[{"author":[{"full_name":"Gemen, Julius","last_name":"Gemen","first_name":"Julius"},{"full_name":"Klajn, Rafal","id":"8e84690e-1e48-11ed-a02b-a1e6fb8bb53b","first_name":"Rafal","last_name":"Klajn"}],"volume":8,"date_updated":"2023-08-02T07:24:57Z","date_created":"2023-08-01T09:32:27Z","year":"2022","publisher":"Elsevier","publication_status":"published","extern":"1","doi":"10.1016/j.chempr.2022.04.022","language":[{"iso":"eng"}],"main_file_link":[{"open_access":"1","url":"https://doi.org/10.1016/j.chempr.2022.04.022"}],"oa":1,"quality_controlled":"1","publication_identifier":{"eissn":["2451-9294"],"issn":["2451-9308"]},"month":"05","oa_version":"Published Version","_id":"13351","user_id":"2DF688A6-F248-11E8-B48F-1D18A9856A87","intvolume":" 8","status":"public","title":"Electron catalysis expands the supramolecular chemist’s toolbox","issue":"5","abstract":[{"lang":"eng","text":"Molecular recognition is at the heart of the noncovalent synthesis of supramolecular assemblies and, at higher length scales, supramolecular materials. In a recent publication in Nature, Stoddart and co-workers demonstrate that the formation of host-guest complexes can be catalyzed by one of the simplest possible catalysts: the electron."}],"type":"journal_article","date_published":"2022-05-12T00:00:00Z","citation":{"ama":"Gemen J, Klajn R. Electron catalysis expands the supramolecular chemist’s toolbox. Chem. 2022;8(5):1183-1186. doi:10.1016/j.chempr.2022.04.022","ista":"Gemen J, Klajn R. 2022. Electron catalysis expands the supramolecular chemist’s toolbox. Chem. 8(5), 1183–1186.","apa":"Gemen, J., & Klajn, R. (2022). Electron catalysis expands the supramolecular chemist’s toolbox. Chem. Elsevier. https://doi.org/10.1016/j.chempr.2022.04.022","ieee":"J. Gemen and R. Klajn, “Electron catalysis expands the supramolecular chemist’s toolbox,” Chem, vol. 8, no. 5. Elsevier, pp. 1183–1186, 2022.","mla":"Gemen, Julius, and Rafal Klajn. “Electron Catalysis Expands the Supramolecular Chemist’s Toolbox.” Chem, vol. 8, no. 5, Elsevier, 2022, pp. 1183–86, doi:10.1016/j.chempr.2022.04.022.","short":"J. Gemen, R. Klajn, Chem 8 (2022) 1183–1186.","chicago":"Gemen, Julius, and Rafal Klajn. “Electron Catalysis Expands the Supramolecular Chemist’s Toolbox.” Chem. Elsevier, 2022. https://doi.org/10.1016/j.chempr.2022.04.022."},"publication":"Chem","page":"1183-1186","article_type":"original","article_processing_charge":"No","day":"12","scopus_import":"1","keyword":["Materials Chemistry","Biochemistry (medical)","General Chemical Engineering","Environmental Chemistry","Biochemistry","General Chemistry"]},{"issue":"9","abstract":[{"text":"Confinement within molecular cages can dramatically modify the physicochemical properties of the encapsulated guest molecules, but such host-guest complexes have mainly been studied in a static context. Combining confinement effects with fast guest exchange kinetics could pave the way toward stimuli-responsive supramolecular systems—and ultimately materials—whose desired properties could be tailored “on demand” rapidly and reversibly. Here, we demonstrate rapid guest exchange between inclusion complexes of an open-window coordination cage that can simultaneously accommodate two guest molecules. Working with two types of guests, anthracene derivatives and BODIPY dyes, we show that the former can substantially modify the optical properties of the latter upon noncovalent heterodimer formation. We also studied the light-induced covalent dimerization of encapsulated anthracenes and found large effects of confinement on reaction rates. By coupling the photodimerization with the rapid guest exchange, we developed a new way to modulate fluorescence using external irradiation.","lang":"eng"}],"type":"journal_article","oa_version":"Published Version","user_id":"2DF688A6-F248-11E8-B48F-1D18A9856A87","_id":"13350","intvolume":" 8","title":"Ternary host-guest complexes with rapid exchange kinetics and photoswitchable fluorescence","status":"public","article_processing_charge":"No","day":"08","scopus_import":"1","keyword":["Materials Chemistry","Biochemistry (medical)","General Chemical Engineering","Environmental Chemistry","Biochemistry","General Chemistry"],"date_published":"2022-09-08T00:00:00Z","citation":{"ista":"Gemen J, Białek MJ, Kazes M, Shimon LJW, Feller M, Semenov SN, Diskin-Posner Y, Oron D, Klajn R. 2022. Ternary host-guest complexes with rapid exchange kinetics and photoswitchable fluorescence. Chem. 8(9), 2362–2379.","apa":"Gemen, J., Białek, M. J., Kazes, M., Shimon, L. J. W., Feller, M., Semenov, S. N., … Klajn, R. (2022). Ternary host-guest complexes with rapid exchange kinetics and photoswitchable fluorescence. Chem. Elsevier. https://doi.org/10.1016/j.chempr.2022.05.008","ieee":"J. Gemen et al., “Ternary host-guest complexes with rapid exchange kinetics and photoswitchable fluorescence,” Chem, vol. 8, no. 9. Elsevier, pp. 2362–2379, 2022.","ama":"Gemen J, Białek MJ, Kazes M, et al. Ternary host-guest complexes with rapid exchange kinetics and photoswitchable fluorescence. Chem. 2022;8(9):2362-2379. doi:10.1016/j.chempr.2022.05.008","chicago":"Gemen, Julius, Michał J. Białek, Miri Kazes, Linda J.W. Shimon, Moran Feller, Sergey N. Semenov, Yael Diskin-Posner, Dan Oron, and Rafal Klajn. “Ternary Host-Guest Complexes with Rapid Exchange Kinetics and Photoswitchable Fluorescence.” Chem. Elsevier, 2022. https://doi.org/10.1016/j.chempr.2022.05.008.","mla":"Gemen, Julius, et al. “Ternary Host-Guest Complexes with Rapid Exchange Kinetics and Photoswitchable Fluorescence.” Chem, vol. 8, no. 9, Elsevier, 2022, pp. 2362–79, doi:10.1016/j.chempr.2022.05.008.","short":"J. Gemen, M.J. Białek, M. Kazes, L.J.W. Shimon, M. Feller, S.N. Semenov, Y. Diskin-Posner, D. Oron, R. Klajn, Chem 8 (2022) 2362–2379."},"publication":"Chem","page":"2362-2379","article_type":"original","extern":"1","author":[{"last_name":"Gemen","first_name":"Julius","full_name":"Gemen, Julius"},{"first_name":"Michał J.","last_name":"Białek","full_name":"Białek, Michał J."},{"full_name":"Kazes, Miri","last_name":"Kazes","first_name":"Miri"},{"last_name":"Shimon","first_name":"Linda J.W.","full_name":"Shimon, Linda J.W."},{"last_name":"Feller","first_name":"Moran","full_name":"Feller, Moran"},{"last_name":"Semenov","first_name":"Sergey N.","full_name":"Semenov, Sergey N."},{"full_name":"Diskin-Posner, Yael","first_name":"Yael","last_name":"Diskin-Posner"},{"full_name":"Oron, Dan","last_name":"Oron","first_name":"Dan"},{"first_name":"Rafal","last_name":"Klajn","id":"8e84690e-1e48-11ed-a02b-a1e6fb8bb53b","full_name":"Klajn, Rafal"}],"volume":8,"date_created":"2023-08-01T09:32:14Z","date_updated":"2023-08-02T09:39:35Z","pmid":1,"year":"2022","publisher":"Elsevier","publication_status":"published","publication_identifier":{"issn":["2451-9308"],"eissn":["2451-9294"]},"month":"09","doi":"10.1016/j.chempr.2022.05.008","language":[{"iso":"eng"}],"oa":1,"external_id":{"pmid":["36133801"]},"main_file_link":[{"open_access":"1","url":"https://doi.org/10.1016/j.chempr.2022.05.008"}],"quality_controlled":"1"},{"license":"https://creativecommons.org/licenses/by/4.0/","file_date_updated":"2023-01-30T07:35:09Z","ec_funded":1,"date_updated":"2023-08-04T09:38:26Z","date_created":"2023-01-16T09:51:26Z","volume":34,"author":[{"id":"bd3fceba-dc74-11ea-a0a7-c17f71817366","last_name":"Fiedler","first_name":"Christine","full_name":"Fiedler, Christine"},{"id":"8BD9DE16-AB3C-11E9-9C8C-2A03E6697425","last_name":"Kleinhanns","first_name":"Tobias","full_name":"Kleinhanns, Tobias"},{"first_name":"Maria","last_name":"Garcia","id":"6e5c50b8-97dc-11ed-be98-b0a74c84cae0","full_name":"Garcia, Maria"},{"first_name":"Seungho","last_name":"Lee","id":"BB243B88-D767-11E9-B658-BC13E6697425","orcid":"0000-0002-6962-8598","full_name":"Lee, Seungho"},{"last_name":"Calcabrini","first_name":"Mariano","id":"45D7531A-F248-11E8-B48F-1D18A9856A87","full_name":"Calcabrini, Mariano"},{"full_name":"Ibáñez, Maria","id":"43C61214-F248-11E8-B48F-1D18A9856A87","orcid":"0000-0001-5013-2843","first_name":"Maria","last_name":"Ibáñez"}],"related_material":{"record":[{"id":"12885","relation":"dissertation_contains","status":"public"}]},"publication_status":"published","department":[{"_id":"MaIb"}],"publisher":"American Chemical Society","year":"2022","acknowledgement":"This work was financially supported by ISTA and the Werner Siemens Foundation. M.C. has received funding from the European Union’s Horizon 2020 research and innovation program under the Marie Skłodowska-Curie Grant Agreement no. 665385.","pmid":1,"month":"09","publication_identifier":{"eissn":["1520-5002"],"issn":["0897-4756"]},"language":[{"iso":"eng"}],"doi":"10.1021/acs.chemmater.2c01967","quality_controlled":"1","isi":1,"project":[{"grant_number":"665385","_id":"2564DBCA-B435-11E9-9278-68D0E5697425","call_identifier":"H2020","name":"International IST Doctoral Program"}],"oa":1,"tmp":{"name":"Creative Commons Attribution 4.0 International Public License (CC-BY 4.0)","legal_code_url":"https://creativecommons.org/licenses/by/4.0/legalcode","short":"CC BY (4.0)","image":"/images/cc_by.png"},"external_id":{"pmid":["36248227"],"isi":["000917837600001"]},"abstract":[{"lang":"eng","text":"Thermoelectric technology requires synthesizing complex materials where not only the crystal structure but also other structural features such as defects, grain size and orientation, and interfaces must be controlled. To date, conventional solid-state techniques are unable to provide this level of control. Herein, we present a synthetic approach in which dense inorganic thermoelectric materials are produced by the consolidation of well-defined nanoparticle powders. The idea is that controlling the characteristics of the powder allows the chemical transformations that take place during consolidation to be guided, ultimately yielding inorganic solids with targeted features. Different from conventional methods, syntheses in solution can produce particles with unprecedented control over their size, shape, crystal structure, composition, and surface chemistry. However, to date, most works have focused only on the low-cost benefits of this strategy. In this perspective, we first cover the opportunities that solution processing of the powder offers, emphasizing the potential structural features that can be controlled by precisely engineering the inorganic core of the particle, the surface, and the organization of the particles before consolidation. We then discuss the challenges of this synthetic approach and more practical matters related to solution processing. Finally, we suggest some good practices for adequate knowledge transfer and improving reproducibility among different laboratories."