---
_id: '14435'
abstract:
- lang: eng
text: Low‐cost, safe, and environmental‐friendly rechargeable aqueous zinc‐ion batteries
(ZIBs) are promising as next‐generation energy storage devices for wearable electronics
among other applications. However, sluggish ionic transport kinetics and the unstable
electrode structure during ionic insertion/extraction hampers their deployment.
Herein, we propose a new cathode material based on a layered metal chalcogenide
(LMC), bismuth telluride (Bi2Te3), coated
with polypyrrole (PPy). Taking advantage of the PPy coating, the Bi2Te3@PPy
composite presents strong ionic absorption affinity, high oxidation resistance,
and high structural stability. The ZIBs based on Bi2Te3@PPy
cathodes exhibit high capacities and ultra‐long lifespans of over 5000 cycles.
They also present outstanding stability even under bending. In addition, we analyze
here the reaction mechanism using in situ X‐ray diffraction, X‐ray photoelectron
spectroscopy, and computational tools and demonstrate that, in the aqueous system,
Zn2+ is not inserted into the cathode as previously assumed.
In contrast, proton charge storage dominates the process. Overall, this work not
only shows the great potential of LMCs as ZIBs cathode materials and the advantages
of PPy coating, but also clarifies the charge/discharge mechanism in rechargeable
ZIBs based on LMCs.
acknowledged_ssus:
- _id: EM-Fac
acknowledgement: G.Z. and Q.S. contributed equally to this work. This work was supported
by the National Natural Science Foundation of China (52105329, 52175300) and the
Heilongjiang Provincial Natural Science Foundation of China (LH2022E059). G.Z.,
X.L., and C.Z. thank the China Scholarship Council (CSC) for the scholarship support.
This research was supported by the Scientific Service Units of ISTA through resources
provided by the Electron Microscopy Facility. S.H. and M.I. acknowledge funding
by ISTA and Werner Siemens.
article_number: '2305128'
article_processing_charge: No
article_type: original
author:
- first_name: Guifang
full_name: Zeng, Guifang
last_name: Zeng
- first_name: Qing
full_name: Sun, Qing
last_name: Sun
- first_name: Sharona
full_name: Horta, Sharona
id: 03a7e858-01b1-11ec-8b71-99ae6c4a05bc
last_name: Horta
- first_name: Shang
full_name: Wang, Shang
last_name: Wang
- first_name: Xuan
full_name: Lu, Xuan
last_name: Lu
- first_name: Chaoyue
full_name: Zhang, Chaoyue
last_name: Zhang
- first_name: Jing
full_name: Li, Jing
last_name: Li
- first_name: Junshan
full_name: Li, Junshan
last_name: Li
- first_name: Lijie
full_name: Ci, Lijie
last_name: Ci
- first_name: Yanhong
full_name: Tian, Yanhong
last_name: Tian
- first_name: Maria
full_name: Ibáñez, Maria
id: 43C61214-F248-11E8-B48F-1D18A9856A87
last_name: Ibáñez
orcid: 0000-0001-5013-2843
- first_name: Andreu
full_name: Cabot, Andreu
last_name: Cabot
citation:
ama: 'Zeng G, Sun Q, Horta S, et al. A layered Bi2Te3@PPy cathode for aqueous zinc
ion batteries: Mechanism and application in printed flexible batteries. Advanced
Materials. 2024;36(1). doi:10.1002/adma.202305128'
apa: 'Zeng, G., Sun, Q., Horta, S., Wang, S., Lu, X., Zhang, C., … Cabot, A. (2024).
A layered Bi2Te3@PPy cathode for aqueous zinc ion batteries: Mechanism and application
in printed flexible batteries. Advanced Materials. Wiley. https://doi.org/10.1002/adma.202305128'
chicago: 'Zeng, Guifang, Qing Sun, Sharona Horta, Shang Wang, Xuan Lu, Chaoyue Zhang,
Jing Li, et al. “A Layered Bi2Te3@PPy Cathode for Aqueous Zinc Ion Batteries:
Mechanism and Application in Printed Flexible Batteries.” Advanced Materials.
Wiley, 2024. https://doi.org/10.1002/adma.202305128.'
ieee: 'G. Zeng et al., “A layered Bi2Te3@PPy cathode for aqueous zinc ion
batteries: Mechanism and application in printed flexible batteries,” Advanced
Materials, vol. 36, no. 1. Wiley, 2024.'
ista: 'Zeng G, Sun Q, Horta S, Wang S, Lu X, Zhang C, Li J, Li J, Ci L, Tian Y,
Ibáñez M, Cabot A. 2024. A layered Bi2Te3@PPy cathode for aqueous zinc ion batteries:
Mechanism and application in printed flexible batteries. Advanced Materials. 36(1),
2305128.'
mla: 'Zeng, Guifang, et al. “A Layered Bi2Te3@PPy Cathode for Aqueous Zinc Ion Batteries:
Mechanism and Application in Printed Flexible Batteries.” Advanced Materials,
vol. 36, no. 1, 2305128, Wiley, 2024, doi:10.1002/adma.202305128.'
short: G. Zeng, Q. Sun, S. Horta, S. Wang, X. Lu, C. Zhang, J. Li, J. Li, L. Ci,
Y. Tian, M. Ibáñez, A. Cabot, Advanced Materials 36 (2024).
date_created: 2023-10-17T10:53:56Z
date_published: 2024-01-04T00:00:00Z
date_updated: 2025-04-15T06:36:40Z
day: '04'
department:
- _id: MaIb
doi: 10.1002/adma.202305128
external_id:
isi:
- '001085681000001'
pmid:
- '37555532'
intvolume: ' 36'
isi: 1
issue: '1'
keyword:
- Mechanical Engineering
- Mechanics of Materials
- General Materials Science
language:
- iso: eng
month: '01'
oa_version: None
pmid: 1
project:
- _id: 9B8F7476-BA93-11EA-9121-9846C619BF3A
name: 'HighTE: The Werner Siemens Laboratory for the High Throughput Discovery of
Semiconductors for Waste Heat Recovery'
publication: Advanced Materials
publication_identifier:
eissn:
- 1521-4095
issn:
- 0935-9648
publication_status: published
publisher: Wiley
quality_controlled: '1'
scopus_import: '1'
status: public
title: 'A layered Bi2Te3@PPy cathode for aqueous zinc ion batteries: Mechanism and
application in printed flexible batteries'
type: journal_article
user_id: 2DF688A6-F248-11E8-B48F-1D18A9856A87
volume: 36
year: '2024'
...
---
OA_place: publisher
OA_type: hybrid
_id: '15018'
abstract:
- lang: eng
text: The epitaxial growth of a strained Ge layer, which is a promising candidate
for the channel material of a hole spin qubit, has been demonstrated on 300 mm
Si wafers using commercially available Si0.3Ge0.7 strain relaxed buffer (SRB)
layers. The assessment of the layer and the interface qualities for a buried strained
Ge layer embedded in Si0.3Ge0.7 layers is reported. The XRD reciprocal space mapping
confirmed that the reduction of the growth temperature enables the 2-dimensional
growth of the Ge layer fully strained with respect to the Si0.3Ge0.7. Nevertheless,
dislocations at the top and/or bottom interface of the Ge layer were observed
by means of electron channeling contrast imaging, suggesting the importance of
the careful dislocation assessment. The interface abruptness does not depend on
the selection of the precursor gases, but it is strongly influenced by the growth
temperature which affects the coverage of the surface H-passivation. The mobility
of 2.7 × 105 cm2/Vs is promising, while the low percolation density of 3 × 1010
/cm2 measured with a Hall-bar device at 7 K illustrates the high quality of the
heterostructure thanks to the high Si0.3Ge0.7 SRB quality.
acknowledgement: The Ge project received funding from the European Union's Horizon
Europe programme under the Grant Agreement 101069515 – IGNITE. Siltronic AG is acknowledged
for providing the SRB wafers. This work was supported by Imec's Industrial Affiliation
Program on Quantum Computing.
article_number: '108231'
article_processing_charge: Yes (in subscription journal)
article_type: original
author:
- first_name: Yosuke
full_name: Shimura, Yosuke
last_name: Shimura
- first_name: Clement
full_name: Godfrin, Clement
last_name: Godfrin
- first_name: Andriy
full_name: Hikavyy, Andriy
last_name: Hikavyy
- first_name: Roy
full_name: Li, Roy
last_name: Li
- first_name: Juan L
full_name: Aguilera Servin, Juan L
id: 2A67C376-F248-11E8-B48F-1D18A9856A87
last_name: Aguilera Servin
orcid: 0000-0002-2862-8372
- first_name: Georgios
full_name: Katsaros, Georgios
id: 38DB5788-F248-11E8-B48F-1D18A9856A87
last_name: Katsaros
orcid: 0000-0001-8342-202X
- first_name: Paola
full_name: Favia, Paola
last_name: Favia
- first_name: Han
full_name: Han, Han
last_name: Han
- first_name: Danny
full_name: Wan, Danny
last_name: Wan
- first_name: Kristiaan
full_name: de Greve, Kristiaan
last_name: de Greve
- first_name: Roger
full_name: Loo, Roger
last_name: Loo
citation:
ama: Shimura Y, Godfrin C, Hikavyy A, et al. Compressively strained epitaxial Ge
layers for quantum computing applications. Materials Science in Semiconductor
Processing. 2024;174(5). doi:10.1016/j.mssp.2024.108231
apa: Shimura, Y., Godfrin, C., Hikavyy, A., Li, R., Aguilera Servin, J. L., Katsaros,
G., … Loo, R. (2024). Compressively strained epitaxial Ge layers for quantum computing
applications. Materials Science in Semiconductor Processing. Elsevier.
https://doi.org/10.1016/j.mssp.2024.108231
chicago: Shimura, Yosuke, Clement Godfrin, Andriy Hikavyy, Roy Li, Juan L Aguilera
Servin, Georgios Katsaros, Paola Favia, et al. “Compressively Strained Epitaxial
Ge Layers for Quantum Computing Applications.” Materials Science in Semiconductor
Processing. Elsevier, 2024. https://doi.org/10.1016/j.mssp.2024.108231.
ieee: Y. Shimura et al., “Compressively strained epitaxial Ge layers for
quantum computing applications,” Materials Science in Semiconductor Processing,
vol. 174, no. 5. Elsevier, 2024.
ista: Shimura Y, Godfrin C, Hikavyy A, Li R, Aguilera Servin JL, Katsaros G, Favia
P, Han H, Wan D, de Greve K, Loo R. 2024. Compressively strained epitaxial Ge
layers for quantum computing applications. Materials Science in Semiconductor
Processing. 174(5), 108231.
