[{"tmp":{"legal_code_url":"https://creativecommons.org/licenses/by/4.0/legalcode","name":"Creative Commons Attribution 4.0 International Public License (CC-BY 4.0)","image":"/images/cc_by.png","short":"CC BY (4.0)"},"project":[{"grant_number":"F100403","_id":"7c040762-9f16-11ee-852c-dd79eeee4ab3","name":"Coherent Optical Metrology Beyond Electric-Dipole-Allowed Transitions"},{"name":"Polarons in Lead Halide Perovskites","grant_number":"12078","_id":"8fa7db46-16d5-11f0-9cad-917600954daf"}],"scopus_import":"1","author":[{"id":"ff19510a-0d2c-11ef-b018-c338ad2f4325","first_name":"Jinglun","last_name":"Li","full_name":"Li, Jinglun"},{"id":"d7b23d3a-9e21-11ec-b482-f76739596b95","first_name":"Georgios","full_name":"Koutentakis, Georgios","last_name":"Koutentakis"},{"full_name":"Hrast, Mateja","last_name":"Hrast","first_name":"Mateja","id":"48dbb294-2a9c-11ef-905d-f56be71f0e5d"},{"first_name":"Mikhail","full_name":"Lemeshko, Mikhail","last_name":"Lemeshko","id":"37CB05FA-F248-11E8-B48F-1D18A9856A87","orcid":"0000-0002-6990-7802"},{"first_name":"Andreas","full_name":"Schindewolf, Andreas","last_name":"Schindewolf"},{"first_name":"Ragheed","full_name":"Al Hyder, Ragheed","last_name":"Al Hyder","id":"d1c405be-ae15-11ed-8510-ccf53278162e"}],"acknowledgement":"J.-L.Li thanks Gaoren Wang for valuable discussions on the absorbing boundary condition. G.M.K. thanks P. Giannakeas for fruitful discussions during the initial stages of this study. G.M.K. was funded by the Austrian Science Fund (FWF) [10.55776/F1004]. R.A. received funding from the Austrian Academy of Science ÖAW grant No. PR1029OEAW03. A.S. acknowledges funding from the European Union’s Horizon Europe research and innovation programme under grant agreement No. 101219560.","status":"public","fulldoi":"https://doi.org/10.1038/s42005-026-02578-8","license":"https://creativecommons.org/licenses/by/4.0/","date_published":"2026-04-14T00:00:00Z","user_id":"2DF688A6-F248-11E8-B48F-1D18A9856A87","oa":1,"file":[{"checksum":"3bf5852b54b9f13ec1679056a5f58c3a","relation":"main_file","date_created":"2026-06-24T06:09:35Z","access_level":"open_access","file_id":"22133","file_name":"2026_CommunicationsPhysics_Li.pdf","content_type":"application/pdf","creator":"dernst","file_size":1161879,"date_updated":"2026-06-24T06:09:35Z","success":1}],"DOAJ_listed":"1","date_created":"2026-06-21T22:02:58Z","supplementarymaterial":"yes","article_processing_charge":"Yes","department":[{"_id":"MiLe"}],"arxiv":1,"oa_version":"Published Version","OA_place":"publisher","quality_controlled":"1","OA_type":"gold","article_type":"original","month":"04","has_accepted_license":"1","dataavailabilitystatement":"The data that support the findings of this study are available from the corresponding authors upon request. The computational codes that were used to generate the figures presented in this study are available from the corresponding authors upon request.","intvolume":"         9","citation":{"ieee":"J. Li, G. Koutentakis, M. Hrast, M. Lemeshko, A. Schindewolf, and R. Al Hyder, “Tunable field-linked s-wave interactions in dipolar fermi mixtures,” <i>Communications Physics</i>, vol. 9. Springer Nature, 2026.","ista":"Li J, Koutentakis G, Hrast M, Lemeshko M, Schindewolf A, Al Hyder R. 2026. Tunable field-linked s-wave interactions in dipolar fermi mixtures. Communications Physics. 9, 201.","chicago":"Li, Jinglun, Georgios Koutentakis, Mateja Hrast, Mikhail Lemeshko, Andreas Schindewolf, and Ragheed Al Hyder. “Tunable Field-Linked s-Wave Interactions in Dipolar Fermi Mixtures.” <i>Communications Physics</i>. Springer Nature, 2026. <a href=\"https://doi.org/10.1038/s42005-026-02578-8\">https://doi.org/10.1038/s42005-026-02578-8</a>.","ama":"Li J, Koutentakis G, Hrast M, Lemeshko M, Schindewolf A, Al Hyder R. Tunable field-linked s-wave interactions in dipolar fermi mixtures. <i>Communications Physics</i>. 