@article{21537, abstract = {Nanophotonics has revolutionized the control of light-matter interactions in various fields of fundamental science and technology. In this work, we propose Implosion Fabrication (ImpFab) as a versatile nanophotonics fabrication platform providing the highest spatial resolution, material versatility, and full volumetric control. ImpFab uniquely combines top-down lithography with bottom-up nanoparticle assembly within a hydrogel scaffold, enabling precise control over optical material properties, such as refractive index, by adjusting printing parameters. We showcase the potential of ImpFab by fabricating three-dimensional photonic crystals and quasicrystals, as well as demonstrating optical structures with spatially modulated unit cell material properties. Our results highlight the potential of ImpFab in producing nanostructures with tailored optical functionalities, which are crucial for applications in sensing, imaging, and information processing, and opening new avenues in developing non-Hermitian photonic systems with spatially controlled gain and loss.}, author = {Salamin, Yannick and Yang, Gaojie and Mills, Brian and Grossi Fonseca, André and Roques-Carmes, Charles and Yang, Quansan and Beroz, Justin and Kooi, Steven E. and de Miguel Comella, Marc and Mak, Kiran and Vaidya, Sachin and Oran, Daniel and Swain, Corban and Sun, Yi and Maayani, Shai and Sloan, Jamison and Amin Elfadil Elawad, Amel and Lopez, Josue J. and Boyden, Edward S. and Soljačić, Marin}, issn = {2047-7538}, journal = {Light: Science & Applications}, publisher = {Springer Nature}, title = {{Three-dimensional nanophotonics with spatially modulated optical properties}}, doi = {10.1038/s41377-025-02166-5}, volume = {15}, year = {2026}, } @article{21536, abstract = {Scintillators have been widely used in X-ray imaging due to their ability to convert high-energy radiation into visible light, making them essential for applications such as medical imaging and high-energy physics. Recent advances in the artificial structuring of scintillators offer new opportunities for improving the energy resolution of scintillator-based X-ray detectors. Here, we present a three-bin energy-resolved X-ray imaging framework based on a three-layer multicolor scintillator used in conjunction with a physics-aware image postprocessing algorithm. The multicolor scintillator is able to preserve X-ray energy information through the combination of emission wavelength multiplexing and energy-dependent isolation of X-ray absorption in specific layers. The dominant emission color and the radius of the spot measured by the detector are used to infer the incident X-ray energy based on prior knowledge of the energy-dependent absorption profiles of the scintillator stack. Through ab initio Monte Carlo simulations, we show that our approach can achieve an energy reconstruction accuracy of 49.7%, which is only 2% below the maximum accuracy achievable with realistic scintillators. We apply our framework to medical phantom imaging simulations where we demonstrate that it can effectively differentiate iodine and gadolinium-based contrast agents from bone, muscle, and soft tissue.}, author = {Min, Seokhwan and Choi, Seou and Pajovic, Simo and Vaidya, Sachin and Rivera, Nicholas and Fan, Shanhui and Soljačić, Marin and Roques-Carmes, Charles}, issn = {2047-7538}, journal = {Light: Science & Applications}, publisher = {Springer Nature}, title = {{End-to-end design of multicolor scintillators for enhanced energy resolution in X-ray imaging}}, doi = {10.1038/s41377-025-01836-8}, volume = {14}, year = {2025}, } @article{21535, abstract = {Optical phenomena always display some degree of partial coherence between their respective degrees of freedom. Partial coherence is of particular interest in multimodal systems, where classical and quantum correlations between spatial, polarization, and spectral degrees of freedom can lead to fascinating phenomena (e.g., entanglement) and be leveraged for advanced imaging and sensing modalities (e.g., in hyperspectral, polarization, and ghost imaging). Here, we present a universal method to analyze, process, and generate spatially partially coherent light in multimode systems by using self-configuring optical networks. Our method relies on cascaded self-configuring layers whose average power outputs are sequentially optimized. Once optimized, the network separates the input light into its mutually incoherent components, which is formally equivalent to a diagonalization of the input density matrix. We illustrate our method with numerical simulations of Mach-Zehnder interferometer arrays and show how this method can be used to perform partially coherent environmental light sensing, generation of multimode partially coherent light with arbitrary coherency matrices, and unscrambling of quantum optical mixtures. We provide guidelines for the experimental realization of this method, including the influence of losses, paving the way for self-configuring photonic devices that can automatically learn optimal modal representations of partially coherent light fields.