mla: Shimura, Yosuke, et al. “Compressively Strained Epitaxial Ge Layers for Quantum
Computing Applications.” Materials Science in Semiconductor Processing,
vol. 174, no. 5, 108231, Elsevier, 2024, doi:10.1016/j.mssp.2024.108231.
short: Y. Shimura, C. Godfrin, A. Hikavyy, R. Li, J.L. Aguilera Servin, G. Katsaros,
P. Favia, H. Han, D. Wan, K. de Greve, R. Loo, Materials Science in Semiconductor
Processing 174 (2024).
date_created: 2024-02-22T14:10:40Z
date_published: 2024-05-20T00:00:00Z
date_updated: 2025-04-14T08:01:27Z
day: '20'
ddc:
- '530'
department:
- _id: GeKa
- _id: NanoFab
doi: 10.1016/j.mssp.2024.108231
external_id:
isi:
- '001188520000001'
file:
- access_level: open_access
checksum: 62e8e9ae960387a3dca32ec7f5e413ab
content_type: application/pdf
creator: dernst
date_created: 2024-07-22T11:56:08Z
date_updated: 2024-07-22T11:56:08Z
file_id: '17312'
file_name: 2024_MaterialsScience_Shimura.pdf
file_size: 4220165
relation: main_file
success: 1
file_date_updated: 2024-07-22T11:56:08Z
has_accepted_license: '1'
intvolume: ' 174'
isi: 1
issue: '5'
keyword:
- Mechanical Engineering
- Mechanics of Materials
- Condensed Matter Physics
- General Materials Science
language:
- iso: eng
month: '05'
oa: 1
oa_version: Published Version
project:
- _id: 34c0acea-11ca-11ed-8bc3-8775e10fd452
grant_number: '101069515'
name: Integrated Germanium Quantum Technology
publication: Materials Science in Semiconductor Processing
publication_identifier:
issn:
- 1369-8001
publication_status: published
publisher: Elsevier
quality_controlled: '1'
scopus_import: '1'
status: public
title: Compressively strained epitaxial Ge layers for quantum computing applications
tmp:
image: /images/cc_by.png
legal_code_url: https://creativecommons.org/licenses/by/4.0/legalcode
name: Creative Commons Attribution 4.0 International Public License (CC-BY 4.0)
short: CC BY (4.0)
type: journal_article
user_id: 2DF688A6-F248-11E8-B48F-1D18A9856A87
volume: 174
year: '2024'
...
---
_id: '14434'
abstract:
- lang: eng
text: High entropy alloys (HEAs) are highly suitable candidate catalysts for oxygen
evolution and reduction reactions (OER/ORR) as they offer numerous parameters
for optimizing the electronic structure and catalytic sites. Herein, FeCoNiMoW
HEA nanoparticles are synthesized using a solution‐based low‐temperature approach.
Such FeCoNiMoW nanoparticles show high entropy properties, subtle lattice distortions,
and modulated electronic structure, leading to superior OER performance with an
overpotential of 233 mV at 10 mA cm−2 and 276 mV at 100 mA cm−2.
Density functional theory calculations reveal the electronic structures of the
FeCoNiMoW active sites with an optimized d‐band center position that enables suitable
adsorption of OOH* intermediates and reduces the Gibbs free energy barrier in
the OER process. Aqueous zinc–air batteries (ZABs) based on this HEA demonstrate
a high open circuit potential of 1.59 V, a peak power density of 116.9 mW cm−2,
a specific capacity of 857 mAh gZn−1,
and excellent stability for over 660 h of continuous charge–discharge cycles.
Flexible and solid ZABs are also assembled and tested, displaying excellent charge–discharge
performance at different bending angles. This work shows the significance of 4d/5d
metal‐modulated electronic structure and optimized adsorption ability to improve
the performance of OER/ORR, ZABs, and beyond.
acknowledged_ssus:
- _id: EM-Fac
acknowledgement: The authors acknowledge funding from Generalitat de Catalunya 2021
SGR 01581; the project COMBENERGY, PID2019-105490RB-C32, from the Spanish Ministerio
de Ciencia e Innovación; the National Natural Science Foundation of China (22102002);
the Anhui Provincial Natural Science Foundation (2108085QE192); Zhejiang Province
key research and development project (2023C01191); the Foundation of State Key Laboratory
of High-efficiency Utilization of Coal and Green Chemical Engineering (GrantNo.2022-K31);
and The Key Research and Development Program of Hebei Province (20314305D). IREC
is funded by the CERCA Programme from the Generalitat de Catalunya. L.L.Y. thanks
the China Scholarship Council (CSC) for the scholarship support (202008130132).
This research was supported by the Scientific Service Units (SSU) of ISTA (Institute
of Science and Technology Austria) through resources provided by the Electron Microscopy
Facility (EMF). S.L., S.H., and M.I. acknowledge funding by ISTA and the Werner
Siemens.
article_number: '2303719'
article_processing_charge: No
article_type: original
author:
- first_name: Ren
full_name: He, Ren
last_name: He
- first_name: Linlin
full_name: Yang, Linlin
last_name: Yang
- first_name: Yu
full_name: Zhang, Yu
last_name: Zhang
- first_name: Daochuan
full_name: Jiang, Daochuan
last_name: Jiang
- first_name: Seungho
full_name: Lee, Seungho
id: BB243B88-D767-11E9-B658-BC13E6697425
last_name: Lee
orcid: 0000-0002-6962-8598
- first_name: Sharona
full_name: Horta, Sharona
id: 03a7e858-01b1-11ec-8b71-99ae6c4a05bc
last_name: Horta
- first_name: Zhifu
full_name: Liang, Zhifu
last_name: Liang
- first_name: Xuan
full_name: Lu, Xuan
last_name: Lu
- first_name: Ahmad
full_name: Ostovari Moghaddam, Ahmad
last_name: Ostovari Moghaddam
- first_name: Junshan
full_name: Li, Junshan
last_name: Li
- first_name: Maria
full_name: Ibáñez, Maria
id: 43C61214-F248-11E8-B48F-1D18A9856A87
last_name: Ibáñez
orcid: 0000-0001-5013-2843
- first_name: Ying
full_name: Xu, Ying
last_name: Xu
- first_name: Yingtang
full_name: Zhou, Yingtang
last_name: Zhou
- first_name: Andreu
full_name: Cabot, Andreu
last_name: Cabot
citation:
ama: He R, Yang L, Zhang Y, et al. A 3d‐4d‐5d high entropy alloy as a bifunctional
oxygen catalyst for robust aqueous zinc–air batteries. Advanced Materials.
2023;35(46). doi:10.1002/adma.202303719
apa: He, R., Yang, L., Zhang, Y., Jiang, D., Lee, S., Horta, S., … Cabot, A. (2023).
A 3d‐4d‐5d high entropy alloy as a bifunctional oxygen catalyst for robust aqueous
zinc–air batteries. Advanced Materials. Wiley. https://doi.org/10.1002/adma.202303719
chicago: He, Ren, Linlin Yang, Yu Zhang, Daochuan Jiang, Seungho Lee, Sharona Horta,
Zhifu Liang, et al. “A 3d‐4d‐5d High Entropy Alloy as a Bifunctional Oxygen Catalyst
for Robust Aqueous Zinc–Air Batteries.” Advanced Materials. Wiley, 2023.
https://doi.org/10.1002/adma.202303719.
ieee: R. He et al., “A 3d‐4d‐5d high entropy alloy as a bifunctional oxygen
catalyst for robust aqueous zinc–air batteries,” Advanced Materials, vol.
35, no. 46. Wiley, 2023.
ista: He R, Yang L, Zhang Y, Jiang D, Lee S, Horta S, Liang Z, Lu X, Ostovari Moghaddam
A, Li J, Ibáñez M, Xu Y, Zhou Y, Cabot A. 2023. A 3d‐4d‐5d high entropy alloy
as a bifunctional oxygen catalyst for robust aqueous zinc–air batteries. Advanced
Materials. 35(46), 2303719.
mla: He, Ren, et al. “A 3d‐4d‐5d High Entropy Alloy as a Bifunctional Oxygen Catalyst
for Robust Aqueous Zinc–Air Batteries.” Advanced Materials, vol. 35, no.
46, 2303719, Wiley, 2023, doi:10.1002/adma.202303719.
short: R. He, L. Yang, Y. Zhang, D. Jiang, S. Lee, S. Horta, Z. Liang, X. Lu, A.
Ostovari Moghaddam, J. Li, M. Ibáñez, Y. Xu, Y. Zhou, A. Cabot, Advanced Materials
35 (2023).
date_created: 2023-10-17T10:52:23Z
date_published: 2023-11-16T00:00:00Z
date_updated: 2025-04-15T06:36:40Z
day: '16'
department:
- _id: MaIb
doi: 10.1002/adma.202303719
external_id:
isi:
- '001083876900001'
pmid:
- '37487245'
intvolume: ' 35'
isi: 1
issue: '46'
keyword:
- Mechanical Engineering
- Mechanics of Materials
- General Materials Science
language:
- iso: eng
month: '11'
oa_version: None
pmid: 1
project:
- _id: 9B8F7476-BA93-11EA-9121-9846C619BF3A
name: 'HighTE: The Werner Siemens Laboratory for the High Throughput Discovery of
Semiconductors for Waste Heat Recovery'
publication: Advanced Materials
publication_identifier:
eissn:
- 1521-4095
issn:
- 0935-9648
publication_status: published
publisher: Wiley
quality_controlled: '1'
scopus_import: '1'
status: public
title: A 3d‐4d‐5d high entropy alloy as a bifunctional oxygen catalyst for robust
aqueous zinc–air batteries
type: journal_article
user_id: 2DF688A6-F248-11E8-B48F-1D18A9856A87
volume: 35
year: '2023'
...