2026;9. doi:<a href=\"https://doi.org/10.1038/s42005-026-02578-8\">10.1038/s42005-026-02578-8</a>","short":"J. Li, G. Koutentakis, M. Hrast, M. Lemeshko, A. Schindewolf, R. Al Hyder, Communications Physics 9 (2026).","apa":"Li, J., Koutentakis, G., Hrast, M., Lemeshko, M., Schindewolf, A., &#38; Al Hyder, R. (2026). Tunable field-linked s-wave interactions in dipolar fermi mixtures. <i>Communications Physics</i>. Springer Nature. <a href=\"https://doi.org/10.1038/s42005-026-02578-8\">https://doi.org/10.1038/s42005-026-02578-8</a>","mla":"Li, Jinglun, et al. “Tunable Field-Linked s-Wave Interactions in Dipolar Fermi Mixtures.” <i>Communications Physics</i>, vol. 9, 201, Springer Nature, 2026, doi:<a href=\"https://doi.org/10.1038/s42005-026-02578-8\">10.1038/s42005-026-02578-8</a>."},"researchdata_availability":"upon request","doi":"10.1038/s42005-026-02578-8","date_updated":"2026-06-24T06:10:44Z","publication_identifier":{"eissn":["2399-3650"]},"article_number":"201","das_tickbox":"1","abstract":[{"lang":"eng","text":"Spin mixtures of degenerate fermions are a cornerstone of quantum many-body physics, enabling superfluidity, polarons, and rich spin dynamics through s-wave scattering resonances. Combining them with strong, long-range dipolar interactions provides highly flexible control schemes promising even more exotic quantum phases. Recently, microwave shielding gave access to spin-polarized degenerate samples of dipolar fermionic molecules, where tunable p-wave interactions were enabled by field-linked resonances available only by compromising the shielding (due to experimental limitations). Here, we study the scattering properties of a fermionic dipolar spin mixture and show that a universal s-wave resonance is readily accessible without compromising the shielding. We develop a universal description of the tunable s-wave interaction and weakly bound tetratomic states based on the microwave-field parameters. The s-wave resonance paves the way to stable, controllable and strongly-interacting dipolar spin mixtures of deeply degenerate fermions and supports favorable conditions to reach this regime via evaporative cooling."}],"ddc":["530"],"type":"journal_article","day":"14","publication_status":"published","language":[{"iso":"eng"}],"PlanS_conform":"1","year":"2026","_id":"22100","file_date_updated":"2026-06-24T06:09:35Z","corr_author":"1","title":"Tunable field-linked s-wave interactions in dipolar fermi mixtures","publication":"Communications Physics","volume":9,"external_id":{"arxiv":["2506.23318"]},"publisher":"Springer Nature"},{"file":[{"checksum":"805c929fff9fd4d0e733293eaace67b8","relation":"main_file","date_created":"2026-02-10T11:25:46Z","access_level":"open_access","file_id":"21210","file_name":"2026_PhysicalReviewLetters_Hrast.pdf","content_type":"application/pdf","creator":"dernst","file_size":511312,"date_updated":"2026-02-10T11:25:46Z","success":1}],"oa":1,"date_created":"2026-02-06T10:53:17Z","status":"public","fulldoi":"https://doi.org/10.1103/fkf1-1jml","date_published":"2026-02-05T00:00:00Z","user_id":"2DF688A6-F248-11E8-B48F-1D18A9856A87","tmp":{"legal_code_url":"https://creativecommons.org/licenses/by/4.0/legalcode","name":"Creative Commons Attribution 4.0 International Public License (CC-BY 4.0)","image":"/images/cc_by.png","short":"CC BY (4.0)"},"project":[{"name":"Coherent Optical Metrology Beyond Electric-Dipole-Allowed