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The life span of nuclear RNAs, which are critical for proper chromatin architecture and transcription regulation, has not been determined in adult tissues. In this work, we identified and characterized nuclear RNAs that do not turn over for at least 2 years in a subset of postnatally born cells in the mouse brain. These long-lived RNAs were stably retained in nuclei in a neural cell type–specific manner and were required for the maintenance of heterochromatin. Thus, the life span of neural cells may depend on both the molecular longevity of DNA for the storage of genetic information and also the extreme stability of RNA for the functional organization of chromatin."}],"fulldoi":"https://doi.org/10.1126/science.adf3481","year":"2024","supplementarymaterial":"yes","issue":"6691","user_id":"317138e5-6ab7-11ef-aa6d-ffef3953e345","article_type":"original","dataavailabilitystatement":"All data are available in the main text, figures, or supplementary materials. EU-RNA-seq data were submitted to the Gene Expression Omnibus (GEO) under accession no. GSE248101.","type":"journal_article","language":[{"iso":"eng"}],"oa_version":"Submitted Version","status":"public","department":[{"_id":"MaHe"}],"main_file_link":[{"open_access":"1","url":"https://www.ncbi.nlm.nih.gov/pmc/articles/PMC7615865"}],"citation":{"chicago":"Zocher, Sara, Asako Mccloskey, Anne Karasinsky, Roberta Schulte, Ulrike Friedrich, Mathias Lesche, Nicole Rund, Fred H. Gage, Martin Hetzer, and Tomohisa Toda. “Lifelong Persistence of Nuclear RNAs in the Mouse Brain.” Science. AAAS, 2024. https://doi.org/10.1126/science.adf3481.","apa":"Zocher, S., Mccloskey, A., Karasinsky, A., Schulte, R., Friedrich, U., Lesche, M., … Toda, T. (2024). Lifelong persistence of nuclear RNAs in the mouse brain. Science. AAAS. https://doi.org/10.1126/science.adf3481","short":"S. Zocher, A. Mccloskey, A. Karasinsky, R. Schulte, U. Friedrich, M. Lesche, N. Rund, F.H. Gage, M. Hetzer, T. Toda, Science 384 (2024) 53–59.","mla":"Zocher, Sara, et al. “Lifelong Persistence of Nuclear RNAs in the Mouse Brain.” Science, vol. 384, no. 6691, AAAS, 2024, pp. 53–59, doi:10.1126/science.adf3481.","ama":"Zocher S, Mccloskey A, Karasinsky A, et al. Lifelong persistence of nuclear RNAs in the mouse brain. Science. 2024;384(6691):53-59. doi:10.1126/science.adf3481","ista":"Zocher S, Mccloskey A, Karasinsky A, Schulte R, Friedrich U, Lesche M, Rund N, Gage FH, Hetzer M, Toda T. 2024. Lifelong persistence of nuclear RNAs in the mouse brain. Science. 384(6691), 53–59.","ieee":"S. Zocher et al., “Lifelong persistence of nuclear RNAs in the mouse brain,” Science, vol. 384, no. 6691. AAAS, pp. 53–59, 2024."},"quality_controlled":"1","date_updated":"2026-10-16T08:59:32Z","_id":"15316","intvolume":" 384","researchdata_availability":"yes","date_created":"2024-04-14T22:01:01Z","OA_type":"green","publication_status":"published","date_published":"2024-04-04T00:00:00Z","author":[{"last_name":"Zocher","first_name":"Sara","full_name":"Zocher, Sara"},{"first_name":"Asako","last_name":"Mccloskey","full_name":"Mccloskey, Asako"},{"first_name":"Anne","last_name":"Karasinsky","full_name":"Karasinsky, Anne"},{"full_name":"Schulte, Roberta","first_name":"Roberta","last_name":"Schulte"},{"full_name":"Friedrich, Ulrike","first_name":"Ulrike","last_name":"Friedrich"},{"first_name":"Mathias","last_name":"Lesche","full_name":"Lesche, Mathias"},{"full_name":"Rund, Nicole","last_name":"Rund","first_name":"Nicole"},{"full_name":"Gage, Fred H.","last_name":"Gage","first_name":"Fred H."},{"full_name":"Hetzer, Martin W","first_name":"Martin W","id":"86c0d31b-b4eb-11ec-ac5a-eae7b2e135ed","orcid":"0000-0002-2111-992X","last_name":"Hetzer"},{"full_name":"Toda, Tomohisa","last_name":"Toda","first_name":"Tomohisa"}],"pmid":1,"page":"53-59","isi":1,"das_tickbox":"1","title":"Lifelong persistence of nuclear RNAs in the mouse brain","doi":"10.1126/science.adf3481"},{"publisher":"Repository","ddc":["570"],"day":"21","_id":"22865","date_updated":"2026-10-16T09:00:15Z","abstract":[{"text":"Dataset for Dos Santos et al, 2024","lang":"eng"}],"date_created":"2026-09-09T08:43:34Z","related_material":{"record":[{"status":"public","relation":"used_in_publication","id":"18480"}]},"month":"10","oa_version":"None","OA_place":"repository","status":"public","main_file_link":[{"url":"https://doi.org/10.5281/zenodo.6491943","open_access":"1"}],"department":[{"_id":"MaHe"}],"oa":1,"article_processing_charge":"No","citation":{"ieee":"R. Arrojo e Drigo, “Calorie restriction increases insulin sensitivity to promote beta cell homeostasis and longevity.” Repository, 2024.","mla":"Arrojo e Drigo, Rafael. Calorie Restriction Increases Insulin Sensitivity to Promote Beta Cell Homeostasis and Longevity. Repository, 2024, doi:10.5281/zenodo.6491943.","ama":"Arrojo e Drigo R. Calorie restriction increases insulin sensitivity to promote beta cell homeostasis and longevity. 2024. doi:10.5281/zenodo.6491943","ista":"Arrojo e Drigo R. 2024. Calorie restriction increases insulin sensitivity to promote beta cell homeostasis and longevity, Repository, 10.5281/zenodo.6491943.","short":"R. Arrojo e Drigo, (2024).","chicago":"Arrojo e Drigo, Rafael. “Calorie Restriction Increases Insulin Sensitivity to Promote Beta Cell Homeostasis and Longevity.” Repository, 2024. https://doi.org/10.5281/zenodo.6491943.","apa":"Arrojo e Drigo, R. (2024). Calorie restriction increases insulin sensitivity to promote beta cell homeostasis and longevity. Repository. https://doi.org/10.5281/zenodo.6491943"},"author":[{"full_name":"Arrojo e Drigo, Rafael","last_name":"Arrojo e Drigo","first_name":"Rafael"}],"date_published":"2024-10-21T00:00:00Z","type":"research_data_reference","title":"Calorie restriction increases insulin sensitivity to promote beta cell homeostasis and longevity","doi":"10.5281/zenodo.6491943","fulldoi":"https://doi.org/10.5281/zenodo.6491943","OA_type":"green","year":"2024","user_id":"317138e5-6ab7-11ef-aa6d-ffef3953e345"},{"date_published":"2024-10-04T00:00:00Z","author":[{"last_name":"Tang","first_name":"Xuechen","full_name":"Tang, Xuechen"}],"doi":"10.5281/zenodo.13889273","title":"The interaction between the DSC2 and the cell membrane","type":"research_data_reference","year":"2024","fulldoi":"https://doi.org/10.5281/zenodo.13889273","OA_type":"green","user_id":"317138e5-6ab7-11ef-aa6d-ffef3953e345","ddc":["570"],"publisher":"Zenodo","date_created":"2026-10-16T09:10:47Z","abstract":[{"lang":"eng","text":"The attached trajectories illustrate the thinning of the membrane by DSC2, the impact of Y53A, R54A mutations on this process.In order to comply with the size limit, the initial conformations as well as one illustrative example of the final productive simulation of each simulated system are provided herewith. The initial conformations are provided in PDB format, while the final productive simulations are uploaded in NetCDF (AMBER) format. "}],"date_updated":"2026-10-16T09:14:37Z","_id":"23143","day":"04","oa_version":"None","month":"10","related_material":{"record":[{"id":"18522","status":"public","relation":"used_in_publication"}]},"article_processing_charge":"No","citation":{"chicago":"Tang, Xuechen. “The Interaction between the DSC2 and the Cell Membrane.” Zenodo, 2024. https://doi.org/10.5281/zenodo.13889273.","apa":"Tang, X. (2024). The interaction between the DSC2 and the cell membrane. Zenodo. https://doi.org/10.5281/zenodo.13889273","short":"X. Tang, (2024).","ama":"Tang X. The interaction between the DSC2 and the cell membrane. 2024. doi:10.5281/zenodo.13889273","ista":"Tang X. 2024. The interaction between the DSC2 and the cell membrane, Zenodo, 10.5281/zenodo.13889273.","mla":"Tang, Xuechen. The Interaction between the DSC2 and the Cell Membrane. Zenodo, 2024, doi:10.5281/zenodo.13889273.","ieee":"X. Tang, “The interaction between the DSC2 and the cell membrane.” Zenodo, 2024."},"main_file_link":[{"open_access":"1","url":"https://doi.org/10.5281/zenodo.13889273"}],"oa":1,"status":"public","OA_place":"repository"},{"doi":"10.1021/acsaelm.3c00055","file_date_updated":"2024-07-16T07:54:21Z","das_tickbox":"0","isi":1,"title":"Engineering of thermoelectric composites based on silver selenide in aqueous solution and ambient temperature","page":"2807-215","date_published":"2024-05-28T00:00:00Z","publication_status":"published","pmid":1,"author":[{"last_name":"Nan","first_name":"Bingfei","full_name":"Nan, Bingfei"},{"first_name":"Mengyao","last_name":"Li","full_name":"Li, Mengyao"},{"full_name":"Zhang, Yu","last_name":"Zhang","first_name":"Yu"},{"first_name":"Ke","last_name":"Xiao","full_name":"Xiao, Ke"},{"last_name":"Lim","first_name":"Khak Ho","full_name":"Lim, Khak Ho"},{"id":"9E331C2E-9F27-11E9-AE48-5033E6697425","last_name":"Chang","orcid":"0000-0002-9515-4277","first_name":"Cheng","full_name":"Chang, Cheng"},{"last_name":"Han","first_name":"Xu","full_name":"Han, Xu"},{"last_name":"Zuo","first_name":"Yong","full_name":"Zuo, Yong"},{"full_name":"Li, Junshan","first_name":"Junshan","last_name":"Li"},{"last_name":"Arbiol","first_name":"Jordi","full_name":"Arbiol, Jordi"},{"full_name":"Llorca, Jordi","last_name":"Llorca","first_name":"Jordi"},{"first_name":"Maria","last_name":"Ibáñez","orcid":"0000-0001-5013-2843","id":"43C61214-F248-11E8-B48F-1D18A9856A87","full_name":"Ibáñez, Maria"},{"last_name":"Cabot","first_name":"Andreu","full_name":"Cabot, Andreu"}],"file":[{"access_level":"open_access","file_id":"17250","file_name":"2024_ACSAppElecMaterials_Nan.pdf","date_updated":"2024-07-16T07:54:21Z","checksum":"1f743eaf4fc988cd30102b7c2f12c15d","relation":"main_file","date_created":"2024-07-16T07:54:21Z","success":1,"creator":"dernst","content_type":"application/pdf","file_size":5851865}],"researchdata_availability":"no","date_created":"2023-05-28T22:01:03Z","intvolume":" 6","tmp":{"name":"Creative Commons Attribution 4.0 International Public License (CC-BY 4.0)","legal_code_url":"https://creativecommons.org/licenses/by/4.0/legalcode","image":"/images/cc_by.png","short":"CC BY (4.0)"},"date_updated":"2026-10-16T09:18:36Z","_id":"13093","quality_controlled":"1","citation":{"mla":"Nan, Bingfei, et al. “Engineering of Thermoelectric Composites Based on Silver Selenide in Aqueous Solution and Ambient Temperature.” ACS Applied Electronic Materials, vol. 6, no. 5, American Chemical Society, 2024, pp. 2807–215, doi:10.1021/acsaelm.3c00055.","ama":"Nan B, Li M, Zhang Y, et al. Engineering of thermoelectric composites based on silver selenide in aqueous solution and ambient temperature. ACS Applied Electronic Materials. 2024;6(5):2807-215. doi:10.1021/acsaelm.3c00055","ista":"Nan B, Li M, Zhang Y, Xiao K, Lim KH, Chang C, Han X, Zuo Y, Li J, Arbiol J, Llorca J, Ibáñez M, Cabot A. 2024. Engineering of thermoelectric composites based on silver selenide in aqueous solution and ambient temperature. ACS Applied Electronic Materials. 6(5), 2807–215.","ieee":"B. Nan et al., “Engineering of thermoelectric composites based on silver selenide in aqueous solution and ambient temperature,” ACS Applied Electronic Materials, vol. 6, no. 5. American Chemical Society, pp. 2807–215, 2024.","apa":"Nan, B., Li, M., Zhang, Y., Xiao, K., Lim, K. H., Chang, C., … Cabot, A. (2024). Engineering of thermoelectric composites based on silver selenide in aqueous solution and ambient temperature. ACS Applied Electronic Materials. American Chemical Society. https://doi.org/10.1021/acsaelm.3c00055","chicago":"Nan, Bingfei, Mengyao Li, Yu Zhang, Ke Xiao, Khak Ho Lim, Cheng Chang, Xu Han, et al. “Engineering of Thermoelectric Composites Based on Silver Selenide in Aqueous Solution and Ambient Temperature.” ACS Applied Electronic Materials. American Chemical Society, 2024. https://doi.org/10.1021/acsaelm.3c00055.","short":"B. Nan, M. Li, Y. Zhang, K. Xiao, K.H. Lim, C. Chang, X. Han, Y. Zuo, J. Li, J. Arbiol, J. Llorca, M. Ibáñez, A. Cabot, ACS Applied Electronic Materials 6 (2024) 2807–215."