---
_id: '12137'
abstract:
- lang: eng
text: We investigate the local self-sustained process underlying spiral turbulence
in counter-rotating Taylor–Couette flow using a periodic annular domain, shaped
as a parallelogram, two of whose sides are aligned with the cylindrical helix
described by the spiral pattern. The primary focus of the study is placed on the
emergence of drifting–rotating waves (DRW) that capture, in a relatively small
domain, the main features of coherent structures typically observed in developed
turbulence. The transitional dynamics of the subcritical region, far below the
first instability of the laminar circular Couette flow, is determined by the upper
and lower branches of DRW solutions originated at saddle-node bifurcations. The
mechanism whereby these solutions self-sustain, and the chaotic dynamics they
induce, are conspicuously reminiscent of other subcritical shear flows. Remarkably,
the flow properties of DRW persist even as the Reynolds number is increased beyond
the linear stability threshold of the base flow. Simulations in a narrow parallelogram
domain stretched in the azimuthal direction to revolve around the apparatus a
full turn confirm that self-sustained vortices eventually concentrate into a localised
pattern. The resulting statistical steady state satisfactorily reproduces qualitatively,
and to a certain degree also quantitatively, the topology and properties of spiral
turbulence as calculated in a large periodic domain of sufficient aspect ratio
that is representative of the real system.
acknowledgement: "K.D.’s research was supported by an Australian Research Council
Discovery Early Career\r\nResearcher Award (DE170100171). B.W., R.A., F.M. and A.M.
research was supported by the Spanish Ministerio de Economía y Competitivdad (grant
numbers FIS2016-77849-R and FIS2017-85794-P) and Ministerio de Ciencia e Innovación
(grant number PID2020-114043GB-I00) and the Generalitat de Catalunya (grant 2017-SGR-785).
B.W.’s research was also supported by the Chinese Scholarship Council (grant CSC
no. 201806440152)."
article_number: A21
article_processing_charge: No
article_type: original
arxiv: 1
author:
- first_name: B.
full_name: Wang, B.
last_name: Wang
- first_name: Roger
full_name: Ayats López, Roger
id: ab77522d-073b-11ed-8aff-e71b39258362
last_name: Ayats López
orcid: 0000-0001-6572-0621
- first_name: K.
full_name: Deguchi, K.
last_name: Deguchi
- first_name: F.
full_name: Mellibovsky, F.
last_name: Mellibovsky
- first_name: A.
full_name: Meseguer, A.
last_name: Meseguer
citation:
ama: Wang B, Ayats López R, Deguchi K, Mellibovsky F, Meseguer A. Self-sustainment
of coherent structures in counter-rotating Taylor–Couette flow. Journal of
Fluid Mechanics. 2022;951. doi:10.1017/jfm.2022.828
apa: Wang, B., Ayats López, R., Deguchi, K., Mellibovsky, F., & Meseguer, A.
(2022). Self-sustainment of coherent structures in counter-rotating Taylor–Couette
flow. Journal of Fluid Mechanics. Cambridge University Press. https://doi.org/10.1017/jfm.2022.828
chicago: Wang, B., Roger Ayats López, K. Deguchi, F. Mellibovsky, and A. Meseguer.
“Self-Sustainment of Coherent Structures in Counter-Rotating Taylor–Couette Flow.”
Journal of Fluid Mechanics. Cambridge University Press, 2022. https://doi.org/10.1017/jfm.2022.828.
ieee: B. Wang, R. Ayats López, K. Deguchi, F. Mellibovsky, and A. Meseguer, “Self-sustainment
of coherent structures in counter-rotating Taylor–Couette flow,” Journal of
Fluid Mechanics, vol. 951. Cambridge University Press, 2022.
ista: Wang B, Ayats López R, Deguchi K, Mellibovsky F, Meseguer A. 2022. Self-sustainment
of coherent structures in counter-rotating Taylor–Couette flow. Journal of Fluid
Mechanics. 951, A21.
mla: Wang, B., et al. “Self-Sustainment of Coherent Structures in Counter-Rotating
Taylor–Couette Flow.” Journal of Fluid Mechanics, vol. 951, A21, Cambridge
University Press, 2022, doi:10.1017/jfm.2022.828.
short: B. Wang, R. Ayats López, K. Deguchi, F. Mellibovsky, A. Meseguer, Journal
of Fluid Mechanics 951 (2022).
date_created: 2023-01-12T12:04:17Z
date_published: 2022-11-07T00:00:00Z
date_updated: 2023-08-04T08:54:16Z
day: '07'
department:
- _id: BjHo
doi: 10.1017/jfm.2022.828
external_id:
arxiv:
- '2207.12990'
isi:
- '000879446900001'
intvolume: ' 951'
isi: 1
keyword:
- Mechanical Engineering
- Mechanics of Materials
- Condensed Matter Physics
- Applied Mathematics
language:
- iso: eng
main_file_link:
- open_access: '1'
url: ' https://doi.org/10.48550/arXiv.2207.12990'
month: '11'
oa: 1
oa_version: Preprint
publication: Journal of Fluid Mechanics
publication_identifier:
eissn:
- 1469-7645
issn:
- 0022-1120
publication_status: published
publisher: Cambridge University Press
quality_controlled: '1'
scopus_import: '1'
status: public
title: Self-sustainment of coherent structures in counter-rotating Taylor–Couette
flow
type: journal_article
user_id: 4359f0d1-fa6c-11eb-b949-802e58b17ae8
volume: 951
year: '2022'
...
---
_id: '12146'
abstract:
- lang: eng
text: 'In this paper, we explore the stability and dynamical relevance of a wide
variety of steady, time-periodic, quasiperiodic, and chaotic flows arising between
orthogonally stretching parallel plates. We first explore the stability of all
the steady flow solution families formerly identified by Ayats et al. [“Flows
between orthogonally stretching parallel plates,” Phys. Fluids 33, 024103 (2021)],
concluding that only the one that originates from the Stokesian approximation
is actually stable. When both plates are shrinking at identical or nearly the
same deceleration rates, this Stokesian flow exhibits a Hopf bifurcation that
leads to stable time-periodic regimes. The resulting time-periodic orbits or flows
are tracked for different Reynolds numbers and stretching rates while monitoring
their Floquet exponents to identify secondary instabilities. It is found that
these time-periodic flows also exhibit Neimark–Sacker bifurcations, generating
stable quasiperiodic flows (tori) that may sometimes give rise to chaotic dynamics
through a Ruelle–Takens–Newhouse scenario. However, chaotic dynamics is unusually
observed, as the quasiperiodic flows generally become phase-locked through a resonance
mechanism before a strange attractor may arise, thus restoring the time-periodicity
of the flow. In this work, we have identified and tracked four different resonance
regions, also known as Arnold tongues or horns. In particular, the 1 : 4 strong
resonance region is explored in great detail, where the identified scenarios are
in very good agreement with normal form theory. '
acknowledgement: "This work was supported by the Spanish MINECO under Grant Nos. FIS2017-85794-P
and PRX18/00179, the Spanish MICINN through Grant No. PID2020-114043GB-I00, and
the\r\nGeneralitat de Catalunya under Grant No. 2017-SGR-785. B.W.’s research was
also supported by the Chinese Scholarship Council through Grant CSC No. 201806440152."
article_number: '114111'
article_processing_charge: No
article_type: original
author:
- first_name: B.
full_name: Wang, B.
last_name: Wang
- first_name: Roger
full_name: Ayats López, Roger
id: ab77522d-073b-11ed-8aff-e71b39258362
last_name: Ayats López
orcid: 0000-0001-6572-0621
- first_name: A.
full_name: Meseguer, A.
last_name: Meseguer
- first_name: F.
full_name: Marques, F.
last_name: Marques
citation:
ama: Wang B, Ayats López R, Meseguer A, Marques F. Phase-locking flows between orthogonally
stretching parallel plates. Physics of Fluids. 2022;34(11). doi:10.1063/5.0124152
apa: Wang, B., Ayats López, R., Meseguer, A., & Marques, F. (2022). Phase-locking
flows between orthogonally stretching parallel plates. Physics of Fluids.
AIP Publishing. https://doi.org/10.1063/5.0124152
chicago: Wang, B., Roger Ayats López, A. Meseguer, and F. Marques. “Phase-Locking
Flows between Orthogonally Stretching Parallel Plates.” Physics of Fluids.
AIP Publishing, 2022. https://doi.org/10.1063/5.0124152.
ieee: B. Wang, R. Ayats López, A. Meseguer, and F. Marques, “Phase-locking flows
between orthogonally stretching parallel plates,” Physics of Fluids, vol.
34, no. 11. AIP Publishing, 2022.
ista: Wang B, Ayats López R, Meseguer A, Marques F. 2022. Phase-locking flows between
orthogonally stretching parallel plates. Physics of Fluids. 34(11), 114111.
mla: Wang, B., et al. “Phase-Locking Flows between Orthogonally Stretching Parallel
Plates.” Physics of Fluids, vol. 34, no. 11, 114111, AIP Publishing, 2022,
doi:10.1063/5.0124152.
short: B. Wang, R. Ayats López, A. Meseguer, F. Marques, Physics of Fluids 34 (2022).
date_created: 2023-01-12T12:06:58Z
date_published: 2022-11-04T00:00:00Z
date_updated: 2023-10-03T11:07:58Z
day: '04'
department:
- _id: BjHo
doi: 10.1063/5.0124152
external_id:
isi:
- '000880665300024'
intvolume: ' 34'
isi: 1
issue: '11'
keyword:
- Condensed Matter Physics
- Fluid Flow and Transfer Processes
- Mechanics of Materials
- Computational Mechanics
- Mechanical Engineering
language:
- iso: eng
main_file_link:
- open_access: '1'
url: https://upcommons.upc.edu/handle/2117/385635
month: '11'
oa: 1
oa_version: Submitted Version
publication: Physics of Fluids
publication_identifier:
eissn:
- 1089-7666
issn:
- 1070-6631
publication_status: published
publisher: AIP Publishing
quality_controlled: '1'
scopus_import: '1'
status: public
title: Phase-locking flows between orthogonally stretching parallel plates
type: journal_article
user_id: 2DF688A6-F248-11E8-B48F-1D18A9856A87
volume: 34
year: '2022'
...
---
_id: '13355'
abstract:
- lang: eng
text: 'Supramolecular self-assembly in biological systems holds promise to convert
and amplify disease-specific signals to physical or mechanical signals that can
direct cell fate. However, it remains challenging to design physiologically stable
self-assembling systems that demonstrate tunable and predictable behavior. Here,
the use of zwitterionic tetrapeptide modalities to direct nanoparticle assembly
under physiological conditions is reported. The self-assembly of gold nanoparticles
can be activated by enzymatic unveiling of surface-bound zwitterionic tetrapeptides
through matrix metalloprotease-9 (MMP-9), which is overexpressed by cancer cells.
This robust nanoparticle assembly is achieved by multivalent, self-complementary
interactions of the zwitterionic tetrapeptides. In cancer cells that overexpress
MMP-9, the nanoparticle assembly process occurs near the cell membrane and causes
size-induced selection of cellular uptake mechanism, resulting in diminished cell
growth. The enzyme responsiveness, and therefore, indirectly, the uptake route
of the system can be programmed by customizing the peptide sequence: a simple
inversion of the two amino acids at the cleavage site completely inactivates the
enzyme responsiveness, self-assembly, and consequently changes the endocytic pathway.
