---
OA_place: repository
OA_type: green
_id: '21955'
abstract:
- lang: eng
  text: 'AgRP neurons cause hunger, the drive to seek and consume food. Their activation
    by fasting is key for survival and is thought to be triggered by feedback when
    energy stores are low. However, we know that environmental cues can also regulate
    AgRP neurons since cues that predict future food intake rapidly inhibit AgRP neurons,
    but is the converse true: can the prediction of future fasting rapidly activate
    AgRP neurons? Here, we show in mice that such rapid fasting activation of AgRP
    neurons does occur. This rapid activation is driven by excitatory input from paraventricular
    hypothalamic (PVH) neurons expressing Sim2, which are bidirectionally sensitive
    to predictions of future energy state. Thus, cognitively processed contextual
    information conveyed by PVHSim2 neurons strongly activates AgRP neurons. Lastly,
    chronic silencing of PVHSim2 neurons causes persistent hypophagia. This PVHSim2-to-AgRP-neuron
    circuit, by anticipating and preventing negative energy balance, provides an important
    new dimension of hunger regulation.'
acknowledgement: "We thank all members of the B.B.L. laboratory for helpful discussions.
  We\r\nthank the BADERC and BNORC transgenic cores (NIH P30DK057521 and\r\nP30DK046200)
  for performing embryo injections to generate knockin mouse\r\nlines. We also thank
  the BIDMC Energy Balance Core (supported by NIH\r\nS10OD028635 and the Boston Area
  Diabetes Endocrinology Research Centers, P30DK135043), where Marissa Cortopassi
  performed indirect calorimetry experiments and Alexander Banks assisted with data
  analysis and interpretation. Confocal imaging was performed at BIDMC’s Confocal
  Imaging\r\nCore. We thank Chen Wu for assistance in designing knockin mouse lines.\r\nThis
  work was supported by the NIH (R01DK134427, R01DK096010, and\r\nR01DK075632 to B.B.L.).
  Authors were supported by an EMBO Long-Term\r\nFellowship (770-2018, S.J.W.), a
  T32 Postdoctoral Training Fellowship\r\n(5T32DK007516, E.D.L.), the Charles A. King
  Trust Postdoctoral Research\r\nFellowship program (A.M.D.), and a K99 Career Development
  Award\r\n(K99HL144923, J.M.R.)."
article_processing_charge: No
article_type: original
author:
- first_name: Samuel J.
  full_name: Walker, Samuel J.
  last_name: Walker
- first_name: Elijah D.
  full_name: Lowenstein, Elijah D.
  last_name: Lowenstein
- first_name: Amelia May Barnett
  full_name: Douglass, Amelia May Barnett
  id: de5f6fda-80fb-11ef-996f-a8c4ecd8e289
  last_name: Douglass
  orcid: 0000-0001-5398-6473
- first_name: Callum M.P.
  full_name: Thomas, Callum M.P.
  last_name: Thomas
- first_name: Joseph C.
  full_name: Madara, Joseph C.
  last_name: Madara
- first_name: Hakan
  full_name: Kucukdereli, Hakan
  last_name: Kucukdereli
- first_name: Eunice A.
  full_name: Barbosa-Meillon, Eunice A.
  last_name: Barbosa-Meillon
- first_name: Jenkang
  full_name: Tao, Jenkang
  last_name: Tao
- first_name: Jon M.
  full_name: Resch, Jon M.
  last_name: Resch
- first_name: Bradford B.
  full_name: Lowell, Bradford B.
  last_name: Lowell
citation:
  ama: Walker SJ, Lowenstein ED, Douglass AM, et al. A hypothalamic circuit for anticipating
    future changes in energy balance. <i>Neuron</i>. doi:<a href="https://doi.org/10.1016/j.neuron.2026.05.010">10.1016/j.neuron.2026.05.010</a>
  apa: Walker, S. J., Lowenstein, E. D., Douglass, A. M., Thomas, C. M. P., Madara,
    J. C., Kucukdereli, H., … Lowell, B. B. (n.d.). A hypothalamic circuit for anticipating
    future changes in energy balance. <i>Neuron</i>. Elsevier. <a href="https://doi.org/10.1016/j.neuron.2026.05.010">https://doi.org/10.1016/j.neuron.2026.05.010</a>
  chicago: Walker, Samuel J., Elijah D. Lowenstein, Amelia M. Douglass, Callum M.P.
    Thomas, Joseph C. Madara, Hakan Kucukdereli, Eunice A. Barbosa-Meillon, Jenkang
    Tao, Jon M. Resch, and Bradford B. Lowell. “A Hypothalamic Circuit for Anticipating
    Future Changes in Energy Balance.” <i>Neuron</i>. Elsevier, n.d. <a href="https://doi.org/10.1016/j.neuron.2026.05.010">https://doi.org/10.1016/j.neuron.2026.05.010</a>.
  ieee: S. J. Walker <i>et al.</i>, “A hypothalamic circuit for anticipating future
    changes in energy balance,” <i>Neuron</i>. Elsevier.
  ista: Walker SJ, Lowenstein ED, Douglass AM, Thomas CMP, Madara JC, Kucukdereli
    H, Barbosa-Meillon EA, Tao J, Resch JM, Lowell BB. A hypothalamic circuit for
    anticipating future changes in energy balance. Neuron.
  mla: Walker, Samuel J., et al. “A Hypothalamic Circuit for Anticipating Future Changes
    in Energy Balance.” <i>Neuron</i>, Elsevier, doi:<a href="https://doi.org/10.1016/j.neuron.2026.05.010">10.1016/j.neuron.2026.05.010</a>.
  short: S.J. Walker, E.D. Lowenstein, A.M. Douglass, C.M.P. Thomas, J.C. Madara,
    H. Kucukdereli, E.A. Barbosa-Meillon, J. Tao, J.M. Resch, B.B. Lowell, Neuron
    (n.d.).
date_created: 2026-06-08T09:24:25Z
date_published: 2026-06-03T00:00:00Z
date_updated: 2026-06-16T08:35:11Z
day: '03'
department:
- _id: AmDo
doi: 10.1016/j.neuron.2026.05.010
external_id:
  pmid:
  - '42235510'
keyword:
- hunger
- hypothalamus
- AGRP neurons
- neuroscience
- metabolism
- homeostasis
- feeding
- food intake
- energy balance
- appetite
language:
- iso: eng
main_file_link:
- open_access: '1'
  url: https://doi.org/10.1101/2025.09.27.678865
month: '06'
oa: 1
oa_version: Preprint
pmid: 1
publication: Neuron
publication_identifier:
  eissn:
  - ' 1097-4199'
  issn:
  - 0896-6273
publication_status: inpress
publisher: Elsevier
quality_controlled: '1'
scopus_import: '1'
status: public
title: A hypothalamic circuit for anticipating future changes in energy balance
type: journal_article
user_id: 2DF688A6-F248-11E8-B48F-1D18A9856A87
year: '2026'
...
---
_id: '14733'
abstract:
- lang: eng
  text: Redox flow batteries (RFBs) rely on the development of cheap, highly soluble,
    and high-energy-density electrolytes. Several candidate quinones have already
    been investigated in the literature as two-electron anolytes or catholytes, benefiting
    from fast kinetics, high tunability, and low cost. Here, an investigation of nitrogen-rich
    fused heteroaromatic quinones was carried out to explore avenues for electrolyte
    development. These quinones were synthesized and screened by using electrochemical
    techniques. The most promising candidate, 4,8-dioxo-4,8-dihydrobenzo[1,2-d:4,5-d′]bis([1,2,3]triazole)-1,5-diide
    (−0.68 V(SHE)), was tested in both an asymmetric and symmetric full-cell setup
    resulting in capacity fade rates of 0.35% per cycle and 0.0124% per cycle, respectively.
    In situ ultraviolet-visible spectroscopy (UV–Vis), nuclear magnetic resonance
    (NMR), and electron paramagnetic resonance (EPR) spectroscopies were used to investigate
    the electrochemical stability of the charged species during operation. UV–Vis
    spectroscopy, supported by density functional theory (DFT) modeling, reaffirmed
    that the two-step charging mechanism observed during battery operation consisted
    of two, single-electron transfers. The radical concentration during battery operation
    and the degree of delocalization of the unpaired electron were quantified with
    NMR and EPR spectroscopy.
article_processing_charge: Yes (in subscription journal)
article_type: original
author:
- first_name: Rajesh B
  full_name: Jethwa, Rajesh B
  id: 4cc538d5-803f-11ed-ab7e-8139573aad8f
  last_name: Jethwa
  orcid: 0000-0002-0404-4356
- first_name: Dominic
  full_name: Hey, Dominic
  last_name: Hey
- first_name: Rachel N.
  full_name: Kerber, Rachel N.
  last_name: Kerber
- first_name: Andrew D.
  full_name: Bond, Andrew D.
  last_name: Bond
- first_name: Dominic S.
  full_name: Wright, Dominic S.
  last_name: Wright
- first_name: Clare P.
  full_name: Grey, Clare P.
  last_name: Grey
citation:
  ama: Jethwa RB, Hey D, Kerber RN, Bond AD, Wright DS, Grey CP. Exploring the landscape
    of heterocyclic quinones for redox flow batteries. <i>ACS Applied Energy Materials</i>.
    2024;7(2):414-426. doi:<a href="https://doi.org/10.1021/acsaem.3c02223">10.1021/acsaem.3c02223</a>
  apa: Jethwa, R. B., Hey, D., Kerber, R. N., Bond, A. D., Wright, D. S., &#38; Grey,
    C. P. (2024). Exploring the landscape of heterocyclic quinones for redox flow
    batteries. <i>ACS Applied Energy Materials</i>. American Chemical Society. <a
    href="https://doi.org/10.1021/acsaem.3c02223">https://doi.org/10.1021/acsaem.3c02223</a>
  chicago: Jethwa, Rajesh B, Dominic Hey, Rachel N. Kerber, Andrew D. Bond, Dominic
    S. Wright, and Clare P. Grey. “Exploring the Landscape of Heterocyclic Quinones
    for Redox Flow Batteries.” <i>ACS Applied Energy Materials</i>. American Chemical
    Society, 2024. <a href="https://doi.org/10.1021/acsaem.3c02223">https://doi.org/10.1021/acsaem.3c02223</a>.
  ieee: R. B. Jethwa, D. Hey, R. N. Kerber, A. D. Bond, D. S. Wright, and C. P. Grey,
    “Exploring the landscape of heterocyclic quinones for redox flow batteries,” <i>ACS
    Applied Energy Materials</i>, vol. 7, no. 2. American Chemical Society, pp. 414–426,
    2024.
  ista: Jethwa RB, Hey D, Kerber RN, Bond AD, Wright DS, Grey CP. 2024. Exploring
    the landscape of heterocyclic quinones for redox flow batteries. ACS Applied Energy
    Materials. 7(2), 414–426.
  mla: Jethwa, Rajesh B., et al. “Exploring the Landscape of Heterocyclic Quinones
    for Redox Flow Batteries.” <i>ACS Applied Energy Materials</i>, vol. 7, no. 2,
    American Chemical Society, 2024, pp. 414–26, doi:<a href="https://doi.org/10.1021/acsaem.3c02223">10.1021/acsaem.3c02223</a>.
  short: R.B. Jethwa, D. Hey, R.N. Kerber, A.D. Bond, D.S. Wright, C.P. Grey, ACS
    Applied Energy Materials 7 (2024) 414–426.
date_created: 2024-01-05T09:20:48Z
date_published: 2024-01-22T00:00:00Z
date_updated: 2025-09-04T11:36:32Z
day: '22'
ddc:
- '540'
department:
- _id: StFr
doi: 10.1021/acsaem.3c02223
ec_funded: 1
external_id:
  isi:
  - '001146733200001'
  pmid:
  - '38273966'
file:
- access_level: open_access
  checksum: 2841e86a041d249ac0df2531b7f9aec1
  content_type: application/pdf
  creator: dernst
  date_created: 2024-07-16T11:59:24Z
  date_updated: 2024-07-16T11:59:24Z
  file_id: '17262'
  file_name: 2024_ACSAppElecMaterials_Jethwa.pdf
  file_size: 5607177
  relation: main_file
  success: 1
file_date_updated: 2024-07-16T11:59:24Z
has_accepted_license: '1'
intvolume: '         7'
isi: 1
issue: '2'
keyword:
- Electrical and Electronic Engineering
- Materials Chemistry
- Electrochemistry
- Energy Engineering and Power Technology
- Chemical Engineering (miscellaneous)
language:
- iso: eng
main_file_link:
- open_access: '1'
  url: https://doi.org/10.1021/acsaem.3c02223
month: '01'
oa: 1
oa_version: Published Version
page: 414-426
pmid: 1
project:
- _id: fc2ed2f7-9c52-11eb-aca3-c01059dda49c
  call_identifier: H2020
  grant_number: '101034413'
  name: 'IST-BRIDGE: International postdoctoral program'
publication: ACS Applied Energy Materials
publication_identifier:
  eissn:
  - 2574-0962
publication_status: published
publisher: American Chemical Society
quality_controlled: '1'
scopus_import: '1'
status: public
title: Exploring the landscape of heterocyclic quinones for redox flow batteries
tmp:
  image: /images/cc_by.png
  legal_code_url: https://creativecommons.org/licenses/by/4.0/legalcode
  name: Creative Commons Attribution 4.0 International Public License (CC-BY 4.0)
  short: CC BY (4.0)
type: journal_article
user_id: 317138e5-6ab7-11ef-aa6d-ffef3953e345
volume: 7
year: '2024'
...
---
_id: '14828'
abstract:
- lang: eng
  text: Production of hydrogen at large scale requires development of non-noble, inexpensive,
    and high-performing catalysts for constructing water-splitting devices. Herein,
    we report the synthesis of Zn-doped NiO heterostructure (ZnNiO) catalysts at room
    temperature via a coprecipitation method followed by drying (at 80 °C, 6 h) and
    calcination at an elevated temperature of 400 °C for 5 h under three distinct
    conditions, namely, air, N2, and vacuum. The vacuum-synthesized catalyst demonstrates
    a low overpotential of 88 mV at −10 mA cm–2 and a small Tafel slope of 73 mV dec–1
    suggesting relatively higher charge transfer kinetics for hydrogen evolution reactions
    (HER) compared with the specimens synthesized under N2 or O2 atmosphere. It also
    demonstrates an oxygen evolution (OER) overpotential of 260 mV at 10 mA cm–2 with
    a low Tafel slope of 63 mV dec–1. In a full-cell water-splitting device, the vacuum-synthesized
    ZnNiO heterostructure demonstrates a cell voltage of 1.94 V at 50 mA cm–2 and
    shows remarkable stability over 24 h at a high current density of 100 mA cm–2.