}],"issue":"19","type":"journal_article","oa_version":"Published Version","file":[{"checksum":"f7143e44ab510519d1949099c3558532","success":1,"date_created":"2023-01-30T07:35:09Z","date_updated":"2023-01-30T07:35:09Z","relation":"main_file","file_id":"12434","file_size":10923495,"content_type":"application/pdf","creator":"dernst","access_level":"open_access","file_name":"2022_ChemistryMaterials_Fiedler.pdf"}],"status":"public","title":"Solution-processed inorganic thermoelectric materials: Opportunities and challenges","ddc":["540"],"intvolume":" 34","user_id":"4359f0d1-fa6c-11eb-b949-802e58b17ae8","_id":"12237","day":"20","article_processing_charge":"Yes (via OA deal)","has_accepted_license":"1","keyword":["Materials Chemistry","General Chemical Engineering","General Chemistry"],"scopus_import":"1","date_published":"2022-09-20T00:00:00Z","article_type":"original","page":"8471-8489","publication":"Chemistry of Materials","citation":{"chicago":"Fiedler, Christine, Tobias Kleinhanns, Maria Garcia, Seungho Lee, Mariano Calcabrini, and Maria Ibáñez. “Solution-Processed Inorganic Thermoelectric Materials: Opportunities and Challenges.” Chemistry of Materials. American Chemical Society, 2022. https://doi.org/10.1021/acs.chemmater.2c01967.","mla":"Fiedler, Christine, et al. “Solution-Processed Inorganic Thermoelectric Materials: Opportunities and Challenges.” Chemistry of Materials, vol. 34, no. 19, American Chemical Society, 2022, pp. 8471–89, doi:10.1021/acs.chemmater.2c01967.","short":"C. Fiedler, T. Kleinhanns, M. Garcia, S. Lee, M. Calcabrini, M. Ibáñez, Chemistry of Materials 34 (2022) 8471–8489.","ista":"Fiedler C, Kleinhanns T, Garcia M, Lee S, Calcabrini M, Ibáñez M. 2022. Solution-processed inorganic thermoelectric materials: Opportunities and challenges. Chemistry of Materials. 34(19), 8471–8489.","apa":"Fiedler, C., Kleinhanns, T., Garcia, M., Lee, S., Calcabrini, M., & Ibáñez, M. (2022). Solution-processed inorganic thermoelectric materials: Opportunities and challenges. Chemistry of Materials. American Chemical Society. https://doi.org/10.1021/acs.chemmater.2c01967","ieee":"C. Fiedler, T. Kleinhanns, M. Garcia, S. Lee, M. Calcabrini, and M. Ibáñez, “Solution-processed inorganic thermoelectric materials: Opportunities and challenges,” Chemistry of Materials, vol. 34, no. 19. American Chemical Society, pp. 8471–8489, 2022.","ama":"Fiedler C, Kleinhanns T, Garcia M, Lee S, Calcabrini M, Ibáñez M. Solution-processed inorganic thermoelectric materials: Opportunities and challenges. Chemistry of Materials. 2022;34(19):8471-8489. doi:10.1021/acs.chemmater.2c01967"}},{"oa_version":"Published Version","file":[{"relation":"main_file","file_id":"12459","date_created":"2023-01-30T11:16:54Z","date_updated":"2023-01-30T11:16:54Z","checksum":"efad6742f89f39a18bec63116dd689a0","success":1,"file_name":"2022_Nanomaterials_Shuvaev.pdf","access_level":"open_access","file_size":464840,"content_type":"application/pdf","creator":"dernst"}],"ddc":["530"],"title":"Band structure near the Dirac Point in HgTe quantum wells with critical thickness","status":"public","intvolume":" 12","user_id":"2DF688A6-F248-11E8-B48F-1D18A9856A87","_id":"12278","abstract":[{"lang":"eng","text":"Mercury telluride (HgTe) thin films with a critical thickness of 6.5 nm are predicted to possess a gapless Dirac-like band structure. We report a comprehensive study on gated and optically doped samples by magnetooptical spectroscopy in the THz range. The quasi-classical analysis of the cyclotron resonance allowed the mapping of the band dispersion of Dirac charge carriers in a broad range of electron and hole doping. A smooth transition through the charge neutrality point between Dirac holes and electrons was observed. An additional peak coming from a second type of holes with an almost density-independent mass of around 0.04m0 was detected in the hole-doping range and attributed to an asymmetric spin splitting of the Dirac cone. Spectroscopic evidence for disorder-induced band energy fluctuations could not be detected in present cyclotron resonance experiments."}],"issue":"14","type":"journal_article","date_published":"2022-07-20T00:00:00Z","article_type":"original","publication":"Nanomaterials","citation":{"ama":"Shuvaev A, Dziom U, Gospodarič J, et al. Band structure near the Dirac Point in HgTe quantum wells with critical thickness. Nanomaterials. 2022;12(14). doi:10.3390/nano12142492","apa":"Shuvaev, A., Dziom, U., Gospodarič, J., Novik, E. G., Dobretsova, A. A., Mikhailov, N. N., … Pimenov, A. (2022). Band structure near the Dirac Point in HgTe quantum wells with critical thickness. Nanomaterials. MDPI. https://doi.org/10.3390/nano12142492","ieee":"A. Shuvaev et al., “Band structure near the Dirac Point in HgTe quantum wells with critical thickness,” Nanomaterials, vol. 12, no. 14. MDPI, 2022.","ista":"Shuvaev A, Dziom U, Gospodarič J, Novik EG, Dobretsova AA, Mikhailov NN, Kvon ZD, Pimenov A. 2022. Band structure near the Dirac Point in HgTe quantum wells with critical thickness. Nanomaterials. 12(14), 2492.","short":"A. Shuvaev, U. Dziom, J. Gospodarič, E.G. Novik, A.A. Dobretsova, N.N. Mikhailov, Z.D. Kvon, A. Pimenov, Nanomaterials 12 (2022).","mla":"Shuvaev, Alexey, et al. “Band Structure near the Dirac Point in HgTe Quantum Wells with Critical Thickness.” Nanomaterials, vol. 12, no. 14, 2492, MDPI, 2022, doi:10.3390/nano12142492.","chicago":"Shuvaev, Alexey, Uladzislau Dziom, Jan Gospodarič, Elena G. Novik, Alena A. Dobretsova, Nikolay N. Mikhailov, Ze Don Kvon, and Andrei Pimenov. “Band Structure near the Dirac Point in HgTe Quantum Wells with Critical Thickness.” Nanomaterials. MDPI, 2022. https://doi.org/10.3390/nano12142492."},"day":"20","article_processing_charge":"Yes","has_accepted_license":"1","keyword":["General Materials Science","General Chemical Engineering"],"scopus_import":"1","date_created":"2023-01-16T10:02:31Z","date_updated":"2023-10-17T11:41:28Z","volume":12,"author":[{"first_name":"Alexey","last_name":"Shuvaev","full_name":"Shuvaev, Alexey"},{"id":"6A9A37C2-8C5C-11E9-AE53-F2FDE5697425","orcid":"0000-0002-1648-0999","first_name":"Uladzislau","last_name":"Dziom","full_name":"Dziom, Uladzislau"},{"first_name":"Jan","last_name":"Gospodarič","full_name":"Gospodarič, Jan"},{"full_name":"Novik, Elena G.","last_name":"Novik","first_name":"Elena G."},{"first_name":"Alena A.","last_name":"Dobretsova","full_name":"Dobretsova, Alena A."},{"first_name":"Nikolay N.","last_name":"Mikhailov","full_name":"Mikhailov, Nikolay N."},{"full_name":"Kvon, Ze Don","last_name":"Kvon","first_name":"Ze Don"},{"full_name":"Pimenov, Andrei","first_name":"Andrei","last_name":"Pimenov"}],"publication_status":"published","publisher":"MDPI","department":[{"_id":"ZhAl"}],"acknowledgement":"This work was supported by the Austrian Science Funds (W1243, I 3456-N27, I 5539-N).\r\nOpen Access Funding by the Austrian Science Fund (FWF).","year":"2022","file_date_updated":"2023-01-30T11:16:54Z","article_number":"2492","language":[{"iso":"eng"}],"doi":"10.3390/nano12142492","isi":1,"quality_controlled":"1","oa":1,"tmp":{"name":"Creative Commons Attribution 4.0 International Public License (CC-BY 4.0)","legal_code_url":"https://creativecommons.org/licenses/by/4.0/legalcode","short":"CC BY (4.0)","image":"/images/cc_by.png"},"external_id":{"isi":["000834401600001"]},"month":"07","publication_identifier":{"issn":["2079-4991"]}},{"oa_version":"Published Version","_id":"13357","user_id":"2DF688A6-F248-11E8-B48F-1D18A9856A87","title":"Electrostatic co-assembly of nanoparticles with oppositely charged small molecules into static and dynamic superstructures","status":"public","intvolume":" 13","abstract":[{"lang":"eng","text":"Coulombic interactions can be used to assemble charged nanoparticles into higher-order structures, but the process requires oppositely charged partners that are similarly sized. The ability to mediate the assembly of such charged nanoparticles using structurally simple small molecules would greatly facilitate the fabrication of nanostructured materials and harnessing their applications in catalysis, sensing and photonics. Here we show that small molecules with as few as three electric charges can effectively induce attractive interactions between oppositely charged nanoparticles in water. These interactions can guide the assembly of charged nanoparticles into colloidal crystals of a quality previously only thought to result from their co-crystallization with oppositely charged nanoparticles of a similar size. Transient nanoparticle assemblies can be generated using positively charged nanoparticles and multiply charged anions that are enzymatically hydrolysed into mono- and/or dianions. Our findings demonstrate an approach for the facile fabrication, manipulation and further investigation of static and dynamic nanostructured materials in aqueous environments."}],"issue":"10","type":"journal_article","date_published":"2021-10-01T00:00:00Z","publication":"Nature Chemistry","citation":{"chicago":"Bian, Tong, Andrea Gardin, Julius Gemen, Lothar Houben, Claudio Perego, Byeongdu Lee, Nadav Elad, Zonglin Chu, Giovanni M. Pavan, and Rafal Klajn. “Electrostatic Co-Assembly of Nanoparticles with Oppositely Charged Small Molecules into Static and Dynamic Superstructures.” Nature Chemistry. Springer Nature, 2021. https://doi.org/10.1038/s41557-021-00752-9.","short":"T. Bian, A. Gardin, J. Gemen, L. Houben, C. Perego, B. Lee, N. Elad, Z. Chu, G.M. Pavan, R. Klajn, Nature Chemistry 13 (2021) 940–949.","mla":"Bian, Tong, et al. “Electrostatic Co-Assembly of Nanoparticles with Oppositely Charged Small Molecules into Static and Dynamic Superstructures.” Nature Chemistry, vol. 13, no. 10, Springer Nature, 2021, pp. 940–49, doi:10.1038/s41557-021-00752-9.","ieee":"T. Bian et al., “Electrostatic co-assembly of nanoparticles with oppositely charged small molecules into static and dynamic superstructures,” Nature Chemistry, vol. 13, no. 10. Springer Nature, pp. 940–949, 2021.","apa":"Bian, T., Gardin, A., Gemen, J., Houben, L., Perego, C., Lee, B., … Klajn, R. (2021). Electrostatic co-assembly of nanoparticles with oppositely charged small molecules into static and dynamic superstructures. Nature Chemistry. Springer Nature. https://doi.org/10.1038/s41557-021-00752-9","ista":"Bian T, Gardin A, Gemen J, Houben L, Perego C, Lee B, Elad N, Chu Z, Pavan GM, Klajn R. 2021. Electrostatic co-assembly of nanoparticles with oppositely charged small molecules into static and dynamic superstructures. Nature Chemistry. 13(10), 940–949.","ama":"Bian T, Gardin A, Gemen J, et al. Electrostatic co-assembly of nanoparticles with oppositely charged small molecules into static and dynamic superstructures. Nature Chemistry. 2021;13(10):940-949. doi:10.1038/s41557-021-00752-9"},"article_type":"original","page":"940-949","day":"01","article_processing_charge":"No","scopus_import":"1","keyword":["General Chemical Engineering","General Chemistry"],"author":[{"full_name":"Bian, Tong","first_name":"Tong","last_name":"Bian"},{"full_name":"Gardin, Andrea","first_name":"Andrea","last_name":"Gardin"},{"full_name":"Gemen, Julius","last_name":"Gemen","first_name":"Julius"},{"full_name":"Houben, Lothar","last_name":"Houben","first_name":"Lothar"},{"full_name":"Perego, Claudio","first_name":"Claudio","last_name":"Perego"},{"full_name":"Lee, Byeongdu","last_name":"Lee","first_name":"Byeongdu"},{"full_name":"Elad, Nadav","first_name":"Nadav","last_name":"Elad"},{"last_name":"Chu","first_name":"Zonglin","full_name":"Chu, Zonglin"},{"last_name":"Pavan","first_name":"Giovanni M.","full_name":"Pavan, Giovanni M."