This robust self-complementary, zwitterionic peptide design demonstrates the use
of enzyme-activated electrostatic side-chain patterns as powerful and customizable
peptide modalities to program nanoparticle self-assembly and alter cellular response
in biological context.'
article_number: '2104962'
article_processing_charge: No
article_type: original
author:
- first_name: Richard H.
full_name: Huang, Richard H.
last_name: Huang
- first_name: Nazia
full_name: Nayeem, Nazia
last_name: Nayeem
- first_name: Ye
full_name: He, Ye
last_name: He
- first_name: Jorge
full_name: Morales, Jorge
last_name: Morales
- first_name: Duncan
full_name: Graham, Duncan
last_name: Graham
- first_name: Rafal
full_name: Klajn, Rafal
id: 8e84690e-1e48-11ed-a02b-a1e6fb8bb53b
last_name: Klajn
- first_name: Maria
full_name: Contel, Maria
last_name: Contel
- first_name: Stephen
full_name: O'Brien, Stephen
last_name: O'Brien
- first_name: Rein V.
full_name: Ulijn, Rein V.
last_name: Ulijn
citation:
ama: Huang RH, Nayeem N, He Y, et al. Self‐complementary zwitterionic peptides direct
nanoparticle assembly and enable enzymatic selection of endocytic pathways. Advanced
Materials. 2022;34(1). doi:10.1002/adma.202104962
apa: Huang, R. H., Nayeem, N., He, Y., Morales, J., Graham, D., Klajn, R., … Ulijn,
R. V. (2022). Self‐complementary zwitterionic peptides direct nanoparticle assembly
and enable enzymatic selection of endocytic pathways. Advanced Materials.
Wiley. https://doi.org/10.1002/adma.202104962
chicago: Huang, Richard H., Nazia Nayeem, Ye He, Jorge Morales, Duncan Graham, Rafal
Klajn, Maria Contel, Stephen O’Brien, and Rein V. Ulijn. “Self‐complementary Zwitterionic
Peptides Direct Nanoparticle Assembly and Enable Enzymatic Selection of Endocytic
Pathways.” Advanced Materials. Wiley, 2022. https://doi.org/10.1002/adma.202104962.
ieee: R. H. Huang et al., “Self‐complementary zwitterionic peptides direct
nanoparticle assembly and enable enzymatic selection of endocytic pathways,” Advanced
Materials, vol. 34, no. 1. Wiley, 2022.
ista: Huang RH, Nayeem N, He Y, Morales J, Graham D, Klajn R, Contel M, O’Brien
S, Ulijn RV. 2022. Self‐complementary zwitterionic peptides direct nanoparticle
assembly and enable enzymatic selection of endocytic pathways. Advanced Materials.
34(1), 2104962.
mla: Huang, Richard H., et al. “Self‐complementary Zwitterionic Peptides Direct
Nanoparticle Assembly and Enable Enzymatic Selection of Endocytic Pathways.” Advanced
Materials, vol. 34, no. 1, 2104962, Wiley, 2022, doi:10.1002/adma.202104962.
short: R.H. Huang, N. Nayeem, Y. He, J. Morales, D. Graham, R. Klajn, M. Contel,
S. O’Brien, R.V. Ulijn, Advanced Materials 34 (2022).
date_created: 2023-08-01T09:33:26Z
date_published: 2022-01-06T00:00:00Z
date_updated: 2023-08-07T09:58:17Z
day: '06'
doi: 10.1002/adma.202104962
extern: '1'
external_id:
pmid:
- '34668253'
intvolume: ' 34'
issue: '1'
keyword:
- Mechanical Engineering
- Mechanics of Materials
- General Materials Science
language:
- iso: eng
main_file_link:
- open_access: '1'
url: https://doi.org/10.1002/adma.202104962
month: '01'
oa: 1
oa_version: Published Version
pmid: 1
publication: Advanced Materials
publication_identifier:
eissn:
- 1521-4095
issn:
- 0935-9648
publication_status: published
publisher: Wiley
quality_controlled: '1'
scopus_import: '1'
status: public
title: Self‐complementary zwitterionic peptides direct nanoparticle assembly and enable
enzymatic selection of endocytic pathways
type: journal_article
user_id: 2DF688A6-F248-11E8-B48F-1D18A9856A87
volume: 34
year: '2022'
...
---
_id: '9282'
abstract:
- lang: eng
text: Several Ising-type magnetic van der Waals (vdW) materials exhibit stable magnetic
ground states. Despite these clear experimental demonstrations, a complete theoretical
and microscopic understanding of their magnetic anisotropy is still lacking. In
particular, the validity limit of identifying their one-dimensional (1-D) Ising
nature has remained uninvestigated in a quantitative way. Here we performed the
complete mapping of magnetic anisotropy for a prototypical Ising vdW magnet FePS3
for the first time. Combining torque magnetometry measurements with their magnetostatic
model analysis and the relativistic density functional total energy calculations,
we successfully constructed the three-dimensional (3-D) mappings of the magnetic
anisotropy in terms of magnetic torque and energy. The results not only quantitatively
confirm that the easy axis is perpendicular to the ab plane, but also reveal the
anisotropies within the ab, ac, and bc planes. Our approach can be applied to
the detailed quantitative study of magnetism in vdW materials.
article_number: '035011'
article_processing_charge: No
article_type: original
arxiv: 1
author:
- first_name: Muhammad
full_name: Nauman, Muhammad
id: 32c21954-2022-11eb-9d5f-af9f93c24e71
last_name: Nauman
orcid: 0000-0002-2111-4846
- first_name: Do Hoon
full_name: Kiem, Do Hoon
last_name: Kiem
- first_name: Sungmin
full_name: Lee, Sungmin
last_name: Lee
- first_name: Suhan
full_name: Son, Suhan
last_name: Son
- first_name: J-G
full_name: Park, J-G
last_name: Park
- first_name: Woun
full_name: Kang, Woun
last_name: Kang
- first_name: Myung Joon
full_name: Han, Myung Joon
last_name: Han
- first_name: Youn Jung
full_name: Jo, Youn Jung
last_name: Jo
citation:
ama: Nauman M, Kiem DH, Lee S, et al. Complete mapping of magnetic anisotropy for
prototype Ising van der Waals FePS3. 2D Materials. 2021;8(3). doi:10.1088/2053-1583/abeed3
apa: Nauman, M., Kiem, D. H., Lee, S., Son, S., Park, J.-G., Kang, W., … Jo, Y.
J. (2021). Complete mapping of magnetic anisotropy for prototype Ising van der
Waals FePS3. 2D Materials. IOP Publishing. https://doi.org/10.1088/2053-1583/abeed3
chicago: Nauman, Muhammad, Do Hoon Kiem, Sungmin Lee, Suhan Son, J-G Park, Woun
Kang, Myung Joon Han, and Youn Jung Jo. “Complete Mapping of Magnetic Anisotropy
for Prototype Ising van Der Waals FePS3.” 2D Materials. IOP Publishing,
2021. https://doi.org/10.1088/2053-1583/abeed3.
ieee: M. Nauman et al., “Complete mapping of magnetic anisotropy for prototype
Ising van der Waals FePS3,” 2D Materials, vol. 8, no. 3. IOP Publishing,
2021.
ista: Nauman M, Kiem DH, Lee S, Son S, Park J-G, Kang W, Han MJ, Jo YJ. 2021. Complete
mapping of magnetic anisotropy for prototype Ising van der Waals FePS3. 2D Materials.
8(3), 035011.
mla: Nauman, Muhammad, et al. “Complete Mapping of Magnetic Anisotropy for Prototype
Ising van Der Waals FePS3.” 2D Materials, vol. 8, no. 3, 035011, IOP Publishing,
2021, doi:10.1088/2053-1583/abeed3.
short: M. Nauman, D.H. Kiem, S. Lee, S. Son, J.-G. Park, W. Kang, M.J. Han, Y.J.
Jo, 2D Materials 8 (2021).
date_created: 2021-03-23T07:10:17Z
date_published: 2021-04-06T00:00:00Z
date_updated: 2021-12-01T10:36:56Z
day: '06'
department:
- _id: KiMo
doi: 10.1088/2053-1583/abeed3
extern: '1'
external_id:
arxiv:
- '2103.09029'
intvolume: ' 8'
issue: '3'
keyword:
- Mechanical Engineering
- General Materials Science
- Mechanics of Materials
- General Chemistry
- Condensed Matter Physics
language:
- iso: eng
main_file_link:
- open_access: '1'
url: https://arxiv.org/abs/2103.09029
month: '04'
oa: 1
oa_version: Preprint
publication: 2D Materials
publication_identifier:
issn:
- 2053-1583
publication_status: published
publisher: IOP Publishing
quality_controlled: '1'
status: public
title: Complete mapping of magnetic anisotropy for prototype Ising van der Waals FePS3
type: journal_article
user_id: 8b945eb4-e2f2-11eb-945a-df72226e66a9
volume: 8
year: '2021'
...
---
_id: '10123'
abstract:
- lang: eng
text: Solution synthesis of particles emerged as an alternative to prepare thermoelectric
materials with less demanding processing conditions than conventional solid-state
synthetic methods. However, solution synthesis generally involves the presence
of additional molecules or ions belonging to the precursors or added to enable
solubility and/or regulate nucleation and growth. These molecules or ions can
end up in the particles as surface adsorbates and interfere in the material properties.
This work demonstrates that ionic adsorbates, in particular Na⁺ ions, are electrostatically
adsorbed in SnSe particles synthesized in water and play a crucial role not only
in directing the material nano/microstructure but also in determining the transport
properties of the consolidated material. In dense pellets prepared by sintering
SnSe particles, Na remains within the crystal lattice as dopant, in dislocations,
precipitates, and forming grain boundary complexions. These results highlight
the importance of considering all the possible unintentional impurities to establish
proper structure-property relationships and control material properties in solution-processed
thermoelectric materials.
acknowledged_ssus:
- _id: EM-Fac
- _id: NanoFab
acknowledgement: 'Y.L. and M.C. contributed equally to this work. This research was
supported by the Scientific Service Units (SSU) of IST Austria through resources
provided by Electron Microscopy Facility (EMF) and the Nanofabrication Facility
(NNF). This work was financially supported by IST Austria and the Werner Siemens
Foundation. Y.L. acknowledges funding from the European Union''s Horizon 2020 research
and innovation program under the Marie Sklodowska-Curie grant agreement No. 754411.