},"department":[{"_id":"MaIb"}],"status":"public","oa_version":"Published Version","language":[{"iso":"eng"}],"type":"journal_article","article_type":"review","license":"https://creativecommons.org/licenses/by/4.0/","user_id":"317138e5-6ab7-11ef-aa6d-ffef3953e345","issue":"5","supplementarymaterial":"yes","year":"2024","project":[{"grant_number":"M02889","_id":"9B8804FC-BA93-11EA-9121-9846C619BF3A","name":"Bottom-up Engineering for Thermoelectric Applications"},{"name":"HighTE: The Werner Siemens Laboratory for the High Throughput Discovery of Semiconductors for Waste Heat Recovery","_id":"9B8F7476-BA93-11EA-9121-9846C619BF3A"}],"fulldoi":"https://doi.org/10.1021/acsaelm.3c00055","abstract":[{"text":"The direct, solid state, and reversible conversion between heat and electricity using thermoelectric devices finds numerous potential uses, especially around room temperature. However, the relatively high material processing cost limits their real applications. Silver selenide (Ag2Se) is one of the very few n-type thermoelectric (TE) materials for room-temperature applications. Herein, we report a room temperature, fast, and aqueous-phase synthesis approach to produce Ag2Se, which can be extended to other metal chalcogenides. These materials reach TE figures of merit (zT) of up to 0.76 at 380 K. To improve these values, bismuth sulfide (Bi2S3) particles also prepared in an aqueous solution are incorporated into the Ag2Se matrix. In this way, a series of Ag2Se/Bi2S3 composites with Bi2S3 wt % of 0.5, 1.0, and 1.5 are prepared by solution blending and hot-press sintering. The presence of Bi2S3 significantly improves the Seebeck coefficient and power factor while at the same time decreasing the thermal conductivity with no apparent drop in electrical conductivity. Thus, a maximum zT value of 0.96 is achieved in the composites with 1.0 wt % Bi2S3 at 370 K. Furthermore, a high average zT value (zTave) of 0.93 in the 300–390 K range is demonstrated.","lang":"eng"}],"scopus_import":"1","publication_identifier":{"eissn":["2637-6113"]},"volume":6,"day":"28","has_accepted_license":"1","ddc":["540"],"acknowledgement":"Open Access is funded by the Austrian Science Fund (FWF). B.N., M.L., Y.Z., K.X., and X.H. thank the China Scholarship Council (CSC) for the scholarship support. C.C. received funding from the FWF “Lise Meitner Fellowship” grant agreement M 2889-N. M.I. acknowledges the financial support from ISTA and the Werner Siemens Foundation. ICN2 acknowledges funding from Generalitat de Catalunya 2021SGR00457 and project NANOGEN (PID2020-116093RB-C43) funded by MCIN/AEI/10.13039/501100011033/. ICN2 was supported by the Severo Ochoa program from Spanish MCIN/AEI (Grant No.: CEX2021-001214-S) and was funded by the CERCA Programme/Generalitat de Catalunya. J.L. is a Serra Húnter Fellow and is grateful to the ICREA Academia program and projects MICINN/FEDER PID2021-124572OB-C31 and 2021 SGR 01061. K.H.L. acknowledges support from the National Natural Science Foundation of China (22208293). This study is part of the Advanced Materials programme and was supported by MCIN with funding from European Union NextGenerationEU (PRTR-C17.I1) and by Generalitat de Catalunya.","publisher":"American Chemical Society","article_processing_charge":"Yes (in subscription journal)","oa":1,"publication":"ACS Applied Electronic Materials","external_id":{"isi":["000986859000001"],"pmid":["38828037"]},"month":"05"},{"oa":1,"article_processing_charge":"Yes (in subscription journal)","publication":"Journal of Visualized Experiments","external_id":{"isi":["001281657200005"],"pmid":["38829127"]},"OA_place":"publisher","related_material":{"record":[{"status":"public","relation":"dissertation_contains","id":"22626"}]},"month":"05","publication_identifier":{"issn":["1940-087X"]},"scopus_import":"1","abstract":[{"text":"In recent years, solution processes have gained considerable traction as a cost-effective and scalable method to produce high-performance thermoelectric materials. The process entails a series of critical steps: synthesis, purification, thermal treatments, and consolidation, each playing a pivotal role in determining performance, stability, and reproducibility. We have noticed a need for more comprehensive details for each of the described steps in most published works. Recognizing the significance of detailed synthetic protocols, we describe here the approach used to synthesize and characterize one of the highest-performing polycrystalline p-type SnSe. In particular, we report the synthesis of SnSe particles in water and the subsequent surface treatment with CdSe molecular complexes that yields CdSe-SnSe nanocomposites upon consolidation. Moreover, the surface treatment inhibits grain growth through Zenner pinning of secondary phase CdSe nanoparticles and enhances defect formation at different length scales. The enhanced complexity in the CdSe-SnSe nanocomposite microstructure with respect to SnSe promotes phonon scattering and thereby significantly reduces the thermal conductivity. Such surface engineering provides opportunities in solution processing for introducing and controlling defects, making it possible to optimize the transport properties and attain a high thermoelectric figure of merit.","lang":"eng"}],"day":"01","volume":2024,"acknowledgement":"The Scientific Service Units (SSU) of ISTA supported this research through resources provided by the Electron Microscopy Facility (EMF) and the Lab Support Facility (LSF). This work was financially supported by the Institute of Science and Technology Austria and the Werner Siemens Foundation.","ddc":["530"],"has_accepted_license":"1","corr_author":"1","publisher":"MyJove Corporation","APC_amount":"4394,84 EUR","license":"https://creativecommons.org/licenses/by-nc-nd/3.0/","supplementarymaterial":"no","issue":"207","user_id":"317138e5-6ab7-11ef-aa6d-ffef3953e345","fulldoi":"https://doi.org/10.3791/66278","project":[{"_id":"9B8F7476-BA93-11EA-9121-9846C619BF3A","name":"HighTE: The Werner Siemens Laboratory for the High Throughput Discovery of Semiconductors for Waste Heat Recovery"}],"year":"2024","type":"journal_article","acknowledged_ssus":[{"_id":"EM-Fac"},{"_id":"LifeSc"}],"article_type":"original","department":[{"_id":"MaIb"}],"citation":{"ieee":"C. Fiedler, Y. Liu, and M. Ibáñez, “Solution-processed, surface-engineered, polycrystalline CdSe-SnSe exhibiting low thermal conductivity,” Journal of Visualized Experiments, vol. 2024, no. 207. MyJove Corporation, 2024.","mla":"Fiedler, Christine, et al. “Solution-Processed, Surface-Engineered, Polycrystalline CdSe-SnSe Exhibiting Low Thermal Conductivity.” Journal of Visualized Experiments, vol. 2024, no. 207, e66278, MyJove Corporation, 2024, doi:10.3791/66278.","ista":"Fiedler C, Liu Y, Ibáñez M. 2024. Solution-processed, surface-engineered, polycrystalline CdSe-SnSe exhibiting low thermal conductivity. Journal of Visualized Experiments. 2024(207), e66278.","ama":"Fiedler C, Liu Y, Ibáñez M. Solution-processed, surface-engineered, polycrystalline CdSe-SnSe exhibiting low thermal conductivity. Journal of Visualized Experiments. 2024;2024(207). doi:10.3791/66278","short":"C. Fiedler, Y. Liu, M. Ibáñez, Journal of Visualized Experiments 2024 (2024).","chicago":"Fiedler, Christine, Yu Liu, and Maria Ibáñez. “Solution-Processed, Surface-Engineered, Polycrystalline CdSe-SnSe Exhibiting Low Thermal Conductivity.” Journal of Visualized Experiments. 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MyJove Corporation. https://doi.org/10.3791/66278"},"status":"public","oa_version":"Published Version","language":[{"iso":"eng"}],"intvolume":" 2024","date_created":"2024-06-09T22:01:02Z","researchdata_availability":"no","quality_controlled":"1","article_number":"e66278","_id":"17124","tmp":{"legal_code_url":"https://creativecommons.org/licenses/by-nc-nd/3.0/legalcode","image":"/images/cc_by_nc_nd.png","name":"Creative Commons Attribution-NonCommercial-NoDerivs 3.0 Unported (CC BY-NC-ND 3.0)","short":"CC BY-NC-ND (3.0)"},"date_updated":"2026-10-16T09:18:16Z","OA_type":"hybrid","das_tickbox":"0","title":"Solution-processed, surface-engineered, polycrystalline CdSe-SnSe exhibiting low thermal conductivity","isi":1,"file_date_updated":"2025-02-17T15:08:55Z","doi":"10.3791/66278","file":[{"relation":"main_file","checksum":"ddb41f1ce2333484ab5cd109ac2941c0","date_updated":"2025-02-17T15:08:55Z","creator":"dernst","date_created":"2025-02-17T15:08:55Z","success":1,"content_type":"application/pdf","file_size":1371995,"access_level":"open_access","file_id":"19047","file_name":"2024_JoVE_Fiedler.pdf"}],"pmid":1,"publication_status":"published","author":[{"full_name":"Fiedler, Christine","first_name":"Christine","id":"bd3fceba-dc74-11ea-a0a7-c17f71817366","last_name":"Fiedler"},{"full_name":"Liu, Yu","first_name":"Yu","id":"2A70014E-F248-11E8-B48F-1D18A9856A87","orcid":"0000-0001-7313-6740","last_name":"Liu"},{"last_name":"Ibáñez","orcid":"0000-0001-5013-2843","id":"43C61214-F248-11E8-B48F-1D18A9856A87","first_name":"Maria","full_name":"Ibáñez, Maria"}],"date_published":"2024-05-01T00:00:00Z"},{"file":[{"file_id":"18870","access_level":"open_access","file_name":"2024_NatureComm_Weyer.pdf","date_created":"2025-01-22T14:36:33Z","success":1,"creator":"dernst","checksum":"32c986fc3babec999c03a5c043310f40","date_updated":"2025-01-22T14:36:33Z","relation":"main_file","file_size":5634494,"content_type":"application/pdf"}],"pmid":1,"date_published":"2024-12-01T00:00:00Z","publication_status":"published","author":[{"first_name":"Yannick","last_name":"Weyer","full_name":"Weyer, Yannick"},{"last_name":"Schwabl","first_name":"Sinead I.","full_name":"Schwabl, Sinead I."},{"first_name":"Xuechen","last_name":"Tang","full_name":"Tang, Xuechen"},{"full_name":"Purwar, Astha","first_name":"Astha","last_name":"Purwar"},{"first_name":"Konstantin","last_name":"Siegmann","full_name":"Siegmann, Konstantin"},{"last_name":"Ruepp","first_name":"Angela","full_name":"Ruepp, Angela"},{"last_name":"Dunzendorfer-Matt","first_name":"Theresia","full_name":"Dunzendorfer-Matt, Theresia"},{"full_name":"Widerin, Michael A.","last_name":"Widerin","first_name":"Michael A."},{"full_name":"Niedrist, Veronika","first_name":"Veronika","last_name":"Niedrist"},{"last_name":"Mutsters","first_name":"Noa J.M.","full_name":"Mutsters, Noa J.M."},{"full_name":"Tettamanti, Maria G.","last_name":"Tettamanti","first_name":"Maria G."},{"full_name":"Weys, Sabine","last_name":"Weys","id":"caffa136-9669-11ed-9092-ceac12ac9c05","first_name":"Sabine"},{"full_name":"Sarg, Bettina","last_name":"Sarg","first_name":"Bettina"},{"first_name":"Leopold","last_name":"Kremser","full_name":"Kremser, Leopold"},{"first_name":"Klaus R.","last_name":"Liedl","full_name":"Liedl, Klaus R."},{"last_name":"Schmidt","first_name":"Oliver","full_name":"Schmidt, Oliver"},{"full_name":"Teis, David","first_name":"David","last_name":"Teis"}],"doi":"10.1038/s41467-024-53676-6","isi":1,"title":"The Dsc ubiquitin ligase complex identifies transmembrane degrons to degrade orphaned proteins at the Golgi","file_date_updated":"2025-01-22T14:36:33Z","das_tickbox":"1","OA_type":"gold","tmp":{"name":"Creative Commons Attribution 4.0 International Public License (CC-BY 4.0)","legal_code_url":"https://creativecommons.org/licenses/by/4.0/legalcode","image":"/images/cc_by.png","short":"CC BY (4.0)"},"date_updated":"2026-10-16T09:15:18Z","_id":"18522","quality_controlled":"1","article_number":"9257","date_created":"2024-11-10T23:01:58Z","researchdata_availability":"yes","intvolume":" 15","language":[{"iso":"eng"}],"oa_version":"Published Version","status":"public","citation":{"short":"Y. Weyer, S.I. Schwabl, X. Tang, A. Purwar, K. Siegmann, A. Ruepp, T. Dunzendorfer-Matt, M.A. Widerin, V. Niedrist, N.J.M. Mutsters, M.G. Tettamanti, S. Weys, B. Sarg, L. Kremser, K.R. Liedl, O. Schmidt, D. Teis, Nature Communications 15 (2024).","chicago":"Weyer, Yannick, Sinead I. Schwabl, Xuechen Tang, Astha Purwar, Konstantin Siegmann, Angela Ruepp, Theresia Dunzendorfer-Matt, et al. “The Dsc Ubiquitin Ligase Complex Identifies Transmembrane Degrons to Degrade Orphaned Proteins at the Golgi.” Nature Communications. Springer Nature, 2024. https://doi.org/10.1038/s41467-024-53676-6.","apa":"Weyer, Y., Schwabl, S. I., Tang, X., Purwar, A., Siegmann, K., Ruepp, A., … Teis, D. (2024). The Dsc ubiquitin ligase complex identifies transmembrane degrons to degrade orphaned proteins at the Golgi. Nature Communications. Springer Nature. https://doi.org/10.1038/s41467-024-53676-6","ieee":"Y. Weyer et al., “The Dsc ubiquitin ligase complex identifies transmembrane degrons to degrade orphaned proteins at the Golgi,” Nature Communications, vol. 15. Springer Nature, 2024.","mla":"Weyer, Yannick, et al. “The Dsc Ubiquitin Ligase Complex Identifies Transmembrane Degrons to Degrade Orphaned Proteins at the Golgi.” Nature Communications, vol. 15, 9257, Springer Nature, 2024, doi:10.1038/s41467-024-53676-6.","ama":"Weyer Y, Schwabl SI, Tang X, et al. The Dsc ubiquitin ligase complex identifies transmembrane degrons to degrade orphaned proteins at the Golgi. Nature Communications. 2024;15. doi:10.1038/s41467-024-53676-6","ista":"Weyer Y, Schwabl SI, Tang X, Purwar A, Siegmann K, Ruepp A, Dunzendorfer-Matt T, Widerin MA, Niedrist V, Mutsters NJM, Tettamanti MG, Weys S, Sarg B, Kremser L, Liedl KR, Schmidt O, Teis D. 2024. The Dsc ubiquitin ligase complex identifies transmembrane degrons to degrade orphaned proteins at the Golgi. Nature Communications. 15, 9257."