},{"full_name":"Klajn, Rafal","id":"8e84690e-1e48-11ed-a02b-a1e6fb8bb53b","last_name":"Klajn","first_name":"Rafal"}],"date_created":"2023-08-01T09:34:54Z","date_updated":"2023-08-02T10:55:29Z","volume":13,"year":"2021","pmid":1,"publication_status":"published","publisher":"Springer Nature","extern":"1","doi":"10.1038/s41557-021-00752-9","language":[{"iso":"eng"}],"main_file_link":[{"url":"https://doi.org/10.1038/s41557-021-00752-9","open_access":"1"}],"oa":1,"external_id":{"pmid":["34489564"]},"quality_controlled":"1","month":"10","publication_identifier":{"eissn":["1755-4349"],"issn":["1755-4330"]}},{"quality_controlled":"1","oa":1,"main_file_link":[{"open_access":"1","url":"https://doi.org/10.1016/j.chempr.2020.11.025"}],"language":[{"iso":"eng"}],"doi":"10.1016/j.chempr.2020.11.025","month":"01","publication_identifier":{"issn":["2451-9294"]},"publication_status":"published","publisher":"Elsevier","year":"2021","date_updated":"2023-08-07T10:04:28Z","date_created":"2023-08-01T09:35:19Z","volume":7,"author":[{"first_name":"Maren","last_name":"Weißenfels","full_name":"Weißenfels, Maren"},{"first_name":"Julius","last_name":"Gemen","full_name":"Gemen, Julius"},{"full_name":"Klajn, Rafal","last_name":"Klajn","first_name":"Rafal","id":"8e84690e-1e48-11ed-a02b-a1e6fb8bb53b"}],"extern":"1","article_type":"original","page":"23-37","publication":"Chem","citation":{"ieee":"M. Weißenfels, J. Gemen, and R. Klajn, “Dissipative self-assembly: Fueling with chemicals versus light,” Chem, vol. 7, no. 1. Elsevier, pp. 23–37, 2021.","apa":"Weißenfels, M., Gemen, J., & Klajn, R. (2021). Dissipative self-assembly: Fueling with chemicals versus light. Chem. Elsevier. https://doi.org/10.1016/j.chempr.2020.11.025","ista":"Weißenfels M, Gemen J, Klajn R. 2021. Dissipative self-assembly: Fueling with chemicals versus light. Chem. 7(1), 23–37.","ama":"Weißenfels M, Gemen J, Klajn R. Dissipative self-assembly: Fueling with chemicals versus light. Chem. 2021;7(1):23-37. doi:10.1016/j.chempr.2020.11.025","chicago":"Weißenfels, Maren, Julius Gemen, and Rafal Klajn. “Dissipative Self-Assembly: Fueling with Chemicals versus Light.” Chem. Elsevier, 2021. https://doi.org/10.1016/j.chempr.2020.11.025.","short":"M. Weißenfels, J. Gemen, R. Klajn, Chem 7 (2021) 23–37.","mla":"Weißenfels, Maren, et al. “Dissipative Self-Assembly: Fueling with Chemicals versus Light.” Chem, vol. 7, no. 1, Elsevier, 2021, pp. 23–37, doi:10.1016/j.chempr.2020.11.025."},"date_published":"2021-01-14T00:00:00Z","keyword":["Materials Chemistry","Biochemistry (medical)","General Chemical Engineering","Environmental Chemistry","Biochemistry","General Chemistry"],"scopus_import":"1","day":"14","article_processing_charge":"No","title":"Dissipative self-assembly: Fueling with chemicals versus light","status":"public","intvolume":" 7","user_id":"2DF688A6-F248-11E8-B48F-1D18A9856A87","_id":"13359","oa_version":"Published Version","type":"journal_article","abstract":[{"lang":"eng","text":"Dissipative self-assembly is ubiquitous in nature, where it gives rise to complex structures and functions such as self-healing, homeostasis, and camouflage. These phenomena are enabled by the continuous conversion of energy stored in chemical fuels, such as ATP. Over the past decade, an increasing number of synthetic chemically driven systems have been reported that mimic the features of their natural counterparts. At the same time, it has been shown that dissipative self-assembly can also be fueled by light; these optically fueled systems have been developed in parallel to the chemically fueled ones. In this perspective, we critically compare these two classes of systems. Despite the complementarity and fundamental differences between these two modes of dissipative self-assembly, our analysis reveals that multiple analogies exist between chemically and light-fueled systems. We hope that these considerations will facilitate further development of the field of dissipative self-assembly."}],"issue":"1"},{"file_date_updated":"2022-03-18T09:53:15Z","ec_funded":1,"article_number":"1827","date_created":"2022-03-18T09:45:02Z","date_updated":"2023-08-17T07:08:30Z","volume":11,"author":[{"first_name":"Mengyao","last_name":"Li","full_name":"Li, Mengyao"},{"last_name":"Zhang","first_name":"Yu","full_name":"Zhang, Yu"},{"full_name":"Zhang, Ting","first_name":"Ting","last_name":"Zhang"},{"first_name":"Yong","last_name":"Zuo","full_name":"Zuo, Yong"},{"full_name":"Xiao, Ke","first_name":"Ke","last_name":"Xiao"},{"first_name":"Jordi","last_name":"Arbiol","full_name":"Arbiol, Jordi"},{"full_name":"Llorca, Jordi","first_name":"Jordi","last_name":"Llorca"},{"full_name":"Liu, Yu","last_name":"Liu","first_name":"Yu","orcid":"0000-0001-7313-6740","id":"2A70014E-F248-11E8-B48F-1D18A9856A87"},{"full_name":"Cabot, Andreu","last_name":"Cabot","first_name":"Andreu"}],"publication_status":"published","publisher":"MDPI","department":[{"_id":"MaIb"}],"acknowledgement":"M.L., Y.Z., T.Z. and K.X. thank the China Scholarship Council for their scholarship\r\nsupport. Y.L. acknowledges funding from the European Union’s Horizon 2020 research and\r\ninnovation program under the Marie Sklodowska-Curie grant agreement No. 754411. J.L. thanks the ICREA Academia program and projects MICINN/FEDER RTI2018-093996-B-C31 and G.C. 2017 SGR 128. ICN2 acknowledges funding from the Generalitat de Catalunya 2017 SGR 327 and the Spanish MINECO ENE2017-85087-C3.","year":"2021","month":"07","publication_identifier":{"issn":["2079-4991"]},"language":[{"iso":"eng"}],"doi":"10.3390/nano11071827","isi":1,"quality_controlled":"1","project":[{"_id":"260C2330-B435-11E9-9278-68D0E5697425","grant_number":"754411","name":"ISTplus - Postdoctoral Fellowships","call_identifier":"H2020"}],"oa":1,"tmp":{"name":"Creative Commons Attribution 4.0 International Public License (CC-BY 4.0)","legal_code_url":"https://creativecommons.org/licenses/by/4.0/legalcode","short":"CC BY (4.0)","image":"/images/cc_by.png"},"external_id":{"isi":["000676570000001"]},"abstract":[{"lang":"eng","text":"The cost-effective conversion of low-grade heat into electricity using thermoelectric devices requires developing alternative materials and material processing technologies able to reduce the currently high device manufacturing costs. In this direction, thermoelectric materials that do not rely on rare or toxic elements such as tellurium or lead need to be produced using high-throughput technologies not involving high temperatures and long processes. Bi2Se3 is an obvious possible Te-free alternative to Bi2Te3 for ambient temperature thermoelectric applications, but its performance is still low for practical applications, and additional efforts toward finding proper dopants are required. Here, we report a scalable method to produce Bi2Se3 nanosheets at low synthesis temperatures. We studied the influence of different dopants on the thermoelectric properties of this material. Among the elements tested, we demonstrated that Sn doping resulted in the best performance. Sn incorporation resulted in a significant improvement to the Bi2Se3 Seebeck coefficient and a reduction in the thermal conductivity in the direction of the hot-press axis, resulting in an overall 60% improvement in the thermoelectric figure of merit of Bi2Se3."}],"issue":"7","type":"journal_article","file":[{"relation":"main_file","file_id":"10859","date_updated":"2022-03-18T09:53:15Z","date_created":"2022-03-18T09:53:15Z","checksum":"f28a8b5cf80f5605828359bb398463b0","success":1,"file_name":"2021_Nanomaterials_Li.pdf","access_level":"open_access","file_size":4867547,"content_type":"application/pdf","creator":"dernst"}],"oa_version":"Published Version","ddc":["540"],"status":"public","title":"Enhanced thermoelectric performance of n-type Bi2Se3 nanosheets through Sn doping","intvolume":" 11","user_id":"4359f0d1-fa6c-11eb-b949-802e58b17ae8","_id":"10858","day":"14","has_accepted_license":"1","article_processing_charge":"No","keyword":["General Materials Science","General Chemical Engineering"],"scopus_import":"1","date_published":"2021-07-14T00:00:00Z","article_type":"original","publication":"Nanomaterials","citation":{"short":"M. Li, Y. Zhang, T. Zhang, Y. Zuo, K. Xiao, J. Arbiol, J. Llorca, Y. Liu, A. Cabot, Nanomaterials 11 (2021).","mla":"Li, Mengyao, et al. “Enhanced Thermoelectric Performance of N-Type Bi2Se3 Nanosheets through Sn Doping.” Nanomaterials, vol. 11, no. 7, 1827, MDPI, 2021, doi:10.3390/nano11071827.","chicago":"Li, Mengyao, Yu Zhang, Ting Zhang, Yong Zuo, Ke Xiao, Jordi Arbiol, Jordi Llorca, Yu Liu, and Andreu Cabot. “Enhanced Thermoelectric Performance of N-Type Bi2Se3 Nanosheets through Sn Doping.” Nanomaterials. MDPI, 2021. https://doi.org/10.3390/nano11071827.","ama":"Li M, Zhang Y, Zhang T, et al. Enhanced thermoelectric performance of n-type Bi2Se3 nanosheets through Sn doping. Nanomaterials. 2021;11(7). doi:10.3390/nano11071827","apa":"Li, M., Zhang, Y., Zhang, T., Zuo, Y., Xiao, K., Arbiol, J., … Cabot, A. (2021). Enhanced thermoelectric performance of n-type Bi2Se3 nanosheets through Sn doping. Nanomaterials. MDPI. https://doi.org/10.3390/nano11071827","ieee":"M. Li et al., “Enhanced thermoelectric performance of n-type Bi2Se3 nanosheets through Sn doping,” Nanomaterials, vol. 11, no. 7. MDPI, 2021.","ista":"Li M, Zhang Y, Zhang T, Zuo Y, Xiao K, Arbiol J, Llorca J, Liu Y, Cabot A. 2021. Enhanced thermoelectric performance of n-type Bi2Se3 nanosheets through Sn doping. Nanomaterials. 11(7), 1827."