Transitions","grant_number":"F100403","_id":"7c040762-9f16-11ee-852c-dd79eeee4ab3"}],"scopus_import":"1","author":[{"id":"48dbb294-2a9c-11ef-905d-f56be71f0e5d","full_name":"Hrast, Mateja","last_name":"Hrast","first_name":"Mateja"},{"id":"d7b23d3a-9e21-11ec-b482-f76739596b95","first_name":"Georgios","full_name":"Koutentakis, Georgios","last_name":"Koutentakis"},{"first_name":"Mikhail","last_name":"Maslov","full_name":"Maslov, Mikhail","id":"2E65BB0E-F248-11E8-B48F-1D18A9856A87","orcid":"0000-0003-4074-2570"},{"id":"37CB05FA-F248-11E8-B48F-1D18A9856A87","orcid":"0000-0002-6990-7802","first_name":"Mikhail","full_name":"Lemeshko, Mikhail","last_name":"Lemeshko"}],"acknowledgement":"This research was funded in whole or in part by the Austrian Science Fund (FWF) [10.55776/F1004].","has_accepted_license":"1","month":"02","department":[{"_id":"MiLe"}],"oa_version":"Published Version","arxiv":1,"OA_place":"publisher","OA_type":"hybrid","quality_controlled":"1","article_type":"original","article_processing_charge":"Yes (via OA deal)","abstract":[{"text":"We present a general theoretical framework for helical dichroism (HD), establishing an explicit link between chiral resolution and orbital angular momentum (OAM) exchange in light–matter interaction. Tracing microscopic mechanisms of the OAM transfer, we derive rotational selection rules, which establish that HD emerges only from the spin–orbit coupling of light, even for beams without the far-field OAM. Our findings refine the conditions for observing HD, provide a tool to re-examine the outcome of prior experiments, and guide future designs for chiral sensing with structured light.","lang":"eng"}],"publication_identifier":{"eissn":["1079-7114"],"issn":["0031-9007"]},"article_number":"053204","doi":"10.1103/fkf1-1jml","issue":"5","date_updated":"2026-02-10T11:30:37Z","intvolume":"       136","citation":{"ama":"Hrast M, Koutentakis G, Maslov M, Lemeshko M. Bottom-up analysis of rovibrational helical dichroism. <i>Physical Review Letters</i>. 2026;136(5). doi:<a href=\"https://doi.org/10.1103/fkf1-1jml\">10.1103/fkf1-1jml</a>","short":"M. Hrast, G. Koutentakis, M. Maslov, M. Lemeshko, Physical Review Letters 136 (2026).","ista":"Hrast M, Koutentakis G, Maslov M, Lemeshko M. 2026. Bottom-up analysis of rovibrational helical dichroism. Physical Review Letters. 136(5), 053204.","chicago":"Hrast, Mateja, Georgios Koutentakis, Mikhail Maslov, and Mikhail Lemeshko. “Bottom-up Analysis of Rovibrational Helical Dichroism.” <i>Physical Review Letters</i>. American Physical Society, 2026. <a href=\"https://doi.org/10.1103/fkf1-1jml\">https://doi.org/10.1103/fkf1-1jml</a>.","ieee":"M. Hrast, G. Koutentakis, M. Maslov, and M. Lemeshko, “Bottom-up analysis of rovibrational helical dichroism,” <i>Physical Review Letters</i>, vol. 136, no. 5. American Physical Society, 2026.","mla":"Hrast, Mateja, et al. “Bottom-up Analysis of Rovibrational Helical Dichroism.” <i>Physical Review Letters</i>, vol. 136, no. 5, 053204, American Physical Society, 2026, doi:<a href=\"https://doi.org/10.1103/fkf1-1jml\">10.1103/fkf1-1jml</a>.","apa":"Hrast, M., Koutentakis, G., Maslov, M., &#38; Lemeshko, M. (2026). Bottom-up analysis of rovibrational helical dichroism. <i>Physical Review Letters</i>. American Physical Society. <a href=\"https://doi.org/10.1103/fkf1-1jml\">https://doi.org/10.1103/fkf1-1jml</a>"},"volume":136,"external_id":{"arxiv":["2505.16393"]},"publisher":"American Physical Society","PlanS_conform":"1","language":[{"iso":"eng"}],"_id":"21149","year":"2026","file_date_updated":"2026-02-10T11:25:46Z","corr_author":"1","title":"Bottom-up analysis of rovibrational helical dichroism","publication":"Physical Review