    It is also demonstrated in this study that Zn-doping, surface, and interface engineering
    in transition-metal oxides play a crucial role in efficient electrocatalytic water
    splitting. Also, the results obtained from density functional theory (DFT + U
    = 0–8 eV), where U is the on-site Coulomb repulsion parameter also known as Hubbard
    U, based electronic structure calculations confirm that Zn doping constructively
    modifies the electronic structure, in both the valence band and the conduction
    band, and found to be suitable in tailoring the carrier’s effective masses of
    electrons and holes. The decrease in electron’s effective masses together with
    large differences between the effective masses of electrons and holes is noticed,
    which is found to be mainly responsible for achieving the best water-splitting
    performance from a 9% Zn-doped NiO sample prepared under vacuum.
acknowledgement: This work was supported by the Technology Innovation Program (20011622,
  Development of Battery System Applied High-Efficiency Heat Control Polymer and Part
  Component) funded by the Ministry of Trade, Industry & Energy (MOTIE, Korea). Author
  acknowledge to Prof. Tsunehiro Takeuchi from Toyota Technological Institute, Nagoya,
  Japan for the support of computational resources.
article_processing_charge: No
article_type: original
author:
- first_name: Gundegowda Kalligowdanadoddi
  full_name: Kiran, Gundegowda Kalligowdanadoddi
  last_name: Kiran
- first_name: Saurabh
  full_name: Singh, Saurabh
  id: 12d625da-9cb3-11ed-9667-af09d37d3f0a
  last_name: Singh
  orcid: 0000-0003-2209-5269
- first_name: Neelima
  full_name: Mahato, Neelima
  last_name: Mahato
- first_name: Thupakula Venkata Madhukar
  full_name: Sreekanth, Thupakula Venkata Madhukar
  last_name: Sreekanth
- first_name: Gowra Raghupathy
  full_name: Dillip, Gowra Raghupathy
  last_name: Dillip
- first_name: Kisoo
  full_name: Yoo, Kisoo
  last_name: Yoo
- first_name: Jonghoon
  full_name: Kim, Jonghoon
  last_name: Kim
citation:
  ama: Kiran GK, Singh S, Mahato N, et al. Interface engineering modulation combined
    with electronic structure modification of Zn-doped NiO heterostructure for efficient
    water-splitting activity. <i>ACS Applied Energy Materials</i>. 2024;7(1):214-229.
    doi:<a href="https://doi.org/10.1021/acsaem.3c02519">10.1021/acsaem.3c02519</a>
  apa: Kiran, G. K., Singh, S., Mahato, N., Sreekanth, T. V. M., Dillip, G. R., Yoo,
    K., &#38; Kim, J. (2024). Interface engineering modulation combined with electronic
    structure modification of Zn-doped NiO heterostructure for efficient water-splitting
    activity. <i>ACS Applied Energy Materials</i>. American Chemical Society. <a href="https://doi.org/10.1021/acsaem.3c02519">https://doi.org/10.1021/acsaem.3c02519</a>
  chicago: Kiran, Gundegowda Kalligowdanadoddi, Saurabh Singh, Neelima Mahato, Thupakula
    Venkata Madhukar Sreekanth, Gowra Raghupathy Dillip, Kisoo Yoo, and Jonghoon Kim.
    “Interface Engineering Modulation Combined with Electronic Structure Modification
    of Zn-Doped NiO Heterostructure for Efficient Water-Splitting Activity.” <i>ACS
    Applied Energy Materials</i>. American Chemical Society, 2024. <a href="https://doi.org/10.1021/acsaem.3c02519">https://doi.org/10.1021/acsaem.3c02519</a>.
  ieee: G. K. Kiran <i>et al.</i>, “Interface engineering modulation combined with
    electronic structure modification of Zn-doped NiO heterostructure for efficient
    water-splitting activity,” <i>ACS Applied Energy Materials</i>, vol. 7, no. 1.
    American Chemical Society, pp. 214–229, 2024.
  ista: Kiran GK, Singh S, Mahato N, Sreekanth TVM, Dillip GR, Yoo K, Kim J. 2024.
    Interface engineering modulation combined with electronic structure modification
    of Zn-doped NiO heterostructure for efficient water-splitting activity. ACS Applied
    Energy Materials. 7(1), 214–229.
  mla: Kiran, Gundegowda Kalligowdanadoddi, et al. “Interface Engineering Modulation
    Combined with Electronic Structure Modification of Zn-Doped NiO Heterostructure
    for Efficient Water-Splitting Activity.” <i>ACS Applied Energy Materials</i>,
    vol. 7, no. 1, American Chemical Society, 2024, pp. 214–29, doi:<a href="https://doi.org/10.1021/acsaem.3c02519">10.1021/acsaem.3c02519</a>.
  short: G.K. Kiran, S. Singh, N. Mahato, T.V.M. Sreekanth, G.R. Dillip, K. Yoo, J.
    Kim, ACS Applied Energy Materials 7 (2024) 214–229.
corr_author: '1'
date_created: 2024-01-17T12:48:35Z
date_published: 2024-01-08T00:00:00Z
date_updated: 2024-10-09T21:07:53Z
day: '08'
department:
- _id: MaIb
doi: 10.1021/acsaem.3c02519
external_id:
  isi:
  - '001138342900001'
intvolume: '         7'
isi: 1
issue: '1'
keyword:
- Electrical and Electronic Engineering
- Materials Chemistry
- Electrochemistry
- Energy Engineering and Power Technology
- Chemical Engineering (miscellaneous)
language:
- iso: eng
month: '01'
oa_version: None
page: 214-229
publication: ACS Applied Energy Materials
publication_identifier:
  issn:
  - 2574-0962
publication_status: published
publisher: American Chemical Society
quality_controlled: '1'
scopus_import: '1'
status: public
title: Interface engineering modulation combined with electronic structure modification
  of Zn-doped NiO heterostructure for efficient water-splitting activity
type: journal_article
user_id: 2DF688A6-F248-11E8-B48F-1D18A9856A87
volume: 7
year: '2024'
...
---
_id: '14938'
abstract:
- lang: eng
  text: High elevation headwater catchments are complex hydrological systems that
    seasonally buffer water and release it in the form of snow and ice melt, modulating
    downstream runoff regimes and water availability. In High Mountain Asia (HMA),
    where a wide range of climates from semi-arid to monsoonal exist, the importance
    of the cryospheric contributions to the water budget varies with the amount and
    seasonal distribution of precipitation. Losses due to evapotranspiration and sublimation
    are to date largely unquantified components of the water budget in such catchments,
    although they can be comparable in magnitude to glacier melt contributions to
    streamflow. &amp;#xD;Here, we simulate the hydrology of three high elevation headwater
    catchments in distinct climates in HMA over 10 years using an ecohydrological
    model geared towards high-mountain areas including snow and glaciers, forced with
    reanalysis data. &amp;#xD;Our results show that evapotranspiration and sublimation
    together are most important at the semi-arid site, Kyzylsu, on the northernmost
    slopes of the Pamir mountain range. Here, the evaporative loss amounts to 28%
    of the water throughput, which we define as the total water added to, or removed
    from the water balance within a year. In comparison, evaporative losses are 19%
    at the Central Himalayan site Langtang and 13% at the wettest site, 24K, on the
    Southeastern Tibetan Plateau. At the three sites, respectively, sublimation removes
    15%, 13% and 6% of snowfall, while evapotranspiration removes the equivalent of
    76%, 28% and 19% of rainfall. In absolute terms, and across a comparable elevation
    range, the highest ET flux is 413 mm yr-1 at 24K, while the highest sublimation
    flux is 91 mm yr-1 at Kyzylsu. During warm and dry years, glacier melt was found
    to only partially compensate for the annual supply deficit.
acknowledgement: "We would like to thank the team at the Center for the Research of
  Glaciers, Tajik National Academy of Sciences, Abduhamid Kayumov, Khusrav Kabutov,
  Ardamehr Halimov, among others, for their invaluable support over multiple field
  seasons in Kyzylsu. We thank Wei Yang, Zhao Xhuanxi and Zhen Cheng from the Institute
  of Tibetan Plateau Research, Chinese Academy of Sciences, for facilitating and supporting
  fieldwork and for sharing crucial data from the Parlung 24K catchment. We thank
  Reeju Shrestha and Himalayan Research Expeditions for their great support in Langtang.
  We extend our thanks to Jakob Steiner and the team at ICIMOD for their relentless
  efforts in data acquisition and curation in Langtang. Additionally, we are indebted
  to Masashi Niwano from the Meteorological Research Institute, Japan Meteorological
  Agency, for providing NHM atmospheric simulation outputs, which proved very valuable
  in the downscaling process.\r\nThis project has received funding from the European
  Research Council (ERC) under the European Union's Horizon 2020 research and innovation
  program Grant Agreements No. 772751 (RAVEN, Rapid mass losses of debris-covered
  glaciers in High Mountain Asia). Further funding was provided by JSPS-SNSF (Japan
  Society for the Promotion of Science and Swiss National Science Foundation) Bilateral
  Programmes project (HOPE, High-elevation precipitation in High Mountain Asia; Grant
  183633). Fieldwork support for Tajikistan was received from the Swiss Polar Institute
  Flagship Programme PAMIR, SPI-FLAG-2021-001. The project also received funding from
  the ESA and NRSCC Dragon 5 cooperation project 'Cryosphere-hydrosphere interactions
  of the Asian water towers: using remote sensing to drive hyper-resolution ecohydrological
  modeling' (grant no. 59199). The National Natural Science Foundation of China (41961134035)
  financially supported the data collection at 24K."
article_number: '044057'
article_processing_charge: Yes
article_type: original
author:
- first_name: Stefan
  full_name: Fugger, Stefan
  id: 86698d64-c4c6-11ee-af02-cdf1e6a7d31f
  last_name: Fugger
- first_name: Thomas
  full_name: Shaw, Thomas
  id: 3caa3f91-1f03-11ee-96ce-e0e553054d6e
  last_name: Shaw
  orcid: 0000-0001-7640-6152
- first_name: Achille
  full_name: Jouberton, Achille
  last_name: Jouberton
- first_name: Evan
  full_name: Miles, Evan
  last_name: Miles
- first_name: Pascal
  full_name: Buri, Pascal
  id: 317987aa-9421-11ee-ac5a-b941b041abba
  last_name: Buri
- first_name: Michael
  full_name: McCarthy, Michael
  id: 22a2674a-61ce-11ee-94b5-d18813baf16f
  last_name: McCarthy
- first_name: Catriona Louise
  full_name: Fyffe, Catriona Louise
  id: 001b0422-8d15-11ed-bc51-cab6c037a228
  last_name: Fyffe
- first_name: Simone
  full_name: Fatichi, Simone
  last_name: Fatichi
- first_name: Marin
  full_name: Kneib, Marin
  last_name: Kneib
- first_name: Peter
  full_name: Molnar, Peter
  last_name: Molnar
- first_name: Francesca
  full_name: Pellicciotti, Francesca
  id: b28f055a-81ea-11ed-b70c-a9fe7f7b0e70
  last_name: Pellicciotti
  orcid: 0000-0002-5554-8087
citation:
  ama: Fugger S, Shaw T, Jouberton A, et al. Hydrological regimes and evaporative
    flux partitioning at the climatic ends of High Mountain Asia. <i>Environmental
    Research Letters</i>. 2024;19. doi:<a href="https://doi.org/10.1088/1748-9326/ad25a0">10.1088/1748-9326/ad25a0</a>
  apa: Fugger, S., Shaw, T., Jouberton, A., Miles, E., Buri, P., McCarthy, M., … Pellicciotti,
    F. (2024). Hydrological regimes and evaporative flux partitioning at the climatic
    ends of High Mountain Asia. <i>Environmental Research Letters</i>. IOP Publishing.
    <a href="https://doi.org/10.1088/1748-9326/ad25a0">https://doi.org/10.1088/1748-9326/ad25a0</a>
  chicago: Fugger, Stefan, Thomas Shaw, Achille Jouberton, Evan Miles, Pascal Buri,
    Michael McCarthy, Catriona Louise Fyffe, et al. “Hydrological Regimes and Evaporative
    Flux Partitioning at the Climatic Ends of High Mountain Asia.” <i>Environmental
    Research Letters</i>. IOP Publishing, 2024. <a href="https://doi.org/10.1088/1748-9326/ad25a0">https://doi.org/10.1088/1748-9326/ad25a0</a>.
  ieee: S. Fugger <i>et al.</i>, “Hydrological regimes and evaporative flux partitioning
    at the climatic ends of High Mountain Asia,” <i>Environmental Research Letters</i>,
    vol. 19. IOP Publishing, 2024.
  ista: Fugger S, Shaw T, Jouberton A, Miles E, Buri P, McCarthy M, Fyffe CL, Fatichi
    S, Kneib M, Molnar P, Pellicciotti F. 2024. Hydrological regimes and evaporative
    flux partitioning at the climatic ends of High Mountain Asia. Environmental Research
    Letters. 19, 044057.
  mla: Fugger, Stefan, et al. “Hydrological Regimes and Evaporative Flux Partitioning
    at the Climatic Ends of High Mountain Asia.” <i>Environmental Research Letters</i>,
    vol. 19, 044057, IOP Publishing, 2024, doi:<a href="https://doi.org/10.1088/1748-9326/ad25a0">10.1088/1748-9326/ad25a0</a>.
  short: S. Fugger, T. Shaw, A. Jouberton, E. Miles, P. Buri, M. McCarthy, C.L. Fyffe,
    S. Fatichi, M. Kneib, P. Molnar, F. Pellicciotti, Environmental Research Letters
    19 (2024).
corr_author: '1'
date_created: 2024-02-05T09:01:11Z
date_published: 2024-04-09T00:00:00Z
date_updated: 2025-09-04T11:57:57Z
day: '09'
ddc:
- '550'
department:
- _id: FrPe
doi: 10.1088/1748-9326/ad25a0
external_id:
  isi:
  - '001198892300001'
file:
- access_level: open_access
  checksum: 27999359b51c30fec6d81e48cdf0ee0d
  content_type: application/pdf
  creator: dernst
  date_created: 2024-07-22T09:14:44Z
  date_updated: 2024-07-22T09:14:44Z
  file_id: '17295'
  file_name: 2024_EnvironmResearch_Fugger.pdf
  file_size: 4433401
  relation: main_file
  success: 1
file_date_updated: 2024-07-22T09:14:44Z
has_accepted_license: '1'
intvolume: '        19'
isi: 1
keyword:
- Public Health
- Environmental and Occupational Health
- General Environmental Science
- Renewable Energy
- Sustainability and the Environment
language:
- iso: eng
month: '04'
oa: 1
oa_version: Published Version
publication: Environmental Research Letters
publication_identifier:
  issn:
  - 1748-9326
publication_status: published
publisher: IOP Publishing
quality_controlled: '1'
scopus_import: '1'
status: public
title: Hydrological regimes and evaporative flux partitioning at the climatic ends
  of High Mountain Asia
tmp:
  image: /images/cc_by.png
  legal_code_url: https://creativecommons.org/licenses/by/4.0/legalcode
  name: Creative Commons Attribution 4.0 International Public License (CC-BY 4.0)
  short: CC BY (4.0)
type: journal_article
user_id: 317138e5-6ab7-11ef-aa6d-ffef3953e345
volume: 19
year: '2024'
...