}},{"_id":"9250","user_id":"c635000d-4b10-11ee-a964-aac5a93f6ac1","intvolume":" 13","ddc":["540"],"status":"public","title":"Mechanism of mediated alkali peroxide oxidation and triplet versus singlet oxygen formation","oa_version":"Submitted Version","file":[{"access_level":"open_access","file_name":"2021_NatureChem_Petit_acceptedVersion.pdf","creator":"dernst","content_type":"application/pdf","file_size":1811448,"embargo":"2021-09-15","file_id":"9276","relation":"main_file","checksum":"3ee3f8dd79ed1b7bb0929fce184c8012","date_created":"2021-03-22T11:46:00Z","date_updated":"2021-09-16T22:30:03Z"}],"type":"journal_article","issue":"5","abstract":[{"text":"Aprotic alkali metal–O2 batteries face two major obstacles to their chemistry occurring efficiently, the insulating nature of the formed alkali superoxides/peroxides and parasitic reactions that are caused by the highly reactive singlet oxygen (1O2). Redox mediators are recognized to be key for improving rechargeability. However, it is unclear how they affect 1O2 formation, which hinders strategies for their improvement. Here we clarify the mechanism of mediated peroxide and superoxide oxidation and thus explain how redox mediators either enhance or suppress 1O2 formation. We show that charging commences with peroxide oxidation to a superoxide intermediate and that redox potentials above ~3.5 V versus Li/Li+ drive 1O2 evolution from superoxide oxidation, while disproportionation always generates some 1O2. We find that 1O2 suppression requires oxidation to be faster than the generation of 1O2 from disproportionation. Oxidation rates decrease with growing driving force following Marcus inverted-region behaviour, establishing a region of maximum rate.","lang":"eng"}],"citation":{"chicago":"Petit, Yann K., Eléonore Mourad, Christian Prehal, Christian Leypold, Andreas Windischbacher, Daniel Mijailovic, Christian Slugovc, et al. “Mechanism of Mediated Alkali Peroxide Oxidation and Triplet versus Singlet Oxygen Formation.” Nature Chemistry. Springer Nature, 2021. https://doi.org/10.1038/s41557-021-00643-z.","mla":"Petit, Yann K., et al. “Mechanism of Mediated Alkali Peroxide Oxidation and Triplet versus Singlet Oxygen Formation.” Nature Chemistry, vol. 13, no. 5, Springer Nature, 2021, pp. 465–71, doi:10.1038/s41557-021-00643-z.","short":"Y.K. Petit, E. Mourad, C. Prehal, C. Leypold, A. Windischbacher, D. Mijailovic, C. Slugovc, S.M. Borisov, E. Zojer, S. Brutti, O. Fontaine, S.A. Freunberger, Nature Chemistry 13 (2021) 465–471.","ista":"Petit YK, Mourad E, Prehal C, Leypold C, Windischbacher A, Mijailovic D, Slugovc C, Borisov SM, Zojer E, Brutti S, Fontaine O, Freunberger SA. 2021. Mechanism of mediated alkali peroxide oxidation and triplet versus singlet oxygen formation. Nature Chemistry. 13(5), 465–471.","ieee":"Y. K. Petit et al., “Mechanism of mediated alkali peroxide oxidation and triplet versus singlet oxygen formation,” Nature Chemistry, vol. 13, no. 5. Springer Nature, pp. 465–471, 2021.","apa":"Petit, Y. K., Mourad, E., Prehal, C., Leypold, C., Windischbacher, A., Mijailovic, D., … Freunberger, S. A. (2021). Mechanism of mediated alkali peroxide oxidation and triplet versus singlet oxygen formation. Nature Chemistry. Springer Nature. https://doi.org/10.1038/s41557-021-00643-z","ama":"Petit YK, Mourad E, Prehal C, et al. Mechanism of mediated alkali peroxide oxidation and triplet versus singlet oxygen formation. Nature Chemistry. 2021;13(5):465-471. doi:10.1038/s41557-021-00643-z"},"publication":"Nature Chemistry","page":"465-471","article_type":"original","date_published":"2021-03-15T00:00:00Z","scopus_import":"1","keyword":["General Chemistry","General Chemical Engineering"],"has_accepted_license":"1","article_processing_charge":"No","day":"15","pmid":1,"acknowledgement":"S.A.F. is indebted to the European Research Council (ERC) under the European Union’s Horizon 2020 research and innovation programme (grant agreement No. 636069) as well as IST Austria. O.F thanks the French National Research Agency (STORE-EX Labex Project ANR-10-LABX-76-01). We thank EL-Cell GmbH (Hamburg, Germany) for the pressure test cell. We thank R. Saf for help with the mass spectrometry, J. Schlegl for manufacturing instrumentation, M. Winkler of Acib GmbH, G. Strohmeier and R. Fürst for HPLC measurements and S. Mondal and S. Stadlbauer for kinetic measurements.","year":"2021","publisher":"Springer Nature","department":[{"_id":"StFr"}],"publication_status":"published","author":[{"last_name":"Petit","first_name":"Yann K.","full_name":"Petit, Yann K."},{"first_name":"Eléonore","last_name":"Mourad","full_name":"Mourad, Eléonore"},{"first_name":"Christian","last_name":"Prehal","full_name":"Prehal, Christian"},{"last_name":"Leypold","first_name":"Christian","full_name":"Leypold, Christian"},{"last_name":"Windischbacher","first_name":"Andreas","full_name":"Windischbacher, Andreas"},{"full_name":"Mijailovic, Daniel","last_name":"Mijailovic","first_name":"Daniel"},{"full_name":"Slugovc, Christian","first_name":"Christian","last_name":"Slugovc"},{"last_name":"Borisov","first_name":"Sergey M.","full_name":"Borisov, Sergey M."},{"first_name":"Egbert","last_name":"Zojer","full_name":"Zojer, Egbert"},{"full_name":"Brutti, Sergio","last_name":"Brutti","first_name":"Sergio"},{"full_name":"Fontaine, Olivier","last_name":"Fontaine","first_name":"Olivier"},{"orcid":"0000-0003-2902-5319","id":"A8CA28E6-CE23-11E9-AD2D-EC27E6697425","last_name":"Freunberger","first_name":"Stefan Alexander","full_name":"Freunberger, Stefan Alexander"}],"volume":13,"date_updated":"2023-09-05T15:34:44Z","date_created":"2021-03-16T11:12:20Z","file_date_updated":"2021-09-16T22:30:03Z","external_id":{"pmid":["33723377"],"isi":["000629296400001"]},"oa":1,"quality_controlled":"1","isi":1,"doi":"10.1038/s41557-021-00643-z","language":[{"iso":"eng"}],"acknowledged_ssus":[{"_id":"M-Shop"}],"publication_identifier":{"issn":["1755-4330"],"eissn":["1755-4349"]},"month":"03"},{"publication_identifier":{"issn":["1755-4330"],"eissn":["1755-4349"]},"month":"04","language":[{"iso":"eng"}],"doi":"10.1038/s41557-020-0452-1","quality_controlled":"1","oa":1,"main_file_link":[{"url":"https://www.biorxiv.org/content/10.1101/2020.01.08.897488","open_access":"1"}],"external_id":{"pmid":["32303714"]},"extern":"1","volume":12,"date_created":"2021-11-26T09:15:13Z","date_updated":"2021-11-26T11:21:08Z","related_material":{"link":[{"relation":"erratum","url":"https://doi.org/10.1038/s41557-020-0468-6"}]},"author":[{"full_name":"Michaels, Thomas C. T.","first_name":"Thomas C. T.","last_name":"Michaels"},{"full_name":"Šarić, Anđela","first_name":"Anđela","last_name":"Šarić","id":"bf63d406-f056-11eb-b41d-f263a6566d8b","orcid":"0000-0002-7854-2139"},{"last_name":"Curk","first_name":"Samo","full_name":"Curk, Samo"},{"last_name":"Bernfur","first_name":"Katja","full_name":"Bernfur, Katja"},{"first_name":"Paolo","last_name":"Arosio","full_name":"Arosio, Paolo"},{"full_name":"Meisl, Georg","last_name":"Meisl","first_name":"Georg"},{"last_name":"Dear","first_name":"Alexander J.","full_name":"Dear, Alexander J."},{"full_name":"Cohen, Samuel I. A.","last_name":"Cohen","first_name":"Samuel I. A."},{"full_name":"Dobson, Christopher M.","first_name":"Christopher M.","last_name":"Dobson"},{"first_name":"Michele","last_name":"Vendruscolo","full_name":"Vendruscolo, Michele"},{"full_name":"Linse, Sara","first_name":"Sara","last_name":"Linse"},{"first_name":"Tuomas P. J.","last_name":"Knowles","full_name":"Knowles, Tuomas P. J."}],"publisher":"Springer Nature","publication_status":"published","pmid":1,"year":"2020","acknowledgement":"We acknowledge support from Peterhouse (T.C.T.M.), the Swiss National Science foundation (T.C.T.M.), the Royal Society (A.Š.), the Academy of Medical Sciences (A.Š.), the UCL Institute for the Physics of Living Systems (S.C.), Sidney Sussex College (G.M.), the Wellcome Trust (A.Š., M.V., C.M.D. and T.P.J.K.), the Schiff Foundation (A.J.D.), the Cambridge Centre for Misfolding Diseases (M.V., C.M.D. and T.P.J.K.), the BBSRC (C.M.D. and T.P.J.K.), the Frances and Augustus Newman Foundation (T.P.J.K.), the Swedish Research Council (S.L.) and the ERC grant MAMBA (S.L., agreement no. 340890). The research that led to these results received funding from the European Research Council under the European Union’s Seventh Framework Programme (FP7/2007-2013) through the ERC grant PhysProt (agreement no. 337969).","article_processing_charge":"No","day":"13","keyword":["general chemical engineering","general chemistry"],"scopus_import":"1","date_published":"2020-04-13T00:00:00Z","page":"445-451","article_type":"original","citation":{"chicago":"Michaels, Thomas C. T., Anđela Šarić, Samo Curk, Katja Bernfur, Paolo Arosio, Georg Meisl, Alexander J. Dear, et al. “Dynamics of Oligomer Populations Formed during the Aggregation of Alzheimer’s Aβ42 Peptide.” Nature Chemistry. Springer Nature, 2020. https://doi.org/10.1038/s41557-020-0452-1.","mla":"Michaels, Thomas C. T., et al. “Dynamics of Oligomer Populations Formed during the Aggregation of Alzheimer’s Aβ42 Peptide.” Nature Chemistry, vol. 12, no. 5, Springer Nature, 2020, pp. 445–51, doi:10.1038/s41557-020-0452-1.","short":"T.C.T. Michaels, A. Šarić, S. Curk, K. Bernfur, P. Arosio, G. Meisl, A.J. Dear, S.I.A. Cohen, C.M. Dobson, M. Vendruscolo, S. Linse, T.P.J. Knowles, Nature Chemistry 12 (2020) 445–451.","ista":"Michaels TCT, Šarić A, Curk S, Bernfur K, Arosio P, Meisl G, Dear AJ, Cohen SIA, Dobson CM, Vendruscolo M, Linse S, Knowles TPJ. 2020. Dynamics of oligomer populations formed during the aggregation of Alzheimer’s Aβ42 peptide. Nature Chemistry. 12(5), 445–451.","apa":"Michaels, T. C. T., Šarić, A., Curk, S., Bernfur, K., Arosio, P., Meisl, G., … Knowles, T. P. J. (2020). Dynamics of oligomer populations formed during the aggregation of Alzheimer’s Aβ42 peptide. Nature Chemistry. Springer Nature. https://doi.org/10.1038/s41557-020-0452-1","ieee":"T. C. T. Michaels et al., “Dynamics of oligomer populations formed during the aggregation of Alzheimer’s Aβ42 peptide,” Nature Chemistry, vol. 12, no. 5. Springer Nature, pp. 445–451, 2020.","ama":"Michaels TCT, Šarić A, Curk S, et al. Dynamics of oligomer populations formed during the aggregation of Alzheimer’s Aβ42 peptide. Nature Chemistry. 2020;12(5):445-451. doi:10.1038/s41557-020-0452-1"},"publication":"Nature Chemistry","issue":"5","abstract":[{"text":"Oligomeric species populated during the aggregation of the Aβ42 peptide have been identified as potent cytotoxins linked to Alzheimer’s disease, but the fundamental molecular pathways that control their dynamics have yet to be elucidated. By developing a general approach that combines theory, experiment and simulation, we reveal, in molecular detail, the mechanisms of Aβ42 oligomer dynamics during amyloid fibril formation. Even though all mature amyloid fibrils must originate as oligomers, we found that most Aβ42 oligomers dissociate into their monomeric precursors without forming new fibrils. Only a minority of oligomers converts into fibrillar structures. Moreover, the heterogeneous ensemble of oligomeric species interconverts on timescales comparable to those of aggregation. Our results identify fundamentally new steps that could be targeted by therapeutic interventions designed to combat protein misfolding diseases.","lang":"eng"}],"type":"journal_article","oa_version":"None","intvolume":" 12","status":"public","title":"Dynamics of oligomer populations formed during the aggregation of Alzheimer’s Aβ42 peptide","_id":"10351","user_id":"8b945eb4-e2f2-11eb-945a-df72226e66a9"},{"keyword":["General Chemistry","General Chemical Engineering"],"day":"29","article_processing_charge":"No","publication":"RSC Advances","citation":{"mla":"Nauman, Muhammad, et al. “Size-Dependent Magnetic and Magnetothermal Properties of Gadolinium Silicide Nanoparticles.” RSC Advances, vol. 10, no. 47, Royal Society of Chemistry, 2020, pp. 28383–89, doi:10.1039/d0ra05394e.","short":"M. Nauman, M.H. Alnasir, M.A. Hamayun, Y. Wang, M. Shatruk, S. Manzoor, RSC Advances 10 (2020) 28383–28389.","chicago":"Nauman, Muhammad, Muhammad Hisham Alnasir, Muhammad Asif Hamayun, YiXu Wang, Michael Shatruk, and Sadia Manzoor. “Size-Dependent Magnetic and Magnetothermal Properties of Gadolinium Silicide Nanoparticles.” RSC Advances. Royal Society of Chemistry, 2020. https://doi.org/10.1039/d0ra05394e.","ama":"Nauman M, Alnasir MH, Hamayun MA, Wang Y, Shatruk M, Manzoor S. Size-dependent magnetic and magnetothermal properties of gadolinium silicide nanoparticles. RSC Advances. 