M.C. has received funding from the European Union''s Horizon 2020 research and innovation
program under the Marie Skłodowska-Curie Grant Agreement No. 665385. Y.Y. and O.C.-M.
acknowledge the financial support from DFG within the project SFB 917: Nanoswitches.
J.L. is a Serra Húnter Fellow and is grateful to ICREA Academia program. C.C. acknowledges
funding from the FWF “Lise Meitner Fellowship” grant agreement M 2889-N.'
article_number: '2106858'
article_processing_charge: Yes (via OA deal)
article_type: original
author:
- first_name: Yu
full_name: Liu, Yu
id: 2A70014E-F248-11E8-B48F-1D18A9856A87
last_name: Liu
orcid: 0000-0001-7313-6740
- first_name: Mariano
full_name: Calcabrini, Mariano
id: 45D7531A-F248-11E8-B48F-1D18A9856A87
last_name: Calcabrini
orcid: 0000-0003-4566-5877
- first_name: Yuan
full_name: Yu, Yuan
last_name: Yu
- first_name: Aziz
full_name: Genç, Aziz
last_name: Genç
- first_name: Cheng
full_name: Chang, Cheng
id: 9E331C2E-9F27-11E9-AE48-5033E6697425
last_name: Chang
orcid: 0000-0002-9515-4277
- first_name: Tommaso
full_name: Costanzo, Tommaso
id: D93824F4-D9BA-11E9-BB12-F207E6697425
last_name: Costanzo
orcid: 0000-0001-9732-3815
- first_name: Tobias
full_name: Kleinhanns, Tobias
id: 8BD9DE16-AB3C-11E9-9C8C-2A03E6697425
last_name: Kleinhanns
orcid: 0000-0003-1537-7436
- first_name: Seungho
full_name: Lee, Seungho
id: BB243B88-D767-11E9-B658-BC13E6697425
last_name: Lee
orcid: 0000-0002-6962-8598
- first_name: Jordi
full_name: Llorca, Jordi
last_name: Llorca
- first_name: Oana
full_name: Cojocaru‐Mirédin, Oana
last_name: Cojocaru‐Mirédin
- first_name: Maria
full_name: Ibáñez, Maria
id: 43C61214-F248-11E8-B48F-1D18A9856A87
last_name: Ibáñez
orcid: 0000-0001-5013-2843
citation:
ama: 'Liu Y, Calcabrini M, Yu Y, et al. The importance of surface adsorbates in
solution‐processed thermoelectric materials: The case of SnSe. Advanced Materials.
2021;33(52). doi:10.1002/adma.202106858'
apa: 'Liu, Y., Calcabrini, M., Yu, Y., Genç, A., Chang, C., Costanzo, T., … Ibáñez,
M. (2021). The importance of surface adsorbates in solution‐processed thermoelectric
materials: The case of SnSe. Advanced Materials. Wiley. https://doi.org/10.1002/adma.202106858'
chicago: 'Liu, Yu, Mariano Calcabrini, Yuan Yu, Aziz Genç, Cheng Chang, Tommaso
Costanzo, Tobias Kleinhanns, et al. “The Importance of Surface Adsorbates in Solution‐processed
Thermoelectric Materials: The Case of SnSe.” Advanced Materials. Wiley,
2021. https://doi.org/10.1002/adma.202106858.'
ieee: 'Y. Liu et al., “The importance of surface adsorbates in solution‐processed
thermoelectric materials: The case of SnSe,” Advanced Materials, vol. 33,
no. 52. Wiley, 2021.'
ista: 'Liu Y, Calcabrini M, Yu Y, Genç A, Chang C, Costanzo T, Kleinhanns T, Lee
S, Llorca J, Cojocaru‐Mirédin O, Ibáñez M. 2021. The importance of surface adsorbates
in solution‐processed thermoelectric materials: The case of SnSe. Advanced Materials.
33(52), 2106858.'
mla: 'Liu, Yu, et al. “The Importance of Surface Adsorbates in Solution‐processed
Thermoelectric Materials: The Case of SnSe.” Advanced Materials, vol. 33,
no. 52, 2106858, Wiley, 2021, doi:10.1002/adma.202106858.'
short: Y. Liu, M. Calcabrini, Y. Yu, A. Genç, C. Chang, T. Costanzo, T. Kleinhanns,
S. Lee, J. Llorca, O. Cojocaru‐Mirédin, M. Ibáñez, Advanced Materials 33 (2021).
corr_author: '1'
date_created: 2021-10-11T20:07:24Z
date_published: 2021-12-29T00:00:00Z
date_updated: 2026-04-07T13:26:13Z
day: '29'
ddc:
- '620'
department:
- _id: EM-Fac
- _id: MaIb
doi: 10.1002/adma.202106858
ec_funded: 1
external_id:
isi:
- '000709899300001'
pmid:
- '34626034'
file:
- access_level: open_access
checksum: 990bccc527c64d85cf1c97885110b5f4
content_type: application/pdf
creator: cchlebak
date_created: 2022-02-03T13:16:14Z
date_updated: 2022-02-03T13:16:14Z
file_id: '10720'
file_name: 2021_AdvancedMaterials_Liu.pdf
file_size: 5595666
relation: main_file
success: 1
file_date_updated: 2022-02-03T13:16:14Z
has_accepted_license: '1'
intvolume: ' 33'
isi: 1
issue: '52'
keyword:
- mechanical engineering
- mechanics of materials
- general materials science
language:
- iso: eng
month: '12'
oa: 1
oa_version: Published Version
pmid: 1
project:
- _id: 2564DBCA-B435-11E9-9278-68D0E5697425
call_identifier: H2020
grant_number: '665385'
name: International IST Doctoral Program
- _id: 260C2330-B435-11E9-9278-68D0E5697425
call_identifier: H2020
grant_number: '754411'
name: ISTplus - Postdoctoral Fellowships
- _id: 9B8804FC-BA93-11EA-9121-9846C619BF3A
grant_number: M02889
name: Bottom-up Engineering for Thermoelectric Applications
- _id: 9B8F7476-BA93-11EA-9121-9846C619BF3A
name: 'HighTE: The Werner Siemens Laboratory for the High Throughput Discovery of
Semiconductors for Waste Heat Recovery'
publication: Advanced Materials
publication_identifier:
eissn:
- 1521-4095
issn:
- 0935-9648
publication_status: published
publisher: Wiley
quality_controlled: '1'
related_material:
record:
- id: '17062'
relation: later_version
status: public
- id: '12885'
relation: dissertation_contains
status: public
scopus_import: '1'
status: public
title: 'The importance of surface adsorbates in solution‐processed thermoelectric
materials: The case of SnSe'
tmp:
image: /images/cc_by.png
legal_code_url: https://creativecommons.org/licenses/by/4.0/legalcode
name: Creative Commons Attribution 4.0 International Public License (CC-BY 4.0)
short: CC BY (4.0)
type: journal_article
user_id: 4359f0d1-fa6c-11eb-b949-802e58b17ae8
volume: 33
year: '2021'
...
---
_id: '13366'
abstract:
- lang: eng
text: The ability to reversibly assemble nanoparticles using light is both fundamentally
interesting and important for applications ranging from reversible data storage
to controlled drug delivery. Here, the diverse approaches that have so far been
developed to control the self-assembly of nanoparticles using light are reviewed
and compared. These approaches include functionalizing nanoparticles with monolayers
of photoresponsive molecules, placing them in photoresponsive media capable of
reversibly protonating the particles under light, and decorating plasmonic nanoparticles
with thermoresponsive polymers, to name just a few. The applicability of these
methods to larger, micrometer-sized particles is also discussed. Finally, several
perspectives on further developments in the field are offered.
article_number: '1905866'
article_processing_charge: No
article_type: original
author:
- first_name: Tong
full_name: Bian, Tong
last_name: Bian
- first_name: Zonglin
full_name: Chu, Zonglin
last_name: Chu
- first_name: Rafal
full_name: Klajn, Rafal
id: 8e84690e-1e48-11ed-a02b-a1e6fb8bb53b
last_name: Klajn
citation:
ama: Bian T, Chu Z, Klajn R. The many ways to assemble nanoparticles using light.
Advanced Materials. 2019;32(20). doi:10.1002/adma.201905866
apa: Bian, T., Chu, Z., & Klajn, R. (2019). The many ways to assemble nanoparticles
using light. Advanced Materials. Wiley. https://doi.org/10.1002/adma.201905866
chicago: Bian, Tong, Zonglin Chu, and Rafal Klajn. “The Many Ways to Assemble Nanoparticles
Using Light.” Advanced Materials. Wiley, 2019. https://doi.org/10.1002/adma.201905866.
ieee: T. Bian, Z. Chu, and R. Klajn, “The many ways to assemble nanoparticles using
light,” Advanced Materials, vol. 32, no. 20. Wiley, 2019.
ista: Bian T, Chu Z, Klajn R. 2019. The many ways to assemble nanoparticles using
light. Advanced Materials. 32(20), 1905866.
mla: Bian, Tong, et al. “The Many Ways to Assemble Nanoparticles Using Light.” Advanced
Materials, vol. 32, no. 20, 1905866, Wiley, 2019, doi:10.1002/adma.201905866.
short: T. Bian, Z. Chu, R. Klajn, Advanced Materials 32 (2019).
date_created: 2023-08-01T09:37:26Z
date_published: 2019-11-19T00:00:00Z
date_updated: 2024-10-14T12:13:25Z
day: '19'
doi: 10.1002/adma.201905866
extern: '1'
external_id:
pmid:
- '31709655'
intvolume: ' 32'
issue: '20'
keyword:
- Mechanical Engineering
- Mechanics of Materials
- General Materials Science
language:
- iso: eng
month: '11'
oa_version: None
pmid: 1
publication: Advanced Materials
publication_identifier:
eissn:
- 1521-4095
issn:
- 0935-9648
publication_status: published
publisher: Wiley
quality_controlled: '1'
scopus_import: '1'
status: public
title: The many ways to assemble nanoparticles using light
type: journal_article
user_id: 2DF688A6-F248-11E8-B48F-1D18A9856A87
volume: 32
year: '2019'
...