---
_id: '13277'
abstract:
- lang: eng
  text: Recent experimental advances have inspired the development of theoretical
    tools to describe the non-equilibrium dynamics of quantum systems. Among them
    an exact representation of quantum spin systems in terms of classical stochastic
    processes has been proposed. Here we provide first steps towards the extension
    of this stochastic approach to bosonic systems by considering the one-dimensional
    quantum quartic oscillator. We show how to exactly parameterize the time evolution
    of this prototypical model via the dynamics of a set of classical variables. We
    interpret these variables as stochastic processes, which allows us to propose
    a novel way to numerically simulate the time evolution of the system. We benchmark
    our findings by considering analytically solvable limits and providing alternative
    derivations of known results.
acknowledgement: 'S. De Nicola acknowledges funding from the Institute of Science
  and Technology Austria (ISTA), and from the European Union’s Horizon 2020 research
  and innovation program under the Marie Skłodowska-Curie Grant Agreement No. 754411.
  S. De Nicola also acknowledges funding from the EPSRC Center for Doctoral Training
  in Cross-Disciplinary Approaches to NonEquilibrium Systems (CANES) under Grant EP/L015854/1. '
article_number: '029'
article_processing_charge: No
article_type: original
arxiv: 1
author:
- first_name: Gennaro
  full_name: Tucci, Gennaro
  last_name: Tucci
- first_name: Stefano
  full_name: De Nicola, Stefano
  id: 42832B76-F248-11E8-B48F-1D18A9856A87
  last_name: De Nicola
  orcid: 0000-0002-4842-6671
- first_name: Sascha
  full_name: Wald, Sascha
  last_name: Wald
- first_name: Andrea
  full_name: Gambassi, Andrea
  last_name: Gambassi
citation:
  ama: Tucci G, De Nicola S, Wald S, Gambassi A. Stochastic representation of the
    quantum quartic oscillator. <i>SciPost Physics Core</i>. 2023;6(2). doi:<a href="https://doi.org/10.21468/scipostphyscore.6.2.029">10.21468/scipostphyscore.6.2.029</a>
  apa: Tucci, G., De Nicola, S., Wald, S., &#38; Gambassi, A. (2023). Stochastic representation
    of the quantum quartic oscillator. <i>SciPost Physics Core</i>. SciPost Foundation.
    <a href="https://doi.org/10.21468/scipostphyscore.6.2.029">https://doi.org/10.21468/scipostphyscore.6.2.029</a>
  chicago: Tucci, Gennaro, Stefano De Nicola, Sascha Wald, and Andrea Gambassi. “Stochastic
    Representation of the Quantum Quartic Oscillator.” <i>SciPost Physics Core</i>.
    SciPost Foundation, 2023. <a href="https://doi.org/10.21468/scipostphyscore.6.2.029">https://doi.org/10.21468/scipostphyscore.6.2.029</a>.
  ieee: G. Tucci, S. De Nicola, S. Wald, and A. Gambassi, “Stochastic representation
    of the quantum quartic oscillator,” <i>SciPost Physics Core</i>, vol. 6, no. 2.
    SciPost Foundation, 2023.
  ista: Tucci G, De Nicola S, Wald S, Gambassi A. 2023. Stochastic representation
    of the quantum quartic oscillator. SciPost Physics Core. 6(2), 029.
  mla: Tucci, Gennaro, et al. “Stochastic Representation of the Quantum Quartic Oscillator.”
    <i>SciPost Physics Core</i>, vol. 6, no. 2, 029, SciPost Foundation, 2023, doi:<a
    href="https://doi.org/10.21468/scipostphyscore.6.2.029">10.21468/scipostphyscore.6.2.029</a>.
  short: G. Tucci, S. De Nicola, S. Wald, A. Gambassi, SciPost Physics Core 6 (2023).
corr_author: '1'
date_created: 2023-07-24T10:47:46Z
date_published: 2023-04-14T00:00:00Z
date_updated: 2025-04-14T07:43:56Z
day: '14'
ddc:
- '530'
department:
- _id: MaSe
doi: 10.21468/scipostphyscore.6.2.029
ec_funded: 1
external_id:
  arxiv:
  - '2211.01923'
file:
- access_level: open_access
  checksum: b472bc82108747eda5d52adf9e2ac7f3
  content_type: application/pdf
  creator: dernst
  date_created: 2023-07-31T09:02:27Z
  date_updated: 2023-07-31T09:02:27Z
  file_id: '13329'
  file_name: 2023_SciPostPhysCore_Tucci.pdf
  file_size: 523236
  relation: main_file
  success: 1
file_date_updated: 2023-07-31T09:02:27Z
has_accepted_license: '1'
intvolume: '         6'
issue: '2'
keyword:
- Statistical and Nonlinear Physics
- Atomic and Molecular Physics
- and Optics
- Nuclear and High Energy Physics
- Condensed Matter Physics
language:
- iso: eng
month: '04'
oa: 1
oa_version: Published Version
project:
- _id: 260C2330-B435-11E9-9278-68D0E5697425
  call_identifier: H2020
  grant_number: '754411'
  name: ISTplus - Postdoctoral Fellowships
publication: SciPost Physics Core
publication_identifier:
  issn:
  - 2666-9366
publication_status: published
publisher: SciPost Foundation
quality_controlled: '1'
scopus_import: '1'
status: public
title: Stochastic representation of the quantum quartic oscillator
tmp:
  image: /images/cc_by.png
  legal_code_url: https://creativecommons.org/licenses/by/4.0/legalcode
  name: Creative Commons Attribution 4.0 International Public License (CC-BY 4.0)
  short: CC BY (4.0)
type: journal_article
user_id: 2DF688A6-F248-11E8-B48F-1D18A9856A87
volume: 6
year: '2023'
...
---
_id: '14753'
abstract:
- lang: eng
  text: "Several fixed-target experiments reported J/ψ and ϒ polarizations, as functions
    of Feynman x (xF) and transverse momentum (PT), in three different frames, using
    different combinations of beam particles, target nuclei, and collision energies.
    Despite the diverse and heterogeneous picture formed by these measurements, a
    detailed look allows us to discern qualitative physical patterns that inspire
    a simple empirical model. This data-driven scenario offers a good quantitative
    description of the J/ψ and ϒ(1S) polarizations measured in proton- and pion-nucleus
    collisions, in the xF 0.5 domain: more than 80 data points (not statistically
    independent) are well reproduced with only one free parameter. This study sets
    the context for future low-PT\r\n quarkonium polarization measurements in proton-
    and pion-nucleus collisions, such as those to be made by the AMBER experiment,
    and shows that such measurements provide significant constraints on the poorly-known
    parton distribution functions of the pion."
acknowledgement: "P.F. and C.L. acknowledge support from Fundação para a Ciência e
  a Tecnologia, Portugal, under contract CERN/FIS-PAR/0010/2019.\r\nOpen Access funded
  by SCOAP3."
article_number: '137871'
article_processing_charge: Yes (via OA deal)
article_type: original
author:
- first_name: Pietro
  full_name: Faccioli, Pietro
  last_name: Faccioli
- first_name: Ilse
  full_name: Krätschmer, Ilse
  id: 30d4014e-7753-11eb-b44b-db6d61112e73
  last_name: Krätschmer
  orcid: 0000-0002-5636-9259
- first_name: Carlos
  full_name: Lourenço, Carlos
  last_name: Lourenço
citation:
  ama: 'Faccioli P, Krätschmer I, Lourenço C. Low-pT quarkonium polarization measurements:
    Challenges and opportunities. <i>Physics Letters B</i>. 2023;840. doi:<a href="https://doi.org/10.1016/j.physletb.2023.137871">10.1016/j.physletb.2023.137871</a>'
  apa: 'Faccioli, P., Krätschmer, I., &#38; Lourenço, C. (2023). Low-pT quarkonium
    polarization measurements: Challenges and opportunities. <i>Physics Letters B</i>.
    Elsevier. <a href="https://doi.org/10.1016/j.physletb.2023.137871">https://doi.org/10.1016/j.physletb.2023.137871</a>'
  chicago: 'Faccioli, Pietro, Ilse Krätschmer, and Carlos Lourenço. “Low-PT Quarkonium
    Polarization Measurements: Challenges and Opportunities.” <i>Physics Letters B</i>.
    Elsevier, 2023. <a href="https://doi.org/10.1016/j.physletb.2023.137871">https://doi.org/10.1016/j.physletb.2023.137871</a>.'
  ieee: 'P. Faccioli, I. Krätschmer, and C. Lourenço, “Low-pT quarkonium polarization
    measurements: Challenges and opportunities,” <i>Physics Letters B</i>, vol. 840.
    Elsevier, 2023.'
  ista: 'Faccioli P, Krätschmer I, Lourenço C. 2023. Low-pT quarkonium polarization
    measurements: Challenges and opportunities. Physics Letters B. 840, 137871.'
  mla: 'Faccioli, Pietro, et al. “Low-PT Quarkonium Polarization Measurements: Challenges
    and Opportunities.” <i>Physics Letters B</i>, vol. 840, 137871, Elsevier, 2023,
    doi:<a href="https://doi.org/10.1016/j.physletb.2023.137871">10.1016/j.physletb.2023.137871</a>.'
  short: P. Faccioli, I. Krätschmer, C. Lourenço, Physics Letters B 840 (2023).
date_created: 2024-01-08T13:09:17Z
date_published: 2023-05-10T00:00:00Z
date_updated: 2025-09-09T14:13:46Z
day: '10'
ddc:
- '530'
department:
- _id: MaRo
doi: 10.1016/j.physletb.2023.137871
external_id:
  isi:
  - '000967947300001'
file:
- access_level: open_access
  checksum: 02dec160dbc81d95985e755869d8afbf
  content_type: application/pdf
  creator: dernst
  date_created: 2024-01-09T08:59:24Z
  date_updated: 2024-01-09T08:59:24Z
  file_id: '14762'
  file_name: 2023_PhysicsLettersB_Faccioli.pdf
  file_size: 855494
  relation: main_file
  success: 1
file_date_updated: 2024-01-09T08:59:24Z
has_accepted_license: '1'
intvolume: '       840'
isi: 1
keyword:
- Nuclear and High Energy Physics
language:
- iso: eng
month: '05'
oa: 1
oa_version: Published Version
publication: Physics Letters B
publication_identifier:
  eissn:
  - 1873-2445
  issn:
  - 0370-2693
publication_status: published
publisher: Elsevier
quality_controlled: '1'
scopus_import: '1'
status: public
title: 'Low-pT quarkonium polarization measurements: Challenges and opportunities'
tmp:
  image: /images/cc_by.png
  legal_code_url: https://creativecommons.org/licenses/by/4.0/legalcode
  name: Creative Commons Attribution 4.0 International Public License (CC-BY 4.0)
  short: CC BY (4.0)
type: journal_article
user_id: 317138e5-6ab7-11ef-aa6d-ffef3953e345
volume: 840
year: '2023'
...
---
_id: '12133'
abstract:
- lang: eng
  text: Social distancing is an effective way to prevent the spread of disease in
    societies, whereas infection elimination is a key element of organismal immunity.
    Here, we discuss how the study of social insects such as ants — which form a superorganism
    of unconditionally cooperative individuals and thus represent a level of organization
    that is intermediate between a classical society of individuals and an organism
    of cells — can help to determine common principles of disease defence across levels
    of organization.
article_processing_charge: No
article_type: letter_note
author:
- first_name: Sylvia
  full_name: Cremer, Sylvia
  id: 2F64EC8C-F248-11E8-B48F-1D18A9856A87
  last_name: Cremer
  orcid: 0000-0002-2193-3868
- first_name: Michael K
  full_name: Sixt, Michael K
  id: 41E9FBEA-F248-11E8-B48F-1D18A9856A87
  last_name: Sixt
  orcid: 0000-0002-6620-9179
citation:
  ama: Cremer S, Sixt MK. Principles of disease defence in organisms, superorganisms
    and societies. <i>Nature Reviews Immunology</i>. 2022;22(12):713-714. doi:<a href="https://doi.org/10.1038/s41577-022-00797-y">10.1038/s41577-022-00797-y</a>
  apa: Cremer, S., &#38; Sixt, M. K. (2022). Principles of disease defence in organisms,
    superorganisms and societies. <i>Nature Reviews Immunology</i>. Springer Nature.
    <a href="https://doi.org/10.1038/s41577-022-00797-y">https://doi.org/10.1038/s41577-022-00797-y</a>
  chicago: Cremer, Sylvia, and Michael K Sixt. “Principles of Disease Defence in Organisms,
    Superorganisms and Societies.” <i>Nature Reviews Immunology</i>. Springer Nature,
    2022. <a href="https://doi.org/10.1038/s41577-022-00797-y">https://doi.org/10.1038/s41577-022-00797-y</a>.
  ieee: S. Cremer and M. K. Sixt, “Principles of disease defence in organisms, superorganisms
    and societies,” <i>Nature Reviews Immunology</i>, vol. 22, no. 12. Springer Nature,
    pp. 713–714, 2022.
  ista: Cremer S, Sixt MK. 2022. Principles of disease defence in organisms, superorganisms
    and societies. Nature Reviews Immunology. 22(12), 713–714.
  mla: Cremer, Sylvia, and Michael K. Sixt. “Principles of Disease Defence in Organisms,
    Superorganisms and Societies.” <i>Nature Reviews Immunology</i>, vol. 22, no.
    12, Springer Nature, 2022, pp. 713–14, doi:<a href="https://doi.org/10.1038/s41577-022-00797-y">10.1038/s41577-022-00797-y</a>.
  short: S. Cremer, M.K. Sixt, Nature Reviews Immunology 22 (2022) 713–714.
corr_author: '1'
date_created: 2023-01-12T12:03:14Z
date_published: 2022-12-01T00:00:00Z
date_updated: 2024-10-09T21:03:33Z
day: '01'
department:
- _id: SyCr
- _id: MiSi
doi: 10.1038/s41577-022-00797-y
external_id:
  isi:
  - '000871836300001'
  pmid:
  - '36284178'
intvolume: '        22'
isi: 1
issue: '12'
keyword:
- Energy Engineering and Power Technology
- Fuel Technology
language:
- iso: eng
month: '12'
oa_version: None
page: 713-714
pmid: 1
publication: Nature Reviews Immunology
publication_identifier:
  eissn:
  - 1474-1741
  issn:
  - 1474-1733
publication_status: published
publisher: Springer Nature
quality_controlled: '1'
scopus_import: '1'
status: public
title: Principles of disease defence in organisms, superorganisms and societies
type: journal_article
user_id: 4359f0d1-fa6c-11eb-b949-802e58b17ae8
volume: 22
year: '2022'
...