Letters","day":"05","publication_status":"published","ddc":["530"],"type":"journal_article"},{"related_material":{"record":[{"status":"public","id":"18716","relation":"research_data"},{"id":"22866","status":"public","relation":"research_data"}]},"oa":1,"file":[{"access_level":"open_access","date_created":"2025-04-16T09:46:45Z","checksum":"d035683179547b41b811107a8649aab0","relation":"main_file","file_name":"2025_PCCP_Hrast.pdf","file_id":"19581","creator":"dernst","content_type":"application/pdf","success":1,"date_updated":"2025-04-16T09:46:45Z","file_size":1270582}],"date_created":"2024-12-29T23:01:58Z","license":"https://creativecommons.org/licenses/by-nc/3.0/","fulldoi":"https://doi.org/10.1039/d4cp03727h","status":"public","user_id":"2DF688A6-F248-11E8-B48F-1D18A9856A87","date_published":"2025-01-21T00:00:00Z","author":[{"full_name":"Hrast, Mateja","last_name":"Hrast","first_name":"Mateja","id":"48dbb294-2a9c-11ef-905d-f56be71f0e5d"},{"id":"F75EE9BE-5C90-11EA-905D-16643DDC885E","orcid":"0000-0003-0038-7068","first_name":"Marko","last_name":"Ljubotina","full_name":"Ljubotina, Marko"},{"full_name":"Zitnik, Matjaz","last_name":"Zitnik","first_name":"Matjaz"}],"scopus_import":"1","tmp":{"name":"Creative Commons Attribution-NonCommercial 3.0 Unported (CC BY-NC 3.0)","legal_code_url":"https://creativecommons.org/licenses/by-nc/3.0/legalcode","image":"/images/cc_by_nc.png","short":"CC BY-NC (3.0)"},"project":[{"grant_number":"801770","_id":"2688CF98-B435-11E9-9278-68D0E5697425","call_identifier":"H2020","name":"Angulon: physics and applications of a new quasiparticle"}],"acknowledgement":"This publication is based upon work from COST Action CA18212 – Molecular Dynamics in the GAS phase (MD-GAS), supported by COST (European Cooperation in Science and Technology). This work was financially supported by the Slovenian Research Agency in the framework of research program P1-0112 Studies of Atoms, Molecules and Structures by Photons and Particles. Part of this work was financed by the European Research Council (ERC) through the Starting Grant No. 801770 (ANGULON). The authors acknowledge P. Lablanquie, H. Iwayama, F. Penent, K. Soejima and E. Shigemasa for sharing their unpublished experimental spectra on HCl.","has_accepted_license":"1","month":"01","OA_type":"hybrid","quality_controlled":"1","OA_place":"publisher","department":[{"_id":"MiLe"},{"_id":"MaSe"}],"oa_version":"Published Version","article_type":"original","article_processing_charge":"Yes (via OA deal)","isi":1,"abstract":[{"text":"We present an ab initio theoretical method to calculate the resonant Auger spectrum in the presence of ultrafast dissociation. The method is demonstrated by deriving the L-VV resonant Auger spectrum mediated by the 2p3/2−1σ* resonance in HCl, where the electronic Auger decay and nuclear dissociation occur on the same time scale. The Auger decay rates are calculated within the one-center approximation and are shown to vary significantly with the inter-nuclear distance. A quantum-mechanical description of dissociation is effectuated by propagating the corresponding Franck–Condon factors. The calculated profiles of Auger spectral lines resemble those of atomic Auger decay but here the characteristic tails extend towards lower electron kinetic energies, which reflect specific features of the potential energy curves. The presented method can describe the resonant Auger spectrum for an arbitrary speed of dissociation and simplifies to known approximations in the limiting cases.","lang":"eng"}],"publication_identifier":{"issn":["1463-9076"]},"doi":"10.1039/d4cp03727h","issue":"3","date_updated":"2026-09-09T09:20:40Z","pmid":1,"citation":{"mla":"Hrast, Mateja, et al. “Ab Initio Auger Spectrum of the Ultrafast Dissociating 2p3/2−1σ* Resonance