2020;10(47):28383-28389. doi:10.1039/d0ra05394e","ista":"Nauman M, Alnasir MH, Hamayun MA, Wang Y, Shatruk M, Manzoor S. 2020. Size-dependent magnetic and magnetothermal properties of gadolinium silicide nanoparticles. RSC Advances. 10(47), 28383–28389.","ieee":"M. Nauman, M. H. Alnasir, M. A. Hamayun, Y. Wang, M. Shatruk, and S. Manzoor, “Size-dependent magnetic and magnetothermal properties of gadolinium silicide nanoparticles,” RSC Advances, vol. 10, no. 47. Royal Society of Chemistry, pp. 28383–28389, 2020.","apa":"Nauman, M., Alnasir, M. H., Hamayun, M. A., Wang, Y., Shatruk, M., & Manzoor, S. (2020). Size-dependent magnetic and magnetothermal properties of gadolinium silicide nanoparticles. RSC Advances. Royal Society of Chemistry. https://doi.org/10.1039/d0ra05394e"},"article_type":"original","page":"28383-28389","date_published":"2020-07-29T00:00:00Z","type":"journal_article","abstract":[{"text":"Gadolinium silicide (Gd5Si4) nanoparticles are an interesting class of materials due to their high magnetization, low Curie temperature, low toxicity in biological environments and their multifunctional properties. We report the magnetic and magnetothermal properties of gadolinium silicide (Gd5Si4) nanoparticles prepared by surfactant-assisted ball milling of arc melted bulk ingots of the compound. Using different milling times and speeds, a wide range of crystallite sizes (13–43 nm) could be produced and a reduction in Curie temperature (TC) from 340 K to 317 K was achieved, making these nanoparticles suitable for self-controlled magnetic hyperthermia applications. The magnetothermal effect was measured in applied AC magnetic fields of amplitude 164–239 Oe and frequencies 163–519 kHz. All particles showed magnetic heating with a strong dependence of the specific absorption rate (SAR) on the average crystallite size. The highest SAR of 3.7 W g−1 was measured for 43 nm sized nanoparticles of Gd5Si4. The high SAR and low TC, (within the therapeutic range for magnetothermal therapy) makes the Gd5Si4 behave like self-regulating heat switches that would be suitable for self-controlled magnetic hyperthermia applications after biocompatibility and cytotoxicity tests.","lang":"eng"}],"issue":"47","_id":"9067","user_id":"2DF688A6-F248-11E8-B48F-1D18A9856A87","status":"public","title":"Size-dependent magnetic and magnetothermal properties of gadolinium silicide nanoparticles","intvolume":" 10","oa_version":"Published Version","month":"07","publication_identifier":{"issn":["2046-2069"]},"main_file_link":[{"url":"https://doi.org/10.1039/d0ra05394e","open_access":"1"}],"oa":1,"quality_controlled":"1","doi":"10.1039/d0ra05394e","language":[{"iso":"eng"}],"extern":"1","year":"2020","publication_status":"published","publisher":"Royal Society of Chemistry","author":[{"id":"32c21954-2022-11eb-9d5f-af9f93c24e71","orcid":"0000-0002-2111-4846","first_name":"Muhammad","last_name":"Nauman","full_name":"Nauman, Muhammad"},{"first_name":"Muhammad Hisham","last_name":"Alnasir","full_name":"Alnasir, Muhammad Hisham"},{"full_name":"Hamayun, Muhammad Asif","first_name":"Muhammad Asif","last_name":"Hamayun"},{"full_name":"Wang, YiXu","first_name":"YiXu","last_name":"Wang"},{"first_name":"Michael","last_name":"Shatruk","full_name":"Shatruk, Michael"},{"full_name":"Manzoor, Sadia","last_name":"Manzoor","first_name":"Sadia"}],"date_created":"2021-02-02T15:51:23Z","date_updated":"2021-02-04T07:16:37Z","volume":10},{"ec_funded":1,"file_date_updated":"2020-12-10T14:07:24Z","article_number":"2001724","volume":7,"date_created":"2020-10-01T09:44:13Z","date_updated":"2023-08-22T09:53:01Z","author":[{"first_name":"Anhao","last_name":"Tian","full_name":"Tian, Anhao"},{"full_name":"Kang, Bo","first_name":"Bo","last_name":"Kang"},{"full_name":"Li, Baizhou","first_name":"Baizhou","last_name":"Li"},{"first_name":"Biying","last_name":"Qiu","full_name":"Qiu, Biying"},{"full_name":"Jiang, Wenhong","first_name":"Wenhong","last_name":"Jiang"},{"full_name":"Shao, Fangjie","first_name":"Fangjie","last_name":"Shao"},{"full_name":"Gao, Qingqing","first_name":"Qingqing","last_name":"Gao"},{"last_name":"Liu","first_name":"Rui","full_name":"Liu, Rui"},{"full_name":"Cai, Chengwei","last_name":"Cai","first_name":"Chengwei"},{"full_name":"Jing, Rui","first_name":"Rui","last_name":"Jing"},{"full_name":"Wang, Wei","last_name":"Wang","first_name":"Wei"},{"first_name":"Pengxiang","last_name":"Chen","full_name":"Chen, Pengxiang"},{"last_name":"Liang","first_name":"Qinghui","full_name":"Liang, Qinghui"},{"last_name":"Bao","first_name":"Lili","full_name":"Bao, Lili"},{"full_name":"Man, Jianghong","first_name":"Jianghong","last_name":"Man"},{"full_name":"Wang, Yan","first_name":"Yan","last_name":"Wang"},{"first_name":"Yu","last_name":"Shi","full_name":"Shi, Yu"},{"full_name":"Li, Jin","last_name":"Li","first_name":"Jin"},{"first_name":"Minmin","last_name":"Yang","full_name":"Yang, Minmin"},{"first_name":"Lisha","last_name":"Wang","full_name":"Wang, Lisha"},{"full_name":"Zhang, Jianmin","last_name":"Zhang","first_name":"Jianmin"},{"id":"37B36620-F248-11E8-B48F-1D18A9856A87","orcid":"0000-0003-2279-1061","first_name":"Simon","last_name":"Hippenmeyer","full_name":"Hippenmeyer, Simon"},{"first_name":"Junming","last_name":"Zhu","full_name":"Zhu, Junming"},{"last_name":"Bian","first_name":"Xiuwu","full_name":"Bian, Xiuwu"},{"last_name":"Wang","first_name":"Ying‐Jie","full_name":"Wang, Ying‐Jie"},{"last_name":"Liu","first_name":"Chong","full_name":"Liu, Chong"}],"department":[{"_id":"SiHi"}],"publisher":"Wiley","publication_status":"published","acknowledgement":"The authors thank Drs. J. Eisen, QR. Lu, S. Duan, Z‐H. Li, W. Mo, and Q. Wu for their critical comments on the manuscript. They also thank Dr. H. Zong for providing the CKO_NG2‐CreER model. This work is supported by the National Key Research and Development Program of China, Stem Cell and Translational Research (2016YFA0101201 to C.L., 2016YFA0100303 to Y.J.W.), the National Natural Science Foundation of China (81673035 and 81972915 to C.L., 81472722 to Y.J.W.), the Science Foundation for Distinguished Young Scientists of Zhejiang Province (LR17H160001 to C.L.), Fundamental Research Funds for the Central Universities (2016QNA7023 and 2017QNA7028 to C.L.) and the Thousand Talent Program for Young Outstanding Scientists, China (to C.L.), IST Austria institutional funds (to S.H.), European Research Council (ERC) under the European Union's Horizon 2020 research and innovation programme (725780 LinPro to S.H.). C.L. is a scholar of K. C. Wong Education Foundation.","year":"2020","publication_identifier":{"issn":["2198-3844"]},"month":"11","language":[{"iso":"eng"}],"doi":"10.1002/advs.202001724","project":[{"call_identifier":"H2020","name":"Principles of Neural Stem Cell Lineage Progression in Cerebral Cortex Development","grant_number":"725780","_id":"260018B0-B435-11E9-9278-68D0E5697425"}],"quality_controlled":"1","isi":1,"tmp":{"name":"Creative Commons Attribution 4.0 International Public License (CC-BY 4.0)","legal_code_url":"https://creativecommons.org/licenses/by/4.0/legalcode","short":"CC BY (4.0)","image":"/images/cc_by.png"},"oa":1,"external_id":{"isi":["000573860700001"]},"issue":"21","abstract":[{"lang":"eng","text":"Glioblastoma is the most malignant cancer in the brain and currently incurable. It is urgent to identify effective targets for this lethal disease. Inhibition of such targets should suppress the growth of cancer cells and, ideally also precancerous cells for early prevention, but minimally affect their normal counterparts. Using genetic mouse models with neural stem cells (NSCs) or oligodendrocyte precursor cells (OPCs) as the cells‐of‐origin/mutation, it is shown that the susceptibility of cells within the development hierarchy of glioma to the knockout of insulin‐like growth factor I receptor (IGF1R) is determined not only by their oncogenic states, but also by their cell identities/states. Knockout of IGF1R selectively disrupts the growth of mutant and transformed, but not normal OPCs, or NSCs. The desirable outcome of IGF1R knockout on cell growth requires the mutant cells to commit to the OPC identity regardless of its development hierarchical status. At the molecular level, oncogenic mutations reprogram the cellular network of OPCs and force them to depend more on IGF1R for their growth. A new‐generation brain‐penetrable, orally available IGF1R inhibitor harnessing tumor OPCs in the brain is also developed. The findings reveal the cellular window of IGF1R targeting and establish IGF1R as an effective target for the prevention and treatment of glioblastoma."}],"type":"journal_article","file":[{"creator":"dernst","content_type":"application/pdf","file_size":7835833,"access_level":"open_access","file_name":"2020_AdvScience_Tian.pdf","success":1,"checksum":"92818c23ecc70e35acfa671f3cfb9909","date_updated":"2020-12-10T14:07:24Z","date_created":"2020-12-10T14:07:24Z","file_id":"8938","relation":"main_file"}],"oa_version":"Published Version","intvolume":" 7","ddc":["570"],"title":"Oncogenic state and cell identity combinatorially dictate the susceptibility of cells within glioma development hierarchy to IGF1R targeting","status":"public","user_id":"4359f0d1-fa6c-11eb-b949-802e58b17ae8","_id":"8592","has_accepted_license":"1","article_processing_charge":"No","day":"04","keyword":["General Engineering","General Physics and Astronomy","General Materials Science","Medicine (miscellaneous)","General Chemical Engineering","Biochemistry","Genetics and Molecular Biology (miscellaneous)"],"date_published":"2020-11-04T00:00:00Z","article_type":"original","citation":{"chicago":"Tian, Anhao, Bo Kang, Baizhou Li, Biying Qiu, Wenhong Jiang, Fangjie Shao, Qingqing Gao, et al. “Oncogenic State and Cell Identity Combinatorially Dictate the Susceptibility of Cells within Glioma Development Hierarchy to IGF1R Targeting.” Advanced Science. Wiley, 2020. https://doi.org/10.1002/advs.202001724.","short":"A. Tian, B. Kang, B. Li, B. Qiu, W. Jiang, F. Shao, Q. Gao, R. Liu, C. Cai, R. Jing, W. Wang, P. Chen, Q. Liang, L. Bao, J. Man, Y. Wang, Y. Shi, J. Li, M. Yang, L. Wang, J. Zhang, S. Hippenmeyer, J. Zhu, X. Bian, Y. Wang, C. Liu, Advanced Science 7 (2020).","mla":"Tian, Anhao, et al. “Oncogenic State and Cell Identity Combinatorially Dictate the Susceptibility of Cells within Glioma Development Hierarchy to IGF1R Targeting.” Advanced Science, vol. 7, no. 21, 2001724, Wiley, 2020, doi:10.1002/advs.202001724.","apa":"Tian, A., Kang, B., Li, B., Qiu, B., Jiang, W., Shao, F., … Liu, C. (2020). Oncogenic state and cell identity combinatorially dictate the susceptibility of cells within glioma development hierarchy to IGF1R targeting. Advanced Science. Wiley. https://doi.org/10.1002/advs.202001724","ieee":"A. Tian et al., “Oncogenic state and cell identity combinatorially dictate the susceptibility of cells within glioma development hierarchy to IGF1R targeting,” Advanced Science, vol. 7, no. 21. Wiley, 2020.","ista":"Tian A, Kang B, Li B, Qiu B, Jiang W, Shao F, Gao Q, Liu R, Cai C, Jing R, Wang W, Chen P, Liang Q, Bao L, Man J, Wang Y, Shi Y, Li J, Yang M, Wang L, Zhang J, Hippenmeyer S, Zhu J, Bian X, Wang Y, Liu C. 2020. Oncogenic state and cell identity combinatorially dictate the susceptibility of cells within glioma development hierarchy to IGF1R targeting. Advanced Science. 