---
_id: '12155'
abstract:
- lang: eng
  text: The growing demand of thermal management in various fields such as miniaturized
    5G chips has motivated researchers to develop new and high-performance solid-state
    refrigeration technologies, typically including multicaloric and thermoelectric
    (TE) cooling. Among them, TE cooling has attracted huge attention owing to its
    advantages of rapid response, large cooling temperature difference, high stability,
    and tunable device size. Bi2Te3-based alloys have long been the only commercialized
    TE cooling materials, while novel systems SnSe and Mg3(Bi,Sb)2 have recently been
    discovered as potential candidates. However, challenges and problems still require
    to be summarized and further resolved for realizing better cooling performance.
    In this review, we systematically investigate TE cooling from its internal mechanism,
    crucial parameters, to device design and applications. Furthermore, we summarize
    the current optimization strategies for existing TE cooling materials, and finally
    provide some personal prospects especially the material-planification concept
    on future research on establishing better TE cooling.
acknowledgement: We acknowledge support from the National Key Research and Development
  Program of China (2018YFA0702100), the National Natural Science Foundation of China
  (51571007, 51772012, 52002011 and 52002042), the Basic Science Center Project of
  National Natural Science Foundation of China (51788104), Beijing Natural Science
  Foundation (JQ18004), 111 Project (B17002), and the National Science Fund for Distinguished
  Young Scholars (51925101).
article_processing_charge: No
article_type: original
author:
- first_name: Yongxin
  full_name: Qin, Yongxin
  last_name: Qin
- first_name: Bingchao
  full_name: Qin, Bingchao
  last_name: Qin
- first_name: Dongyang
  full_name: Wang, Dongyang
  last_name: Wang
- first_name: Cheng
  full_name: Chang, Cheng
  id: 9E331C2E-9F27-11E9-AE48-5033E6697425
  last_name: Chang
  orcid: 0000-0002-9515-4277
- first_name: Li-Dong
  full_name: Zhao, Li-Dong
  last_name: Zhao
citation:
  ama: 'Qin Y, Qin B, Wang D, Chang C, Zhao L-D. Solid-state cooling: Thermoelectrics.
    <i>Energy &#38; Environmental Science</i>. 2022;15(11):4527-4541. doi:<a href="https://doi.org/10.1039/d2ee02408j">10.1039/d2ee02408j</a>'
  apa: 'Qin, Y., Qin, B., Wang, D., Chang, C., &#38; Zhao, L.-D. (2022). Solid-state
    cooling: Thermoelectrics. <i>Energy &#38; Environmental Science</i>. Royal Society
    of Chemistry. <a href="https://doi.org/10.1039/d2ee02408j">https://doi.org/10.1039/d2ee02408j</a>'
  chicago: 'Qin, Yongxin, Bingchao Qin, Dongyang Wang, Cheng Chang, and Li-Dong Zhao.
    “Solid-State Cooling: Thermoelectrics.” <i>Energy &#38; Environmental Science</i>.
    Royal Society of Chemistry, 2022. <a href="https://doi.org/10.1039/d2ee02408j">https://doi.org/10.1039/d2ee02408j</a>.'
  ieee: 'Y. Qin, B. Qin, D. Wang, C. Chang, and L.-D. Zhao, “Solid-state cooling:
    Thermoelectrics,” <i>Energy &#38; Environmental Science</i>, vol. 15, no. 11.
    Royal Society of Chemistry, pp. 4527–4541, 2022.'
  ista: 'Qin Y, Qin B, Wang D, Chang C, Zhao L-D. 2022. Solid-state cooling: Thermoelectrics.
    Energy &#38; Environmental Science. 15(11), 4527–4541.'
  mla: 'Qin, Yongxin, et al. “Solid-State Cooling: Thermoelectrics.” <i>Energy &#38;
    Environmental Science</i>, vol. 15, no. 11, Royal Society of Chemistry, 2022,
    pp. 4527–41, doi:<a href="https://doi.org/10.1039/d2ee02408j">10.1039/d2ee02408j</a>.'
  short: Y. Qin, B. Qin, D. Wang, C. Chang, L.-D. Zhao, Energy &#38; Environmental
    Science 15 (2022) 4527–4541.
date_created: 2023-01-12T12:08:41Z
date_published: 2022-11-01T00:00:00Z
date_updated: 2024-01-22T08:13:43Z
day: '01'
department:
- _id: MaIb
doi: 10.1039/d2ee02408j
external_id:
  isi:
  - '000863642400001'
intvolume: '        15'
isi: 1
issue: '11'
keyword:
- Pollution
- Nuclear Energy and Engineering
- Renewable Energy
- Sustainability and the Environment
- Environmental Chemistry
language:
- iso: eng
month: '11'
oa_version: None
page: 4527-4541
publication: Energy & Environmental Science
publication_identifier:
  eissn:
  - 1754-5706
  issn:
  - 1754-5692
publication_status: published
publisher: Royal Society of Chemistry
quality_controlled: '1'
related_material:
  link:
  - relation: erratum
    url: https://doi.org/10.1039/d3ee90067c
scopus_import: '1'
status: public
title: 'Solid-state cooling: Thermoelectrics'
type: journal_article
user_id: 2DF688A6-F248-11E8-B48F-1D18A9856A87
volume: 15
year: '2022'
...
---
_id: '12227'
abstract:
- lang: eng
  text: Polydicyclopentadiene (pDCPD), a thermoset with excellent mechanical properties,
    has enormous potential as a lightweight, tough, and stable matrix material owing
    to its highly cross-linked macromolecular network. This work describes generating
    pDCPD-based foams and hierarchically porous carbons derived therefrom by combining
    ring-opening metathesis polymerization (ROMP) of DCPD, high internal phase emulsions
    (HIPEs) as structural templates, and subsequent carbonization. The structure and
    function of the carbon foams were characterized and discussed in detail using
    scanning electron, transmission electron, or atomic force microscopy (SEM, TEM,
    AFM), electron energy-loss spectroscopy (TEM-EELS), N2 sorption, and analyses
    of electrical conductivity as well as mechanical properties. The resulting materials
    exhibited uniform, shape-retaining shrinkage of only ∼1/3 after carbonization.
    No structural failure was observed even when the pDCPD precursor foams were heated
    to 1400 °C. Instead, the high porosity, void size, and 3D interconnectivity were
    fully preserved, and the void diameters could be adjusted between 87 and 2.5 μm.
    Moreover, foams have a carbon content >97%, an electronic conductivity of up to
    2800 S·m–1, a Young’s modulus of up to 2.1 GPa, and a specific surface area of
    up to 1200 m2·g–1. Surprisingly, the pDCPD foams were carbonized into shapes other
    than monoliths, such as 10’s of micron thick membranes or foamy coatings adhered
    to a metal foil or grid substrate. The latter coatings even adhere upon bending.
    Finally, as a use case, carbonized foams were applied as porous cathodes for Li–O2
    batteries where the foams show a favorable combination of porosity, active surface
    area, and pore size for outstanding capacity.
acknowledgement: S.K. acknowledges the financial support from the Slovenian Research
  Agency (grants P1-0021, P2-0150). Support by Graz University of Technology (LP-03
  – Porous Materials@Work) and from VARTA Innovation GmbH is kindly acknowledged.
  We thank Umicore for providing the initiator and Matjaž Mazaj (National Institute
  of Chemistry, Ljubljana) and Karel Jerabek (Czech Academy of Sciences) for measurements
  and fruitful discussions. S.A.F. is indebted to the Austrian Federal Ministry of
  Science, Research and Economy; the Austrian Research Promotion Agency (Grant No.
  845364); and ISTA for support.
article_processing_charge: No
article_type: original
author:
- first_name: Sebastijan
  full_name: Kovačič, Sebastijan
  last_name: Kovačič
- first_name: Bettina
  full_name: Schafzahl, Bettina
  last_name: Schafzahl
- first_name: Nadejda B.
  full_name: Matsko, Nadejda B.
  last_name: Matsko
- first_name: Katharina
  full_name: Gruber, Katharina
  last_name: Gruber
- first_name: Martin
  full_name: Schmuck, Martin
  last_name: Schmuck
- first_name: Stefan
  full_name: Koller, Stefan
  last_name: Koller
- first_name: Stefan Alexander
  full_name: Freunberger, Stefan Alexander
  id: A8CA28E6-CE23-11E9-AD2D-EC27E6697425
  last_name: Freunberger
  orcid: 0000-0003-2902-5319
- first_name: Christian
  full_name: Slugovc, Christian
  last_name: Slugovc
citation:
  ama: 'Kovačič S, Schafzahl B, Matsko NB, et al. Carbon foams via ring-opening metathesis
    polymerization of emulsion templates: A facile method to make carbon current collectors
    for battery applications. <i>ACS Applied Energy Materials</i>. 2022;5(11):14381-14390.
    doi:<a href="https://doi.org/10.1021/acsaem.2c02787">10.1021/acsaem.2c02787</a>'
  apa: 'Kovačič, S., Schafzahl, B., Matsko, N. B., Gruber, K., Schmuck, M., Koller,
    S., … Slugovc, C. (2022). Carbon foams via ring-opening metathesis polymerization
    of emulsion templates: A facile method to make carbon current collectors for battery
    applications. <i>ACS Applied Energy Materials</i>. American Chemical Society.
    <a href="https://doi.org/10.1021/acsaem.2c02787">https://doi.org/10.1021/acsaem.2c02787</a>'
  chicago: 'Kovačič, Sebastijan, Bettina Schafzahl, Nadejda B. Matsko, Katharina Gruber,
    Martin Schmuck, Stefan Koller, Stefan Alexander Freunberger, and Christian Slugovc.
    “Carbon Foams via Ring-Opening Metathesis Polymerization of Emulsion Templates:
    A Facile Method to Make Carbon Current Collectors for Battery Applications.” <i>ACS
    Applied Energy Materials</i>. American Chemical Society, 2022. <a href="https://doi.org/10.1021/acsaem.2c02787">https://doi.org/10.1021/acsaem.2c02787</a>.'
  ieee: 'S. Kovačič <i>et al.</i>, “Carbon foams via ring-opening metathesis polymerization
    of emulsion templates: A facile method to make carbon current collectors for battery
    applications,” <i>ACS Applied Energy Materials</i>, vol. 5, no. 11. American Chemical
    Society, pp. 14381–14390, 2022.'
  ista: 'Kovačič S, Schafzahl B, Matsko NB, Gruber K, Schmuck M, Koller S, Freunberger
    SA, Slugovc C. 2022. Carbon foams via ring-opening metathesis polymerization of
    emulsion templates: A facile method to make carbon current collectors for battery
    applications. ACS Applied Energy Materials. 5(11), 14381–14390.'
  mla: 'Kovačič, Sebastijan, et al. “Carbon Foams via Ring-Opening Metathesis Polymerization
    of Emulsion Templates: A Facile Method to Make Carbon Current Collectors for Battery
    Applications.” <i>ACS Applied Energy Materials</i>, vol. 5, no. 11, American Chemical
    Society, 2022, pp. 14381–90, doi:<a href="https://doi.org/10.1021/acsaem.2c02787">10.1021/acsaem.2c02787</a>.'
  short: S. Kovačič, B. Schafzahl, N.B. Matsko, K. Gruber, M. Schmuck, S. Koller,
    S.A. Freunberger, C. Slugovc, ACS Applied Energy Materials 5 (2022) 14381–14390.
corr_author: '1'
date_created: 2023-01-16T09:48:53Z
date_published: 2022-10-16T00:00:00Z
date_updated: 2024-10-09T21:03:48Z
day: '16'
ddc:
- '540'
department:
- _id: StFr
doi: 10.1021/acsaem.2c02787
external_id:
  isi:
  - '000875635900001'
file:
- access_level: open_access
  checksum: 572d15c250ab83d44f4e2c3aeb5f7388
  content_type: application/pdf
  creator: dernst
  date_created: 2023-01-27T09:09:15Z
  date_updated: 2023-01-27T09:09:15Z
  file_id: '12420'
  file_name: 2022_AppliedEnergyMaterials_Kovacic.pdf
  file_size: 13105589
  relation: main_file
  success: 1
file_date_updated: 2023-01-27T09:09:15Z
has_accepted_license: '1'
intvolume: '         5'
isi: 1
issue: '11'
keyword:
- Electrical and Electronic Engineering
- Materials Chemistry
- Electrochemistry
- Energy Engineering and Power Technology
- Chemical Engineering (miscellaneous)
language:
- iso: eng
month: '10'
oa: 1
oa_version: Published Version
page: 14381-14390
publication: ACS Applied Energy Materials
publication_identifier:
  issn:
  - 2574-0962
publication_status: published
publisher: American Chemical Society
quality_controlled: '1'
scopus_import: '1'
status: public
title: 'Carbon foams via ring-opening metathesis polymerization of emulsion templates:
  A facile method to make carbon current collectors for battery applications'
tmp:
  image: /images/cc_by.png
  legal_code_url: https://creativecommons.org/licenses/by/4.0/legalcode
  name: Creative Commons Attribution 4.0 International Public License (CC-BY 4.0)
  short: CC BY (4.0)
type: journal_article
user_id: 4359f0d1-fa6c-11eb-b949-802e58b17ae8
volume: 5
year: '2022'
...
---
_id: '12232'
abstract:
- lang: eng
  text: We derive a precise asymptotic formula for the density of the small singular
    values of the real Ginibre matrix ensemble shifted by a complex parameter z as
    the dimension tends to infinity. For z away from the real axis the formula coincides
    with that for the complex Ginibre ensemble we derived earlier in Cipolloni et
    al. (Prob Math Phys 1:101–146, 2020). On the level of the one-point function of
    the low lying singular values we thus confirm the transition from real to complex
    Ginibre ensembles as the shift parameter z becomes genuinely complex; the analogous
    phenomenon has been well known for eigenvalues. We use the superbosonization formula
    (Littelmann et al. in Comm Math Phys 283:343–395, 2008) in a regime where the
    main contribution comes from a three dimensional saddle manifold.
acknowledgement: Open access funding provided by Swiss Federal Institute of Technology
  Zurich. Supported by Dr. Max Rössler, the Walter Haefner Foundation and the ETH
  Zürich Foundation.
article_processing_charge: No
article_type: original
author:
- first_name: Giorgio
  full_name: Cipolloni, Giorgio
  id: 42198EFA-F248-11E8-B48F-1D18A9856A87
  last_name: Cipolloni
  orcid: 0000-0002-4901-7992
- first_name: László
  full_name: Erdös, László
  id: 4DBD5372-F248-11E8-B48F-1D18A9856A87
  last_name: Erdös
  orcid: 0000-0001-5366-9603
- first_name: Dominik J
  full_name: Schröder, Dominik J
  id: 408ED176-F248-11E8-B48F-1D18A9856A87
  last_name: Schröder
  orcid: 0000-0002-2904-1856
citation:
  ama: Cipolloni G, Erdös L, Schröder DJ. Density of small singular values of the
    shifted real Ginibre ensemble. <i>Annales Henri Poincaré</i>. 2022;23(11):3981-4002.
    doi:<a href="https://doi.org/10.1007/s00023-022-01188-8">10.1007/s00023-022-01188-8</a>
  apa: Cipolloni, G., Erdös, L., &#38; Schröder, D. J. (2022). Density of small singular
    values of the shifted real Ginibre ensemble. <i>Annales Henri Poincaré</i>. Springer
    Nature. <a href="https://doi.org/10.1007/s00023-022-01188-8">https://doi.org/10.1007/s00023-022-01188-8</a>
  chicago: Cipolloni, Giorgio, László Erdös, and Dominik J Schröder. “Density of Small
    Singular Values of the Shifted Real Ginibre Ensemble.” <i>Annales Henri Poincaré</i>.