---
_id: '13375'
abstract:
- lang: eng
text: 'Dissipative self-assembly leads to structures and materials that exist away
from equilibrium by continuously exchanging energy and materials with the external
environment. Although this mode of self-assembly is ubiquitous in nature, where
it gives rise to functions such as signal processing, motility, self-healing,
self-replication, and ultimately life, examples of dissipative self-assembly processes
in man-made systems are few and far between. Herein, recent progress in developing
diverse synthetic dissipative self-assembly systems is discussed. The systems
reported thus far can be categorized into three classes, in which: i) the fuel
chemically modifies the building blocks, thus triggering their self-assembly,
ii) the fuel acts as a template interacting with the building blocks noncovalently,
and iii) transient states are induced by the addition of two mutually exclusive
stimuli. These early studies give rise to materials that would be difficult to
obtain otherwise, including hydrogels with programmable lifetimes, vesicular nanoreactors,
and membranes exhibiting transient conductivity.'
article_number: '1706750'
article_processing_charge: No
article_type: original
author:
- first_name: Soumen
full_name: De, Soumen
last_name: De
- first_name: Rafal
full_name: Klajn, Rafal
id: 8e84690e-1e48-11ed-a02b-a1e6fb8bb53b
last_name: Klajn
citation:
ama: De S, Klajn R. Dissipative self-assembly driven by the consumption of chemical
fuels. Advanced Materials. 2018;30(41). doi:10.1002/adma.201706750
apa: De, S., & Klajn, R. (2018). Dissipative self-assembly driven by the consumption
of chemical fuels. Advanced Materials. Wiley. https://doi.org/10.1002/adma.201706750
chicago: De, Soumen, and Rafal Klajn. “Dissipative Self-Assembly Driven by the Consumption
of Chemical Fuels.” Advanced Materials. Wiley, 2018. https://doi.org/10.1002/adma.201706750.
ieee: S. De and R. Klajn, “Dissipative self-assembly driven by the consumption of
chemical fuels,” Advanced Materials, vol. 30, no. 41. Wiley, 2018.
ista: De S, Klajn R. 2018. Dissipative self-assembly driven by the consumption of
chemical fuels. Advanced Materials. 30(41), 1706750.
mla: De, Soumen, and Rafal Klajn. “Dissipative Self-Assembly Driven by the Consumption
of Chemical Fuels.” Advanced Materials, vol. 30, no. 41, 1706750, Wiley,
2018, doi:10.1002/adma.201706750.
short: S. De, R. Klajn, Advanced Materials 30 (2018).
date_created: 2023-08-01T09:39:46Z
date_published: 2018-10-11T00:00:00Z
date_updated: 2024-10-14T12:14:43Z
day: '11'
doi: 10.1002/adma.201706750
extern: '1'
external_id:
pmid:
- '29520846'
intvolume: ' 30'
issue: '41'
keyword:
- Mechanical Engineering
- Mechanics of Materials
- General Materials Science
language:
- iso: eng
month: '10'
oa_version: None
pmid: 1
publication: Advanced Materials
publication_identifier:
eissn:
- 1521-4095
issn:
- 0935-9648
publication_status: published
publisher: Wiley
quality_controlled: '1'
scopus_import: '1'
status: public
title: Dissipative self-assembly driven by the consumption of chemical fuels
type: journal_article
user_id: 2DF688A6-F248-11E8-B48F-1D18A9856A87
volume: 30
year: '2018'
...
---
_id: '9066'
abstract:
- lang: eng
text: The novel electronic state of the canted antiferromagnetic (AFM) insulator,
strontium iridate (Sr2IrO4) has been well described by the spin-orbit-entangled
isospin Jeff = 1/2, but the role of isospin in transport phenomena remains poorly
understood. In this study, antiferromagnet-based spintronic functionality is demonstrated
by combining unique characteristics of the isospin state in Sr2IrO4. Based on
magnetic and transport measurements, large and highly anisotropic magnetoresistance
(AMR) is obtained by manipulating the antiferromagnetic isospin domains. First-principles
calculations suggest that electrons whose isospin directions are strongly coupled
to in-plane net magnetic moment encounter the isospin mismatch when moving across
antiferromagnetic domain boundaries, which generates a high resistance state.
By rotating a magnetic field that aligns in-plane net moments and removes domain
boundaries, the macroscopically-ordered isospins govern dynamic transport through
the system, which leads to the extremely angle-sensitive AMR. As with this work
that establishes a link between isospins and magnetotransport in strongly spin-orbit-coupled
AFM Sr2IrO4, the peculiar AMR effect provides a beneficial foundation for fundamental
and applied research on AFM spintronics.
article_number: '1805564'
article_processing_charge: No
article_type: original
arxiv: 1
author:
- first_name: Nara
full_name: Lee, Nara
last_name: Lee
- first_name: Eunjung
full_name: Ko, Eunjung
last_name: Ko
- first_name: Hwan Young
full_name: Choi, Hwan Young
last_name: Choi
- first_name: Yun Jeong
full_name: Hong, Yun Jeong
last_name: Hong
- first_name: Muhammad
full_name: Nauman, Muhammad
id: 32c21954-2022-11eb-9d5f-af9f93c24e71
last_name: Nauman
orcid: 0000-0002-2111-4846
- first_name: Woun
full_name: Kang, Woun
last_name: Kang
- first_name: Hyoung Joon
full_name: Choi, Hyoung Joon
last_name: Choi
- first_name: Young Jai
full_name: Choi, Young Jai
last_name: Choi
- first_name: Younjung
full_name: Jo, Younjung
last_name: Jo
citation:
ama: Lee N, Ko E, Choi HY, et al. Antiferromagnet‐based spintronic functionality
by controlling isospin domains in a layered perovskite iridate. Advanced Materials.
2018;30(52). doi:10.1002/adma.201805564
apa: Lee, N., Ko, E., Choi, H. Y., Hong, Y. J., Nauman, M., Kang, W., … Jo, Y. (2018).
Antiferromagnet‐based spintronic functionality by controlling isospin domains
in a layered perovskite iridate. Advanced Materials. Wiley. https://doi.org/10.1002/adma.201805564
chicago: Lee, Nara, Eunjung Ko, Hwan Young Choi, Yun Jeong Hong, Muhammad Nauman,
Woun Kang, Hyoung Joon Choi, Young Jai Choi, and Younjung Jo. “Antiferromagnet‐based
Spintronic Functionality by Controlling Isospin Domains in a Layered Perovskite
Iridate.” Advanced Materials. Wiley, 2018. https://doi.org/10.1002/adma.201805564.
ieee: N. Lee et al., “Antiferromagnet‐based spintronic functionality by controlling
isospin domains in a layered perovskite iridate,” Advanced Materials, vol.
30, no. 52. Wiley, 2018.
ista: Lee N, Ko E, Choi HY, Hong YJ, Nauman M, Kang W, Choi HJ, Choi YJ, Jo Y. 2018.
Antiferromagnet‐based spintronic functionality by controlling isospin domains
in a layered perovskite iridate. Advanced Materials. 30(52), 1805564.
mla: Lee, Nara, et al. “Antiferromagnet‐based Spintronic Functionality by Controlling
Isospin Domains in a Layered Perovskite Iridate.” Advanced Materials, vol.
30, no. 52, 1805564, Wiley, 2018, doi:10.1002/adma.201805564.
short: N. Lee, E. Ko, H.Y. Choi, Y.J. Hong, M. Nauman, W. Kang, H.J. Choi, Y.J.
Choi, Y. Jo, Advanced Materials 30 (2018).
date_created: 2021-02-02T15:50:58Z
date_published: 2018-10-29T00:00:00Z
date_updated: 2021-02-03T13:58:39Z
day: '29'
doi: 10.1002/adma.201805564
extern: '1'
external_id:
arxiv:
- '1811.04562'
intvolume: ' 30'
issue: '52'
keyword:
- Mechanical Engineering
- General Materials Science
- Mechanics of Materials
language:
- iso: eng
month: '10'
oa_version: Preprint
publication: Advanced Materials
publication_identifier:
issn:
- 0935-9648
- 1521-4095
publication_status: published
publisher: Wiley
quality_controlled: '1'
status: public
title: Antiferromagnet‐based spintronic functionality by controlling isospin domains
in a layered perovskite iridate
type: journal_article
user_id: 2DF688A6-F248-11E8-B48F-1D18A9856A87
volume: 30
year: '2018'
...
---
_id: '13406'
abstract:
- lang: eng
text: Dual-responsive nanoparticles are designed by functionalizing magnetic cores
with light-responsive ligands. These materials respond to both light and magnetic
fields and can be assembled into various higher-order structures, depending on
the relative contributions of these two stimuli.
article_processing_charge: No
article_type: original
author:
- first_name: Sanjib
full_name: Das, Sanjib
last_name: Das
- first_name: Priyadarshi
full_name: Ranjan, Priyadarshi
last_name: Ranjan
- first_name: Pradipta Sankar
full_name: Maiti, Pradipta Sankar
last_name: Maiti
- first_name: Gurvinder
full_name: Singh, Gurvinder
last_name: Singh
- first_name: Gregory
full_name: Leitus, Gregory
last_name: Leitus
- first_name: Rafal
full_name: Klajn, Rafal
id: 8e84690e-1e48-11ed-a02b-a1e6fb8bb53b
last_name: Klajn
citation:
ama: Das S, Ranjan P, Maiti PS, Singh G, Leitus G, Klajn R. Dual-responsive nanoparticles
and their self-assembly. Advanced Materials. 2013;25(3):422-426. doi:10.1002/adma.201201734
apa: Das, S., Ranjan, P., Maiti, P. S., Singh, G., Leitus, G., & Klajn, R. (2013).
Dual-responsive nanoparticles and their self-assembly. Advanced Materials.
Wiley. https://doi.org/10.1002/adma.201201734
chicago: Das, Sanjib, Priyadarshi Ranjan, Pradipta Sankar Maiti, Gurvinder Singh,
Gregory Leitus, and Rafal Klajn. “Dual-Responsive Nanoparticles and Their Self-Assembly.”
Advanced Materials. Wiley, 2013. https://doi.org/10.1002/adma.201201734.
ieee: S. Das, P. Ranjan, P. S. Maiti, G. Singh, G. Leitus, and R. Klajn, “Dual-responsive
nanoparticles and their self-assembly,” Advanced Materials, vol. 25, no.
3. Wiley, pp. 422–426, 2013.
ista: Das S, Ranjan P, Maiti PS, Singh G, Leitus G, Klajn R. 2013. Dual-responsive
nanoparticles and their self-assembly. Advanced Materials. 25(3), 422–426.
mla: Das, Sanjib, et al. “Dual-Responsive Nanoparticles and Their Self-Assembly.”