in HCl.” <i>Physical Chemistry Chemical Physics</i>, vol. 27, no. 3, Royal Society of Chemistry, 2025, pp. 1473–82, doi:<a href=\"https://doi.org/10.1039/d4cp03727h\">10.1039/d4cp03727h</a>.","apa":"Hrast, M., Ljubotina, M., &#38; Zitnik, M. (2025). Ab initio Auger spectrum of the ultrafast dissociating 2p3/2−1σ* resonance in HCl. <i>Physical Chemistry Chemical Physics</i>. Royal Society of Chemistry. <a href=\"https://doi.org/10.1039/d4cp03727h\">https://doi.org/10.1039/d4cp03727h</a>","short":"M. Hrast, M. Ljubotina, M. Zitnik, Physical Chemistry Chemical Physics 27 (2025) 1473–1482.","ama":"Hrast M, Ljubotina M, Zitnik M. Ab initio Auger spectrum of the ultrafast dissociating 2p3/2−1σ* resonance in HCl. <i>Physical Chemistry Chemical Physics</i>. 2025;27(3):1473-1482. doi:<a href=\"https://doi.org/10.1039/d4cp03727h\">10.1039/d4cp03727h</a>","chicago":"Hrast, Mateja, Marko Ljubotina, and Matjaz Zitnik. “Ab Initio Auger Spectrum of the Ultrafast Dissociating 2p3/2−1σ* Resonance in HCl.” <i>Physical Chemistry Chemical Physics</i>. Royal Society of Chemistry, 2025. <a href=\"https://doi.org/10.1039/d4cp03727h\">https://doi.org/10.1039/d4cp03727h</a>.","ieee":"M. Hrast, M. Ljubotina, and M. Zitnik, “Ab initio Auger spectrum of the ultrafast dissociating 2p3/2−1σ* resonance in HCl,” <i>Physical Chemistry Chemical Physics</i>, vol. 27, no. 3. Royal Society of Chemistry, pp. 1473–1482, 2025.","ista":"Hrast M, Ljubotina M, Zitnik M. 2025. Ab initio Auger spectrum of the ultrafast dissociating 2p3/2−1σ* resonance in HCl. Physical Chemistry Chemical Physics. 27(3), 1473–1482."},"intvolume":"        27","external_id":{"isi":["001379819100001"],"pmid":["39698879"]},"ec_funded":1,"volume":27,"publisher":"Royal Society of Chemistry","_id":"18710","file_date_updated":"2025-04-16T09:46:45Z","year":"2025","page":"1473-1482","language":[{"iso":"eng"}],"publication":"Physical Chemistry Chemical Physics","title":"Ab initio Auger spectrum of the ultrafast dissociating 2p3/2−1σ* resonance in HCl","corr_author":"1","day":"21","publication_status":"published","ddc":["530"],"type":"journal_article"},{"month":"09","corr_author":"1","title":"Data for: Ab initio Auger spectrum of the ultrafast dissociating 2p3/2−1σ* resonance in HCl","year":"2024","_id":"18716","main_file_link":[{"open_access":"1","url":"https://doi.org/10.5281/zenodo.13833474"}],"publisher":"Zenodo","type":"research_data_reference","article_processing_charge":"No","ddc":["530"],"day":"24","oa_version":"None","department":[{"_id":"MiLe"}],"date_created":"2025-01-02T08:21:55Z","related_material":{"record":[{"relation":"used_in_publication","id":"18710","status":"public"}]},"oa":1,"abstract":[{"lang":"eng","text":"Data for publication 10.1039/d4cp03727h"}],"citation":{"mla":"Hrast, Mateja. <i>Data for: Ab Initio Auger Spectrum of the Ultrafast Dissociating 2p3/2−1σ* Resonance in HCl</i>. Zenodo, 2024, doi:<a href=\"https://doi.org/10.5281/ZENODO.13833474\">10.5281/ZENODO.13833474</a>.","apa":"Hrast, M. (2024). Data for: Ab initio Auger spectrum of the ultrafast dissociating 2p3/2−1σ* resonance in HCl. Zenodo. <a href=\"https://doi.org/10.5281/ZENODO.13833474\">https://doi.org/10.5281/ZENODO.13833474</a>","ama":"Hrast M. Data for: Ab initio Auger spectrum of the ultrafast dissociating 2p3/2−1σ* resonance in HCl. 2024. doi:<a href=\"https://doi.org/10.5281/ZENODO.13833474\">10.5281/ZENODO.13833474</a>","short":"M. Hrast, (2024).","ieee":"M. Hrast, “Data for: Ab initio Auger spectrum of the ultrafast dissociating 2p3/2−1σ* resonance in HCl.” Zenodo, 2024.","chicago":"Hrast, Mateja. “Data for: Ab Initio Auger Spectrum of the Ultrafast Dissociating 2p3/2−1σ* Resonance in HCl.” Zenodo, 2024. <a href=\"https://doi.org/10.5281/ZENODO.13833474\">https://doi.org/10.5281/ZENODO.13833474</a>.","ista":"Hrast M. 2024. Data for: Ab initio Auger spectrum of the ultrafast dissociating 2p3/2−1σ* resonance in HCl, Zenodo, <a href=\"https://doi.org/10.5281/ZENODO.13833474\">10.5281/ZENODO.13833474</a>."