},"article_type":"original","dataavailabilitystatement":"All relevant data has been included in the paper in the main figures and in supplementary data 1–4, supplementary tables 1 and 2, and figures. The proteomics data have been deposited in PRIDE (accession number: PXD055553). The original trajectories for the MD simulations have been deposited in Zenodo and are available under 10.5281/zenodo.13889274 and 10.5281/zenodo.13889576. All other data that support the findings of this study are available from the corresponding author upon request. Source data are provided with this paper.","type":"journal_article","year":"2024","fulldoi":"https://doi.org/10.1038/s41467-024-53676-6","user_id":"317138e5-6ab7-11ef-aa6d-ffef3953e345","supplementarymaterial":"yes","publisher":"Springer Nature","has_accepted_license":"1","ddc":["570"],"acknowledgement":"We thank Snezhana Oliferenko, Hesso Farhan, Chris Dunworth, and Lukas A Huber for critically reading the manuscript, Ming Li, Peter Espenshade, Sebastien Leon, and Scott Emr for reagents, Bob Kaufmann for help in characterizing the Dsc2 L1 loop mutant. This research was funded in part by the Austrian Science Fund (FWF) (10.55776/P32161, 10.55776/P34907, 10.55776/DOC82 to DT, and 10.55776/P36187 to OS), by a Lipotype lipidomics excellence award (LEA 2019) to OS, by a Luxembourg National Research Fund (FNR): Grant #13571826 to YW, and by European Union’s Horizon 2020 research and innovation program under the Marie Skłodowska-Curie grant agreement No. 847681 (to KRL). For open access purposes, the author has applied a CC BY public copyright license to any author accepted manuscript version arising from this submission.","volume":15,"day":"01","abstract":[{"text":"The Golgi apparatus is essential for protein sorting, yet its quality control mechanisms are poorly understood. Here we show that the Dsc ubiquitin ligase complex uses its rhomboid pseudo-protease subunit, Dsc2, to assess the hydrophobic length of α-helical transmembrane domains (TMDs) at the Golgi. Thereby the Dsc complex likely interacts with orphaned ER and Golgi proteins that have shorter TMDs and ubiquitinates them for targeted degradation. Some Dsc substrates will be extracted by Cdc48 for endosome and Golgi associated proteasomal degradation (EGAD), while others will undergo ESCRT dependent vacuolar degradation. Some substrates are degraded by both, EGAD- or ESCRT pathways. The accumulation of Dsc substrates entails a specific increase in glycerophospholipids with shorter and asymmetric fatty acyl chains. Hence, the Dsc complex mediates the selective degradation of orphaned proteins at the sorting center of cells, which prevents their spreading across other organelles and thereby preserves cellular membrane protein and lipid composition.","lang":"eng"}],"scopus_import":"1","publication_identifier":{"eissn":["2041-1723"]},"month":"12","related_material":{"record":[{"relation":"research_data","status":"public","id":"23143"},{"id":"23144","relation":"research_data","status":"public"}]},"OA_place":"publisher","external_id":{"pmid":["39461958"],"isi":["001345548100007"]},"publication":"Nature Communications","article_processing_charge":"Yes","oa":1,"DOAJ_listed":"1"},{"publication_identifier":{"issn":["0935-9648"],"eissn":["1521-4095"]},"scopus_import":"1","abstract":[{"text":"Low‐cost, safe, and environmental‐friendly rechargeable aqueous zinc‐ion batteries (ZIBs) are promising as next‐generation energy storage devices for wearable electronics among other applications. However, sluggish ionic transport kinetics and the unstable electrode structure during ionic insertion/extraction hampers their deployment. Herein, we propose a new cathode material based on a layered metal chalcogenide (LMC), bismuth telluride (Bi2Te3), coated with polypyrrole (PPy). Taking advantage of the PPy coating, the Bi2Te3@PPy composite presents strong ionic absorption affinity, high oxidation resistance, and high structural stability. The ZIBs based on Bi2Te3@PPy cathodes exhibit high capacities and ultra‐long lifespans of over 5000 cycles. They also present outstanding stability even under bending. In addition, we analyze here the reaction mechanism using in situ X‐ray diffraction, X‐ray photoelectron spectroscopy, and computational tools and demonstrate that, in the aqueous system, Zn2+ is not inserted into the cathode as previously assumed. In contrast, proton charge storage dominates the process. Overall, this work not only shows the great potential of LMCs as ZIBs cathode materials and the advantages of PPy coating, but also clarifies the charge/discharge mechanism in rechargeable ZIBs based on LMCs.","lang":"eng"}],"day":"04","volume":36,"acknowledgement":"G.Z. and Q.S. contributed equally to this work. This work was supported by the National Natural Science Foundation of China (52105329, 52175300) and the Heilongjiang Provincial Natural Science Foundation of China (LH2022E059). G.Z., X.L., and C.Z. thank the China Scholarship Council (CSC) for the scholarship support. This research was supported by the Scientific Service Units of ISTA through resources provided by the Electron Microscopy Facility. S.H. and M.I. acknowledge funding by ISTA and Werner Siemens.","publisher":"Wiley","article_processing_charge":"No","external_id":{"pmid":["37555532"],"isi":["001085681000001"]},"publication":"Advanced Materials","month":"01","type":"journal_article","acknowledged_ssus":[{"_id":"EM-Fac"}],"dataavailabilitystatement":"The data that support the findings of this study are available from the corresponding author upon reasonable request.","article_type":"original","supplementarymaterial":"yes","issue":"1","user_id":"317138e5-6ab7-11ef-aa6d-ffef3953e345","project":[{"_id":"9B8F7476-BA93-11EA-9121-9846C619BF3A","name":"HighTE: The Werner Siemens Laboratory for the High Throughput Discovery of Semiconductors for Waste Heat Recovery"}],"fulldoi":"https://doi.org/10.1002/adma.202305128","year":"2024","intvolume":" 36","researchdata_availability":"upon request","date_created":"2023-10-17T10:53:56Z","quality_controlled":"1","article_number":"2305128","date_updated":"2026-10-16T09:17:57Z","_id":"14435","department":[{"_id":"MaIb"}],"citation":{"apa":"Zeng, G., Sun, Q., Horta, S., Wang, S., Lu, X., Zhang, C., … Cabot, A. (2024). A layered Bi2Te3@PPy cathode for aqueous zinc ion batteries: Mechanism and application in printed flexible batteries. Advanced Materials. Wiley. https://doi.org/10.1002/adma.202305128","chicago":"Zeng, Guifang, Qing Sun, Sharona Horta, Shang Wang, Xuan Lu, Chaoyue Zhang, Jing Li, et al. “A Layered Bi2Te3@PPy Cathode for Aqueous Zinc Ion Batteries: Mechanism and Application in Printed Flexible Batteries.” Advanced Materials. Wiley, 2024. https://doi.org/10.1002/adma.202305128.","short":"G. Zeng, Q. Sun, S. Horta, S. Wang, X. Lu, C. Zhang, J. Li, J. Li, L. Ci, Y. Tian, M. Ibáñez, A. Cabot, Advanced Materials 36 (2024).","ama":"Zeng G, Sun Q, Horta S, et al. A layered Bi2Te3@PPy cathode for aqueous zinc ion batteries: Mechanism and application in printed flexible batteries. Advanced Materials. 2024;36(1). doi:10.1002/adma.202305128","ista":"Zeng G, Sun Q, Horta S, Wang S, Lu X, Zhang C, Li J, Li J, Ci L, Tian Y, Ibáñez M, Cabot A. 2024. A layered Bi2Te3@PPy cathode for aqueous zinc ion batteries: Mechanism and application in printed flexible batteries. Advanced Materials. 36(1), 2305128.","mla":"Zeng, Guifang, et al. “A Layered Bi2Te3@PPy Cathode for Aqueous Zinc Ion Batteries: Mechanism and Application in Printed Flexible Batteries.” Advanced Materials, vol. 36, no. 1, 2305128, Wiley, 2024, doi:10.1002/adma.202305128.","ieee":"G. Zeng et al., “A layered Bi2Te3@PPy cathode for aqueous zinc ion batteries: Mechanism and application in printed flexible batteries,” Advanced Materials, vol. 36, no. 1. Wiley, 2024."},"status":"public","oa_version":"None","language":[{"iso":"eng"}],"isi":1,"das_tickbox":"1","title":"A layered Bi2Te3@PPy cathode for aqueous zinc ion batteries: Mechanism and application in printed flexible batteries","doi":"10.1002/adma.202305128","publication_status":"published","date_published":"2024-01-04T00:00:00Z","author":[{"first_name":"Guifang","last_name":"Zeng","full_name":"Zeng, Guifang"},{"full_name":"Sun, Qing","last_name":"Sun","first_name":"Qing"},{"full_name":"Horta, Sharona","first_name":"Sharona","last_name":"Horta","id":"03a7e858-01b1-11ec-8b71-99ae6c4a05bc"},{"full_name":"Wang, Shang","last_name":"Wang","first_name":"Shang"},{"full_name":"Lu, Xuan","first_name":"Xuan","last_name":"Lu"},{"full_name":"Zhang, Chaoyue","first_name":"Chaoyue","last_name":"Zhang"},{"first_name":"Jing","last_name":"Li","full_name":"Li, Jing"},{"full_name":"Li, Junshan","last_name":"Li","first_name":"Junshan"},{"last_name":"Ci","first_name":"Lijie","full_name":"Ci, Lijie"},{"first_name":"Yanhong","last_name":"Tian","full_name":"Tian, Yanhong"},{"last_name":"Ibáñez","orcid":"0000-0001-5013-2843","id":"43C61214-F248-11E8-B48F-1D18A9856A87","first_name":"Maria","full_name":"Ibáñez, Maria"},{"first_name":"Andreu","last_name":"Cabot","full_name":"Cabot, Andreu"}],"pmid":1,"keyword":["Mechanical Engineering","Mechanics of Materials","General Materials Science"]},{"doi":"10.1021/acsaem.3c02519","isi":1,"das_tickbox":"0","title":"Interface engineering modulation combined with electronic structure modification of Zn-doped NiO heterostructure for efficient water-splitting activity","page":"214-229","publication_status":"published","author":[{"full_name":"Kiran, Gundegowda Kalligowdanadoddi","last_name":"Kiran","first_name":"Gundegowda Kalligowdanadoddi"},{"full_name":"Singh, Saurabh","first_name":"Saurabh","id":"12d625da-9cb3-11ed-9667-af09d37d3f0a","orcid":"0000-0003-2209-5269","last_name":"Singh"},{"full_name":"Mahato, Neelima","first_name":"Neelima","last_name":"Mahato"},{"first_name":"Thupakula Venkata Madhukar","last_name":"Sreekanth","full_name":"Sreekanth, Thupakula Venkata Madhukar"},{"first_name":"Gowra Raghupathy","last_name":"Dillip","full_name":"Dillip, Gowra Raghupathy"},{"full_name":"Yoo, Kisoo","first_name":"Kisoo","last_name":"Yoo"},{"full_name":"Kim, Jonghoon","first_name":"Jonghoon","last_name":"Kim"}],"date_published":"2024-01-08T00:00:00Z","keyword":["Electrical and Electronic Engineering","Materials Chemistry","Electrochemistry","Energy Engineering and Power Technology","Chemical Engineering (miscellaneous)"],"researchdata_availability":"no","date_created":"2024-01-17T12:48:35Z","intvolume":" 7","_id":"14828","date_updated":"2026-10-16T09:20:00Z","quality_controlled":"1","citation":{"short":"G.K. Kiran, S. Singh, N. Mahato, T.V.M. Sreekanth, G.R. Dillip, K. Yoo, J. Kim, ACS Applied Energy Materials 7 (2024) 214–229.","chicago":"Kiran, Gundegowda Kalligowdanadoddi, Saurabh Singh, Neelima Mahato, Thupakula Venkata Madhukar Sreekanth, Gowra Raghupathy Dillip, Kisoo Yoo, and Jonghoon Kim. “Interface Engineering Modulation Combined with Electronic Structure Modification of Zn-Doped NiO Heterostructure for Efficient Water-Splitting Activity.” ACS Applied Energy Materials. American Chemical Society, 2024. https://doi.org/10.1021/acsaem.3c02519.","apa":"Kiran, G. K., Singh, S., Mahato, N., Sreekanth, T. V. M., Dillip, G. R., Yoo, K., & Kim, J. (2024). Interface engineering modulation combined with electronic structure modification of Zn-doped NiO heterostructure for efficient water-splitting activity. ACS Applied Energy Materials. American Chemical Society. https://doi.org/10.1021/acsaem.3c02519","ieee":"G. K. Kiran et al., “Interface engineering modulation combined with electronic structure modification of Zn-doped NiO heterostructure for efficient water-splitting activity,” ACS Applied Energy Materials, vol. 7, no. 1. American Chemical Society, pp. 214–229, 2024.","mla":"Kiran, Gundegowda Kalligowdanadoddi, et al. “Interface Engineering Modulation Combined with Electronic Structure Modification of Zn-Doped NiO Heterostructure for Efficient Water-Splitting Activity.” ACS Applied Energy Materials, vol. 7, no. 1, American Chemical Society, 2024, pp. 214–29, doi:10.1021/acsaem.3c02519.","ista":"Kiran GK, Singh S, Mahato N, Sreekanth TVM, Dillip GR, Yoo K, Kim J. 2024. Interface engineering modulation combined with electronic structure modification of Zn-doped NiO heterostructure for efficient water-splitting activity. ACS Applied Energy Materials. 7(1), 214–229.","ama":"Kiran GK, Singh S, Mahato N, et al. Interface engineering modulation combined with electronic structure modification of Zn-doped NiO heterostructure for efficient water-splitting activity. ACS Applied Energy Materials. 2024;7(1):214-229. doi:10.1021/acsaem.3c02519"},"department":[{"_id":"MaIb"}],"status":"public","oa_version":"None","language":[{"iso":"eng"}],"type":"journal_article","article_type":"original","user_id":"317138e5-6ab7-11ef-aa6d-ffef3953e345","issue":"1","supplementarymaterial":"yes","year":"2024","fulldoi":"https://doi.org/10.1021/acsaem.3c02519","abstract":[{"text":"Production of hydrogen at large scale requires development of non-noble, inexpensive, and high-performing catalysts for constructing water-splitting devices. Herein, we report the synthesis of Zn-doped NiO heterostructure (ZnNiO) catalysts at room temperature via a coprecipitation method followed by drying (at 80 °C, 6 h) and calcination at an elevated temperature of 400 °C for 5 h under three distinct conditions, namely, air, N2, and vacuum. The vacuum-synthesized catalyst demonstrates a low overpotential of 88 mV at −10 mA cm–2 and a small Tafel slope of 73 mV dec–1 suggesting relatively higher charge transfer kinetics for hydrogen evolution reactions (HER) compared with the specimens synthesized under N2 or O2 atmosphere. It also demonstrates an oxygen evolution (OER) overpotential of 260 mV at 10 mA cm–2 with a low Tafel slope of 63 mV dec–1. In a full-cell water-splitting device, the vacuum-synthesized ZnNiO heterostructure demonstrates a cell voltage of 1.94 V at 50 mA cm–2 and shows remarkable stability over 24 h at a high current density of 100 mA cm–2. It is also demonstrated in this study that Zn-doping, surface, and interface engineering in transition-metal oxides play a crucial role in efficient electrocatalytic water splitting. Also, the results obtained from density functional theory (DFT + U = 0–8 eV), where U is the on-site Coulomb repulsion parameter also known as Hubbard U, based electronic structure calculations confirm that Zn doping constructively modifies the electronic structure, in both the valence band and the conduction band, and found to be suitable in tailoring the carrier’s effective masses of electrons and holes. The decrease in electron’s effective masses together with large differences between the effective masses of electrons and holes is noticed, which is found to be mainly responsible for achieving the best water-splitting performance from a 9% Zn-doped NiO sample prepared under vacuum.","lang":"eng"}],"scopus_import":"1","publication_identifier":{"issn":["2574-0962"]},"volume":7,"day":"08","acknowledgement":"This work was supported by the Technology Innovation Program (20011622, Development of Battery System Applied High-Efficiency Heat Control Polymer and Part Component) funded by the Ministry of Trade, Industry & Energy (MOTIE, Korea). Author acknowledge to Prof. Tsunehiro Takeuchi from Toyota Technological Institute, Nagoya, Japan for the support of computational resources.","publisher":"American Chemical Society","corr_author":"1","article_processing_charge":"No","external_id":{"isi":["001138342900001"]},"publication":"ACS Applied Energy Materials","month":"01"},{"doi":"10.1016/j.ces.2024.119959","das_tickbox":"1","title":"Unravelling the reaction mechanism for H2 production via formic acid decomposition over Pd: Coverage-dependent microkinetic modeling","isi":1,"author":[{"last_name":"Yao","first_name":"Zihao","full_name":"Yao, Zihao"},{"full_name":"Liu, Xu","last_name":"Liu","first_name":"Xu"},{"id":"91deeae8-1207-11ec-b130-c194ad5b50c6","orcid":"0000-0001-6928-074X","last_name":"Bunting","first_name":"Rhys","full_name":"Bunting, Rhys"},{"first_name":"Jianguo","last_name":"Wang","full_name":"Wang, Jianguo"}],"publication_status":"published","date_published":"2024-06-05T00:00:00Z","OA_type":"free access","date_updated":"2026-10-16T09:20:35Z","_id":"15114","article_number":"119959","quality_controlled":"1","researchdata_availability":"upon request","date_created":"2024-03-17T23:00:57Z","intvolume":" 291","status":"public","citation":{"mla":"Yao, Zihao, et al. “Unravelling the Reaction Mechanism for H2 Production via Formic Acid Decomposition over Pd: Coverage-Dependent Microkinetic Modeling.” Chemical Engineering Science, vol. 291, 119959, Elsevier, 2024, doi:10.1016/j.ces.2024.119959.","ista":"Yao Z, Liu X, Bunting R, Wang J. 2024. Unravelling the reaction mechanism for H2 production via formic acid decomposition over Pd: Coverage-dependent microkinetic modeling. Chemical Engineering Science. 