Advanced Materials, vol. 25, no. 3, Wiley, 2013, pp. 422–26, doi:10.1002/adma.201201734.
short: S. Das, P. Ranjan, P.S. Maiti, G. Singh, G. Leitus, R. Klajn, Advanced Materials
25 (2013) 422–426.
date_created: 2023-08-01T09:47:30Z
date_published: 2013-01-18T00:00:00Z
date_updated: 2024-10-14T12:21:16Z
day: '18'
doi: 10.1002/adma.201201734
extern: '1'
external_id:
pmid:
- '22933327'
intvolume: ' 25'
issue: '3'
keyword:
- Mechanical Engineering
- Mechanics of Materials
- General Materials Science
language:
- iso: eng
month: '01'
oa_version: None
page: 422-426
pmid: 1
publication: Advanced Materials
publication_identifier:
issn:
- 0935-9648
publication_status: published
publisher: Wiley
quality_controlled: '1'
scopus_import: '1'
status: public
title: Dual-responsive nanoparticles and their self-assembly
type: journal_article
user_id: 2DF688A6-F248-11E8-B48F-1D18A9856A87
volume: 25
year: '2013'
...
---
_id: '13419'
abstract:
- lang: eng
text: Reaction-diffusion (RD) processes initiated from the surfaces of mesoscopic
particles can fabricate complex core-and-shell structures. The propagation of
a sharp RD front selectively removes metal colloids or nanoparticles from the
supporting gel or polymer matrix. Once fabricated, the core structures can be
processed “remotely” via galvanic replacement reactions, and the composite particles
can be assembled into open-lattice crystals.
article_processing_charge: No
article_type: original
author:
- first_name: Paul J.
full_name: Wesson, Paul J.
last_name: Wesson
- first_name: Siowling
full_name: Soh, Siowling
last_name: Soh
- first_name: Rafal
full_name: Klajn, Rafal
id: 8e84690e-1e48-11ed-a02b-a1e6fb8bb53b
last_name: Klajn
- first_name: Kyle J. M.
full_name: Bishop, Kyle J. M.
last_name: Bishop
- first_name: Timothy P.
full_name: Gray, Timothy P.
last_name: Gray
- first_name: Bartosz A.
full_name: Grzybowski, Bartosz A.
last_name: Grzybowski
citation:
ama: 'Wesson PJ, Soh S, Klajn R, Bishop KJM, Gray TP, Grzybowski BA. “Remote” fabrication
via three-dimensional reaction-diffusion: Making complex core-and-shell particles
and assembling them into open-lattice crystals. Advanced Materials. 2009;21(19):1911-1915.
doi:10.1002/adma.200802964'
apa: 'Wesson, P. J., Soh, S., Klajn, R., Bishop, K. J. M., Gray, T. P., & Grzybowski,
B. A. (2009). “Remote” fabrication via three-dimensional reaction-diffusion: Making
complex core-and-shell particles and assembling them into open-lattice crystals.
Advanced Materials. Wiley. https://doi.org/10.1002/adma.200802964'
chicago: 'Wesson, Paul J., Siowling Soh, Rafal Klajn, Kyle J. M. Bishop, Timothy
P. Gray, and Bartosz A. Grzybowski. “‘Remote’ Fabrication via Three-Dimensional
Reaction-Diffusion: Making Complex Core-and-Shell Particles and Assembling Them
into Open-Lattice Crystals.” Advanced Materials. Wiley, 2009. https://doi.org/10.1002/adma.200802964.'
ieee: 'P. J. Wesson, S. Soh, R. Klajn, K. J. M. Bishop, T. P. Gray, and B. A. Grzybowski,
“‘Remote’ fabrication via three-dimensional reaction-diffusion: Making complex
core-and-shell particles and assembling them into open-lattice crystals,” Advanced
Materials, vol. 21, no. 19. Wiley, pp. 1911–1915, 2009.'
ista: 'Wesson PJ, Soh S, Klajn R, Bishop KJM, Gray TP, Grzybowski BA. 2009. “Remote”
fabrication via three-dimensional reaction-diffusion: Making complex core-and-shell
particles and assembling them into open-lattice crystals. Advanced Materials.
21(19), 1911–1915.'
mla: 'Wesson, Paul J., et al. “‘Remote’ Fabrication via Three-Dimensional Reaction-Diffusion:
Making Complex Core-and-Shell Particles and Assembling Them into Open-Lattice
Crystals.” Advanced Materials, vol. 21, no. 19, Wiley, 2009, pp. 1911–15,
doi:10.1002/adma.200802964.'
short: P.J. Wesson, S. Soh, R. Klajn, K.J.M. Bishop, T.P. Gray, B.A. Grzybowski,
Advanced Materials 21 (2009) 1911–1915.
date_created: 2023-08-01T10:30:04Z
date_published: 2009-05-18T00:00:00Z
date_updated: 2023-08-08T09:04:07Z
day: '18'
doi: 10.1002/adma.200802964
extern: '1'
intvolume: ' 21'
issue: '19'
keyword:
- Mechanical Engineering
- Mechanics of Materials
- General Materials Science
language:
- iso: eng
month: '05'
oa_version: None
page: 1911-1915
publication: Advanced Materials
publication_identifier:
eissn:
- 1521-4095
issn:
- 0935-9648
publication_status: published
publisher: Wiley
quality_controlled: '1'
scopus_import: '1'
status: public
title: '“Remote” fabrication via three-dimensional reaction-diffusion: Making complex
core-and-shell particles and assembling them into open-lattice crystals'
type: journal_article
user_id: 2DF688A6-F248-11E8-B48F-1D18A9856A87
volume: 21
year: '2009'
...
---
_id: '9149'
abstract:
- lang: eng
text: "The interaction of tidal currents with sea-floor topography results in the
radiation of internal gravity waves into the ocean interior. These waves are called
internal tides and their dissipation due to nonlinear wave breaking and concomitant
three-dimensional turbulence could play an important role in the mixing of the
abyssal ocean, and hence in controlling the large-scale ocean circulation.\r\nAs
part of on-going work aimed at providing a theory for the vertical distribution
of wave breaking over sea-floor topography, in this paper we investigate the instability
of internal tides in a very simple linear model that helps us to relate the formation
of unstable regions to simple features in the sea-floor topography. For two-dimensional
tides over one-dimensional topography we find that the formation of overturning
instabilities is closely linked to the singularities in the topography shape and
that it is possible to have stable waves at the sea floor and unstable waves in
the ocean interior above.\r\nFor three-dimensional tides over two-dimensional
topography there is in addition an effect of geometric focusing of wave energy
into localized regions of high wave amplitude, and we investigate this focusing
effect in simple examples. Overall, we find that the distribution of unstable
wave breaking regions can be highly non-uniform even for very simple idealized
topography shapes."
article_processing_charge: No
article_type: original
author:
- first_name: Oliver
full_name: Bühler, Oliver
last_name: Bühler
- first_name: Caroline J
full_name: Muller, Caroline J
id: f978ccb0-3f7f-11eb-b193-b0e2bd13182b
last_name: Muller
orcid: 0000-0001-5836-5350
citation:
ama: Bühler O, Muller CJ. Instability and focusing of internal tides in the deep
ocean. Journal of Fluid Mechanics. 2007;588:1-28. doi:10.1017/s0022112007007410
apa: Bühler, O., & Muller, C. J. (2007). Instability and focusing of internal
tides in the deep ocean. Journal of Fluid Mechanics. Cambridge University
Press. https://doi.org/10.1017/s0022112007007410
chicago: Bühler, Oliver, and Caroline J Muller. “Instability and Focusing of Internal
Tides in the Deep Ocean.” Journal of Fluid Mechanics. Cambridge University
Press, 2007. https://doi.org/10.1017/s0022112007007410.
ieee: O. Bühler and C. J. Muller, “Instability and focusing of internal tides in
the deep ocean,” Journal of Fluid Mechanics, vol. 588. Cambridge University
Press, pp. 1–28, 2007.
ista: Bühler O, Muller CJ. 2007. Instability and focusing of internal tides in the
deep ocean. Journal of Fluid Mechanics. 588, 1–28.
mla: Bühler, Oliver, and Caroline J. Muller. “Instability and Focusing of Internal
Tides in the Deep Ocean.” Journal of Fluid Mechanics, vol. 588, Cambridge
University Press, 2007, pp. 1–28, doi:10.1017/s0022112007007410.
short: O. Bühler, C.J. Muller, Journal of Fluid Mechanics 588 (2007) 1–28.
date_created: 2021-02-15T14:41:45Z
date_published: 2007-10-10T00:00:00Z
date_updated: 2022-01-24T13:43:36Z
day: '10'
doi: 10.1017/s0022112007007410
extern: '1'
intvolume: ' 588'
keyword:
- mechanical engineering
- mechanics of materials
- condensed matter physics
language:
- iso: eng
main_file_link:
- open_access: '1'
url: https://doi.org/10.1017/S0022112007007410
month: '10'
oa: 1
oa_version: None
page: 1-28
publication: Journal of Fluid Mechanics
publication_identifier:
issn:
- 0022-1120
- 1469-7645
publication_status: published
publisher: Cambridge University Press
quality_controlled: '1'
status: public
title: Instability and focusing of internal tides in the deep ocean
type: journal_article
user_id: 8b945eb4-e2f2-11eb-945a-df72226e66a9
volume: 588
year: '2007'
...
---
_id: '13431'
abstract:
- lang: eng
text: 'Hydrogel stamps can microstructure solid surfaces, i.e., modify the surface
topology of metals, glasses, and crystals. It is demonstrated that stamps soaked
in an appropriate etchant can remove material with micrometer-scale precision.
The Figure shows an array of concentric circles etched in glass using the immersion
wet stamping process described (scale bar: 500 μm).'
article_processing_charge: No
article_type: original
author:
- first_name: S. K.
full_name: Smoukov, S. K.
last_name: Smoukov
- first_name: K. J. M.
full_name: Bishop, K. J. M.
last_name: Bishop
- first_name: Rafal
full_name: Klajn, Rafal
id: 8e84690e-1e48-11ed-a02b-a1e6fb8bb53b
last_name: Klajn
- first_name: C. J.
full_name: Campbell, C. J.
last_name: Campbell
- first_name: B. A.
full_name: Grzybowski, B. A.
last_name: Grzybowski
citation:
ama: Smoukov SK, Bishop KJM, Klajn R, Campbell CJ, Grzybowski BA. Cutting into solids
with micropatterned gels. Advanced Materials. 2005;17(11):1361-1365. doi:10.1002/adma.200402086
apa: Smoukov, S. K., Bishop, K. J. M., Klajn, R., Campbell, C. J., & Grzybowski,
B. A. (2005). Cutting into solids with micropatterned gels. Advanced Materials.
Wiley. https://doi.org/10.1002/adma.200402086
chicago: Smoukov, S. K., K. J. M. Bishop, Rafal Klajn, C. J. Campbell, and B. A.