},"author":[{"id":"48dbb294-2a9c-11ef-905d-f56be71f0e5d","first_name":"Mateja","last_name":"Hrast","full_name":"Hrast, Mateja"}],"user_id":"2DF688A6-F248-11E8-B48F-1D18A9856A87","date_updated":"2025-05-19T14:03:18Z","date_published":"2024-09-24T00:00:00Z","doi":"10.5281/ZENODO.13833474","fulldoi":"https://doi.org/10.5281/ZENODO.13833474","status":"public"},{"date_created":"2024-09-18T11:43:16Z","related_material":{"record":[{"status":"public","id":"19048","relation":"dissertation_contains"}]},"DOAJ_listed":"1","file":[{"success":1,"date_updated":"2024-09-23T09:46:20Z","file_size":1563824,"creator":"dernst","content_type":"application/pdf","file_name":"2024_PhysicalReviewResearch_Maslov.pdf","file_id":"18125","access_level":"open_access","date_created":"2024-09-23T09:46:20Z","checksum":"8f744d94956a1683b473b1cf9b411a37","relation":"main_file"}],"oa":1,"date_published":"2024-09-10T00:00:00Z","user_id":"2DF688A6-F248-11E8-B48F-1D18A9856A87","fulldoi":"https://doi.org/10.1103/physrevresearch.6.033277","status":"public","acknowledgement":"We are grateful to Emilio Pisanty and Philipp Lunt for valuable discussions. This research was funded wholly or in part by the Austrian Science Fund (FWF) [10.55776/F1004]. G.M.K. gratefully acknowledges funding from the European Union’s Horizon 2020 research and innovation programme under the Marie Skłodowska-Curie Grant Agreement No. 101034413. M.L. acknowledges support by the European Research Council (ERC) Starting Grant No. 801770 (ANGULON). O.H.H. acknowledges support by the Austrian Science Fund (FWF) [10.55776/P36040]. Furthermore, the financial support by the Austrian Federal Ministry for Digital and Economic Affairs, the National Foundation for Research, Technology and Development, and the Christian Doppler Research Association is gratefully acknowledged.","author":[{"last_name":"Maslov","full_name":"Maslov, Mikhail","first_name":"Mikhail","orcid":"0000-0003-4074-2570","id":"2E65BB0E-F248-11E8-B48F-1D18A9856A87"},{"last_name":"Koutentakis","full_name":"Koutentakis, Georgios","first_name":"Georgios","id":"d7b23d3a-9e21-11ec-b482-f76739596b95"},{"first_name":"Mateja","last_name":"Hrast","full_name":"Hrast, Mateja","id":"48dbb294-2a9c-11ef-905d-f56be71f0e5d"},{"last_name":"Heckl","full_name":"Heckl, Oliver H.","first_name":"Oliver H."},{"orcid":"0000-0002-6990-7802","id":"37CB05FA-F248-11E8-B48F-1D18A9856A87","last_name":"Lemeshko","full_name":"Lemeshko, Mikhail","first_name":"Mikhail"}],"scopus_import":"1","tmp":{"legal_code_url":"https://creativecommons.org/licenses/by/4.0/legalcode","name":"Creative Commons Attribution 4.0 International Public License (CC-BY 4.0)","image":"/images/cc_by.png","short":"CC BY (4.0)"},"project":[{"name":"Coherent Optical Metrology Beyond Electric-Dipole-Allowed Transitions","grant_number":"F100403","_id":"7c040762-9f16-11ee-852c-dd79eeee4ab3"},{"name":"IST-BRIDGE: International postdoctoral program","call_identifier":"H2020","grant_number":"101034413","_id":"fc2ed2f7-9c52-11eb-aca3-c01059dda49c"},{"call_identifier":"H2020","name":"Angulon: physics and applications of a new quasiparticle","_id":"2688CF98-B435-11E9-9278-68D0E5697425","grant_number":"801770"},{"name":"FWF Open Access Fund","call_identifier":"FWF","_id":"3AC91DDA-15DF-11EA-824D-93A3E7B544D1"}],"has_accepted_license":"1","month":"09","article_type":"original","OA_place":"publisher","OA_type":"gold","quality_controlled":"1","arxiv":1,"oa_version":"Published