    Springer Nature, 2022. <a href="https://doi.org/10.1007/s00023-022-01188-8">https://doi.org/10.1007/s00023-022-01188-8</a>.
  ieee: G. Cipolloni, L. Erdös, and D. J. Schröder, “Density of small singular values
    of the shifted real Ginibre ensemble,” <i>Annales Henri Poincaré</i>, vol. 23,
    no. 11. Springer Nature, pp. 3981–4002, 2022.
  ista: Cipolloni G, Erdös L, Schröder DJ. 2022. Density of small singular values
    of the shifted real Ginibre ensemble. Annales Henri Poincaré. 23(11), 3981–4002.
  mla: Cipolloni, Giorgio, et al. “Density of Small Singular Values of the Shifted
    Real Ginibre Ensemble.” <i>Annales Henri Poincaré</i>, vol. 23, no. 11, Springer
    Nature, 2022, pp. 3981–4002, doi:<a href="https://doi.org/10.1007/s00023-022-01188-8">10.1007/s00023-022-01188-8</a>.
  short: G. Cipolloni, L. Erdös, D.J. Schröder, Annales Henri Poincaré 23 (2022) 3981–4002.
date_created: 2023-01-16T09:50:26Z
date_published: 2022-11-01T00:00:00Z
date_updated: 2023-08-04T09:33:52Z
day: '01'
ddc:
- '510'
department:
- _id: LaEr
doi: 10.1007/s00023-022-01188-8
external_id:
  isi:
  - '000796323500001'
file:
- access_level: open_access
  checksum: 5582f059feeb2f63e2eb68197a34d7dc
  content_type: application/pdf
  creator: dernst
  date_created: 2023-01-27T11:06:47Z
  date_updated: 2023-01-27T11:06:47Z
  file_id: '12424'
  file_name: 2022_AnnalesHenriP_Cipolloni.pdf
  file_size: 1333638
  relation: main_file
  success: 1
file_date_updated: 2023-01-27T11:06:47Z
has_accepted_license: '1'
intvolume: '        23'
isi: 1
issue: '11'
keyword:
- Mathematical Physics
- Nuclear and High Energy Physics
- Statistical and Nonlinear Physics
language:
- iso: eng
month: '11'
oa: 1
oa_version: Published Version
page: 3981-4002
publication: Annales Henri Poincaré
publication_identifier:
  eissn:
  - 1424-0661
  issn:
  - 1424-0637
publication_status: published
publisher: Springer Nature
quality_controlled: '1'
scopus_import: '1'
status: public
title: Density of small singular values of the shifted real Ginibre ensemble
tmp:
  image: /images/cc_by.png
  legal_code_url: https://creativecommons.org/licenses/by/4.0/legalcode
  name: Creative Commons Attribution 4.0 International Public License (CC-BY 4.0)
  short: CC BY (4.0)
type: journal_article
user_id: 4359f0d1-fa6c-11eb-b949-802e58b17ae8
volume: 23
year: '2022'
...
---
_id: '12576'
abstract:
- lang: eng
  text: Glacier health across High Mountain Asia (HMA) is highly heterogeneous and
    strongly governed by regional climate, which is variably influenced by monsoon
    dynamics and the westerlies. We explore four decades of glacier energy and mass
    balance at three climatically distinct sites across HMA by utilising a detailed
    land surface model driven by bias-corrected Weather Research and Forecasting meteorological
    forcing. All three glaciers have experienced long-term mass losses (ranging from
    −0.04 ± 0.09 to −0.59 ± 0.20 m w.e. a<jats:sup>−1</jats:sup>) consistent with
    widespread warming across the region. However, complex and contrasting responses
    of glacier energy and mass balance to the patterns of the Indian Summer Monsoon
    were evident, largely driven by the role snowfall timing, amount and phase. A
    later monsoon onset generates less total snowfall to the glacier in the southeastern
    Tibetan Plateau during May–June, augmenting net shortwave radiation and affecting
    annual mass balance (−0.5 m w.e. on average compared to early onset years). Conversely,
    timing of the monsoon’s arrival has limited impact for the Nepalese Himalaya which
    is more strongly governed by the temperature and snowfall amount during the core
    monsoon season. In the arid central Tibetan Plateau, a later monsoon arrival results
    in a 40 mm (58%) increase of May–June snowfall on average compared to early onset
    years, likely driven by the greater interaction of westerly storm events. Meanwhile,
    a late monsoon cessation at this site sees an average 200 mm (192%) increase in
    late summer precipitation due to monsoonal storms. A trend towards weaker intensity
    monsoon conditions in recent decades, combined with long-term warming patterns,
    has produced predominantly negative glacier mass balances for all sites (up to
    1 m w.e. more mass loss in the Nepalese Himalaya compared to strong monsoon intensity
    years) but sub-regional variability in monsoon timing can additionally complicate
    this response.
article_number: '104001'
article_processing_charge: No
article_type: letter_note
author:
- first_name: T E
  full_name: Shaw, T E
  last_name: Shaw
- first_name: E S
  full_name: Miles, E S
  last_name: Miles
- first_name: D
  full_name: Chen, D
  last_name: Chen
- first_name: A
  full_name: Jouberton, A
  last_name: Jouberton
- first_name: M
  full_name: Kneib, M
  last_name: Kneib
- first_name: S
  full_name: Fugger, S
  last_name: Fugger
- first_name: T
  full_name: Ou, T
  last_name: Ou
- first_name: H-W
  full_name: Lai, H-W
  last_name: Lai
- first_name: K
  full_name: Fujita, K
  last_name: Fujita
- first_name: W
  full_name: Yang, W
  last_name: Yang
- first_name: S
  full_name: Fatichi, S
  last_name: Fatichi
- first_name: Francesca
  full_name: Pellicciotti, Francesca
  id: b28f055a-81ea-11ed-b70c-a9fe7f7b0e70
  last_name: Pellicciotti
citation:
  ama: Shaw TE, Miles ES, Chen D, et al. Multi-decadal monsoon characteristics and
    glacier response in High Mountain Asia. <i>Environmental Research Letters</i>.
    2022;17(10). doi:<a href="https://doi.org/10.1088/1748-9326/ac9008">10.1088/1748-9326/ac9008</a>
  apa: Shaw, T. E., Miles, E. S., Chen, D., Jouberton, A., Kneib, M., Fugger, S.,
    … Pellicciotti, F. (2022). Multi-decadal monsoon characteristics and glacier response
    in High Mountain Asia. <i>Environmental Research Letters</i>. IOP Publishing.
    <a href="https://doi.org/10.1088/1748-9326/ac9008">https://doi.org/10.1088/1748-9326/ac9008</a>
  chicago: Shaw, T E, E S Miles, D Chen, A Jouberton, M Kneib, S Fugger, T Ou, et
    al. “Multi-Decadal Monsoon Characteristics and Glacier Response in High Mountain
    Asia.” <i>Environmental Research Letters</i>. IOP Publishing, 2022. <a href="https://doi.org/10.1088/1748-9326/ac9008">https://doi.org/10.1088/1748-9326/ac9008</a>.
  ieee: T. E. Shaw <i>et al.</i>, “Multi-decadal monsoon characteristics and glacier
    response in High Mountain Asia,” <i>Environmental Research Letters</i>, vol. 17,
    no. 10. IOP Publishing, 2022.
  ista: Shaw TE, Miles ES, Chen D, Jouberton A, Kneib M, Fugger S, Ou T, Lai H-W,
    Fujita K, Yang W, Fatichi S, Pellicciotti F. 2022. Multi-decadal monsoon characteristics
    and glacier response in High Mountain Asia. Environmental Research Letters. 17(10),
    104001.
  mla: Shaw, T. E., et al. “Multi-Decadal Monsoon Characteristics and Glacier Response
    in High Mountain Asia.” <i>Environmental Research Letters</i>, vol. 17, no. 10,
    104001, IOP Publishing, 2022, doi:<a href="https://doi.org/10.1088/1748-9326/ac9008">10.1088/1748-9326/ac9008</a>.
  short: T.E. Shaw, E.S. Miles, D. Chen, A. Jouberton, M. Kneib, S. Fugger, T. Ou,
    H.-W. Lai, K. Fujita, W. Yang, S. Fatichi, F. Pellicciotti, Environmental Research
    Letters 17 (2022).
date_created: 2023-02-20T08:09:56Z
date_published: 2022-09-16T00:00:00Z
date_updated: 2023-02-28T13:53:16Z
day: '16'
doi: 10.1088/1748-9326/ac9008
extern: '1'
intvolume: '        17'
issue: '10'
keyword:
- Public Health
- Environmental and Occupational Health
- General Environmental Science
- Renewable Energy
- Sustainability and the Environment
language:
- iso: eng
main_file_link:
- open_access: '1'
  url: https://doi.org/10.1088/1748-9326/ac9008
month: '09'
oa: 1
oa_version: Published Version
publication: Environmental Research Letters
publication_identifier:
  issn:
  - 1748-9326
publication_status: published
publisher: IOP Publishing
quality_controlled: '1'
scopus_import: '1'
status: public
title: Multi-decadal monsoon characteristics and glacier response in High Mountain
  Asia
type: journal_article
user_id: 2DF688A6-F248-11E8-B48F-1D18A9856A87
volume: 17
year: '2022'
...
---
_id: '12582'
abstract:
- lang: eng
  text: Supraglacial debris covers 7% of mountain glacier area globally and generally
    reduces glacier surface melt. Enhanced energy absorption at ice cliffs and supraglacial
    ponds scattered across the debris surface leads these features to contribute disproportionately
    to glacier-wide ablation. However, the degree to which cliffs and ponds actually
    increase melt rates remains unclear, as these features have only been studied
    in a detailed manner for selected locations, almost exclusively in High Mountain
    Asia. In this study we model the surface energy balance for debris-covered ice,
    ice cliffs, and supraglacial ponds with a set of automatic weather station records
    representing the global prevalence of debris-covered glacier ice. We generate
    5000 random sets of values for physical parameters using probability distributions
    derived from literature, which we use to investigate relative melt rates and to
    isolate the melt responses of debris, cliffs and ponds to the site-specific meteorological
    forcing. Modelled sub-debris melt rates are primarily controlled by debris thickness
    and thermal conductivity. At a reference thickness of 0.1 m, sub-debris melt rates
    vary considerably, differing by up to a factor of four between sites, mainly attributable
    to air temperature differences. We find that melt rates for ice cliffs are consistently
    2–3× the melt rate for clean glacier ice, but this melt enhancement decays with
    increasing clean ice melt rates. Energy absorption at supraglacial ponds is dominated
    by latent heat exchange and is therefore highly sensitive to wind speed and relative
    humidity, but is generally less than for clean ice. Our results provide reference
    melt enhancement factors for melt modelling of debris-covered glacier sites, globally,
    while highlighting the need for direct measurement of debris-covered glacier surface
    characteristics, physical parameters, and local meteorological conditions at a
    variety of sites around the world.
article_number: '064004'
article_processing_charge: No
article_type: letter_note
author:
- first_name: E S
  full_name: Miles, E S
  last_name: Miles
- first_name: J F
  full_name: Steiner, J F
  last_name: Steiner
- first_name: P
  full_name: Buri, P
  last_name: Buri
- first_name: W W
  full_name: Immerzeel, W W
  last_name: Immerzeel
- first_name: Francesca
  full_name: Pellicciotti, Francesca
  id: b28f055a-81ea-11ed-b70c-a9fe7f7b0e70
  last_name: Pellicciotti
citation:
  ama: Miles ES, Steiner JF, Buri P, Immerzeel WW, Pellicciotti F. Controls on the
    relative melt rates of debris-covered glacier surfaces. <i>Environmental Research
    Letters</i>. 2022;17(6). doi:<a href="https://doi.org/10.1088/1748-9326/ac6966">10.1088/1748-9326/ac6966</a>
  apa: Miles, E. S., Steiner, J. F., Buri, P., Immerzeel, W. W., &#38; Pellicciotti,
    F. (2022). Controls on the relative melt rates of debris-covered glacier surfaces.
    <i>Environmental Research Letters</i>. IOP Publishing. <a href="https://doi.org/10.1088/1748-9326/ac6966">https://doi.org/10.1088/1748-9326/ac6966</a>
  chicago: Miles, E S, J F Steiner, P Buri, W W Immerzeel, and Francesca Pellicciotti.
    “Controls on the Relative Melt Rates of Debris-Covered Glacier Surfaces.” <i>Environmental
    Research Letters</i>. IOP Publishing, 2022. <a href="https://doi.org/10.1088/1748-9326/ac6966">https://doi.org/10.1088/1748-9326/ac6966</a>.
  ieee: E. S. Miles, J. F. Steiner, P. Buri, W. W. Immerzeel, and F. Pellicciotti,
    “Controls on the relative melt rates of debris-covered glacier surfaces,” <i>Environmental
    Research Letters</i>, vol. 17, no. 6. IOP Publishing, 2022.
  ista: Miles ES, Steiner JF, Buri P, Immerzeel WW, Pellicciotti F. 2022. Controls
    on the relative melt rates of debris-covered glacier surfaces. Environmental Research
    Letters. 17(6), 064004.
  mla: Miles, E. S., et al. “Controls on the Relative Melt Rates of Debris-Covered
    Glacier Surfaces.” <i>Environmental Research Letters</i>, vol. 17, no. 6, 064004,
    IOP Publishing, 2022, doi:<a href="https://doi.org/10.1088/1748-9326/ac6966">10.1088/1748-9326/ac6966</a>.
  short: E.S. Miles, J.F. Steiner, P. Buri, W.W. Immerzeel, F. Pellicciotti, Environmental
    Research Letters 17 (2022).
date_created: 2023-02-20T08:10:37Z
date_published: 2022-06-01T00:00:00Z
date_updated: 2023-02-28T13:34:25Z
day: '01'
doi: 10.1088/1748-9326/ac6966
extern: '1'
intvolume: '        17'
issue: '6'
keyword:
- Public Health
- Environmental and Occupational Health
- General Environmental Science
- Renewable Energy
- Sustainability and the Environment
language:
- iso: eng
main_file_link:
- open_access: '1'
  url: https://doi.org/10.1088/1748-9326/ac6966
month: '06'
oa: 1
oa_version: Published Version
publication: Environmental Research Letters
publication_identifier:
  issn:
  - 1748-9326
publication_status: published
publisher: IOP Publishing
quality_controlled: '1'
scopus_import: '1'
status: public
title: Controls on the relative melt rates of debris-covered glacier surfaces
type: journal_article
user_id: 2DF688A6-F248-11E8-B48F-1D18A9856A87
volume: 17
year: '2022'
...