Grzybowski. “Cutting into Solids with Micropatterned Gels.” Advanced Materials.
Wiley, 2005. https://doi.org/10.1002/adma.200402086.
ieee: S. K. Smoukov, K. J. M. Bishop, R. Klajn, C. J. Campbell, and B. A. Grzybowski,
“Cutting into solids with micropatterned gels,” Advanced Materials, vol.
17, no. 11. Wiley, pp. 1361–1365, 2005.
ista: Smoukov SK, Bishop KJM, Klajn R, Campbell CJ, Grzybowski BA. 2005. Cutting
into solids with micropatterned gels. Advanced Materials. 17(11), 1361–1365.
mla: Smoukov, S. K., et al. “Cutting into Solids with Micropatterned Gels.” Advanced
Materials, vol. 17, no. 11, Wiley, 2005, pp. 1361–65, doi:10.1002/adma.200402086.
short: S.K. Smoukov, K.J.M. Bishop, R. Klajn, C.J. Campbell, B.A. Grzybowski, Advanced
Materials 17 (2005) 1361–1365.
date_created: 2023-08-01T10:38:01Z
date_published: 2005-06-24T00:00:00Z
date_updated: 2023-08-08T11:53:16Z
day: '24'
doi: 10.1002/adma.200402086
extern: '1'
external_id:
pmid:
- '34412440'
intvolume: ' 17'
issue: '11'
keyword:
- Mechanical Engineering
- Mechanics of Materials
- General Materials Science
language:
- iso: eng
month: '06'
oa_version: None
page: 1361-1365
pmid: 1
publication: Advanced Materials
publication_identifier:
eissn:
- 1521-4095
issn:
- 0935-9648
publication_status: published
publisher: Wiley
quality_controlled: '1'
scopus_import: '1'
status: public
title: Cutting into solids with micropatterned gels
type: journal_article
user_id: 2DF688A6-F248-11E8-B48F-1D18A9856A87
volume: 17
year: '2005'
...
---
_id: '13434'
abstract:
- lang: eng
text: Thin films of ionically doped gelatin have been color-patterned with submicrometer
precision using the wet-stamping technique. Inorganic salts are delivered onto
the gelatin surface from an agarose stamp, and diffuse into the gelatine layer,
producting deeply colored precipitates. Reaction fronts originating from different
features of the stamp cease within < 1 μm of each other, leaving sharp, transparent
regions in between.
article_processing_charge: No
article_type: original
author:
- first_name: C. J.
full_name: Campbell, C. J.
last_name: Campbell
- first_name: M.
full_name: Fialkowski, M.
last_name: Fialkowski
- first_name: Rafal
full_name: Klajn, Rafal
id: 8e84690e-1e48-11ed-a02b-a1e6fb8bb53b
last_name: Klajn
- first_name: I. T.
full_name: Bensemann, I. T.
last_name: Bensemann
- first_name: B. A.
full_name: Grzybowski, B. A.
last_name: Grzybowski
citation:
ama: Campbell CJ, Fialkowski M, Klajn R, Bensemann IT, Grzybowski BA. Color micro-
and nanopatterning with counter-propagating reaction-diffusion fronts. Advanced
Materials. 2004;16(21):1912-1917. doi:10.1002/adma.200400383
apa: Campbell, C. J., Fialkowski, M., Klajn, R., Bensemann, I. T., & Grzybowski,
B. A. (2004). Color micro- and nanopatterning with counter-propagating reaction-diffusion
fronts. Advanced Materials. Wiley. https://doi.org/10.1002/adma.200400383
chicago: Campbell, C. J., M. Fialkowski, Rafal Klajn, I. T. Bensemann, and B. A.
Grzybowski. “Color Micro- and Nanopatterning with Counter-Propagating Reaction-Diffusion
Fronts.” Advanced Materials. Wiley, 2004. https://doi.org/10.1002/adma.200400383.
ieee: C. J. Campbell, M. Fialkowski, R. Klajn, I. T. Bensemann, and B. A. Grzybowski,
“Color micro- and nanopatterning with counter-propagating reaction-diffusion fronts,”
Advanced Materials, vol. 16, no. 21. Wiley, pp. 1912–1917, 2004.
ista: Campbell CJ, Fialkowski M, Klajn R, Bensemann IT, Grzybowski BA. 2004. Color
micro- and nanopatterning with counter-propagating reaction-diffusion fronts.
Advanced Materials. 16(21), 1912–1917.
mla: Campbell, C. J., et al. “Color Micro- and Nanopatterning with Counter-Propagating
Reaction-Diffusion Fronts.” Advanced Materials, vol. 16, no. 21, Wiley,
2004, pp. 1912–17, doi:10.1002/adma.200400383.
short: C.J. Campbell, M. Fialkowski, R. Klajn, I.T. Bensemann, B.A. Grzybowski,
Advanced Materials 16 (2004) 1912–1917.
date_created: 2023-08-01T10:39:09Z
date_published: 2004-11-14T00:00:00Z
date_updated: 2023-08-08T12:41:23Z
day: '14'
doi: 10.1002/adma.200400383
extern: '1'
intvolume: ' 16'
issue: '21'
keyword:
- Mechanical Engineering
- Mechanics of Materials
- General Materials Science
language:
- iso: eng
month: '11'
oa_version: None
page: 1912-1917
publication: Advanced Materials
publication_identifier:
eissn:
- 1521-4095
issn:
- 0935-9648
publication_status: published
publisher: Wiley
quality_controlled: '1'
scopus_import: '1'
status: public
title: Color micro- and nanopatterning with counter-propagating reaction-diffusion
fronts
type: journal_article
user_id: 2DF688A6-F248-11E8-B48F-1D18A9856A87
volume: 16
year: '2004'
...
---
_id: '13435'
abstract:
- lang: eng
text: Micropatterning of surfaces with several chemicals at different spatial locations
usually requires multiple stamping and registration steps. Here, we describe an
experimental method based on reaction–diffusion phenomena that allows for simultaneous
micropatterning of a substrate with several coloured chemicals. In this method,
called wet stamping (WETS), aqueous solutions of two or more inorganic salts are
delivered onto a film of dry, ionically doped gelatin from an agarose stamp patterned
in bas relief. Once in conformal contact, these salts diffuse into the gelatin,
where they react to give deeply coloured precipitates. Separation of colours in
the plane of the surface is the consequence of the differences in the diffusion
coefficients, the solubility products, and the amounts of different salts delivered
from the stamp, and is faithfully reproduced by a theoretical model based on a
system of reaction–diffusion partial differential equations. The multicolour micropatterns
are useful as non-binary optical elements, and could potentially form the basis
of new applications in microseparations and in controlled delivery.
article_processing_charge: No
article_type: original
author:
- first_name: Rafal
full_name: Klajn, Rafal
id: 8e84690e-1e48-11ed-a02b-a1e6fb8bb53b
last_name: Klajn
- first_name: Marcin
full_name: Fialkowski, Marcin
last_name: Fialkowski
- first_name: Igor T.
full_name: Bensemann, Igor T.
last_name: Bensemann
- first_name: Agnieszka
full_name: Bitner, Agnieszka
last_name: Bitner
- first_name: C. J.
full_name: Campbell, C. J.
last_name: Campbell
- first_name: Kyle
full_name: Bishop, Kyle
last_name: Bishop
- first_name: Stoyan
full_name: Smoukov, Stoyan
last_name: Smoukov
- first_name: Bartosz A.
full_name: Grzybowski, Bartosz A.
last_name: Grzybowski
citation:
ama: Klajn R, Fialkowski M, Bensemann IT, et al. Multicolour micropatterning of
thin films of dry gels. Nature Materials. 2004;3:729-735. doi:10.1038/nmat1231
apa: Klajn, R., Fialkowski, M., Bensemann, I. T., Bitner, A., Campbell, C. J., Bishop,
K., … Grzybowski, B. A. (2004). Multicolour micropatterning of thin films of dry
gels. Nature Materials. Springer Nature. https://doi.org/10.1038/nmat1231
chicago: Klajn, Rafal, Marcin Fialkowski, Igor T. Bensemann, Agnieszka Bitner, C.
J. Campbell, Kyle Bishop, Stoyan Smoukov, and Bartosz A. Grzybowski. “Multicolour
Micropatterning of Thin Films of Dry Gels.” Nature Materials. Springer
Nature, 2004. https://doi.org/10.1038/nmat1231.
ieee: R. Klajn et al., “Multicolour micropatterning of thin films of dry
gels,” Nature Materials, vol. 3. Springer Nature, pp. 729–735, 2004.
ista: Klajn R, Fialkowski M, Bensemann IT, Bitner A, Campbell CJ, Bishop K, Smoukov
S, Grzybowski BA. 2004. Multicolour micropatterning of thin films of dry gels.
Nature Materials. 3, 729–735.
mla: Klajn, Rafal, et al. “Multicolour Micropatterning of Thin Films of Dry Gels.”
Nature Materials, vol. 3, Springer Nature, 2004, pp. 729–35, doi:10.1038/nmat1231.
short: R. Klajn, M. Fialkowski, I.T. Bensemann, A. Bitner, C.J. Campbell, K. Bishop,
S. Smoukov, B.A. Grzybowski, Nature Materials 3 (2004) 729–735.
date_created: 2023-08-01T10:39:23Z
date_published: 2004-09-19T00:00:00Z
date_updated: 2023-08-08T12:42:51Z
day: '19'
doi: 10.1038/nmat1231
extern: '1'
external_id:
pmid:
- '15378052'
intvolume: ' 3'
keyword:
- Mechanical Engineering
- Mechanics of Materials
- Condensed Matter Physics
- General Materials Science
- General Chemistry
language:
- iso: eng
month: '09'
oa_version: None
page: 729-735
pmid: 1
publication: Nature Materials
publication_identifier:
eissn:
- 1476-4660
issn:
- 1476-1122
publication_status: published
publisher: Springer Nature
quality_controlled: '1'
scopus_import: '1'
status: public
title: Multicolour micropatterning of thin films of dry gels
type: journal_article
user_id: 2DF688A6-F248-11E8-B48F-1D18A9856A87
volume: 3
year: '2004'
...