}, author = {Roques-Carmes, Charles and Fan, Shanhui and Miller, David A. B.}, issn = {2047-7538}, journal = {Light: Science & Applications}, publisher = {Springer Nature}, title = {{Measuring, processing, and generating partially coherent light with self-configuring optics}}, doi = {10.1038/s41377-024-01622-y}, volume = {13}, year = {2024}, } @article{6102, abstract = {Light is a union of electric and magnetic fields, and nowhere is the complex relationship between these fields more evident than in the near fields of nanophotonic structures. There, complicated electric and magnetic fields varying over subwavelength scales are generally present, which results in photonic phenomena such as extraordinary optical momentum, superchiral fields, and a complex spatial evolution of optical singularities. An understanding of such phenomena requires nanoscale measurements of the complete optical field vector. Although the sensitivity of near- field scanning optical microscopy to the complete electromagnetic field was recently demonstrated, a separation of different components required a priori knowledge of the sample. Here, we introduce a robust algorithm that can disentangle all six electric and magnetic field components from a single near-field measurement without any numerical modeling of the structure. As examples, we unravel the fields of two prototypical nanophotonic structures: a photonic crystal waveguide and a plasmonic nanowire. These results pave the way for new studies of complex photonic phenomena at the nanoscale and for the design of structures that optimize their optical behavior.}, author = {Le Feber, B. and Sipe, J. E. and Wulf, Matthias and Kuipers, L. and Rotenberg, N.}, issn = {2047-7538}, journal = {Light: Science and Applications}, number = {1}, publisher = {Springer Nature}, title = {{A full vectorial mapping of nanophotonic light fields}}, doi = {10.1038/s41377-019-0124-3}, volume = {8}, year = {2019}, } @article{14012, abstract = {Monochromatization of high-harmonic sources has opened fascinating perspectives regarding time-resolved photoemission from all phases of matter. Such studies have invariably involved the use of spectral filters or spectrally dispersive optical components that are inherently lossy and technically complex. Here we present a new technique for the spectral selection of near-threshold harmonics and their spatial separation from the driving beams without any optical elements. We discover the existence of a narrow phase-matching gate resulting from the combination of the non-collinear generation geometry in an extended medium, atomic resonances and absorption. Our technique offers a filter contrast of up to 104 for the selected harmonics against the adjacent ones and offers multiple temporally synchronized beamlets in a single unified scheme. We demonstrate the selective generation of 133, 80 or 56 nm femtosecond pulses from a 400-nm driver, which is specific to the target gas. These results open new pathways towards phase-sensitive multi-pulse spectroscopy in the vacuum- and extreme-ultraviolet, and frequency-selective output coupling from enhancement cavities.}, author = {Rajeev, Rajendran and Hellwagner, Johannes and Schumacher, Anne and Jordan, Inga and Huppert, Martin and Tehlar, Andres and Niraghatam, Bhargava Ram and Baykusheva, Denitsa Rangelova and Lin, Nan and von Conta, Aaron and Wörner, Hans Jakob}, issn = {2047-7538}, journal = {Light: Science & Applications}, keywords = {Atomic and Molecular Physics, and Optics, Electronic, Optical and Magnetic Materials}, number = {11}, pages = {e16170--e16170}, publisher = {Springer Nature}, title = {{In situ frequency gating and beam splitting of vacuum- and extreme-ultraviolet pulses}}, doi = {10.1038/lsa.2016.170}, volume = {5}, year = {2016}, }