---
_id: '10547'
abstract:
- lang: eng
  text: "We establish global-in-time existence results for thermodynamically consistent
    reaction-(cross-)diffusion systems coupled to an equation describing heat transfer.
    Our main interest is to model species-dependent diffusivities,\r\nwhile at the
    same time ensuring thermodynamic consistency. A key difficulty of the non-isothermal
    case lies in the intrinsic presence of cross-diffusion type phenomena like the
    Soret and the Dufour effect: due to the temperature/energy dependence of the thermodynamic
    equilibria, a nonvanishing temperature gradient may drive a concentration flux
    even in a situation with constant concentrations; likewise, a nonvanishing concentration
    gradient may drive a heat flux even in a case of spatially constant temperature.
    We use time discretisation and regularisation techniques and derive a priori estimates
    based on a suitable entropy and the associated entropy production. Renormalised
    solutions are used in cases where non-integrable diffusion fluxes or reaction
    terms appear."
acknowledgement: M.K. gratefully acknowledges the hospitality of WIAS Berlin, where
  a major part of the project was carried out. The research stay of M.K. at WIAS Berlin
  was funded by the Austrian Federal Ministry of Education, Science and Research through
  a research fellowship for graduates of a promotio sub auspiciis. The research of
  A.M. has been partially supported by Deutsche Forschungsgemeinschaft (DFG) through
  the Collaborative Research Center SFB 1114 “Scaling Cascades in Complex Systems”
  (Project no. 235221301), Subproject C05 “Effective models for materials and interfaces
  with multiple scales”. J.F. and A.M. are grateful for the hospitality of the Erwin
  Schrödinger Institute in Vienna, where some ideas for this work have been developed.
  The authors are grateful to two anonymous referees for several helpful comments,
  in particular for the short proof of estimate (2.7).
article_processing_charge: No
article_type: original
arxiv: 1
author:
- first_name: Julian L
  full_name: Fischer, Julian L
  id: 2C12A0B0-F248-11E8-B48F-1D18A9856A87
  last_name: Fischer
  orcid: 0000-0002-0479-558X
- first_name: Katharina
  full_name: Hopf, Katharina
  last_name: Hopf
- first_name: Michael
  full_name: Kniely, Michael
  id: 2CA2C08C-F248-11E8-B48F-1D18A9856A87
  last_name: Kniely
  orcid: 0000-0001-5645-4333
- first_name: Alexander
  full_name: Mielke, Alexander
  last_name: Mielke
citation:
  ama: Fischer JL, Hopf K, Kniely M, Mielke A. Global existence analysis of energy-reaction-diffusion
    systems. <i>SIAM Journal on Mathematical Analysis</i>. 2022;54(1):220-267. doi:<a
    href="https://doi.org/10.1137/20M1387237">10.1137/20M1387237</a>
  apa: Fischer, J. L., Hopf, K., Kniely, M., &#38; Mielke, A. (2022). Global existence
    analysis of energy-reaction-diffusion systems. <i>SIAM Journal on Mathematical
    Analysis</i>. Society for Industrial and Applied Mathematics. <a href="https://doi.org/10.1137/20M1387237">https://doi.org/10.1137/20M1387237</a>
  chicago: Fischer, Julian L, Katharina Hopf, Michael Kniely, and Alexander Mielke.
    “Global Existence Analysis of Energy-Reaction-Diffusion Systems.” <i>SIAM Journal
    on Mathematical Analysis</i>. Society for Industrial and Applied Mathematics,
    2022. <a href="https://doi.org/10.1137/20M1387237">https://doi.org/10.1137/20M1387237</a>.
  ieee: J. L. Fischer, K. Hopf, M. Kniely, and A. Mielke, “Global existence analysis
    of energy-reaction-diffusion systems,” <i>SIAM Journal on Mathematical Analysis</i>,
    vol. 54, no. 1. Society for Industrial and Applied Mathematics, pp. 220–267, 2022.
  ista: Fischer JL, Hopf K, Kniely M, Mielke A. 2022. Global existence analysis of
    energy-reaction-diffusion systems. SIAM Journal on Mathematical Analysis. 54(1),
    220–267.
  mla: Fischer, Julian L., et al. “Global Existence Analysis of Energy-Reaction-Diffusion
    Systems.” <i>SIAM Journal on Mathematical Analysis</i>, vol. 54, no. 1, Society
    for Industrial and Applied Mathematics, 2022, pp. 220–67, doi:<a href="https://doi.org/10.1137/20M1387237">10.1137/20M1387237</a>.
  short: J.L. Fischer, K. Hopf, M. Kniely, A. Mielke, SIAM Journal on Mathematical
    Analysis 54 (2022) 220–267.
date_created: 2021-12-16T12:08:56Z
date_published: 2022-01-04T00:00:00Z
date_updated: 2023-08-02T13:37:03Z
day: '04'
department:
- _id: JuFi
doi: 10.1137/20M1387237
external_id:
  arxiv:
  - '2012.03792 '
  isi:
  - '000762768000006'
intvolume: '        54'
isi: 1
issue: '1'
keyword:
- Energy-Reaction-Diffusion Systems
- Cross Diffusion
- Global-In-Time Existence of Weak/Renormalised Solutions
- Entropy Method
- Onsager System
- Soret/Dufour Effect
language:
- iso: eng
main_file_link:
- open_access: '1'
  url: https://arxiv.org/abs/2012.03792
month: '01'
oa: 1
oa_version: Preprint
page: 220-267
publication: SIAM Journal on Mathematical Analysis
publication_identifier:
  issn:
  - 0036-1410
publication_status: published
publisher: Society for Industrial and Applied Mathematics
quality_controlled: '1'
scopus_import: '1'
status: public
title: Global existence analysis of energy-reaction-diffusion systems
type: journal_article
user_id: 4359f0d1-fa6c-11eb-b949-802e58b17ae8
volume: 54
year: '2022'
...
---
_id: '15265'
abstract:
- lang: eng
  text: 'The highly enhanced thermoelectric figure of merit, zT ≈ 2.6 at 573 K, obtained
    recently in Cd-doped polycrystalline AgSbTe2 by Roychowdhury et al. ( Science
    2021, 371, 722) brings it to the forefront of thermoelectric and energy materials
    research. Ag/Sb cationic ordering in polycrystalline AgSbTe2 was a challenging
    issue for a long time: their ordered arrangement in the cationic sublattice in
    polycrystalline samples remained elusive despite multiple theoretical predictions
    and experimental studies. Recently, selective cation doping has been used to enhance
    the Ag/Sb ordering, and cation ordered nanoscale (2–4 nm) domains were observed
    in polycrystalline AgSbTe2, which reduce lattice thermal conductivity. The enhanced
    cation ordering also delocalizes disorder-induced localized electronic states,
    and consequently the electronic transport enhances. In this Focus Review, we provide
    the details of the rational design of a high-performance thermoelectric material
    using the recently developed atomic order–disorder optimization strategy with
    AgSbTe2 as an example. Atomic disorder is ubiquitous in most thermoelectric materials,
    and the atomic order–disorder optimization strategy applies to a large variety
    of thermoelectric materials.'
article_processing_charge: No
article_type: original
author:
- first_name: Tanmoy
  full_name: Ghosh, Tanmoy
  id: a5fc9bc3-feff-11ea-93fe-e8015a3c7e9d
  last_name: Ghosh
- first_name: Subhajit
  full_name: Roychowdhury, Subhajit
  last_name: Roychowdhury
- first_name: Moinak
  full_name: Dutta, Moinak
  last_name: Dutta
- first_name: Kanishka
  full_name: Biswas, Kanishka
  last_name: Biswas
citation:
  ama: 'Ghosh T, Roychowdhury S, Dutta M, Biswas K. High-performance thermoelectric
    energy conversion: A tale of atomic ordering in AgSbTe2. <i>ACS Energy Letters</i>.
    2021;6(8):2825-2837. doi:<a href="https://doi.org/10.1021/acsenergylett.1c01184">10.1021/acsenergylett.1c01184</a>'
  apa: 'Ghosh, T., Roychowdhury, S., Dutta, M., &#38; Biswas, K. (2021). High-performance
    thermoelectric energy conversion: A tale of atomic ordering in AgSbTe2. <i>ACS
    Energy Letters</i>. American Chemical Society. <a href="https://doi.org/10.1021/acsenergylett.1c01184">https://doi.org/10.1021/acsenergylett.1c01184</a>'
  chicago: 'Ghosh, Tanmoy, Subhajit Roychowdhury, Moinak Dutta, and Kanishka Biswas.
    “High-Performance Thermoelectric Energy Conversion: A Tale of Atomic Ordering
    in AgSbTe2.” <i>ACS Energy Letters</i>. American Chemical Society, 2021. <a href="https://doi.org/10.1021/acsenergylett.1c01184">https://doi.org/10.1021/acsenergylett.1c01184</a>.'
  ieee: 'T. Ghosh, S. Roychowdhury, M. Dutta, and K. Biswas, “High-performance thermoelectric
    energy conversion: A tale of atomic ordering in AgSbTe2,” <i>ACS Energy Letters</i>,
    vol. 6, no. 8. American Chemical Society, pp. 2825–2837, 2021.'
  ista: 'Ghosh T, Roychowdhury S, Dutta M, Biswas K. 2021. High-performance thermoelectric
    energy conversion: A tale of atomic ordering in AgSbTe2. ACS Energy Letters. 6(8),
    2825–2837.'
  mla: 'Ghosh, Tanmoy, et al. “High-Performance Thermoelectric Energy Conversion:
    A Tale of Atomic Ordering in AgSbTe2.” <i>ACS Energy Letters</i>, vol. 6, no.
    8, American Chemical Society, 2021, pp. 2825–37, doi:<a href="https://doi.org/10.1021/acsenergylett.1c01184">10.1021/acsenergylett.1c01184</a>.'
  short: T. Ghosh, S. Roychowdhury, M. Dutta, K. Biswas, ACS Energy Letters 6 (2021)
    2825–2837.
date_created: 2024-04-03T07:36:10Z
date_published: 2021-07-21T00:00:00Z
date_updated: 2024-04-29T06:56:57Z
day: '21'
department:
- _id: MaIb
doi: 10.1021/acsenergylett.1c01184
intvolume: '         6'
issue: '8'
keyword:
- Materials Chemistry
- Energy Engineering and Power Technology
- Fuel Technology
- Renewable Energy
- Sustainability and the Environment
- Chemistry (miscellaneous)
language:
- iso: eng
month: '07'
oa_version: None
page: 2825-2837
publication: ACS Energy Letters
publication_identifier:
  issn:
  - 2380-8195
publication_status: published
publisher: American Chemical Society
quality_controlled: '1'
status: public
title: 'High-performance thermoelectric energy conversion: A tale of atomic ordering
  in AgSbTe2'
type: journal_article
user_id: 2DF688A6-F248-11E8-B48F-1D18A9856A87
volume: 6
year: '2021'
...
---
_id: '15269'
abstract:
- lang: eng
  text: We study different aspects of quantum field theory at finite density using
    methods from quantum information theory. For simplicity we focus on massive Dirac
    fermions with nonzero chemical potential, and work in 1 + 1 space-time dimensions.
    Using the entanglement entropy on an interval, we construct an entropic <jats:italic>c</jats:italic>-function
    that is finite. Unlike what happens in Lorentz-invariant theories, this <jats:italic>c</jats:italic>-function
    exhibits a strong violation of monotonicity; it also encodes the creation of long-range
    entanglement from the Fermi surface. Motivated by previous works on lattice models,
    we next calculate numerically the Renyi entropies and find Friedel-type oscillations;
    these are understood in terms of a defect operator product expansion. Furthermore,
    we consider the mutual information as a measure of correlation functions between
    different regions. Using a long-distance expansion previously developed by Cardy,
    we argue that the mutual information detects Fermi surface correlations already
    at leading order in the expansion. We also analyze the relative entropy and its
    Renyi generalizations in order to distinguish states with different charge and/or
    mass. In particular, we show that states in different superselection sectors give
    rise to a super-extensive behavior in the relative entropy. Finally, we discuss
    possible extensions to interacting theories, and argue for the relevance of some
    of these measures for probing non-Fermi liquids.
acknowledgement: "We thank H. Casini for many interesting discussions and comments
  on the manuscript.\r\nLD is supported by CNEA and UNCuyo, Inst. Balseiro. RM is
  supported by IST Austria.\r\nMS is supported by CONICET and UNCuyo, Inst. Balseiro.
  GT is supported by CONICET\r\n(PIP grant 11220150100299), ANPCyT (PICT 2018-2517),
  CNEA, and UNCuyo,\r\nInst. Balseiro."
article_number: '79'
article_processing_charge: Yes
article_type: original
arxiv: 1
author:
- first_name: Lucas
  full_name: Daguerre, Lucas
  last_name: Daguerre
- first_name: Raimel A
  full_name: Medina Ramos, Raimel A
  id: CE680B90-D85A-11E9-B684-C920E6697425
  last_name: Medina Ramos
  orcid: 0000-0002-5383-2869
- first_name: Mario
  full_name: Solís, Mario
  last_name: Solís
- first_name: Gonzalo
  full_name: Torroba, Gonzalo
  last_name: Torroba
citation:
  ama: Daguerre L, Medina Ramos RA, Solís M, Torroba G. Aspects of quantum information
    in finite density field theory. <i>Journal of High Energy Physics</i>. 2021;2021(3).
    doi:<a href="https://doi.org/10.1007/jhep03(2021)079">10.1007/jhep03(2021)079</a>
  apa: Daguerre, L., Medina Ramos, R. A., Solís, M., &#38; Torroba, G. (2021). Aspects
    of quantum information in finite density field theory. <i>Journal of High Energy
    Physics</i>. Springer Nature. <a href="https://doi.org/10.1007/jhep03(2021)079">https://doi.org/10.1007/jhep03(2021)079</a>
  chicago: Daguerre, Lucas, Raimel A Medina Ramos, Mario Solís, and Gonzalo Torroba.