291, 119959.","ama":"Yao Z, Liu X, Bunting R, Wang J. Unravelling the reaction mechanism for H2 production via formic acid decomposition over Pd: Coverage-dependent microkinetic modeling. Chemical Engineering Science. 2024;291. doi:10.1016/j.ces.2024.119959","ieee":"Z. Yao, X. Liu, R. Bunting, and J. Wang, “Unravelling the reaction mechanism for H2 production via formic acid decomposition over Pd: Coverage-dependent microkinetic modeling,” Chemical Engineering Science, vol. 291. Elsevier, 2024.","chicago":"Yao, Zihao, Xu Liu, Rhys Bunting, and Jianguo Wang. “Unravelling the Reaction Mechanism for H2 Production via Formic Acid Decomposition over Pd: Coverage-Dependent Microkinetic Modeling.” Chemical Engineering Science. Elsevier, 2024. https://doi.org/10.1016/j.ces.2024.119959.","apa":"Yao, Z., Liu, X., Bunting, R., & Wang, J. (2024). Unravelling the reaction mechanism for H2 production via formic acid decomposition over Pd: Coverage-dependent microkinetic modeling. Chemical Engineering Science. Elsevier. https://doi.org/10.1016/j.ces.2024.119959","short":"Z. Yao, X. Liu, R. Bunting, J. Wang, Chemical Engineering Science 291 (2024)."},"department":[{"_id":"MaIb"}],"main_file_link":[{"url":"https://doi.org/10.1016/j.ces.2024.119959","open_access":"1"}],"language":[{"iso":"eng"}],"oa_version":"None","type":"journal_article","article_type":"original","dataavailabilitystatement":"Data will be made available on request.","user_id":"317138e5-6ab7-11ef-aa6d-ffef3953e345","supplementarymaterial":"yes","year":"2024","fulldoi":"https://doi.org/10.1016/j.ces.2024.119959","volume":291,"day":"05","abstract":[{"lang":"eng","text":"As a key liquid organic hydrogen carrier, investigating the decomposition of formic acid (HCOOH) on the Pd (1 1 1) transition metal surface is imperative for harnessing hydrogen energy. Despite a multitude of studies, the major mechanisms and key intermediates involved in the dehydrogenation process of formic acid remain a great topic of debate due to ambiguous adsorbate interactions. In this research, we develop an advanced microkinetic model based on first-principles calculations, accounting for adsorbate–adsorbate interactions. Our study unveils a comprehensive mechanism for the Pd (1 1 1) surface, highlighting the significance of coverage effects in formic acid dehydrogenation. Our findings unequivocally demonstrate that H coverage on the Pd (1 1 1) surface renders formic acid more susceptible to decompose into H2 and CO2 through COOH intermediates. Consistent with experimental results, the selectivity of H2 in the decomposition of formic acid on the Pd (1 1 1) surface approaches 100 %. Considering the influence of H coverage, our kinetic analysis aligns perfectly with experimental values at a temperature of 373 K."}],"scopus_import":"1","publication_identifier":{"issn":["0009-2509"]},"publisher":"Elsevier","acknowledgement":"The authors acknowledge the financial support from the National Key Research and Development Project of China (2021YFA1500900, 2022YFE0113800), the National Natural Science Foundation of China (22141001, U21A20298), Zhejiang Innovation Team (2017R5203).","external_id":{"isi":["001203872000001"]},"publication":"Chemical Engineering Science","article_processing_charge":"No","oa":1,"month":"06"},{"month":"02","article_processing_charge":"No","publication":"Physica B: Condensed Matter","external_id":{"isi":["001127429000001"]},"publisher":"Elsevier","abstract":[{"text":"In order to demonstrate the stability of newly proposed iridium-based Ir2Cr(In,Sn) and IrRhCr(In,Sn) heusler alloys, we present ab-initio analysis of these alloys by examining various properties to prove their stability. The stability of these alloys can be inferred from different cohesive and formation energies as well as positive phonon frequencies. Their electronic structure results indicate that they are semi-metals in nature. The magnetic moments are computed using the Slater-Pauling formula and exhibit a high value, with the Cr atom contributing the most in all alloys. Mulliken’s charge analysis results show that our alloys contain a range of linkages, mainly ionic and covalent ones. The ductility and mechanical stability of these alloys are confirmed by elastic constants viz. Poisson’s ratio, Pugh’s ratio, and many different types of elastic moduli.","lang":"eng"}],"scopus_import":"1","publication_identifier":{"issn":["0921-4526"]},"volume":674,"day":"01","year":"2024","fulldoi":"https://doi.org/10.1016/j.physb.2023.415539","issue":"2","user_id":"317138e5-6ab7-11ef-aa6d-ffef3953e345","supplementarymaterial":"no","dataavailabilitystatement":"No data was used for the research described in the article.","article_type":"original","type":"journal_article","oa_version":"None","language":[{"iso":"eng"}],"citation":{"ieee":"S. L. Gupta et al., “Ab-initio stability of Iridium based newly proposed full and quaternary heusler alloys,” Physica B: Condensed Matter, vol. 674, no. 2. Elsevier, 2024.","mla":"Gupta, Shyam Lal, et al. “Ab-Initio Stability of Iridium Based Newly Proposed Full and Quaternary Heusler Alloys.” Physica B: Condensed Matter, vol. 674, no. 2, 415539, Elsevier, 2024, doi:10.1016/j.physb.2023.415539.","ama":"Gupta SL, Singh S, Kumar S, et al. Ab-initio stability of Iridium based newly proposed full and quaternary heusler alloys. Physica B: Condensed Matter. 2024;674(2). doi:10.1016/j.physb.2023.415539","ista":"Gupta SL, Singh S, Kumar S, Anupam U, Thakur SS, Kumar A, Panwar S, Diwaker D. 2024. Ab-initio stability of Iridium based newly proposed full and quaternary heusler alloys. Physica B: Condensed Matter. 674(2), 415539.","short":"S.L. Gupta, S. Singh, S. Kumar, U. Anupam, S.S. Thakur, A. Kumar, S. Panwar, D. Diwaker, Physica B: Condensed Matter 674 (2024).","apa":"Gupta, S. L., Singh, S., Kumar, S., Anupam, U., Thakur, S. S., Kumar, A., … Diwaker, D. (2024). Ab-initio stability of Iridium based newly proposed full and quaternary heusler alloys. Physica B: Condensed Matter. Elsevier. https://doi.org/10.1016/j.physb.2023.415539","chicago":"Gupta, Shyam Lal, Saurabh Singh, Sumit Kumar, Unknown Anupam, Samjeet Singh Thakur, Ashish Kumar, Sanjay Panwar, and D. Diwaker. “Ab-Initio Stability of Iridium Based Newly Proposed Full and Quaternary Heusler Alloys.” Physica B: Condensed Matter. Elsevier, 2024. https://doi.org/10.1016/j.physb.2023.415539."},"department":[{"_id":"MaIb"}],"status":"public","date_created":"2023-12-10T23:00:56Z","researchdata_availability":"not applicable","intvolume":" 674","date_updated":"2026-10-16T09:19:32Z","_id":"14652","article_number":"415539","quality_controlled":"1","publication_status":"published","author":[{"first_name":"Shyam Lal","last_name":"Gupta","full_name":"Gupta, Shyam Lal"},{"full_name":"Singh, Saurabh","id":"12d625da-9cb3-11ed-9667-af09d37d3f0a","last_name":"Singh","orcid":"0000-0003-2209-5269","first_name":"Saurabh"},{"first_name":"Sumit","last_name":"Kumar","full_name":"Kumar, Sumit"},{"full_name":"Anupam, Unknown","first_name":"Unknown","last_name":"Anupam"},{"last_name":"Thakur","first_name":"Samjeet Singh","full_name":"Thakur, Samjeet Singh"},{"full_name":"Kumar, Ashish","last_name":"Kumar","first_name":"Ashish"},{"first_name":"Sanjay","last_name":"Panwar","full_name":"Panwar, Sanjay"},{"first_name":"D.","last_name":"Diwaker","full_name":"Diwaker, D."}],"date_published":"2024-02-01T00:00:00Z","doi":"10.1016/j.physb.2023.415539","das_tickbox":"1","title":"Ab-initio stability of Iridium based newly proposed full and quaternary heusler alloys","isi":1},{"publisher":"Zenodo","ddc":["570"],"day":"04","date_updated":"2026-10-16T09:15:19Z","_id":"23144","abstract":[{"lang":"eng","text":"The attached trajectories illustrate the preference for the association of saturated asymmetric lipids over unsaturated ones with DSC2. In order to comply with the size limit, the initial conformations as well as one illustrative example of the final productive simulation with complete number of frames and all others sliced by 100 frames of each simulated system are provided herewith. Two illustrative example trajectories in the equilibrated but not yet converged phases are attached in additon, to demonstrate the dynamic rearrangement of asymmetric lipids before the stable states. The first example is that of the saturated asymmetric lipid, which is used to illustrate the association of the trucated saturated chain with the DSC2. The second example depicts the dissociation of an analogous unsaturated chain from the DSC2. The initial conformations are provided in PDB format, while the final productive simulations are uploaded in NetCDF (AMBER) format. "}],"date_created":"2026-10-16T09:14:55Z","related_material":{"record":[{"relation":"used_in_publication","status":"public","id":"18522"}]},"month":"10","oa_version":"None","OA_place":"repository","status":"public","oa":1,"main_file_link":[{"open_access":"1","url":"https://doi.org/10.5281/zenodo.13889575"}],"citation":{"ieee":"X. Tang, “The interaction between the DSC2 and the asymmetric lipids.” Zenodo, 2024.","ista":"Tang X. 2024. The interaction between the DSC2 and the asymmetric lipids, Zenodo, 10.5281/zenodo.13889575.","ama":"Tang X. The interaction between the DSC2 and the asymmetric lipids. 2024. doi:10.5281/zenodo.13889575","mla":"Tang, Xuechen. The Interaction between the DSC2 and the Asymmetric Lipids. Zenodo, 2024, doi:10.5281/zenodo.13889575.","short":"X. Tang, (2024).","chicago":"Tang, Xuechen. “The Interaction between the DSC2 and the Asymmetric Lipids.” Zenodo, 2024. https://doi.org/10.5281/zenodo.13889575.","apa":"Tang, X. (2024). The interaction between the DSC2 and the asymmetric lipids. Zenodo. https://doi.org/10.5281/zenodo.13889575"},"article_processing_charge":"No","author":[{"full_name":"Tang, Xuechen","first_name":"Xuechen","last_name":"Tang"}],"date_published":"2024-10-04T00:00:00Z","type":"research_data_reference","title":"The interaction between the DSC2 and the asymmetric lipids","doi":"10.5281/zenodo.13889575","OA_type":"green","fulldoi":"https://doi.org/10.5281/zenodo.13889575","year":"2024","user_id":"317138e5-6ab7-11ef-aa6d-ffef3953e345"},{"article_type":"original","acknowledged_ssus":[{"_id":"EM-Fac"},{"_id":"NMR"},{"_id":"LifeSc"}],"dataavailabilitystatement":"The data that support the findings of this study are available from the corresponding author upon reasonable request.","type":"journal_article","year":"2024","project":[{"grant_number":"754411","_id":"260C2330-B435-11E9-9278-68D0E5697425","call_identifier":"H2020","name":"ISTplus - Postdoctoral Fellowships"},{"grant_number":"665385","_id":"2564DBCA-B435-11E9-9278-68D0E5697425","call_identifier":"H2020","name":"International IST Doctoral Program"},{"_id":"9B8F7476-BA93-11EA-9121-9846C619BF3A","name":"HighTE: The Werner Siemens Laboratory for the High Throughput Discovery of Semiconductors for Waste Heat Recovery"}],"fulldoi":"https://doi.org/10.1002/anie.202402628","issue":"25","user_id":"317138e5-6ab7-11ef-aa6d-ffef3953e345","supplementarymaterial":"yes","license":"https://creativecommons.org/licenses/by-nc-nd/4.0/","publisher":"Wiley","corr_author":"1","has_accepted_license":"1","ddc":["540"],"acknowledgement":"ISTA and the Werner Siemens Foundation financially supported this work. The Scientific Service Units (SSU) of ISTA supported this research through resources provided by the Electron Microscopy Facility (EMF), NMR Facility and the Lab Support Facility (LSF). Dr. Krishnendu Maji at ISTA aided in this work through XRD analysis of the crystal phase of SnSe. Y.L. acknowledges funding from the European Union's Horizon 2020 research and innovation program under the Marie Sklodowska-Curie grant agreement No. 754411, the