7(21), 2001724.","ama":"Tian A, Kang B, Li B, et al. Oncogenic state and cell identity combinatorially dictate the susceptibility of cells within glioma development hierarchy to IGF1R targeting. Advanced Science. 2020;7(21). doi:10.1002/advs.202001724"},"publication":"Advanced Science"},{"month":"09","publication_identifier":{"issn":["2451-9308"],"eissn":["2451-9294"]},"quality_controlled":"1","oa":1,"main_file_link":[{"url":"https://doi.org/10.1016/j.chempr.2019.08.012","open_access":"1"}],"language":[{"iso":"eng"}],"doi":"10.1016/j.chempr.2019.08.012","extern":"1","publication_status":"published","publisher":"Elsevier","year":"2019","date_created":"2023-08-01T09:38:38Z","date_updated":"2023-08-07T10:46:50Z","volume":5,"author":[{"full_name":"Białek, Michał J.","first_name":"Michał J.","last_name":"Białek"},{"full_name":"Klajn, Rafal","first_name":"Rafal","last_name":"Klajn","id":"8e84690e-1e48-11ed-a02b-a1e6fb8bb53b"}],"keyword":["Materials Chemistry","Biochemistry (medical)","General Chemical Engineering","Environmental Chemistry","Biochemistry","General Chemistry"],"scopus_import":"1","day":"12","article_processing_charge":"No","article_type":"original","page":"2283-2285","publication":"Chem","citation":{"ista":"Białek MJ, Klajn R. 2019. Diamond grows up. Chem. 5(9), 2283–2285.","ieee":"M. J. Białek and R. Klajn, “Diamond grows up,” Chem, vol. 5, no. 9. Elsevier, pp. 2283–2285, 2019.","apa":"Białek, M. J., & Klajn, R. (2019). Diamond grows up. Chem. Elsevier. https://doi.org/10.1016/j.chempr.2019.08.012","ama":"Białek MJ, Klajn R. Diamond grows up. Chem. 2019;5(9):2283-2285. doi:10.1016/j.chempr.2019.08.012","chicago":"Białek, Michał J., and Rafal Klajn. “Diamond Grows Up.” Chem. Elsevier, 2019. https://doi.org/10.1016/j.chempr.2019.08.012.","mla":"Białek, Michał J., and Rafal Klajn. “Diamond Grows Up.” Chem, vol. 5, no. 9, Elsevier, 2019, pp. 2283–85, doi:10.1016/j.chempr.2019.08.012.","short":"M.J. Białek, R. Klajn, Chem 5 (2019) 2283–2285."},"date_published":"2019-09-12T00:00:00Z","type":"journal_article","abstract":[{"lang":"eng","text":"Diamondoid nanoporous crystals represent a synthetically challenging class of materials that typically have been obtained from tetrahedral building blocks. In this issue of Chem, Stoddart and coworkers demonstrate that it is possible to generate diamondoid frameworks from a hexacationic building block lacking a tetrahedral symmetry. These results highlight the great potential of self-assembly for rapidly transforming small molecules into structurally complex functional materials."}],"issue":"9","title":"Diamond grows up","status":"public","intvolume":" 5","_id":"13371","user_id":"2DF688A6-F248-11E8-B48F-1D18A9856A87","oa_version":"Published Version"},{"user_id":"8b945eb4-e2f2-11eb-945a-df72226e66a9","_id":"10360","status":"public","title":"Distinct thermodynamic signatures of oligomer generation in the aggregation of the amyloid-β peptide","intvolume":" 10","oa_version":"None","type":"journal_article","abstract":[{"lang":"eng","text":"Mapping free-energy landscapes has proved to be a powerful tool for studying reaction mechanisms. Many complex biomolecular assembly processes, however, have remained challenging to access using this approach, including the aggregation of peptides and proteins into amyloid fibrils implicated in a range of disorders. Here, we generalize the strategy used to probe free-energy landscapes in protein folding to determine the activation energies and entropies that characterize each of the molecular steps in the aggregation of the amyloid-β peptide (Aβ42), which is associated with Alzheimer’s disease. Our results reveal that interactions between monomeric Aβ42 and amyloid fibrils during fibril-dependent secondary nucleation fundamentally reverse the thermodynamic signature of this process relative to primary nucleation, even though both processes generate aggregates from soluble peptides. By mapping the energetic and entropic contributions along the reaction trajectories, we show that the catalytic efficiency of Aβ42 fibril surfaces results from the enthalpic stabilization of adsorbing peptides in conformations amenable to nucleation, resulting in a dramatic lowering of the activation energy for nucleation."}],"issue":"5","publication":"Nature Chemistry","citation":{"ama":"Cohen SIA, Cukalevski R, Michaels TCT, et al. Distinct thermodynamic signatures of oligomer generation in the aggregation of the amyloid-β peptide. Nature Chemistry. 2018;10(5):523-531. doi:10.1038/s41557-018-0023-x","ista":"Cohen SIA, Cukalevski R, Michaels TCT, Šarić A, Törnquist M, Vendruscolo M, Dobson CM, Buell AK, Knowles TPJ, Linse S. 2018. Distinct thermodynamic signatures of oligomer generation in the aggregation of the amyloid-β peptide. Nature Chemistry. 10(5), 523–531.","ieee":"S. I. A. Cohen et al., “Distinct thermodynamic signatures of oligomer generation in the aggregation of the amyloid-β peptide,” Nature Chemistry, vol. 10, no. 5. Springer Nature, pp. 523–531, 2018.","apa":"Cohen, S. I. A., Cukalevski, R., Michaels, T. C. T., Šarić, A., Törnquist, M., Vendruscolo, M., … Linse, S. (2018). Distinct thermodynamic signatures of oligomer generation in the aggregation of the amyloid-β peptide. Nature Chemistry. Springer Nature. https://doi.org/10.1038/s41557-018-0023-x","mla":"Cohen, Samuel I. A., et al. “Distinct Thermodynamic Signatures of Oligomer Generation in the Aggregation of the Amyloid-β Peptide.” Nature Chemistry, vol. 10, no. 5, Springer Nature, 2018, pp. 523–31, doi:10.1038/s41557-018-0023-x.","short":"S.I.A. Cohen, R. Cukalevski, T.C.T. Michaels, A. Šarić, M. Törnquist, M. Vendruscolo, C.M. Dobson, A.K. Buell, T.P.J. Knowles, S. Linse, Nature Chemistry 10 (2018) 523–531.","chicago":"Cohen, Samuel I. A., Risto Cukalevski, Thomas C. T. Michaels, Anđela Šarić, Mattias Törnquist, Michele Vendruscolo, Christopher M. Dobson, Alexander K. Buell, Tuomas P. J. Knowles, and Sara Linse. “Distinct Thermodynamic Signatures of Oligomer Generation in the Aggregation of the Amyloid-β Peptide.” Nature Chemistry. Springer Nature, 2018. https://doi.org/10.1038/s41557-018-0023-x."},"article_type":"original","page":"523-531","date_published":"2018-03-26T00:00:00Z","scopus_import":"1","keyword":["general chemical engineering","general chemistry"],"day":"26","article_processing_charge":"No","acknowledgement":"We thank B. Jönsson and I. André for helpful discussions. We acknowledge financial support from the Schiff Foundation (S.I.A.C.), St John’s College, Cambridge (S.I.A.C.), the Royal Physiographic Society (R.C.), the Research School FLÄK of Lund University (S.L., R.C.), the Swedish Research Council (S.L.) and its Linneaus Centre Organizing Molecular Matter (S.L.), the Crafoord Foundation (S.L.), Alzheimerfonden (S.L.), the European Research Council (S.L.), NanoLund (S.L.), Knut and Alice Wallenberg Foundation (S.L.), Peterhouse, Cambridge (T.C.T.M.), the Swiss National Science Foundation (T.C.T.M.), Magdalene College, Cambridge (A.K.B.), the Leverhulme Trust (A.K.B.), the Royal Society (A.Š.), the Academy of Medical Sciences (A.Š.), the Wellcome Trust (C.M.D., T.P.J.K., A.Š.), and the Centre for Misfolding Diseases (C.M.D., T.P.J.K, M.V.). A.K.B. thanks the Alzheimer Forschung Initiative (AFI).","year":"2018","pmid":1,"publication_status":"published","publisher":"Springer Nature","author":[{"full_name":"Cohen, Samuel I. A.","first_name":"Samuel I. A.","last_name":"Cohen"},{"last_name":"Cukalevski","first_name":"Risto","full_name":"Cukalevski, Risto"},{"full_name":"Michaels, Thomas C. T.","last_name":"Michaels","first_name":"Thomas C. T."},{"full_name":"Šarić, Anđela","first_name":"Anđela","last_name":"Šarić","id":"bf63d406-f056-11eb-b41d-f263a6566d8b","orcid":"0000-0002-7854-2139"},{"last_name":"Törnquist","first_name":"Mattias","full_name":"Törnquist, Mattias"},{"first_name":"Michele","last_name":"Vendruscolo","full_name":"Vendruscolo, Michele"},{"full_name":"Dobson, Christopher M.","first_name":"Christopher M.","last_name":"Dobson"},{"full_name":"Buell, Alexander K.","first_name":"Alexander K.","last_name":"Buell"},{"first_name":"Tuomas P. J.","last_name":"Knowles","full_name":"Knowles, Tuomas P. J."},{"first_name":"Sara","last_name":"Linse","full_name":"Linse, Sara"}],"date_updated":"2021-11-26T15:14:00Z","date_created":"2021-11-26T12:41:38Z","volume":10,"extern":"1","external_id":{"pmid":["29581486"]},"quality_controlled":"1","doi":"10.1038/s41557-018-0023-x","language":[{"iso":"eng"}],"month":"03","publication_identifier":{"issn":["1755-4330"],"eissn":["1755-4349"]}},{"page":"8415-8419","quality_controlled":"1","article_type":"review","citation":{"ama":"Roy S, Roy S, Rao A, Devatha G, Pillai PP. Precise nanoparticle–reactant interaction outplays ligand poisoning in visible-light photocatalysis. Chemistry of Materials. 2018;30(23):8415-8419. doi:10.1021/acs.chemmater.8b03108","ista":"Roy S, Roy S, Rao A, Devatha G, Pillai PP. 2018. Precise nanoparticle–reactant interaction outplays ligand poisoning in visible-light photocatalysis. Chemistry of Materials. 30(23), 8415–8419.","ieee":"S. Roy, S. Roy, A. Rao, G. Devatha, and P. P. Pillai, “Precise nanoparticle–reactant interaction outplays ligand poisoning in visible-light photocatalysis,” Chemistry of Materials, vol. 30, no. 23. American Chemical Society, pp. 8415–8419, 2018.","apa":"Roy, S., Roy, S., Rao, A., Devatha, G., & Pillai, P. P. (2018). Precise nanoparticle–reactant interaction outplays ligand poisoning in visible-light photocatalysis. Chemistry of Materials. American Chemical Society. https://doi.org/10.1021/acs.chemmater.8b03108","mla":"Roy, Soumendu, et al. “Precise Nanoparticle–Reactant Interaction Outplays Ligand Poisoning in Visible-Light Photocatalysis.” Chemistry of Materials, vol. 30, no. 23, American Chemical Society, 2018, pp. 8415–19, doi:10.1021/acs.chemmater.8b03108.","short":"S. Roy, S. Roy, A. Rao, G. Devatha, P.P. Pillai, Chemistry of Materials 30 (2018) 8415–8419.","chicago":"Roy, Soumendu, Sumit Roy, Anish Rao, Gayathri Devatha, and Pramod P. Pillai. “Precise Nanoparticle–Reactant Interaction Outplays Ligand Poisoning in Visible-Light Photocatalysis.” Chemistry of Materials. American Chemical Society, 2018. https://doi.org/10.1021/acs.chemmater.8b03108."