    “Aspects of Quantum Information in Finite Density Field Theory.” <i>Journal of
    High Energy Physics</i>. Springer Nature, 2021. <a href="https://doi.org/10.1007/jhep03(2021)079">https://doi.org/10.1007/jhep03(2021)079</a>.
  ieee: L. Daguerre, R. A. Medina Ramos, M. Solís, and G. Torroba, “Aspects of quantum
    information in finite density field theory,” <i>Journal of High Energy Physics</i>,
    vol. 2021, no. 3. Springer Nature, 2021.
  ista: Daguerre L, Medina Ramos RA, Solís M, Torroba G. 2021. Aspects of quantum
    information in finite density field theory. Journal of High Energy Physics. 2021(3),
    79.
  mla: Daguerre, Lucas, et al. “Aspects of Quantum Information in Finite Density Field
    Theory.” <i>Journal of High Energy Physics</i>, vol. 2021, no. 3, 79, Springer
    Nature, 2021, doi:<a href="https://doi.org/10.1007/jhep03(2021)079">10.1007/jhep03(2021)079</a>.
  short: L. Daguerre, R.A. Medina Ramos, M. Solís, G. Torroba, Journal of High Energy
    Physics 2021 (2021).
corr_author: '1'
date_created: 2024-04-03T07:51:06Z
date_published: 2021-03-08T00:00:00Z
date_updated: 2025-09-10T10:15:02Z
day: '08'
ddc:
- '530'
department:
- _id: MaSe
doi: 10.1007/jhep03(2021)079
external_id:
  arxiv:
  - '2011.01252'
  isi:
  - '000627376600004'
file:
- access_level: open_access
  checksum: 4f540e63988ee87173e02f51a19a6672
  content_type: application/pdf
  creator: dernst
  date_created: 2024-04-10T09:18:38Z
  date_updated: 2024-04-10T09:18:38Z
  file_id: '15310'
  file_name: 2021_JourHighEnergyPhysics_Daguerre.pdf
  file_size: 5389195
  relation: main_file
  success: 1
file_date_updated: 2024-04-10T09:18:38Z
has_accepted_license: '1'
intvolume: '      2021'
isi: 1
issue: '3'
keyword:
- Nuclear and High Energy Physics
language:
- iso: eng
month: '03'
oa: 1
oa_version: Published Version
publication: Journal of High Energy Physics
publication_identifier:
  issn:
  - 1029-8479
publication_status: published
publisher: Springer Nature
quality_controlled: '1'
scopus_import: '1'
status: public
title: Aspects of quantum information in finite density field theory
tmp:
  image: /images/cc_by.png
  legal_code_url: https://creativecommons.org/licenses/by/4.0/legalcode
  name: Creative Commons Attribution 4.0 International Public License (CC-BY 4.0)
  short: CC BY (4.0)
type: journal_article
user_id: 317138e5-6ab7-11ef-aa6d-ffef3953e345
volume: 2021
year: '2021'
...
---
_id: '10327'
abstract:
- lang: eng
  text: Composite materials offer numerous advantages in a wide range of applications,
    including thermoelectrics. Here, semiconductor–metal composites are produced by
    just blending nanoparticles of a sulfide semiconductor obtained in aqueous solution
    and at room temperature with a metallic Cu powder. The obtained blend is annealed
    in a reducing atmosphere and afterward consolidated into dense polycrystalline
    pellets through spark plasma sintering (SPS). We observe that, during the annealing
    process, the presence of metallic copper activates a partial reduction of the
    PbS, resulting in the formation of PbS–Pb–CuxS composites. The presence of metallic
    lead during the SPS process habilitates the liquid-phase sintering of the composite.
    Besides, by comparing the transport properties of PbS, the PbS–Pb–CuxS composites,
    and PbS–CuxS composites obtained by blending PbS and CuxS nanoparticles, we demonstrate
    that the presence of metallic lead decisively contributes to a strong increase
    of the charge carrier concentration through spillover of charge carriers enabled
    by the low work function of lead. The increase in charge carrier concentration
    translates into much higher electrical conductivities and moderately lower Seebeck
    coefficients. These properties translate into power factors up to 2.1 mW m–1 K–2
    at ambient temperature, well above those of PbS and PbS + CuxS. Additionally,
    the presence of multiple phases in the final composite results in a notable decrease
    in the lattice thermal conductivity. Overall, the introduction of metallic copper
    in the initial blend results in a significant improvement of the thermoelectric
    performance of PbS, reaching a dimensionless thermoelectric figure of merit ZT
    = 1.1 at 750 K, which represents about a 400% increase over bare PbS. Besides,
    an average ZTave = 0.72 in the temperature range 320–773 K is demonstrated.
acknowledgement: This work was supported by the European Regional Development Funds.
  M.L., Y.Z., X.H., and K.X. thank the China Scholarship Council for scholarship support.
  M. I. has been financially supported by IST Austria and the Werner Siemens Foundation.
  Y.L. acknowledges funding from the European Union’s Horizon 2020 research and innovation
  program under the Marie Sklodowska-Curie grant agreement No. 754411. J.L. is a Serra
  Húnter fellow and is grateful to ICREA Academia program and projects MICINN/FEDER
  RTI2018-093996-B-C31 and GC 2017 SGR 128. ICN2 acknowledges funding from Generalitat
  de Catalunya 2017 SGR 327 and the Spanish MINECO project NANOGEN (PID2020-116093RB-C43).
  ICN2 was supported by the Severo Ochoa program from Spanish MINECO (grant no. SEV-2017-0706)
  and was funded by the CERCA Programme/Generalitat de Catalunya. X.H. thanks China
  Scholarship Council for scholarship support (201804910551). Part of the present
  work was performed in the framework of Universitat Autònoma de Barcelona Materials
  Science Ph.D. program.
article_processing_charge: No
article_type: original
author:
- first_name: Mengyao
  full_name: Li, Mengyao
  last_name: Li
- first_name: Yu
  full_name: Liu, Yu
  id: 2A70014E-F248-11E8-B48F-1D18A9856A87
  last_name: Liu
  orcid: 0000-0001-7313-6740
- first_name: Yu
  full_name: Zhang, Yu
  last_name: Zhang
- first_name: Xu
  full_name: Han, Xu
  last_name: Han
- first_name: Ke
  full_name: Xiao, Ke
  last_name: Xiao
- first_name: Mehran
  full_name: Nabahat, Mehran
  last_name: Nabahat
- first_name: Jordi
  full_name: Arbiol, Jordi
  last_name: Arbiol
- first_name: Jordi
  full_name: Llorca, Jordi
  last_name: Llorca
- first_name: Maria
  full_name: Ibáñez, Maria
  id: 43C61214-F248-11E8-B48F-1D18A9856A87
  last_name: Ibáñez
  orcid: 0000-0001-5013-2843
- first_name: Andreu
  full_name: Cabot, Andreu
  last_name: Cabot
citation:
  ama: Li M, Liu Y, Zhang Y, et al. PbS–Pb–CuxS composites for thermoelectric application.
    <i>ACS Applied Materials and Interfaces</i>. 2021;13(43):51373–51382. doi:<a href="https://doi.org/10.1021/acsami.1c15609">10.1021/acsami.1c15609</a>
  apa: Li, M., Liu, Y., Zhang, Y., Han, X., Xiao, K., Nabahat, M., … Cabot, A. (2021).
    PbS–Pb–CuxS composites for thermoelectric application. <i>ACS Applied Materials
    and Interfaces</i>. American Chemical Society . <a href="https://doi.org/10.1021/acsami.1c15609">https://doi.org/10.1021/acsami.1c15609</a>
  chicago: Li, Mengyao, Yu Liu, Yu Zhang, Xu Han, Ke Xiao, Mehran Nabahat, Jordi Arbiol,
    Jordi Llorca, Maria Ibáñez, and Andreu Cabot. “PbS–Pb–CuxS Composites for Thermoelectric
    Application.” <i>ACS Applied Materials and Interfaces</i>. American Chemical Society
    , 2021. <a href="https://doi.org/10.1021/acsami.1c15609">https://doi.org/10.1021/acsami.1c15609</a>.
  ieee: M. Li <i>et al.</i>, “PbS–Pb–CuxS composites for thermoelectric application,”
    <i>ACS Applied Materials and Interfaces</i>, vol. 13, no. 43. American Chemical
    Society , pp. 51373–51382, 2021.
  ista: Li M, Liu Y, Zhang Y, Han X, Xiao K, Nabahat M, Arbiol J, Llorca J, Ibáñez
    M, Cabot A. 2021. PbS–Pb–CuxS composites for thermoelectric application. ACS Applied
    Materials and Interfaces. 13(43), 51373–51382.
  mla: Li, Mengyao, et al. “PbS–Pb–CuxS Composites for Thermoelectric Application.”
    <i>ACS Applied Materials and Interfaces</i>, vol. 13, no. 43, American Chemical
    Society , 2021, pp. 51373–51382, doi:<a href="https://doi.org/10.1021/acsami.1c15609">10.1021/acsami.1c15609</a>.
  short: M. Li, Y. Liu, Y. Zhang, X. Han, K. Xiao, M. Nabahat, J. Arbiol, J. Llorca,
    M. Ibáñez, A. Cabot, ACS Applied Materials and Interfaces 13 (2021) 51373–51382.
corr_author: '1'
date_created: 2021-11-21T23:01:30Z
date_published: 2021-10-19T00:00:00Z
date_updated: 2025-04-14T07:43:47Z
day: '19'
department:
- _id: MaIb
doi: 10.1021/acsami.1c15609
ec_funded: 1
external_id:
  isi:
  - '000715852100070'
  pmid:
  - '34665616'
intvolume: '        13'
isi: 1
issue: '43'
keyword:
- CuxS
- PbS
- energy conversion
- nanocomposite
- nanoparticle
- solution synthesis
- thermoelectric
language:
- iso: eng
main_file_link:
- open_access: '1'
  url: https://upcommons.upc.edu/bitstream/2117/363528/1/Pb%20mengyao.pdf
month: '10'
oa: 1
oa_version: Submitted Version
page: 51373–51382
pmid: 1
project:
- _id: 260C2330-B435-11E9-9278-68D0E5697425
  call_identifier: H2020
  grant_number: '754411'
  name: ISTplus - Postdoctoral Fellowships
- _id: 9B8F7476-BA93-11EA-9121-9846C619BF3A
  name: 'HighTE: The Werner Siemens Laboratory for the High Throughput Discovery of
    Semiconductors for Waste Heat Recovery'
publication: ACS Applied Materials and Interfaces
publication_identifier:
  eissn:
  - 1944-8252
  issn:
  - 1944-8244
publication_status: published
publisher: 'American Chemical Society '
quality_controlled: '1'
scopus_import: '1'
status: public
title: PbS–Pb–CuxS composites for thermoelectric application
type: journal_article
user_id: 2DF688A6-F248-11E8-B48F-1D18A9856A87
volume: 13
year: '2021'
...
---
_id: '9447'
abstract:
- lang: eng
  text: 'Lithium bis(trifluoromethylsulfonyl)imide (LiTFSI) based water-in-salt electrolytes
    (WiSEs) has recently emerged as a new promising class of electrolytes, primarily
    owing to their wide electrochemical stability windows (~3–4 V), that by far exceed
    the thermodynamic stability window of water (1.23 V). Upon increasing the salt
    concentration towards superconcentration the onset of the oxygen evolution reaction
    (OER) shifts more significantly than the hydrogen evolution reaction (HER) does.
    The OER shift has been explained by the accumulation of hydrophobic anions blocking
    water access to the electrode surface, hence by double layer theory. Here we demonstrate
    that the processes during oxidation are much more complex, involving OER, carbon
    and salt decomposition by OER intermediates, and salt precipitation upon local
    oversaturation. The positive shift in the onset potential of oxidation currents
    was elucidated by combining several advanced analysis techniques: rotating ring-disk
    electrode voltammetry, online electrochemical mass spectrometry, and X-ray photoelectron
    spectroscopy, using both dilute and superconcentrated electrolytes. The results
    demonstrate the importance of reactive OER intermediates and surface films for
    electrolyte and electrode stability and motivate further studies of the nature
    of the electrode.'
article_number: '050550'
article_processing_charge: No
author:
- first_name: Marion
  full_name: Maffre, Marion
  last_name: Maffre
- first_name: Roza
  full_name: Bouchal, Roza
  last_name: Bouchal
- first_name: Stefan Alexander
  full_name: Freunberger, Stefan Alexander
  id: A8CA28E6-CE23-11E9-AD2D-EC27E6697425
  last_name: Freunberger
  orcid: 0000-0003-2902-5319
- first_name: Niklas
  full_name: Lindahl, Niklas
  last_name: Lindahl
- first_name: Patrik
  full_name: Johansson, Patrik
  last_name: Johansson
- first_name: Frédéric
  full_name: Favier, Frédéric
  last_name: Favier
- first_name: Olivier
  full_name: Fontaine, Olivier
  last_name: Fontaine
- first_name: Daniel
  full_name: Bélanger, Daniel
  last_name: Bélanger
citation:
  ama: Maffre M, Bouchal R, Freunberger SA, et al. Investigation of electrochemical
    and chemical processes occurring at positive potentials in “Water-in-Salt” electrolytes.
    <i>Journal of The Electrochemical Society</i>. 2021;168(5). doi:<a href="https://doi.org/10.1149/1945-7111/ac0300">10.1149/1945-7111/ac0300</a>
  apa: Maffre, M., Bouchal, R., Freunberger, S. A., Lindahl, N., Johansson, P., Favier,
    F., … Bélanger, D. (2021). Investigation of electrochemical and chemical processes
    occurring at positive potentials in “Water-in-Salt” electrolytes. <i>Journal of
    The Electrochemical Society</i>. IOP Publishing. <a href="https://doi.org/10.1149/1945-7111/ac0300">https://doi.org/10.1149/1945-7111/ac0300</a>
  chicago: Maffre, Marion, Roza Bouchal, Stefan Alexander Freunberger, Niklas Lindahl,
    Patrik Johansson, Frédéric Favier, Olivier Fontaine, and Daniel Bélanger. “Investigation
    of Electrochemical and Chemical Processes Occurring at Positive Potentials in
    ‘Water-in-Salt’ Electrolytes.” <i>Journal of The Electrochemical Society</i>.