National Natural Science Foundation of China (NSFC) (Grants No. 22209034). M.C. received funding from the European Union's Horizon 2020 research and innovation program under the Marie Skłodowska-Curie Grant Agreement No. 665385.","volume":63,"day":"17","scopus_import":"1","abstract":[{"text":"Production of thermoelectric materials from solution-processed particles involves the synthesis of particles, their purification and densification into pelletized material. Chemical changes that occur during each one of these steps render them performance determining. Particularly the purification steps, bypassed in conventional solid-state synthesis, are the cause for large discrepancies among similar solution-processed materials. In present work, the investigation focuses on a water-based surfactant free solution synthesis of SnSe, a highly relevant thermoelectric material. We show and rationalize that the number of leaching steps, purification solvent, annealing, and annealing atmosphere have significant influence on the Sn : Se ratio and impurity content in the powder. Such compositional changes that are undetectable by conventional characterization techniques lead to distinct consolidated materials with different types and concentration of defects. Additionally, the profound effect on their transport properties is demonstrated. We emphasize that understanding the chemistry and identifying key chemical species and their role throughout the process is paramount for optimizing material performance. Furthermore, we aim to demonstrate the necessity of comprehensive reporting of these steps as a standard practice to ensure material reproducibility.","lang":"eng"}],"publication_identifier":{"eissn":["1521-3773"],"issn":["1433-7851"]},"month":"06","related_material":{"record":[{"relation":"dissertation_contains","status":"public","id":"22626"}]},"publication":"Angewandte Chemie International Edition","external_id":{"pmid":["38623865"],"isi":["001223768400001"]},"OA_place":"publisher","article_processing_charge":"Yes (via OA deal)","oa":1,"pmid":1,"file":[{"content_type":"application/pdf","file_size":16347226,"date_updated":"2025-01-09T09:12:07Z","checksum":"1572a0f4d2df55751761efeb2d11c7fc","relation":"main_file","date_created":"2025-01-09T09:12:07Z","success":1,"creator":"dernst","file_name":"2024_AngewChemieIntern_Fiedler.pdf","access_level":"open_access","file_id":"18797"}],"author":[{"full_name":"Fiedler, Christine","first_name":"Christine","id":"bd3fceba-dc74-11ea-a0a7-c17f71817366","last_name":"Fiedler"},{"first_name":"Mariano","id":"45D7531A-F248-11E8-B48F-1D18A9856A87","last_name":"Calcabrini","orcid":"0000-0003-4566-5877","full_name":"Calcabrini, Mariano"},{"first_name":"Yu","id":"2A70014E-F248-11E8-B48F-1D18A9856A87","last_name":"Liu","orcid":"0000-0001-7313-6740","full_name":"Liu, Yu"},{"first_name":"Maria","id":"43C61214-F248-11E8-B48F-1D18A9856A87","last_name":"Ibáñez","orcid":"0000-0001-5013-2843","full_name":"Ibáñez, Maria"}],"date_published":"2024-06-17T00:00:00Z","publication_status":"published","doi":"10.1002/anie.202402628","title":"Unveiling crucial chemical processing parameters influencing the performance of solution-processed inorganic thermoelectric materials","file_date_updated":"2025-01-09T09:12:07Z","isi":1,"das_tickbox":"1","OA_type":"hybrid","tmp":{"legal_code_url":"https://creativecommons.org/licenses/by-nc-nd/4.0/legalcode","image":"/images/cc_by_nc_nd.png","name":"Creative Commons Attribution-NonCommercial-NoDerivatives 4.0 International (CC BY-NC-ND 4.0)","short":"CC BY-NC-ND (4.0)"},"_id":"17052","date_updated":"2026-10-16T09:30:27Z","article_number":"e202402628","quality_controlled":"1","date_created":"2024-05-26T22:00:58Z","researchdata_availability":"upon request","intvolume":" 63","language":[{"iso":"eng"}],"oa_version":"Published Version","ec_funded":1,"status":"public","citation":{"short":"C. Fiedler, M. Calcabrini, Y. Liu, M. Ibáñez, Angewandte Chemie International Edition 63 (2024).","chicago":"Fiedler, Christine, Mariano Calcabrini, Yu Liu, and Maria Ibáñez. “Unveiling Crucial Chemical Processing Parameters Influencing the Performance of Solution-Processed Inorganic Thermoelectric Materials.” Angewandte Chemie International Edition. Wiley, 2024. https://doi.org/10.1002/anie.202402628.","apa":"Fiedler, C., Calcabrini, M., Liu, Y., & Ibáñez, M. (2024). Unveiling crucial chemical processing parameters influencing the performance of solution-processed inorganic thermoelectric materials. Angewandte Chemie International Edition. Wiley. https://doi.org/10.1002/anie.202402628","ieee":"C. Fiedler, M. Calcabrini, Y. Liu, and M. Ibáñez, “Unveiling crucial chemical processing parameters influencing the performance of solution-processed inorganic thermoelectric materials,” Angewandte Chemie International Edition, vol. 63, no. 25. Wiley, 2024.","mla":"Fiedler, Christine, et al. “Unveiling Crucial Chemical Processing Parameters Influencing the Performance of Solution-Processed Inorganic Thermoelectric Materials.” Angewandte Chemie International Edition, vol. 63, no. 25, e202402628, Wiley, 2024, doi:10.1002/anie.202402628.","ista":"Fiedler C, Calcabrini M, Liu Y, Ibáñez M. 2024. Unveiling crucial chemical processing parameters influencing the performance of solution-processed inorganic thermoelectric materials. Angewandte Chemie International Edition. 63(25), e202402628.","ama":"Fiedler C, Calcabrini M, Liu Y, Ibáñez M. Unveiling crucial chemical processing parameters influencing the performance of solution-processed inorganic thermoelectric materials. Angewandte Chemie International Edition. 2024;63(25). doi:10.1002/anie.202402628"},"department":[{"_id":"MaIb"}]},{"article_processing_charge":"No","external_id":{"pmid":["38152986"],"isi":["001133369800001"]},"publication":"Small Methods","month":"08","abstract":[{"text":"Developing cost-effective and high-performance thermoelectric (TE) materials to assemble efficient TE devices presents a multitude of challenges and opportunities. Cu3SbSe4 is a promising p-type TE material based on relatively earth abundant elements. However, the challenge lies in its poor electrical conductivity. Herein, an efficient and scalable solution-based approach is developed to synthesize high-quality Cu3SbSe4 nanocrystals doped with Pb at the Sb site. After ligand displacement and annealing treatments, the dried powders are consolidated into dense pellets, and their TE properties are investigated. Pb doping effectively increases the charge carrier concentration, resulting in a significant increase in electrical conductivity, while the Seebeck coefficients remain consistently high. The calculated band structure shows that Pb doping induces band convergence, thereby increasing the effective mass. Furthermore, the large ionic radius of Pb2+ results in the generation of additional point and plane defects and interphases, dramatically enhancing phonon scattering, which significantly decreases the lattice thermal conductivity at high temperatures. Overall, a maximum figure of merit (zTmax) ≈ 0.85 at 653 K is obtained in Cu3Sb0.97Pb0.03Se4. This represents a 1.6-fold increase compared to the undoped sample and exceeds most doped Cu3SbSe4-based materials produced by solid-state, demonstrating advantages of versatility and cost-effectiveness using a solution-based technology.","lang":"eng"}],"scopus_import":"1","publication_identifier":{"eissn":["2366-9608"]},"volume":8,"day":"01","acknowledgement":"Y.L. acknowledges funding from the National Natural Science Foundation of China (NSFC) (Grants No. 22209034), the Innovation and Entrepreneurship Project of Overseas Returnees in Anhui Province (Grant No. 2022LCX002). K.H.L. acknowledges financial support from the National Natural Science Foundation of China (NSFC) (Grant No. 22208293). M.I. acknowledges financial support from ISTA and the Werner Siemens Foundation.","publisher":"Wiley","issue":"8","user_id":"317138e5-6ab7-11ef-aa6d-ffef3953e345","supplementarymaterial":"yes","year":"2024","fulldoi":"https://doi.org/10.1002/smtd.202301377","project":[{"name":"HighTE: The Werner Siemens Laboratory for the High Throughput Discovery of Semiconductors for Waste Heat Recovery","_id":"9B8F7476-BA93-11EA-9121-9846C619BF3A"}],"type":"journal_article","dataavailabilitystatement":"The data that support the findings of this study are available in the supplementary material of this article. Support","article_type":"original","citation":{"short":"S. Wan, S. Xiao, M. Li, X. Wang, K.H. Lim, M. Hong, M. Ibáñez, A. Cabot, Y. Liu, Small Methods 8 (2024).","apa":"Wan, S., Xiao, S., Li, M., Wang, X., Lim, K. H., Hong, M., … Liu, Y. (2024). Band engineering through Pb-doping of nanocrystal building blocks to enhance thermoelectric performance in Cu3SbSe4. Small Methods. Wiley. https://doi.org/10.1002/smtd.202301377","chicago":"Wan, Shanhong, Shanshan Xiao, Mingquan Li, Xin Wang, Khak Ho Lim, Min Hong, Maria Ibáñez, Andreu Cabot, and Yu Liu. “Band Engineering through Pb-Doping of Nanocrystal Building Blocks to Enhance Thermoelectric Performance in Cu3SbSe4.” Small Methods. Wiley, 2024. https://doi.org/10.1002/smtd.202301377.","ieee":"S. Wan et al., “Band engineering through Pb-doping of nanocrystal building blocks to enhance thermoelectric performance in Cu3SbSe4,” Small Methods, vol. 8, no. 8. Wiley, 2024.","mla":"Wan, Shanhong, et al. “Band Engineering through Pb-Doping of Nanocrystal Building Blocks to Enhance Thermoelectric Performance in Cu3SbSe4.” Small Methods, vol. 8, no. 8, 2301377, Wiley, 2024, doi:10.1002/smtd.202301377.","ama":"Wan S, Xiao S, Li M, et al. Band engineering through Pb-doping of nanocrystal building blocks to enhance thermoelectric performance in Cu3SbSe4. Small Methods. 2024;8(8). doi:10.1002/smtd.202301377","ista":"Wan S, Xiao S, Li M, Wang X, Lim KH, Hong M, Ibáñez M, Cabot A, Liu Y. 2024. Band engineering through Pb-doping of nanocrystal building blocks to enhance thermoelectric performance in Cu3SbSe4. Small Methods. 8(8), 2301377."},"department":[{"_id":"MaIb"}],"status":"public","oa_version":"None","language":[{"iso":"eng"}],"date_created":"2024-01-07T23:00:51Z","researchdata_availability":"yes (supplementary data)","intvolume":" 8","date_updated":"2026-10-16T09:29:55Z","_id":"14734","quality_controlled":"1","article_number":"2301377","OA_type":"closed access","doi":"10.1002/smtd.202301377","title":"Band engineering through Pb-doping of nanocrystal building blocks to enhance thermoelectric performance in Cu3SbSe4","das_tickbox":"1","isi":1,"author":[{"full_name":"Wan, Shanhong","first_name":"Shanhong","last_name":"Wan"},{"full_name":"Xiao, Shanshan","first_name":"Shanshan","last_name":"Xiao"},{"full_name":"Li, Mingquan","first_name":"Mingquan","last_name":"Li"},{"first_name":"Xin","last_name":"Wang","full_name":"Wang, Xin"},{"first_name":"Khak Ho","last_name":"Lim","full_name":"Lim, Khak Ho"},{"full_name":"Hong, Min","last_name":"Hong","first_name":"Min"},{"orcid":"0000-0001-5013-2843","last_name":"Ibáñez","id":"43C61214-F248-11E8-B48F-1D18A9856A87","first_name":"Maria","full_name":"Ibáñez, Maria"},{"last_name":"Cabot","first_name":"Andreu","full_name":"Cabot, Andreu"},{"full_name":"Liu, Yu","last_name":"Liu","orcid":"0000-0001-7313-6740","id":"2A70014E-F248-11E8-B48F-1D18A9856A87","first_name":"Yu"}],"pmid":1,"date_published":"2024-08-01T00:00:00Z","publication_status":"published"},{"article_processing_charge":"No","publication":"Journal of Energy Storage","external_id":{"isi":["001287584100001"]},"month":"05","publication_identifier":{"eissn":["2352-152X"]},"scopus_import":"1","abstract":[{"lang":"eng","text":"Development of electroactive materials exhibiting high performance with superior stability is crucial in the field of supercapacitors and battery research. We report on synthesis of highly stable composite of semi-polycrystalline polyaniline and graphene (SPani-graphene) and its application in supercapacitor electrodes. The electrochemical behavior and device performance of the electrodes were investigated through cyclic voltammetry (CV), galvanostatic charge-discharge GCD) and electrochemical impedance spectroscopy (EIS) in a 3-electrode and a 2-electrode (device) cell configurations, repectively. The cell specific capacitance (Cell Csp) achieved from the 2-electrode symmetric cell configuration was 525.5 F g−1 at 0.1 A g−1 using polymer gel electrolyte (PGE). The PGE in this work is xanthan gum jellied in 1 M aq. Na2SO4. The maximum energy density and power density achieved from the device was 46.7 Wh kg−1 and 16.16 kW kg−1, respectively, at 0.4 A g−1. Furthermore, the device exhibits an excellent retention of cell specific capacitance and coulombic efficiency of 97 % and 94 %, respectively, over 10,000 continuous GCD cycles, indicating an excellent rate capability as well as a promising power management. To investigate the material's electrochemical durability, a detailed EIS study has been carried out using both, 3-electrode, and 2-electrode cell configurations, before and after long cycling test (over 10,000 continuous GCD cycles). Our thorough experimentation delivers satisfactory results and has been explained in detail in the manuscript. Hereby, we propose that the EIS technique can be adopted for investigating materials' electrochemical stability, in addition to long CV and GCD cycles in the field of supercapacitors and battery research."