},"publication":"Chemistry of Materials","language":[{"iso":"eng"}],"doi":"10.1021/acs.chemmater.8b03108","date_published":"2018-11-19T00:00:00Z","keyword":["Materials Chemistry","General Chemical Engineering","General Chemistry"],"scopus_import":"1","publication_identifier":{"eissn":["1520-5002"],"issn":["0897-4756"]},"article_processing_charge":"No","day":"19","month":"11","publisher":"American Chemical Society","intvolume":" 30","status":"public","publication_status":"published","title":"Precise nanoparticle–reactant interaction outplays ligand poisoning in visible-light photocatalysis","_id":"15107","year":"2018","user_id":"2DF688A6-F248-11E8-B48F-1D18A9856A87","oa_version":"None","volume":30,"date_updated":"2024-03-20T07:50:07Z","date_created":"2024-03-12T12:54:30Z","author":[{"first_name":"Soumendu","last_name":"Roy","full_name":"Roy, Soumendu"},{"id":"67a1dc7d-cffb-11ee-b082-e15ca6a616d9","orcid":"0000-0002-6883-4939","first_name":"Sumit","last_name":"Roy","full_name":"Roy, Sumit"},{"full_name":"Rao, Anish","last_name":"Rao","first_name":"Anish"},{"last_name":"Devatha","first_name":"Gayathri","full_name":"Devatha, Gayathri"},{"full_name":"Pillai, Pramod P.","first_name":"Pramod P.","last_name":"Pillai"}],"type":"journal_article","extern":"1","issue":"23"},{"file_date_updated":"2021-11-29T09:00:40Z","extern":"1","author":[{"full_name":"Simunovic, Mijo","first_name":"Mijo","last_name":"Simunovic"},{"full_name":"Šarić, Anđela","first_name":"Anđela","last_name":"Šarić","id":"bf63d406-f056-11eb-b41d-f263a6566d8b","orcid":"0000-0002-7854-2139"},{"first_name":"J. Michael","last_name":"Henderson","full_name":"Henderson, J. Michael"},{"full_name":"Lee, Ka Yee C.","first_name":"Ka Yee C.","last_name":"Lee"},{"full_name":"Voth, Gregory A.","last_name":"Voth","first_name":"Gregory A."}],"volume":3,"date_created":"2021-11-29T08:49:50Z","date_updated":"2021-11-29T09:28:06Z","pmid":1,"year":"2017","acknowledgement":"M.S. and G.A.V. acknowledge their research reported in this publication as being supported by the National Institute of General Medical Sciences of the National Institutes of Health under Award Number R01-GM063796. Computational resources were provided to M.S. and G.A.V. by the National Science Foundation through XSEDE (Grant TG-MCA94P017, supercomputers Stampede and Gordon), and also by the Blue Waters computing project at the National Center for Supercomputing Applications (University of Illinois at Urbana–Champaign, NSF Awards OCI-0725070 and ACI-1238993). A.Š. acknowledges support from the Human Frontier Science Program and Royal Society. J.M.H. and K.Y.C.L. acknowledge the support from the National Science Foundation (Grant MCB-1413613) and the NSF-supported MRSEC program at the University of Chicago (Grant DMR-1420709). We are grateful to Carsten Mim and Vinzenz Unger of Northwestern University for generously providing us with the protein. We thank all the members of the Voth group for fruitful discussions, especially John M. A. Grime.","publisher":"American Chemical Society","publication_status":"published","publication_identifier":{"eissn":["2374-7951"],"issn":["2374-7943"]},"month":"11","doi":"10.1021/acscentsci.7b00392","language":[{"iso":"eng"}],"tmp":{"name":"Creative Commons Attribution 4.0 International Public License (CC-BY 4.0)","legal_code_url":"https://creativecommons.org/licenses/by/4.0/legalcode","short":"CC BY (4.0)","image":"/images/cc_by.png"},"main_file_link":[{"open_access":"1","url":"https://pubs.acs.org/doi/10.1021/acscentsci.7b00392"}],"external_id":{"pmid":["29296664"]},"oa":1,"quality_controlled":"1","issue":"12","abstract":[{"lang":"eng","text":"Biological membranes have a central role in mediating the organization of membrane-curving proteins, a dynamic process that has proven to be challenging to probe experimentally. Using atomic force microscopy, we capture the hierarchically organized assemblies of Bin/amphiphysin/Rvs (BAR) proteins on supported lipid membranes. Their structure reveals distinct long linear aggregates of proteins, regularly spaced by up to 300 nm. Employing accurate free-energy calculations from large-scale coarse-grained computer simulations, we found that the membrane mediates the interaction among protein filaments as a combination of short- and long-ranged interactions. The long-ranged component acts at strikingly long distances, giving rise to a variety of micron-sized ordered patterns. This mechanism may contribute to the long-ranged spatiotemporal control of membrane remodeling by proteins in the cell."}],"type":"journal_article","oa_version":"Published Version","file":[{"date_created":"2021-11-29T09:00:40Z","date_updated":"2021-11-29T09:00:40Z","checksum":"1cf3e5e5342f2d728f47560acc3ec560","success":1,"relation":"main_file","file_id":"10371","file_size":2635263,"content_type":"application/pdf","creator":"cchlebak","file_name":"2017_ACSCentSci_Simunovic.pdf","access_level":"open_access"}],"user_id":"8b945eb4-e2f2-11eb-945a-df72226e66a9","_id":"10369","intvolume":" 3","ddc":["540"],"status":"public","title":"Long-range organization of membrane-curving proteins","has_accepted_license":"1","article_processing_charge":"No","day":"21","scopus_import":"1","keyword":["general chemical engineering","general chemistry"],"date_published":"2017-11-21T00:00:00Z","citation":{"mla":"Simunovic, Mijo, et al. “Long-Range Organization of Membrane-Curving Proteins.” ACS Central Science, vol. 3, no. 12, American Chemical Society, 2017, pp. 1246–53, doi:10.1021/acscentsci.7b00392.","short":"M. Simunovic, A. Šarić, J.M. Henderson, K.Y.C. Lee, G.A. Voth, ACS Central Science 3 (2017) 1246–1253.","chicago":"Simunovic, Mijo, Anđela Šarić, J. Michael Henderson, Ka Yee C. Lee, and Gregory A. Voth. “Long-Range Organization of Membrane-Curving Proteins.” ACS Central Science. American Chemical Society, 2017. https://doi.org/10.1021/acscentsci.7b00392.","ama":"Simunovic M, Šarić A, Henderson JM, Lee KYC, Voth GA. Long-range organization of membrane-curving proteins. ACS Central Science. 2017;3(12):1246-1253. doi:10.1021/acscentsci.7b00392","ista":"Simunovic M, Šarić A, Henderson JM, Lee KYC, Voth GA. 2017. Long-range organization of membrane-curving proteins. ACS Central Science. 3(12), 1246–1253.","apa":"Simunovic, M., Šarić, A., Henderson, J. M., Lee, K. Y. C., & Voth, G. A. (2017). Long-range organization of membrane-curving proteins. ACS Central Science. American Chemical Society. https://doi.org/10.1021/acscentsci.7b00392","ieee":"M. Simunovic, A. Šarić, J. M. Henderson, K. Y. C. Lee, and G. A. Voth, “Long-range organization of membrane-curving proteins,” ACS Central Science, vol. 3, no. 12. American Chemical Society, pp. 1246–1253, 2017."},"publication":"ACS Central Science","page":"1246-1253","article_type":"original"},{"publication_identifier":{"issn":["1631-0748"]},"month":"02","quality_controlled":"1","tmp":{"name":"Creative Commons Attribution-NonCommercial-NoDerivatives 4.0 International (CC BY-NC-ND 4.0)","legal_code_url":"https://creativecommons.org/licenses/by-nc-nd/4.0/legalcode","short":"CC BY-NC-ND (4.0)","image":"/images/cc_by_nc_nd.png"},"oa":1,"language":[{"iso":"eng"}],"doi":"10.1016/j.crci.2015.12.004","license":"https://creativecommons.org/licenses/by-nc-nd/4.0/","extern":"1","file_date_updated":"2021-01-22T12:36:52Z","publisher":"Elsevier","publication_status":"published","year":"2016","volume":19,"date_created":"2021-01-19T11:11:54Z","date_updated":"2023-02-23T13:46:55Z","author":[{"last_name":"Bakail","first_name":"May M","orcid":"0000-0002-9592-1587","id":"FB3C3F8E-522F-11EA-B186-22963DDC885E","full_name":"Bakail, May M"},{"full_name":"Ochsenbein, Francoise","first_name":"Francoise","last_name":"Ochsenbein"}],"keyword":["General Chemistry","General Chemical Engineering"],"article_processing_charge":"No","has_accepted_license":"1","day":"06","page":"19-27","article_type":"original","citation":{"ama":"Bakail MM, Ochsenbein F. Targeting protein–protein interactions, a wide open field for drug design. Comptes Rendus Chimie. 2016;19(1-2):19-27. doi:10.1016/j.crci.2015.12.004","ista":"Bakail MM, Ochsenbein F. 2016. Targeting protein–protein interactions, a wide open field for drug design. Comptes Rendus Chimie. 19(1–2), 19–27.","ieee":"M. M. Bakail and F. Ochsenbein, “Targeting protein–protein interactions, a wide open field for drug design,” Comptes Rendus Chimie, vol. 19, no. 1–2. Elsevier, pp. 19–27, 2016.","apa":"Bakail, M. M., & Ochsenbein, F. (2016). Targeting protein–protein interactions, a wide open field for drug design. Comptes Rendus Chimie. Elsevier. https://doi.org/10.1016/j.crci.2015.12.004","mla":"Bakail, May M., and Francoise Ochsenbein. “Targeting Protein–Protein Interactions, a Wide Open Field for Drug Design.” Comptes Rendus Chimie, vol. 19, no. 1–2, Elsevier, 2016, pp. 19–27, doi:10.1016/j.crci.2015.12.004.","short":"M.M. Bakail, F. Ochsenbein, Comptes Rendus Chimie 19 (2016) 19–27.","chicago":"Bakail, May M, and Francoise Ochsenbein. “Targeting Protein–Protein Interactions, a Wide Open Field for Drug Design.” Comptes Rendus Chimie. Elsevier, 2016. https://doi.org/10.1016/j.crci.2015.12.004."},"publication":"Comptes Rendus Chimie","date_published":"2016-02-06T00:00:00Z","type":"journal_article","issue":"1-2","abstract":[{"text":"Targeting protein–protein interactions has long been considered as a very difficult if impossible task, but over the past decade, front lines have moved. The number of successful examples is exponentially growing. This review presents a rapid overview of recent advances in this field considering the strengths and weaknesses of the small molecule approaches and alternative strategies such as the selection or design of artificial antibodies, peptides or peptidomimetics.","lang":"eng"},{"text":"Cibler les interactions protéine–protéine a longtemps été considéré comme une tâche très difficile, voire impossible, mais, depuis les dix dernières années, les lignes ont bougé. Le nombre d’exemples de réussites s’accroît exponentiellement. Cette revue présente un rapide panorama des avancées récentes dans ce domaine, considérant les forces et les faiblesses de l’approche « petite molécule » ainsi que des stratégies alternatives comme la sélection ou le design d’anticorps artificiels, de peptides ou de peptidomimétiques.","lang":"fre"}],"intvolume":" 19","title":"Targeting protein–protein interactions, a wide open field for drug design","status":"public","ddc":["570"],"user_id":"2DF688A6-F248-11E8-B48F-1D18A9856A87","_id":"9019","file":[{"date_created":"2021-01-22T12:36:52Z","date_updated":"2021-01-22T12:36:52Z","success":1,"checksum":"c262814ffdbfe95900256ab9ff42cdf5","file_id":"9035","relation":"main_file","creator":"dernst","file_size":2045260,"content_type":"application/pdf","file_name":"2016_ComptesRendueChimie_Bakail.pdf","access_level":"open_access"}],"oa_version":"Published Version"},{"intvolume":" 7","status":"public","title":"Light-controlled self-assembly of non-photoresponsive nanoparticles","_id":"13394","user_id":"2DF688A6-F248-11E8-B48F-1D18A9856A87","oa_version":"None","type":"journal_article","abstract":[{"lang":"eng","text":"The ability to guide the assembly of nanosized objects reversibly with external stimuli, in particular light, is of fundamental importance, and it contributes to the development of applications as diverse as nanofabrication and controlled drug delivery. However, all the systems described to date are based on nanoparticles (NPs) that are inherently photoresponsive, which makes their preparation cumbersome and can markedly hamper their performance. Here we describe a conceptually new methodology to assemble NPs reversibly using light that does not require the particles to be functionalized with light-responsive ligands. Our strategy is based on the use of a photoswitchable medium that responds to light in such a way that it modulates the interparticle interactions. NP assembly proceeds quantitatively and without apparent fatigue, both in solution and in gels. Exposing the gels to light in a spatially controlled manner allowed us to draw images that spontaneously disappeared after a specific period of time."