Version","department":[{"_id":"GradSch"},{"_id":"MiLe"}],"article_processing_charge":"Yes","abstract":[{"text":"We present a theory describing the interaction of structured light, such as light carrying orbital angular momentum, with molecules. The light-matter interaction Hamiltonian we derive is expressed through couplings between spherical gradients of the electric field and the (transition) electric multipole moments of a particle of any nontrivial rotation point group. Our model can therefore accommodate an arbitrary complexity of the molecular and electric field structure, and it can be straightforwardly extended to atoms or nanostructures. Applying this framework to rovibrational spectroscopy of molecules, we uncover the general mechanism of angular momentum exchange between the spin and orbital angular momenta of light, molecular rotation, and its center-of-mass motion. We show that the nonzero vorticity of Laguerre-Gaussian beams can strongly enhance certain rovibrational transitions that are considered forbidden in the case of nonhelical light. We discuss the experimental requirements for the observation of these forbidden transitions in state-of-the-art spatially resolved spectroscopy measurements.","lang":"eng"}],"article_number":"033277","publication_identifier":{"eissn":["2643-1564"]},"issue":"3","date_updated":"2026-04-07T11:52:53Z","doi":"10.1103/physrevresearch.6.033277","citation":{"apa":"Maslov, M., Koutentakis, G., Hrast, M., Heckl, O. H., &#38; Lemeshko, M. (2024). Theory of angular momentum transfer from light to molecules. <i>Physical Review Research</i>. American Physical Society. <a href=\"https://doi.org/10.1103/physrevresearch.6.033277\">https://doi.org/10.1103/physrevresearch.6.033277</a>","mla":"Maslov, Mikhail, et al. “Theory of Angular Momentum Transfer from Light to Molecules.” <i>Physical Review Research</i>, vol. 6, no. 3, 033277, American Physical Society, 2024, doi:<a href=\"https://doi.org/10.1103/physrevresearch.6.033277\">10.1103/physrevresearch.6.033277</a>.","ieee":"M. Maslov, G. Koutentakis, M. Hrast, O. H. Heckl, and M. Lemeshko, “Theory of angular momentum transfer from light to molecules,” <i>Physical Review Research</i>, vol. 6, no. 3. American Physical Society, 2024.","ista":"Maslov M, Koutentakis G, Hrast M, Heckl OH, Lemeshko M. 2024. Theory of angular momentum transfer from light to molecules. Physical Review Research. 6(3), 033277.","chicago":"Maslov, Mikhail, Georgios Koutentakis, Mateja Hrast, Oliver H. Heckl, and Mikhail Lemeshko. “Theory of Angular Momentum Transfer from Light to Molecules.” <i>Physical Review Research</i>. American Physical Society, 2024. <a href=\"https://doi.org/10.1103/physrevresearch.6.033277\">https://doi.org/10.1103/physrevresearch.6.033277</a>.","short":"M. Maslov, G. Koutentakis, M. Hrast, O.H. Heckl, M. Lemeshko, Physical Review Research 6 (2024).","ama":"Maslov M, Koutentakis G, Hrast M, Heckl OH, Lemeshko M. Theory of angular momentum transfer from light to molecules. <i>Physical Review Research</i>. 2024;6(3). doi:<a href=\"https://doi.org/10.1103/physrevresearch.6.033277\">10.1103/physrevresearch.6.033277</a>"},"intvolume":"         6","APC_amount":"3028,31 EUR","publisher":"American Physical Society","external_id":{"arxiv":["2310.00095"]},"volume":6,"ec_funded":1,"publication":"Physical Review Research","title":"Theory of angular momentum transfer from light to molecules","corr_author":"1","_id":"18087","file_date_updated":"2024-09-23T09:46:20Z","year":"2024","language":[{"iso":"eng"}],"publication_status":"published","day":"10","type":"journal_article","ddc":["530"]}]