    IOP Publishing, 2021. <a href="https://doi.org/10.1149/1945-7111/ac0300">https://doi.org/10.1149/1945-7111/ac0300</a>.
  ieee: M. Maffre <i>et al.</i>, “Investigation of electrochemical and chemical processes
    occurring at positive potentials in ‘Water-in-Salt’ electrolytes,” <i>Journal
    of The Electrochemical Society</i>, vol. 168, no. 5. IOP Publishing, 2021.
  ista: Maffre M, Bouchal R, Freunberger SA, Lindahl N, Johansson P, Favier F, Fontaine
    O, Bélanger D. 2021. Investigation of electrochemical and chemical processes occurring
    at positive potentials in “Water-in-Salt” electrolytes. Journal of The Electrochemical
    Society. 168(5), 050550.
  mla: Maffre, Marion, et al. “Investigation of Electrochemical and Chemical Processes
    Occurring at Positive Potentials in ‘Water-in-Salt’ Electrolytes.” <i>Journal
    of The Electrochemical Society</i>, vol. 168, no. 5, 050550, IOP Publishing, 2021,
    doi:<a href="https://doi.org/10.1149/1945-7111/ac0300">10.1149/1945-7111/ac0300</a>.
  short: M. Maffre, R. Bouchal, S.A. Freunberger, N. Lindahl, P. Johansson, F. Favier,
    O. Fontaine, D. Bélanger, Journal of The Electrochemical Society 168 (2021).
date_created: 2021-06-03T09:58:38Z
date_published: 2021-05-01T00:00:00Z
date_updated: 2024-10-21T06:02:10Z
day: '01'
department:
- _id: StFr
doi: 10.1149/1945-7111/ac0300
external_id:
  isi:
  - '000657724200001'
intvolume: '       168'
isi: 1
issue: '5'
keyword:
- Renewable Energy
- Sustainability and the Environment
- Electrochemistry
- Materials Chemistry
- Electronic
- Optical and Magnetic Materials
- Surfaces
- Coatings and Films
- Condensed Matter Physics
language:
- iso: eng
month: '05'
oa_version: None
publication: Journal of The Electrochemical Society
publication_identifier:
  eissn:
  - 1945-7111
  issn:
  - 0013-4651
publication_status: published
publisher: IOP Publishing
quality_controlled: '1'
scopus_import: '1'
status: public
title: Investigation of electrochemical and chemical processes occurring at positive
  potentials in “Water-in-Salt” electrolytes
type: journal_article
user_id: c635000d-4b10-11ee-a964-aac5a93f6ac1
volume: 168
year: '2021'
...
---
_id: '9978'
abstract:
- lang: eng
  text: Redox mediators could catalyse otherwise slow and energy-inefficient cycling
    of Li-S and Li-O 2 batteries by shuttling electrons/holes between the electrode
    and the solid insulating storage materials. For mediators to work efficiently
    they need to oxidize the solid with fast kinetics yet the lowest possible overpotential.
    Here, we found that when the redox potentials of mediators are tuned via, e.g.,
    Li + concentration in the electrolyte, they exhibit distinct threshold potentials,
    where the kinetics accelerate several-fold within a range as small as 10 mV. This
    phenomenon is independent of types of mediators and electrolyte. The acceleration
    originates from the overpotentials required to activate fast Li + /e – extraction
    and the following chemical step at specific abundant surface facets. Efficient
    redox catalysis at insulating solids requires therefore carefully considering
    the surface conditions of the storage materials and electrolyte-dependent redox
    potentials, which may be tuned by salt concentrations or solvents.
acknowledgement: 'This work was financially supported by the National Natural Science
  Foundation of China (51773092, 21975124, 11874254, 51802187, U2030206). S.A.F. is
  indebted to IST Austria for support. '
article_processing_charge: No
author:
- first_name: Deqing
  full_name: Cao, Deqing
  last_name: Cao
- first_name: Xiaoxiao
  full_name: Shen, Xiaoxiao
  last_name: Shen
- first_name: Aiping
  full_name: Wang, Aiping
  last_name: Wang
- first_name: Fengjiao
  full_name: Yu, Fengjiao
  last_name: Yu
- first_name: Yuping
  full_name: Wu, Yuping
  last_name: Wu
- first_name: Siqi
  full_name: Shi, Siqi
  last_name: Shi
- first_name: Stefan Alexander
  full_name: Freunberger, Stefan Alexander
  id: A8CA28E6-CE23-11E9-AD2D-EC27E6697425
  last_name: Freunberger
  orcid: 0000-0003-2902-5319
- first_name: Yuhui
  full_name: Chen, Yuhui
  last_name: Chen
citation:
  ama: Cao D, Shen X, Wang A, et al. Sharp kinetic acceleration potentials during
    mediated redox catalysis of insulators. <i>Research Square</i>. doi:<a href="https://doi.org/10.21203/rs.3.rs-750965/v1">10.21203/rs.3.rs-750965/v1</a>
  apa: Cao, D., Shen, X., Wang, A., Yu, F., Wu, Y., Shi, S., … Chen, Y. (n.d.). Sharp
    kinetic acceleration potentials during mediated redox catalysis of insulators.
    <i>Research Square</i>. Research Square. <a href="https://doi.org/10.21203/rs.3.rs-750965/v1">https://doi.org/10.21203/rs.3.rs-750965/v1</a>
  chicago: Cao, Deqing, Xiaoxiao Shen, Aiping Wang, Fengjiao Yu, Yuping Wu, Siqi Shi,
    Stefan Alexander Freunberger, and Yuhui Chen. “Sharp Kinetic Acceleration Potentials
    during Mediated Redox Catalysis of Insulators.” <i>Research Square</i>. Research
    Square, n.d. <a href="https://doi.org/10.21203/rs.3.rs-750965/v1">https://doi.org/10.21203/rs.3.rs-750965/v1</a>.
  ieee: D. Cao <i>et al.</i>, “Sharp kinetic acceleration potentials during mediated
    redox catalysis of insulators,” <i>Research Square</i>. Research Square.
  ista: Cao D, Shen X, Wang A, Yu F, Wu Y, Shi S, Freunberger SA, Chen Y. Sharp kinetic
    acceleration potentials during mediated redox catalysis of insulators. Research
    Square, <a href="https://doi.org/10.21203/rs.3.rs-750965/v1">10.21203/rs.3.rs-750965/v1</a>.
  mla: Cao, Deqing, et al. “Sharp Kinetic Acceleration Potentials during Mediated
    Redox Catalysis of Insulators.” <i>Research Square</i>, Research Square, doi:<a
    href="https://doi.org/10.21203/rs.3.rs-750965/v1">10.21203/rs.3.rs-750965/v1</a>.
  short: D. Cao, X. Shen, A. Wang, F. Yu, Y. Wu, S. Shi, S.A. Freunberger, Y. Chen,
    Research Square (n.d.).
corr_author: '1'
date_created: 2021-08-31T12:54:16Z
date_published: 2021-08-18T00:00:00Z
date_updated: 2024-10-09T21:01:46Z
day: '18'
ddc:
- '541'
department:
- _id: StFr
doi: 10.21203/rs.3.rs-750965/v1
file:
- access_level: open_access
  checksum: 1878e91c29d5769ed5a827b0b7addf00
  content_type: application/pdf
  creator: cchlebak
  date_created: 2021-08-31T14:02:19Z
  date_updated: 2021-08-31T14:02:19Z
  file_id: '9979'
  file_name: 2021_ResearchSquare_Cao.pdf
  file_size: 1019662
  relation: main_file
  success: 1
file_date_updated: 2021-08-31T14:02:19Z
has_accepted_license: '1'
keyword:
- Catalysis
- Energy engineering
- Materials theory and modeling
language:
- iso: eng
month: '08'
oa: 1
oa_version: Preprint
page: '21'
publication: Research Square
publication_identifier:
  eissn:
  - 2693-5015
publication_status: submitted
publisher: Research Square
related_material:
  record:
  - id: '10813'
    relation: later_version
    status: public
status: public
title: Sharp kinetic acceleration potentials during mediated redox catalysis of insulators
tmp:
  image: /images/cc_by.png
  legal_code_url: https://creativecommons.org/licenses/by/4.0/legalcode
  name: Creative Commons Attribution 4.0 International Public License (CC-BY 4.0)
  short: CC BY (4.0)
type: preprint
user_id: 2DF688A6-F248-11E8-B48F-1D18A9856A87
year: '2021'
...
---
DOAJ_listed: '1'
OA_place: publisher
OA_type: gold
_id: '9128'
abstract:
- lang: eng
  text: This paper reviews recent important advances in our understanding of the response
    of precipitation extremes to warming from theory and from idealized cloud-resolving
    simulations. A theoretical scaling for precipitation extremes has been proposed
    and refined in the past decades, allowing to address separately the contributions
    from the thermodynamics, the dynamics and the microphysics. Theoretical constraints,
    as well as remaining uncertainties, associated with each of these three contributions
    to precipitation extremes, are discussed. Notably, although to leading order precipitation
    extremes seem to follow the thermodynamic theoretical expectation in idealized
    simulations, considerable uncertainty remains regarding the response of the dynamics
    and of the microphysics to warming, and considerable departure from this theoretical
    expectation is found in observations and in more realistic simulations. We also
    emphasize key outstanding questions, in particular the response of mesoscale convective
    organization to warming. Observations suggest that extreme rainfall often comes
    from an organized system in very moist environments. Improved understanding of
    the physical processes behind convective organization is needed in order to achieve
    accurate extreme rainfall prediction in our current, and in a warming climate.
article_number: '035001'
article_processing_charge: No
article_type: letter_note
author:
- first_name: Caroline J
  full_name: Muller, Caroline J
  id: f978ccb0-3f7f-11eb-b193-b0e2bd13182b
  last_name: Muller
  orcid: 0000-0001-5836-5350
- first_name: Yukari
  full_name: Takayabu, Yukari
  last_name: Takayabu
citation:
  ama: 'Muller CJ, Takayabu Y. Response of precipitation extremes to warming: What
    have we learned from theory and idealized cloud-resolving simulations, and what
    remains to be learned? <i>Environmental Research Letters</i>. 2020;15(3). doi:<a
    href="https://doi.org/10.1088/1748-9326/ab7130">10.1088/1748-9326/ab7130</a>'
  apa: 'Muller, C. J., &#38; Takayabu, Y. (2020). Response of precipitation extremes
    to warming: What have we learned from theory and idealized cloud-resolving simulations,
    and what remains to be learned? <i>Environmental Research Letters</i>. IOP Publishing.
    <a href="https://doi.org/10.1088/1748-9326/ab7130">https://doi.org/10.1088/1748-9326/ab7130</a>'
  chicago: 'Muller, Caroline J, and Yukari Takayabu. “Response of Precipitation Extremes
    to Warming: What Have We Learned from Theory and Idealized Cloud-Resolving Simulations,
    and What Remains to Be Learned?” <i>Environmental Research Letters</i>. IOP Publishing,
    2020. <a href="https://doi.org/10.1088/1748-9326/ab7130">https://doi.org/10.1088/1748-9326/ab7130</a>.'
  ieee: 'C. J. Muller and Y. Takayabu, “Response of precipitation extremes to warming:
    What have we learned from theory and idealized cloud-resolving simulations, and
    what remains to be learned?,” <i>Environmental Research Letters</i>, vol. 15,
    no. 3. IOP Publishing, 2020.'
  ista: 'Muller CJ, Takayabu Y. 2020. Response of precipitation extremes to warming:
    What have we learned from theory and idealized cloud-resolving simulations, and
    what remains to be learned? Environmental Research Letters. 15(3), 035001.'
  mla: 'Muller, Caroline J., and Yukari Takayabu. “Response of Precipitation Extremes
    to Warming: What Have We Learned from Theory and Idealized Cloud-Resolving Simulations,
    and What Remains to Be Learned?” <i>Environmental Research Letters</i>, vol. 15,
    no. 3, 035001, IOP Publishing, 2020, doi:<a href="https://doi.org/10.1088/1748-9326/ab7130">10.1088/1748-9326/ab7130</a>.'
  short: C.J. Muller, Y. Takayabu, Environmental Research Letters 15 (2020).
date_created: 2021-02-15T14:07:14Z
date_published: 2020-02-18T00:00:00Z
date_updated: 2024-10-15T13:49:06Z
day: '18'
doi: 10.1088/1748-9326/ab7130
extern: '1'
intvolume: '        15'
issue: '3'
keyword:
- Renewable Energy
- Sustainability and the Environment
- Public Health
- Environmental and Occupational Health
- General Environmental Science
language:
- iso: eng
main_file_link:
- open_access: '1'
  url: https://doi.org/10.1088/1748-9326/ab7130
month: '02'
oa: 1
oa_version: Published Version
publication: Environmental Research Letters
publication_identifier:
  issn:
  - 1748-9326
publication_status: published
publisher: IOP Publishing
quality_controlled: '1'
status: public
title: 'Response of precipitation extremes to warming: What have we learned from theory
  and idealized cloud-resolving simulations, and what remains to be learned?'
type: journal_article
user_id: 0043cee0-e5fc-11ee-9736-f83bc23afbf0
volume: 15
year: '2020'
...
---
_id: '8407'
article_processing_charge: No
article_type: original
author:
- first_name: Paul
  full_name: Schanda, Paul
  id: 7B541462-FAF6-11E9-A490-E8DFE5697425
  last_name: Schanda
  orcid: 0000-0002-9350-7606
citation:
  ama: Schanda P. Relaxing with liquids and solids – A perspective on biomolecular
    dynamics. <i>Journal of Magnetic Resonance</i>. 2019;306:180-186. doi:<a href="https://doi.org/10.1016/j.jmr.2019.07.025">10.1016/j.jmr.2019.07.025</a>
  apa: Schanda, P. (2019). Relaxing with liquids and solids – A perspective on biomolecular
    dynamics. <i>Journal of Magnetic Resonance</i>. Elsevier. <a href="https://doi.org/10.1016/j.jmr.2019.07.025">https://doi.org/10.1016/j.jmr.2019.07.025</a>
  chicago: Schanda, Paul. “Relaxing with Liquids and Solids – A Perspective on Biomolecular
    Dynamics.” <i>Journal of Magnetic Resonance</i>. Elsevier, 2019. <a href="https://doi.org/10.1016/j.jmr.2019.07.025">https://doi.org/10.1016/j.jmr.2019.07.025</a>.
  ieee: P. Schanda, “Relaxing with liquids and solids – A perspective on biomolecular
    dynamics,” <i>Journal of Magnetic Resonance</i>, vol. 306. Elsevier, pp. 180–186,
    2019.
  ista: Schanda P. 2019. Relaxing with liquids and solids – A perspective on biomolecular
    dynamics. Journal of Magnetic Resonance. 306, 180–186.
  mla: Schanda, Paul. “Relaxing with Liquids and Solids – A Perspective on Biomolecular
    Dynamics.” <i>Journal of Magnetic Resonance</i>, vol. 306, Elsevier, 2019, pp.
    180–86, doi:<a href="https://doi.org/10.1016/j.jmr.2019.07.025">10.1016/j.jmr.2019.07.025</a>.
  short: P. Schanda, Journal of Magnetic Resonance 306 (2019) 180–186.
date_created: 2020-09-17T10:28:47Z
date_published: 2019-09-01T00:00:00Z
date_updated: 2021-01-12T08:19:04Z
day: '01'
doi: 10.1016/j.jmr.2019.07.025
extern: '1'
external_id:
  pmid:
  - '31350165'
intvolume: '       306'
keyword:
- Nuclear and High Energy Physics
- Biophysics
- Biochemistry
- Condensed Matter Physics
language:
- iso: eng
month: '09'
oa_version: Submitted Version
page: 180-186
pmid: 1
publication: Journal of Magnetic Resonance
publication_identifier:
  issn:
  - 1090-7807
publication_status: published
publisher: Elsevier
quality_controlled: '1'
status: public
title: Relaxing with liquids and solids – A perspective on biomolecular dynamics
type: journal_article
user_id: 2DF688A6-F248-11E8-B48F-1D18A9856A87
volume: 306
year: '2019'
...