}],"day":"30","volume":88,"acknowledgement":"This work was supported by Korea Institute of Energy Technology Evaluation and Planning (KETEP); and Ministry of Trade, Industry & Energy (MOTIE), Republic of Korea (Grant No. \r\n20210501010020).","publisher":"Elsevier","supplementarymaterial":"yes","user_id":"317138e5-6ab7-11ef-aa6d-ffef3953e345","fulldoi":"https://doi.org/10.1016/j.est.2024.111464","year":"2024","type":"journal_article","dataavailabilitystatement":"Data will be made available on request.","article_type":"original","department":[{"_id":"MaIb"}],"citation":{"ieee":"N. Mahato, S. Singh, T. V. M. Sreekanth, K. Yoo, and J. Kim, “Polycrystalline phases engineered in-situ in polyaniline-graphene composite evoluting an exceptional stability and high charge storage capacity: An EIS investigative approach to evaluate material’s stability,” Journal of Energy Storage, vol. 88. Elsevier, 2024.","mla":"Mahato, Neelima, et al. “Polycrystalline Phases Engineered In-Situ in Polyaniline-Graphene Composite Evoluting an Exceptional Stability and High Charge Storage Capacity: An EIS Investigative Approach to Evaluate Material’s Stability.” Journal of Energy Storage, vol. 88, 111464, Elsevier, 2024, doi:10.1016/j.est.2024.111464.","ama":"Mahato N, Singh S, Sreekanth TVM, Yoo K, Kim J. Polycrystalline phases engineered in-situ in polyaniline-graphene composite evoluting an exceptional stability and high charge storage capacity: An EIS investigative approach to evaluate material’s stability. Journal of Energy Storage. 2024;88. doi:10.1016/j.est.2024.111464","ista":"Mahato N, Singh S, Sreekanth TVM, Yoo K, Kim J. 2024. Polycrystalline phases engineered in-situ in polyaniline-graphene composite evoluting an exceptional stability and high charge storage capacity: An EIS investigative approach to evaluate material’s stability. Journal of Energy Storage. 88, 111464.","short":"N. Mahato, S. Singh, T.V.M. Sreekanth, K. Yoo, J. Kim, Journal of Energy Storage 88 (2024).","apa":"Mahato, N., Singh, S., Sreekanth, T. V. M., Yoo, K., & Kim, J. (2024). Polycrystalline phases engineered in-situ in polyaniline-graphene composite evoluting an exceptional stability and high charge storage capacity: An EIS investigative approach to evaluate material’s stability. Journal of Energy Storage. Elsevier. https://doi.org/10.1016/j.est.2024.111464","chicago":"Mahato, Neelima, Saurabh Singh, T. V.M. Sreekanth, Kisoo Yoo, and Jonghoon Kim. “Polycrystalline Phases Engineered In-Situ in Polyaniline-Graphene Composite Evoluting an Exceptional Stability and High Charge Storage Capacity: An EIS Investigative Approach to Evaluate Material’s Stability.” Journal of Energy Storage. Elsevier, 2024. https://doi.org/10.1016/j.est.2024.111464."},"status":"public","oa_version":"None","language":[{"iso":"eng"}],"intvolume":" 88","date_created":"2024-04-14T22:01:01Z","researchdata_availability":"upon request","quality_controlled":"1","article_number":"111464","date_updated":"2026-10-16T09:21:29Z","_id":"15314","title":"Polycrystalline phases engineered in-situ in polyaniline-graphene composite evoluting an exceptional stability and high charge storage capacity: An EIS investigative approach to evaluate material's stability","isi":1,"das_tickbox":"1","doi":"10.1016/j.est.2024.111464","date_published":"2024-05-30T00:00:00Z","publication_status":"published","author":[{"full_name":"Mahato, Neelima","first_name":"Neelima","last_name":"Mahato"},{"last_name":"Singh","orcid":"0000-0003-2209-5269","id":"12d625da-9cb3-11ed-9667-af09d37d3f0a","first_name":"Saurabh","full_name":"Singh, Saurabh"},{"last_name":"Sreekanth","first_name":"T. V.M.","full_name":"Sreekanth, T. V.M."},{"full_name":"Yoo, Kisoo","first_name":"Kisoo","last_name":"Yoo"},{"last_name":"Kim","first_name":"Jonghoon","full_name":"Kim, Jonghoon"}]},{"volume":383,"day":"14","abstract":[{"lang":"eng","text":"Reducing defects boosts room-temperature performance of a thermoelectric device"}],"scopus_import":"1","publication_identifier":{"issn":["0036-8075"],"eissn":["1095-9203"]},"corr_author":"1","publisher":"American Association for the Advancement of Science","acknowledgement":"The authors thank the Werner-Siemens-Stiftung and the Institute of Science and Technology Austria for financial support.","external_id":{"isi":["001273082800019"],"pmid":["38484066"]},"publication":"Science","article_processing_charge":"No","month":"03","type":"journal_article","article_type":"letter_note","user_id":"317138e5-6ab7-11ef-aa6d-ffef3953e345","issue":"6688","supplementarymaterial":"no","year":"2024","fulldoi":"https://doi.org/10.1126/science.ado4077","project":[{"name":"HighTE: The Werner Siemens Laboratory for the High Throughput Discovery of Semiconductors for Waste Heat Recovery","_id":"9B8F7476-BA93-11EA-9121-9846C619BF3A"}],"date_updated":"2026-10-16T09:20:57Z","_id":"15166","quality_controlled":"1","researchdata_availability":"no","date_created":"2024-03-24T23:00:58Z","intvolume":" 383","status":"public","citation":{"short":"N. Jakhar, M. Ibáñez, Science 383 (2024) 1184.","chicago":"Jakhar, Navita, and Maria Ibáñez. “Electron Highways Are Cooler.” Science. American Association for the Advancement of Science, 2024. https://doi.org/10.1126/science.ado4077.","apa":"Jakhar, N., & Ibáñez, M. (2024). Electron highways are cooler. Science. American Association for the Advancement of Science. https://doi.org/10.1126/science.ado4077","ieee":"N. Jakhar and M. Ibáñez, “Electron highways are cooler,” Science, vol. 383, no. 6688. American Association for the Advancement of Science, p. 1184, 2024.","mla":"Jakhar, Navita, and Maria Ibáñez. “Electron Highways Are Cooler.” Science, vol. 383, no. 6688, American Association for the Advancement of Science, 2024, p. 1184, doi:10.1126/science.ado4077.","ista":"Jakhar N, Ibáñez M. 2024. Electron highways are cooler. Science. 383(6688), 1184.","ama":"Jakhar N, Ibáñez M. Electron highways are cooler. Science. 2024;383(6688):1184. doi:10.1126/science.ado4077"},"department":[{"_id":"MaIb"}],"language":[{"iso":"eng"}],"oa_version":"None","doi":"10.1126/science.ado4077","das_tickbox":"0","isi":1,"title":"Electron highways are cooler","page":"1184","publication_status":"published","pmid":1,"date_published":"2024-03-14T00:00:00Z","author":[{"first_name":"Navita","orcid":"0000-0001-7408-8197","last_name":"Navita","id":"6ebe278d-ba0b-11ee-8184-f34cdc671de4","full_name":"Navita, Navita"},{"first_name":"Maria","orcid":"0000-0001-5013-2843","last_name":"Ibáñez","id":"43C61214-F248-11E8-B48F-1D18A9856A87","full_name":"Ibáñez, Maria"}]},{"abstract":[{"lang":"eng","text":"The electroreduction of biomass-derived benzaldehyde (BZH) provides a potentially cost-effective route to produce benzyl alcohol (BA). This reaction competes with the electrochemical self-coupling of BZH to hydrobenzoin (HDB), which holds significance as a biofuel. Herein, we demonstrate the selectivity towards one or the other product strongly depends on the surface chemistry of the catalyst, specifically on its ability to adsorb hydrogen, as showcased with Cu2S electrocatalysts. We particularly analyze the effect of surface ligands, oleylamine (OAm), on the selective conversion of BZH to BA or HDB. The effect of the electrode potential, electrolyte pH, and temperature are studied. Results indicate that bare Cu2S exhibits higher selectivity towards BA, while OAm-capped Cu2S promotes HDB formation. This difference is explained by the competing adsorption of protons and BZH. During the BZH electrochemical conversion, electrons first transfer to the C in the C[double bond, length as m-dash]O group to form a ketyl radical. Then the radical either couples with surrounding H+ to form BA or self-couple to produce HDB, depending on the H+ availability that is affected by the electrocatalyst surface properties. The presence of OAm inhibits the H adsorption on the electrode surface therefore reducing the formation of high-energy state Had and its combination with ketyl radicals to form BA. Instead, the presence of OAm promotes the outer sphere reaction for obtaining HDB."}],"scopus_import":"1","publication_identifier":{"eissn":["2753-1457"]},"volume":3,"day":"01","has_accepted_license":"1","ddc":["540"],"acknowledgement":"L. Gong and J. Yu thank the China Scholarship Council for the scholarship support. ICN2 acknowledges funding from Generalitat de Catalunya 2021SGR00457. This study is part of the Advanced Materials programme and was supported by MCIN with funding from European Union NextGenerationEU (PRTR-C17.I1) and by Generalitat de Catalunya. The authors thank support from the project NANOGEN (PID2020-116093RB-C43), funded by MCIN/AEI/10.13039/501100011033/and by “ERDF A way of making Europe”, by the “European Union”. ICN2 is supported by the Severo Ochoa program from Spanish MCIN/AEI (Grant No.: CEX2021-001214-S) and is funded by the CERCA Programme/Generalitat de Catalunya. Part of the present work has been performed in the framework of Universitat Autònoma de Barcelona Materials Science PhD program. Authors acknowledge the use of instrumentation as well as the technical advice provided by the Joint Electron Microscopy Center at ALBA (JEMCA). ICN2 acknowledges funding from Grant IU16-014206 (METCAM-FIB) funded by the European Union through the European Regional Development Fund (ERDF), with the support of the Ministry of Research and Universities, Generalitat de Catalunya. ICN2 is founding member of e-DREAM.","publisher":"Royal Society of Chemistry","article_processing_charge":"Yes","oa":1,"DOAJ_listed":"1","OA_place":"publisher","publication":"Energy Advances","month":"09","type":"journal_article","dataavailabilitystatement":"The data supporting this article have been included as part of the ESI.†","article_type":"original","license":"https://creativecommons.org/licenses/by-nc/3.0/","user_id":"317138e5-6ab7-11ef-aa6d-ffef3953e345","issue":"9","supplementarymaterial":"yes","year":"2024","fulldoi":"https://doi.org/10.1039/d4ya00334a","researchdata_availability":"yes (supplementary data)","date_created":"2024-08-11T22:01:12Z","intvolume":" 3","_id":"17412","tmp":{"short":"CC BY-NC (3.0)","name":"Creative Commons Attribution-NonCommercial 3.0 Unported (CC BY-NC 3.0)","legal_code_url":"https://creativecommons.org/licenses/by-nc/3.0/legalcode","image":"/images/cc_by_nc.png"},"date_updated":"2026-10-16T10:04:01Z","quality_controlled":"1","citation":{"apa":"Gong, L., Zhao, S., Yu, J., Li, J., Arbiol, J., Kallio, T., … Cabot, A. (2024). Influence of the catalyst surface chemistry on the electrochemical self-coupling of biomass-derived benzaldehyde into hydrobenzoin. Energy Advances. Royal Society of Chemistry. https://doi.org/10.1039/d4ya00334a","chicago":"Gong, Li, Shiling Zhao, Jing Yu, Junshan Li, Jordi Arbiol, Tanja Kallio, Mariano Calcabrini, Paulina R. Martínez-Alanis, Maria Ibáñez, and Andreu Cabot. “Influence of the Catalyst Surface Chemistry on the Electrochemical Self-Coupling of Biomass-Derived Benzaldehyde into Hydrobenzoin.” Energy Advances. Royal Society of Chemistry, 2024. https://doi.org/10.1039/d4ya00334a.","short":"L. Gong, S. Zhao, J. Yu, J. Li, J. Arbiol, T. Kallio, M. Calcabrini, P.R. Martínez-Alanis, M. Ibáñez, A. Cabot, Energy Advances 3 (2024) 2287–2294.","mla":"Gong, Li, et al. “Influence of the Catalyst Surface Chemistry on the Electrochemical Self-Coupling of Biomass-Derived Benzaldehyde into Hydrobenzoin.” Energy Advances, vol. 3, no. 9, Royal Society of Chemistry, 2024, pp. 2287–94, doi:10.1039/d4ya00334a.","ista":"Gong L, Zhao S, Yu J, Li J, Arbiol J, Kallio T, Calcabrini M, Martínez-Alanis PR, Ibáñez M, Cabot A. 2024. Influence of the catalyst surface chemistry on the electrochemical self-coupling of biomass-derived benzaldehyde into hydrobenzoin. Energy Advances. 3(9), 2287–2294.","ama":"Gong L, Zhao S, Yu J, et al. Influence of the catalyst surface chemistry on the electrochemical self-coupling of biomass-derived benzaldehyde into hydrobenzoin. Energy Advances. 2024;3(9):2287-2294. doi:10.1039/d4ya00334a","ieee":"L. Gong et al., “Influence of the catalyst surface chemistry on the electrochemical self-coupling of biomass-derived benzaldehyde into hydrobenzoin,” Energy Advances, vol. 3, no. 9. Royal Society of Chemistry, pp. 2287–2294, 2024."},"department":[{"_id":"MaIb"}],"status":"public","oa_version":"Published Version","language":[{"iso":"eng"}],"doi":"10.1039/d4ya00334a","file_date_updated":"2025-01-09T12:29:09Z","das_tickbox":"1","title":"Influence of the catalyst surface chemistry on the electrochemical self-coupling of biomass-derived benzaldehyde into hydrobenzoin","page":"2287-2294","author":[{"full_name":"Gong, Li","last_name":"Gong","first_name":"Li"},{"full_name":"Zhao, Shiling","last_name":"Zhao","first_name":"Shiling"},{"last_name":"Yu","first_name":"Jing","full_name":"Yu, Jing"},{"full_name":"Li, Junshan","first_name":"Junshan","last_name":"Li"},{"last_name":"Arbiol","first_name":"Jordi","full_name":"Arbiol, Jordi"},{"first_name":"Tanja","last_name":"Kallio","full_name":"Kallio, Tanja"},{"first_name":"Mariano","id":"45D7531A-F248-11E8-B48F-1D18A9856A87","orcid":"0000-0003-4566-5877","last_name":"Calcabrini","full_name":"Calcabrini, Mariano"},{"full_name":"Martínez-Alanis, Paulina R.","last_name":"Martínez-Alanis","first_name":"Paulina R."