}],"page":"646-652","article_type":"original","citation":{"ama":"Kundu PK, Samanta D, Leizrowice R, et al. Light-controlled self-assembly of non-photoresponsive nanoparticles. Nature Chemistry. 2015;7:646-652. doi:10.1038/nchem.2303","ieee":"P. K. Kundu et al., “Light-controlled self-assembly of non-photoresponsive nanoparticles,” Nature Chemistry, vol. 7. Springer Nature, pp. 646–652, 2015.","apa":"Kundu, P. K., Samanta, D., Leizrowice, R., Margulis, B., Zhao, H., Börner, M., … Klajn, R. (2015). Light-controlled self-assembly of non-photoresponsive nanoparticles. Nature Chemistry. Springer Nature. https://doi.org/10.1038/nchem.2303","ista":"Kundu PK, Samanta D, Leizrowice R, Margulis B, Zhao H, Börner M, Udayabhaskararao T, Manna D, Klajn R. 2015. Light-controlled self-assembly of non-photoresponsive nanoparticles. Nature Chemistry. 7, 646–652.","short":"P.K. Kundu, D. Samanta, R. Leizrowice, B. Margulis, H. Zhao, M. Börner, T. Udayabhaskararao, D. Manna, R. Klajn, Nature Chemistry 7 (2015) 646–652.","mla":"Kundu, Pintu K., et al. “Light-Controlled Self-Assembly of Non-Photoresponsive Nanoparticles.” Nature Chemistry, vol. 7, Springer Nature, 2015, pp. 646–52, doi:10.1038/nchem.2303.","chicago":"Kundu, Pintu K., Dipak Samanta, Ron Leizrowice, Baruch Margulis, Hui Zhao, Martin Börner, T. Udayabhaskararao, Debasish Manna, and Rafal Klajn. “Light-Controlled Self-Assembly of Non-Photoresponsive Nanoparticles.” Nature Chemistry. Springer Nature, 2015. https://doi.org/10.1038/nchem.2303."},"publication":"Nature Chemistry","date_published":"2015-07-20T00:00:00Z","keyword":["General Chemical Engineering","General Chemistry"],"scopus_import":"1","article_processing_charge":"No","day":"20","publisher":"Springer Nature","publication_status":"published","pmid":1,"year":"2015","volume":7,"date_created":"2023-08-01T09:44:33Z","date_updated":"2023-08-07T13:00:15Z","author":[{"full_name":"Kundu, Pintu K.","first_name":"Pintu K.","last_name":"Kundu"},{"full_name":"Samanta, Dipak","last_name":"Samanta","first_name":"Dipak"},{"full_name":"Leizrowice, Ron","first_name":"Ron","last_name":"Leizrowice"},{"full_name":"Margulis, Baruch","last_name":"Margulis","first_name":"Baruch"},{"full_name":"Zhao, Hui","first_name":"Hui","last_name":"Zhao"},{"first_name":"Martin","last_name":"Börner","full_name":"Börner, Martin"},{"last_name":"Udayabhaskararao","first_name":"T.","full_name":"Udayabhaskararao, T."},{"last_name":"Manna","first_name":"Debasish","full_name":"Manna, Debasish"},{"full_name":"Klajn, Rafal","id":"8e84690e-1e48-11ed-a02b-a1e6fb8bb53b","last_name":"Klajn","first_name":"Rafal"}],"extern":"1","quality_controlled":"1","external_id":{"pmid":["26201741"]},"language":[{"iso":"eng"}],"doi":"10.1038/nchem.2303","publication_identifier":{"issn":["1755-4330"],"eissn":["1755-4349"]},"month":"07"},{"date_published":"2010-10-15T00:00:00Z","page":"2247-2279","article_type":"original","citation":{"chicago":"Klajn, Rafal. “Immobilized Azobenzenes for the Construction of Photoresponsive Materials.” Pure and Applied Chemistry. De Gruyter, 2010. https://doi.org/10.1351/pac-con-10-09-04.","mla":"Klajn, Rafal. “Immobilized Azobenzenes for the Construction of Photoresponsive Materials.” Pure and Applied Chemistry, vol. 82, no. 12, De Gruyter, 2010, pp. 2247–79, doi:10.1351/pac-con-10-09-04.","short":"R. Klajn, Pure and Applied Chemistry 82 (2010) 2247–2279.","ista":"Klajn R. 2010. Immobilized azobenzenes for the construction of photoresponsive materials. Pure and Applied Chemistry. 82(12), 2247–2279.","ieee":"R. Klajn, “Immobilized azobenzenes for the construction of photoresponsive materials,” Pure and Applied Chemistry, vol. 82, no. 12. De Gruyter, pp. 2247–2279, 2010.","apa":"Klajn, R. (2010). Immobilized azobenzenes for the construction of photoresponsive materials. Pure and Applied Chemistry. De Gruyter. https://doi.org/10.1351/pac-con-10-09-04","ama":"Klajn R. Immobilized azobenzenes for the construction of photoresponsive materials. Pure and Applied Chemistry. 2010;82(12):2247-2279. doi:10.1351/pac-con-10-09-04"},"publication":"Pure and Applied Chemistry","article_processing_charge":"No","day":"15","keyword":["General Chemical Engineering","General Chemistry"],"scopus_import":"1","oa_version":"Published Version","intvolume":" 82","title":"Immobilized azobenzenes for the construction of photoresponsive materials","status":"public","_id":"13409","user_id":"2DF688A6-F248-11E8-B48F-1D18A9856A87","issue":"12","abstract":[{"text":"The immobilization of molecular switches onto inorganic supports has recently become a hot topic as it can give rise to novel hybrid materials in which the properties of the two components are mutually enhanced. Even more attractive is the concept of “transferring” the switchable characteristics of single layers of organic molecules onto the underlying inorganic components, rendering them responsive to external stimuli as well. Of the various molecular switches studied, azobenzene (AB) has arguably attracted most attention due to its simple molecular structure, and because its “trigger” (light) is a noninvasive one, it can be delivered instantaneously, and into a precise location. In order to fully realize its potential, however, it is necessary to immobilize AB onto solid supports. It is the goal of this manuscript to comprehensively yet concisely review such hybrid systems which comprise AB forming well-defined self-assembled monolayers (SAMs) on planar and curved (colloidal and nanoporous) inorganic surfaces. I discuss methods to immobilize AB derivatives onto surfaces, strategies to ensure efficient AB isomerization, ways to monitor the switching process, properties of these switchable hybrid materials, and, last but not least, their emerging applications.","lang":"eng"}],"type":"journal_article","language":[{"iso":"eng"}],"doi":"10.1351/pac-con-10-09-04","quality_controlled":"1","oa":1,"main_file_link":[{"url":"https://doi.org/10.1351/pac-con-10-09-04","open_access":"1"}],"publication_identifier":{"issn":["0033-4545"],"eissn":["1365-3075"]},"month":"10","volume":82,"date_created":"2023-08-01T09:48:11Z","date_updated":"2023-08-08T07:58:13Z","author":[{"full_name":"Klajn, Rafal","first_name":"Rafal","last_name":"Klajn","id":"8e84690e-1e48-11ed-a02b-a1e6fb8bb53b"}],"publisher":"De Gruyter","publication_status":"published","year":"2010","extern":"1"},{"publication_identifier":{"issn":["1755-4330"],"eissn":["1755-4349"]},"month":"12","external_id":{"pmid":["21124361"]},"quality_controlled":"1","doi":"10.1038/nchem.432","language":[{"iso":"eng"}],"extern":"1","pmid":1,"year":"2009","publisher":"Springer Nature","publication_status":"published","author":[{"full_name":"Klajn, Rafal","first_name":"Rafal","last_name":"Klajn","id":"8e84690e-1e48-11ed-a02b-a1e6fb8bb53b"},{"last_name":"Olson","first_name":"Mark A.","full_name":"Olson, Mark A."},{"first_name":"Paul J.","last_name":"Wesson","full_name":"Wesson, Paul J."},{"last_name":"Fang","first_name":"Lei","full_name":"Fang, Lei"},{"first_name":"Ali","last_name":"Coskun","full_name":"Coskun, Ali"},{"first_name":"Ali","last_name":"Trabolsi","full_name":"Trabolsi, Ali"},{"last_name":"Soh","first_name":"Siowling","full_name":"Soh, Siowling"},{"first_name":"J. Fraser","last_name":"Stoddart","full_name":"Stoddart, J. Fraser"},{"full_name":"Grzybowski, Bartosz A.","first_name":"Bartosz A.","last_name":"Grzybowski"}],"volume":1,"date_created":"2023-08-01T09:50:23Z","date_updated":"2023-08-08T08:55:36Z","scopus_import":"1","keyword":["General Chemical Engineering","General Chemistry"],"article_processing_charge":"No","day":"01","citation":{"short":"R. Klajn, M.A. Olson, P.J. Wesson, L. Fang, A. Coskun, A. Trabolsi, S. Soh, J.F. Stoddart, B.A. Grzybowski, Nature Chemistry 1 (2009) 733–738.","mla":"Klajn, Rafal, et al. “Dynamic Hook-and-Eye Nanoparticle Sponges.” Nature Chemistry, vol. 1, Springer Nature, 2009, pp. 733–38, doi:10.1038/nchem.432.","chicago":"Klajn, Rafal, Mark A. Olson, Paul J. Wesson, Lei Fang, Ali Coskun, Ali Trabolsi, Siowling Soh, J. Fraser Stoddart, and Bartosz A. Grzybowski. “Dynamic Hook-and-Eye Nanoparticle Sponges.” Nature Chemistry. Springer Nature, 2009. https://doi.org/10.1038/nchem.432.","ama":"Klajn R, Olson MA, Wesson PJ, et al. Dynamic hook-and-eye nanoparticle sponges. Nature Chemistry. 2009;1:733-738. doi:10.1038/nchem.432","apa":"Klajn, R., Olson, M. A., Wesson, P. J., Fang, L., Coskun, A., Trabolsi, A., … Grzybowski, B. A. (2009). Dynamic hook-and-eye nanoparticle sponges. Nature Chemistry. Springer Nature. https://doi.org/10.1038/nchem.432","ieee":"R. Klajn et al., “Dynamic hook-and-eye nanoparticle sponges,” Nature Chemistry, vol. 1. Springer Nature, pp. 733–738, 2009.","ista":"Klajn R, Olson MA, Wesson PJ, Fang L, Coskun A, Trabolsi A, Soh S, Stoddart JF, Grzybowski BA. 2009. Dynamic hook-and-eye nanoparticle sponges. Nature Chemistry. 1, 733–738."},"publication":"Nature Chemistry","page":"733-738","article_type":"original","date_published":"2009-12-01T00:00:00Z","type":"journal_article","abstract":[{"lang":"eng","text":"Systems in which nanoscale components of different types can be captured and/or released from organic scaffolds provide a fertile basis for the construction of dynamic, exchangeable functional materials. In such heterogeneous systems, the components interact with one another by means of programmable, noncovalent bonding interactions. Herein, we describe polymers that capture and release functionalized nanoparticles selectively during redox-controlled aggregation and disaggregation, respectively. The interactions between the polymer and the NPs are mediated by the reversible formation of polypseudorotaxanes, and give rise to architectures ranging from short chains composed of few nanoparticles to extended networks of nanoparticles crosslinked by the polymer. In the latter case, the polymer/nanoparticle aggregates precipitate from solution such that the polymer acts as a selective ‘sponge’ for the capture/release of the nanoparticles of different types."}],"user_id":"2DF688A6-F248-11E8-B48F-1D18A9856A87","_id":"13415","intvolume":" 1","title":"Dynamic hook-and-eye nanoparticle sponges","status":"public","oa_version":"None"}]