},{"full_name":"Ibáñez, Maria","first_name":"Maria","last_name":"Ibáñez","orcid":"0000-0001-5013-2843","id":"43C61214-F248-11E8-B48F-1D18A9856A87"},{"last_name":"Cabot","first_name":"Andreu","full_name":"Cabot, Andreu"}],"date_published":"2024-09-01T00:00:00Z","publication_status":"published","file":[{"file_name":"2024_EnergyAdvances_Gong.pdf","access_level":"open_access","file_id":"18812","content_type":"application/pdf","file_size":1448762,"date_updated":"2025-01-09T12:29:09Z","checksum":"4a49515ec90354d005852e741bff1d29","relation":"main_file","date_created":"2025-01-09T12:29:09Z","success":1,"creator":"dernst"}],"OA_type":"gold"},{"researchdata_availability":"upon request","date_created":"2024-09-08T22:01:13Z","intvolume":" 17","_id":"17897","date_updated":"2026-10-16T10:04:37Z","quality_controlled":"1","citation":{"mla":"He, Ren, et al. “Active Site Switching on High Entropy Phosphides as Bifunctional Oxygen Electrocatalysts for Rechargeable/Robust Zn-Air Battery.” Energy and Environmental Science, vol. 17, no. 19, Royal Society of Chemistry, 2024, pp. 7193–208, doi:10.1039/d4ee01912a.","ista":"He R, Wang S, Yang L, Horta S, Ding Y, Di C, Zhang X, Xu Y, Ibáñez M, Zhou Y, Mebs S, Dau H, Hausmann JN, Huo W, Menezes PW, Cabot A. 2024. Active site switching on high entropy phosphides as bifunctional oxygen electrocatalysts for rechargeable/robust Zn-air battery. Energy and Environmental Science. 17(19), 7193–7208.","ama":"He R, Wang S, Yang L, et al. Active site switching on high entropy phosphides as bifunctional oxygen electrocatalysts for rechargeable/robust Zn-air battery. Energy and Environmental Science. 2024;17(19):7193-7208. doi:10.1039/d4ee01912a","ieee":"R. He et al., “Active site switching on high entropy phosphides as bifunctional oxygen electrocatalysts for rechargeable/robust Zn-air battery,” Energy and Environmental Science, vol. 17, no. 19. Royal Society of Chemistry, pp. 7193–7208, 2024.","chicago":"He, Ren, Shiqi Wang, Linlin Yang, Sharona Horta, Yang Ding, Chong Di, Xuesong Zhang, et al. “Active Site Switching on High Entropy Phosphides as Bifunctional Oxygen Electrocatalysts for Rechargeable/Robust Zn-Air Battery.” Energy and Environmental Science. Royal Society of Chemistry, 2024. https://doi.org/10.1039/d4ee01912a.","apa":"He, R., Wang, S., Yang, L., Horta, S., Ding, Y., Di, C., … Cabot, A. (2024). Active site switching on high entropy phosphides as bifunctional oxygen electrocatalysts for rechargeable/robust Zn-air battery. Energy and Environmental Science. Royal Society of Chemistry. https://doi.org/10.1039/d4ee01912a","short":"R. He, S. Wang, L. Yang, S. Horta, Y. Ding, C. Di, X. Zhang, Y. Xu, M. Ibáñez, Y. Zhou, S. Mebs, H. Dau, J.N. Hausmann, W. Huo, P.W. Menezes, A. Cabot, Energy and Environmental Science 17 (2024) 7193–7208."},"department":[{"_id":"MaIb"}],"status":"public","oa_version":"None","language":[{"iso":"eng"}],"doi":"10.1039/d4ee01912a","das_tickbox":"1","isi":1,"title":"Active site switching on high entropy phosphides as bifunctional oxygen electrocatalysts for rechargeable/robust Zn-air battery","page":"7193-7208","date_published":"2024-08-22T00:00:00Z","author":[{"last_name":"He","first_name":"Ren","full_name":"He, Ren"},{"full_name":"Wang, Shiqi","first_name":"Shiqi","last_name":"Wang"},{"first_name":"Linlin","last_name":"Yang","full_name":"Yang, Linlin"},{"full_name":"Horta, Sharona","last_name":"Horta","id":"03a7e858-01b1-11ec-8b71-99ae6c4a05bc","first_name":"Sharona"},{"full_name":"Ding, Yang","first_name":"Yang","last_name":"Ding"},{"full_name":"Di, Chong","first_name":"Chong","last_name":"Di"},{"first_name":"Xuesong","last_name":"Zhang","full_name":"Zhang, Xuesong"},{"full_name":"Xu, Ying","first_name":"Ying","last_name":"Xu"},{"full_name":"Ibáñez, Maria","first_name":"Maria","id":"43C61214-F248-11E8-B48F-1D18A9856A87","last_name":"Ibáñez","orcid":"0000-0001-5013-2843"},{"last_name":"Zhou","first_name":"Yingtang","full_name":"Zhou, Yingtang"},{"last_name":"Mebs","first_name":"Stefan","full_name":"Mebs, Stefan"},{"full_name":"Dau, Holger","last_name":"Dau","first_name":"Holger"},{"full_name":"Hausmann, Jan Niklas","last_name":"Hausmann","first_name":"Jan Niklas"},{"full_name":"Huo, Wenyi","first_name":"Wenyi","last_name":"Huo"},{"last_name":"Menezes","first_name":"Prashanth W.","full_name":"Menezes, Prashanth W."},{"last_name":"Cabot","first_name":"Andreu","full_name":"Cabot, Andreu"}],"publication_status":"published","OA_type":"closed access","abstract":[{"lang":"eng","text":"High-entropy materials (HEMs) offer a quasi-continuous spectrum of active sites and have generated great expectations in fields such as electrocatalysis and energy storage. Despite their potential, the complex composition and associated surface phenomena of HEMs pose challenges to their rational design and development. In this context, we have synthesized FeCoNiPdWP high entropy phosphide (HEP) nanoparticles using a low-temperature colloidal method, and explored their application as bifunctional electrocatalysts for the oxygen evolution and reduction reactions (OER/ORR). Our analysis provides a detailed understanding of the individual roles and transformations of each element during OER/ORR operation. Notably, the HEPs exhibit an exceptionally low OER overpotential of 227 mV at 10 mA cm−2, attributed to the reconstructed HEP surface into a FeCoNiPdW high entropy oxyhydroxide with high oxidation states of Fe, Co, and Ni serving as the active sites. Additionally, Pd and W play crucial roles in modulating the electronic structure to optimize the adsorption energy of oxygen intermediates. For the ORR, Pd emerges as the most active component. In the reconstructed catalyst, the strong d–d orbital coupling of especially Pd, Co, and W fine-tunes ORR electron transfer pathways, delivering an ORR half-wave potential of 0.81 V with a pure four-electron reduction mechanism. The practicality of these HEPs catalysts is showcased through the assembly of aqueous zinc–air batteries. These batteries demonstrate a superior specific capacity of 886 mA h gZn−1 and maintain excellent stability over more than 700 hours of continuous operation. Overall, this study not only elucidates the role of each element in HEMs but also establishes a foundational framework for the design and development of next-generation bifunctional oxygen catalysts, broadening the potential applications of these complex materials in advanced energy systems."}],"scopus_import":"1","publication_identifier":{"eissn":["1754-5706"],"issn":["1754-5692"]},"volume":17,"day":"22","acknowledgement":"This work was financially supported by the SyDEC at project from the Spanish MCIN/AEI/FEDER (PID2022-136883OB-C22) and Generalitat de Catalunya 2021SGR01581. J. N. H. and P. W. M. acknowledge support from the German Federal Ministry of Education and Research in the framework of the project “Catlab” (03EW0015A/B). L. Yang thanks the China Scholarship Council (CSC) for the scholarship support (202008130132). This work was supported by the European Union Horizon 2020 research and innovation program (No. 857470) and the European Regional Development Fund via the Foundation for Polish Science International Research Agenda PLUS program (No. MAB PLUS/2018/8). The publication was created within the framework of the project of the Minister of Science and Higher Education, Poland “Support for the activities of Centres of Excellence established in Poland under Horizon 2020” under contract no. MEiN/2023/DIR/3795. H. D. and S. M. thank the German Federal Ministry of Education and Research (BMBF) for supporting the Live-XAS project (05K22KE1) and the Deutsche Forschungsgemeinschaft (DFG, German Research Foundation) for support under Germany's Excellence Strategy – EXC 2008/1 – 390540038 – UniSysCat. The authors thank the Helmholtz-Zentrum Berlin (HZB) for beamtime allocation at the KMC-3 synchrotron beamline of the BESSY synchrotron in Berlin-Adlershof and Dr Ivo Zizak as well as Dr Michael Haumann for technical support.","publisher":"Royal Society of Chemistry","article_processing_charge":"No","publication":"Energy and Environmental Science","external_id":{"isi":["001298924700001"]},"month":"08","type":"journal_article","dataavailabilitystatement":"The data that support the findings of this study are available from the corresponding author upon reasonable request.","article_type":"original","user_id":"317138e5-6ab7-11ef-aa6d-ffef3953e345","issue":"19","supplementarymaterial":"yes","year":"2024","fulldoi":"https://doi.org/10.1039/d4ee01912a"},{"doi":"10.1021/acsnano.3c10201","isi":1,"das_tickbox":"0","title":"Nanocrystal assemblies: Current advances and open problems","page":"14791-14840","publication_status":"published","author":[{"last_name":"Bassani","first_name":"Carlos L.","full_name":"Bassani, Carlos L."},{"full_name":"Van Anders, Greg","first_name":"Greg","last_name":"Van Anders"},{"last_name":"Banin","first_name":"Uri","full_name":"Banin, Uri"},{"last_name":"Baranov","first_name":"Dmitry","full_name":"Baranov, Dmitry"},{"full_name":"Chen, Qian","last_name":"Chen","first_name":"Qian"},{"last_name":"Dijkstra","first_name":"Marjolein","full_name":"Dijkstra, Marjolein"},{"first_name":"Michael S.","last_name":"Dimitriyev","full_name":"Dimitriyev, Michael S."},{"full_name":"Efrati, Efi","last_name":"Efrati","first_name":"Efi"},{"last_name":"Faraudo","first_name":"Jordi","full_name":"Faraudo, Jordi"},{"last_name":"Gang","first_name":"Oleg","full_name":"Gang, Oleg"},{"full_name":"Gaston, Nicola","first_name":"Nicola","last_name":"Gaston"},{"full_name":"Golestanian, Ramin","first_name":"Ramin","last_name":"Golestanian"},{"full_name":"Guerrero-Garcia, G. Ivan","last_name":"Guerrero-Garcia","first_name":"G. Ivan"},{"full_name":"Gruenwald, Michael","last_name":"Gruenwald","first_name":"Michael"},{"first_name":"Amir","last_name":"Haji-Akbari","full_name":"Haji-Akbari, Amir"},{"id":"43C61214-F248-11E8-B48F-1D18A9856A87","last_name":"Ibáñez","orcid":"0000-0001-5013-2843","first_name":"Maria","full_name":"Ibáñez, Maria"},{"last_name":"Karg","first_name":"Matthias","full_name":"Karg, Matthias"},{"full_name":"Kraus, Tobias","last_name":"Kraus","first_name":"Tobias"},{"full_name":"Lee, Byeongdu","last_name":"Lee","first_name":"Byeongdu"},{"last_name":"Van Lehn","first_name":"Reid C.","full_name":"Van Lehn, Reid C."},{"full_name":"Macfarlane, Robert J.","last_name":"Macfarlane","first_name":"Robert J."},{"full_name":"Mognetti, Bortolo M.","first_name":"Bortolo M.","last_name":"Mognetti"},{"last_name":"Nikoubashman","first_name":"Arash","full_name":"Nikoubashman, Arash"},{"first_name":"Saeed","last_name":"Osat","full_name":"Osat, Saeed"},{"full_name":"Prezhdo, Oleg V.","first_name":"Oleg V.","last_name":"Prezhdo"},{"first_name":"Grant M.","last_name":"Rotskoff","full_name":"Rotskoff, Grant M."},{"first_name":"Leonor","last_name":"Saiz","full_name":"Saiz, Leonor"},{"first_name":"An Chang","last_name":"Shi","full_name":"Shi, An Chang"},{"last_name":"Skrabalak","first_name":"Sara","full_name":"Skrabalak, Sara"},{"full_name":"Smalyukh, Ivan I.","last_name":"Smalyukh","first_name":"Ivan I."},{"first_name":"Mario","last_name":"Tagliazucchi","full_name":"Tagliazucchi, Mario"},{"last_name":"Talapin","first_name":"Dmitri V.","full_name":"Talapin, Dmitri V."},{"first_name":"Alexei V.","last_name":"Tkachenko","full_name":"Tkachenko, Alexei V."},{"last_name":"Tretiak","first_name":"Sergei","full_name":"Tretiak, Sergei"},{"first_name":"David","last_name":"Vaknin","full_name":"Vaknin, David"},{"last_name":"Widmer-Cooper","first_name":"Asaph","full_name":"Widmer-Cooper, Asaph"},{"full_name":"Wong, Gerard C.L.","first_name":"Gerard C.L.","last_name":"Wong"},{"full_name":"Ye, Xingchen","last_name":"Ye","first_name":"Xingchen"},{"full_name":"Zhou, Shan","last_name":"Zhou","first_name":"Shan"},{"full_name":"Rabani, Eran","last_name":"Rabani","first_name":"Eran"},{"full_name":"Engel, Michael","first_name":"Michael","last_name":"Engel"},{"full_name":"Travesset, Alex","last_name":"Travesset","first_name":"Alex"}],"date_published":"2024-05-30T00:00:00Z","pmid":1,"OA_type":"closed access","_id":"17125","date_updated":"2026-10-16T10:03:25Z","quality_controlled":"1","researchdata_availability":"no","date_created":"2024-06-09T22:01:02Z","intvolume":" 18","status":"public","citation":{"apa":"Bassani, C. L., Van Anders, G., Banin, U., Baranov, D., Chen, Q., Dijkstra, M., … Travesset, A. (2024). Nanocrystal assemblies: Current advances and open problems. ACS Nano. American Chemical Society. https://doi.org/10.1021/acsnano.3c10201","chicago":"Bassani, Carlos L., Greg Van Anders, Uri Banin, Dmitry Baranov, Qian Chen, Marjolein Dijkstra, Michael S. Dimitriyev, et al. “Nanocrystal Assemblies: Current Advances and Open Problems.” ACS Nano. American Chemical Society, 2024. https://doi.org/10.1021/acsnano.3c10201.","short":"C.L. Bassani, G. Van Anders, U. Banin, D. Baranov, Q. Chen, M. Dijkstra, M.S. Dimitriyev, E. Efrati, J. Faraudo, O. Gang, N. Gaston, R. Golestanian, G.I. Guerrero-Garcia, M. Gruenwald, A. Haji-Akbari, M. Ibáñez, M. Karg, T. Kraus, B. Lee, R.C. Van Lehn, R.J. Macfarlane, B.M. Mognetti, A. Nikoubashman, S. Osat, O.V. Prezhdo, G.M. Rotskoff, L. Saiz, A.C. Shi, S. Skrabalak, I.I. Smalyukh, M. Tagliazucchi, D.V. Talapin, A.V. Tkachenko, S. Tretiak, D. Vaknin, A. Widmer-Cooper, G.C.L. Wong, X. Ye, S. Zhou, E. Rabani, M. Engel, A. Travesset, ACS Nano 18 (2024) 14791–14840.","ama":"Bassani CL, Van Anders G, Banin U, et al. Nanocrystal assemblies: Current advances and open problems. ACS Nano. 2024;18(23):14791-14840. doi:10.1021/acsnano.3c10201","ista":"Bassani CL, Van Anders G, Banin U, Baranov D, Chen Q, Dijkstra M, Dimitriyev MS, Efrati E, Faraudo J, Gang O, Gaston N, Golestanian R, Guerrero-Garcia GI, Gruenwald M, Haji-Akbari A, Ibáñez M, Karg M, Kraus T, Lee B, Van Lehn RC, Macfarlane RJ, Mognetti BM, Nikoubashman A, Osat S, Prezhdo OV, Rotskoff GM, Saiz L, Shi AC, Skrabalak S, Smalyukh II, Tagliazucchi M, Talapin DV, Tkachenko AV, Tretiak S, Vaknin D, Widmer-Cooper A, Wong GCL, Ye X, Zhou S, Rabani E, Engel M, Travesset A. 2024. Nanocrystal assemblies: Current advances and open problems. ACS Nano. 18(23), 14791–14840.","mla":"Bassani, Carlos L., et al. “Nanocrystal Assemblies: Current Advances and Open Problems.” ACS Nano, vol. 18, no. 23, American Chemical Society, 2024, pp. 14791–840, doi:10.1021/acsnano.3c10201.","ieee":"C. L. Bassani et al., “Nanocrystal assemblies: Current advances and open problems,” ACS Nano, vol. 18, no. 23. American Chemical Society, pp. 14791–14840, 2024."},"department":[{"_id":"MaIb"}],"language":[{"iso":"eng"}],"oa_version":"None","type":"journal_article","article_type":"review","user_id":"317138e5-6ab7-11ef-aa6d-ffef3953e345","issue":"23","supplementarymaterial":"no","year":"2024","fulldoi":"https://doi.org/10.1021/acsnano.3c10201","volume":18,"day":"30","scopus_import":"1","abstract":[{"text":"We explore the potential of nanocrystals (a term used equivalently to nanoparticles) as building blocks for nanomaterials, and the current advances and open challenges for fundamental science developments and applications. Nanocrystal assemblies are inherently multiscale, and the generation of revolutionary material properties requires a precise understanding of the relationship between structure and function, the former being determined by classical effects and the latter often by quantum effects. With an emphasis on theory and computation, we discuss challenges that hamper current assembly strategies and to what extent nanocrystal assemblies represent thermodynamic equilibrium or kinetically trapped metastable states. We also examine dynamic effects and optimization of assembly protocols. Finally, we discuss promising material functions and examples of their realization with nanocrystal assemblies.","lang":"eng"}],"publication_identifier":{"issn":["1936-0851"],"eissn":["1936-086X"]},"publisher":"American Chemical Society","acknowledgement":"This research was supported in part by the National Science Foundation under Grant No. NSF PHY-1748958 to the Kavli Institute for Theoretical Physics. The biophysics part of this paper was supported in part by the Gordon and Betty Moore Foundation Grant No. 2919.02. CLB acknowledges the sponsorship of the Alexander von Humboldt Foundation through the Humboldt Research Fellowship for postdoctoral researchers, and the support of the Emerging Talents Initiative (ETI) and the EAM Starting Grant (EAM-SG23-1) of the Competence Center Engineering of Advanced Materials of the Friedrich-Alexander-Universität Erlangen-Nürnberg. CLB and ME acknowledge the support of the Deutsche Forschungsgemeinschaft (DFG, German Research Foundation) Project-ID 416229255-SFB 1411. The research of AT was supported by the U.S. Department of Energy (U.S. DOE), Office of Basic Energy Sciences, Division of Materials Sciences and Engineering. Iowa State University operates Ames National Laboratory for the U.S. DOE under Contract DE-AC02-07CH11358.","publication":"ACS Nano","external_id":{"isi":["001236199900001"],"pmid":["38814908"]},"article_processing_charge":"No","month":"05"},{"volume":16,"day":"11","abstract":[{"lang":"eng","text":"Broadband photodetectors that can decipher the wavelength (λ) and intensity (I) of an unknown incident light are urgently demanded. Photothermoelectric (PTE) detectors can achieve ultrabroadband photodetection surpassing the bandgap limitation; however, their practical application is severely hampered by the lack of deciphering strategy. In this work, we report a variable elimination method to decipher λ and I of the incident lights based on an integrated Ag2Se film-based PTE detector. Nanostructured Ag2Se films with controlled thickness are synthesized using an ion sputtering of Ag and a room-temperature selenization method and then assembled into a detector. Under identical illumination, Ag2Se films of different thicknesses produce varying output photothermal voltages, influenced by factors including λ. By establishing a direct relationship between the photothermal voltage and the absorption of Ag2Se films of varied thickness, we successfully eliminate variables independent of λ, thus determining λ. Subsequently, I is determined by the calibrated responsivity relationship using obtained λ. Our PTE detector achieves a broadband spectrum from 400 to 950 nm and high accuracy, with deviations as low as ∼2.63 and ∼0.53% for deciphered λ and I, respectively. This method allows for self-powered broadband decipherable photodetection without a complex device architecture or computational assistance, which could boost the research enthusiasm and promote the commercialization of PTE broadband detectors."}],"scopus_import":"1","publication_identifier":{"eissn":["1944-8252"],"issn":["1944-8244"]},"publisher":"American Chemical Society","acknowledgement":"The authors appreciate the Analytical & Testing Center of Sichuan University and Ceshigo Research Service for their supports on material characterization. This study is financial supported by the fund of the State Key Laboratory of Solidification Processing in Northwestern Polytechnical University (NWPU, Grant SKLSP202315), the State Key Laboratory for Mechanical Behavior of Materials (Grant 20232509), and the International Scientific and Technological Innovation Cooperation of Sichuan Province (2024YFHZ0309).","external_id":{"pmid":["39194354"],"isi":["001300770000001"]},"publication":"ACS Applied Materials and Interfaces","article_processing_charge":"No","month":"09","type":"journal_article","article_type":"original","user_id":"317138e5-6ab7-11ef-aa6d-ffef3953e345","issue":"36","supplementarymaterial":"yes","year":"2024","fulldoi":"https://doi.org/10.1021/acsami.4c10489","date_updated":"2026-10-16T10:04:56Z","_id":"17896","quality_controlled":"1","date_created":"2024-09-08T22:01:13Z","researchdata_availability":"no","intvolume":" 16","status":"public","citation":{"mla":"Zhou, Jiamin, et al. “Decipher the Wavelength and Intensity Using Photothermoelectric Detectors.” ACS Applied Materials and Interfaces, vol. 16, no. 36, American Chemical Society, 2024, pp. 47923–30, doi:10.1021/acsami.4c10489.","ama":"Zhou J, Xu S, Shuai Y, et al. Decipher the wavelength and intensity using photothermoelectric detectors. ACS Applied Materials and Interfaces. 2024;16(36):47923-47930. doi:10.1021/acsami.4c10489","ista":"Zhou J, Xu S, Shuai Y, Sun Q, Ma H, Wang C, Wu H, Tan S, Wang Z, Yang L. 2024. Decipher the wavelength and intensity using photothermoelectric detectors. ACS Applied Materials and Interfaces. 16(36), 47923–47930.","ieee":"J. Zhou et al., “Decipher the wavelength and intensity using photothermoelectric detectors,” ACS Applied Materials and Interfaces, vol. 16, no. 36. American Chemical Society, pp. 47923–47930, 2024.","chicago":"Zhou, Jiamin, Shengduo Xu, Yi Shuai, Qiang Sun, Huangshui Ma, Chao Wang, Haijuan Wu, Shanshan Tan, Zegao Wang, and Lei Yang. “Decipher the Wavelength and Intensity Using Photothermoelectric Detectors.” ACS Applied Materials and Interfaces. American Chemical Society, 2024. https://doi.org/10.1021/acsami.4c10489.","apa":"Zhou, J., Xu, S., Shuai, Y., Sun, Q., Ma, H., Wang, C., … Yang, L. (2024). Decipher the wavelength and intensity using photothermoelectric detectors. ACS Applied Materials and Interfaces. American Chemical Society. https://doi.org/10.1021/acsami.4c10489","short":"J. Zhou, S. Xu, Y. Shuai, Q. Sun, H. Ma, C. Wang, H. Wu, S. Tan, Z. Wang, L. Yang, ACS Applied Materials and Interfaces 16 (2024) 47923–47930."},"department":[{"_id":"MaIb"}],"language":[{"iso":"eng"}],"oa_version":"None","doi":"10.1021/acsami.4c10489","isi":1,"das_tickbox":"0","title":"Decipher the wavelength and intensity using photothermoelectric detectors","page":"47923-47930","pmid":1,"author":[{"full_name":"Zhou, Jiamin","first_name":"Jiamin","last_name":"Zhou"},{"full_name":"Xu, Shengduo","first_name":"Shengduo","id":"12ab8624-4c8a-11ec-9e11-e1ac2438f22f","last_name":"Xu"},{"full_name":"Shuai, Yi","first_name":"Yi","last_name":"Shuai"},{"full_name":"Sun, Qiang","first_name":"Qiang","last_name":"Sun"},{"last_name":"Ma","first_name":"Huangshui","full_name":"Ma, Huangshui"},{"last_name":"Wang","first_name":"Chao","full_name":"Wang, Chao"},{"last_name":"Wu","first_name":"Haijuan","full_name":"Wu, Haijuan"},{"first_name":"Shanshan","last_name":"Tan","full_name":"Tan, Shanshan"},{"last_name":"Wang","first_name":"Zegao","full_name":"Wang, Zegao"},{"full_name":"Yang, Lei","last_name":"Yang","first_name":"Lei"}],"date_published":"2024-09-11T00:00:00Z","publication_status":"published","OA_type":"closed access"},{"date_published":"2024-06-15T00:00:00Z","publication_status":"published","author":[{"full_name":"Mahato, Neelima","first_name":"Neelima","last_name":"Mahato"},{"id":"12d625da-9cb3-11ed-9667-af09d37d3f0a","orcid":"0000-0003-2209-5269","last_name":"Singh","first_name":"Saurabh","full_name":"Singh, Saurabh"},{"full_name":"Sreekanth, T. V.M.","last_name":"Sreekanth","first_name":"T. V.M."},{"full_name":"Yoo, Kisoo","last_name":"Yoo","first_name":"Kisoo"},{"full_name":"Kim, Jonghoon","first_name":"Jonghoon","last_name":"Kim"}],"isi":1,"das_tickbox":"1","title":"In-situ engineered highly crystalline polythiophene empowered electrochemical capacitor-I: Synthesis, characterization, and electrochemical charge storage","doi":"10.1016/j.matlet.2024.136483","OA_type":"closed access","intvolume":" 365","date_created":"2024-04-28T22:00:56Z","researchdata_availability":"upon request","quality_controlled":"1","article_number":"136483","date_updated":"2026-10-16T10:01:50Z","_id":"15348","oa_version":"None","language":[{"iso":"eng"}],"department":[{"_id":"MaIb"}],"citation":{"chicago":"Mahato, Neelima, Saurabh Singh, T. V.M. Sreekanth, Kisoo Yoo, and Jonghoon Kim. “In-Situ Engineered Highly Crystalline Polythiophene Empowered Electrochemical Capacitor-I: Synthesis, Characterization, and Electrochemical Charge Storage.” Materials Letters. Elsevier, 2024. https://doi.org/10.1016/j.matlet.2024.136483.","apa":"Mahato, N., Singh, S., Sreekanth, T. V. M., Yoo, K., & Kim, J. (2024). In-situ engineered highly crystalline polythiophene empowered electrochemical capacitor-I: Synthesis, characterization, and electrochemical charge storage. Materials Letters. Elsevier. https://doi.org/10.1016/j.matlet.2024.136483","short":"N. Mahato, S. Singh, T.V.M. Sreekanth, K. Yoo, J. Kim, Materials Letters 365 (2024).","ama":"Mahato N, Singh S, Sreekanth TVM, Yoo K, Kim J. In-situ engineered highly crystalline polythiophene empowered electrochemical capacitor-I: Synthesis, characterization, and electrochemical charge storage. Materials Letters. 2024;365. doi:10.1016/j.matlet.2024.136483","ista":"Mahato N, Singh S, Sreekanth TVM, Yoo K, Kim J. 2024. In-situ engineered highly crystalline polythiophene empowered electrochemical capacitor-I: Synthesis, characterization, and electrochemical charge storage. Materials Letters. 365, 136483.","mla":"Mahato, Neelima, et al. “In-Situ Engineered Highly Crystalline Polythiophene Empowered Electrochemical Capacitor-I: Synthesis, Characterization, and Electrochemical Charge Storage.” Materials Letters, vol. 365, 136483, Elsevier, 2024, doi:10.1016/j.matlet.2024.136483.","ieee":"N. Mahato, S. Singh, T. V. M. Sreekanth, K. Yoo, and J. Kim, “In-situ engineered highly crystalline polythiophene empowered electrochemical capacitor-I: Synthesis, characterization, and electrochemical charge storage,” Materials Letters, vol. 365. Elsevier, 2024."},"status":"public","dataavailabilitystatement":"Data will be made available on request.","article_type":"original","type":"journal_article","fulldoi":"https://doi.org/10.1016/j.matlet.2024.136483","year":"2024","supplementarymaterial":"yes","user_id":"317138e5-6ab7-11ef-aa6d-ffef3953e345","acknowledgement":"This research was supported by the Korea Evaluation Institute of Industrial Technology (No. 200116167, Development of Battery Safety Diagnosis System (BDS) SoC that predicts the internal state, explosion risk, remaining useful life, and replacement timing of electric vehicle batteries).","corr_author":"1","publisher":"Elsevier","publication_identifier":{"eissn":["1873-4979"],"issn":["0167-577X"]},"abstract":[{"text":"We report on synthesis of highly crystalline polythiophene and its application in supercapacitor electrodes. The material exhibits a remarkably stable electrochemical behavior and an excellent device performance. The device delivers an electrode specific capacitance (Csp) of 129.13F g−1, Cell Csp of 32.28F g−1 at 0.5 A/g; energy, and power densities of ∼ 3 Wh kg−1 and 250 W kg -1, respectively at 0.5 A/g. Also, it exhibits an excellent retention of Cell Csp and coulombic efficiency up to ∼ 95 % over 10,000 continuous galvanostatic charge discharge (GCD) cycles indicating a remarkable performance by a standalone, pristine and undoped polythiophene. Electrochemical impedance spectroscopy (EIS) studies further suggest material’s stable capacitive behavior. The material’s enhanced electrochemical properties, stable behavior and outstanding performance in device application are attributed to the crystalline phases present in the polymer matrix achievable via a slow rate of synthesis; overall, an edge over other conventional synthesis methods.","lang":"eng"}],"scopus_import":"1","day":"15","volume":365,"month":"06","article_processing_charge":"No","external_id":{"isi":["001300025600001"]},"publication":"Materials Letters"}]