[{"date_created":"2023-08-01T09:44:04Z","publisher":"Springer Nature","intvolume":"        11","type":"journal_article","citation":{"apa":"Zhao, H., Sen, S., Udayabhaskararao, T., Sawczyk, M., Kučanda, K., Manna, D., … Klajn, R. (2015). Reversible trapping and reaction acceleration within dynamically self-assembling nanoflasks. <i>Nature Nanotechnology</i>. Springer Nature. <a href=\"https://doi.org/10.1038/nnano.2015.256\">https://doi.org/10.1038/nnano.2015.256</a>","short":"H. Zhao, S. Sen, T. Udayabhaskararao, M. Sawczyk, K. Kučanda, D. Manna, P.K. Kundu, J.-W. Lee, P. Král, R. Klajn, Nature Nanotechnology 11 (2015) 82–88.","ama":"Zhao H, Sen S, Udayabhaskararao T, et al. Reversible trapping and reaction acceleration within dynamically self-assembling nanoflasks. <i>Nature Nanotechnology</i>. 2015;11:82-88. doi:<a href=\"https://doi.org/10.1038/nnano.2015.256\">10.1038/nnano.2015.256</a>","ista":"Zhao H, Sen S, Udayabhaskararao T, Sawczyk M, Kučanda K, Manna D, Kundu PK, Lee J-W, Král P, Klajn R. 2015. Reversible trapping and reaction acceleration within dynamically self-assembling nanoflasks. Nature Nanotechnology. 11, 82–88.","mla":"Zhao, Hui, et al. “Reversible Trapping and Reaction Acceleration within Dynamically Self-Assembling Nanoflasks.” <i>Nature Nanotechnology</i>, vol. 11, Springer Nature, 2015, pp. 82–88, doi:<a href=\"https://doi.org/10.1038/nnano.2015.256\">10.1038/nnano.2015.256</a>.","ieee":"H. Zhao <i>et al.</i>, “Reversible trapping and reaction acceleration within dynamically self-assembling nanoflasks,” <i>Nature Nanotechnology</i>, vol. 11. Springer Nature, pp. 82–88, 2015.","chicago":"Zhao, Hui, Soumyo Sen, T. Udayabhaskararao, Michał Sawczyk, Kristina Kučanda, Debasish Manna, Pintu K. Kundu, Ji-Woong Lee, Petr Král, and Rafal Klajn. “Reversible Trapping and Reaction Acceleration within Dynamically Self-Assembling Nanoflasks.” <i>Nature Nanotechnology</i>. Springer Nature, 2015. <a href=\"https://doi.org/10.1038/nnano.2015.256\">https://doi.org/10.1038/nnano.2015.256</a>."},"publication_status":"published","day":"23","doi":"10.1038/nnano.2015.256","date_published":"2015-11-23T00:00:00Z","publication":"Nature Nanotechnology","language":[{"iso":"eng"}],"scopus_import":"1","publication_identifier":{"issn":["1748-3387"],"eissn":["1748-3395"]},"keyword":["Electrical and Electronic Engineering","Condensed Matter Physics","General Materials Science","Biomedical Engineering","Atomic and Molecular Physics","and Optics","Bioengineering"],"external_id":{"pmid":["26595335"]},"extern":"1","pmid":1,"oa_version":"None","date_updated":"2024-10-14T12:17:26Z","abstract":[{"text":"The chemical behaviour of molecules can be significantly modified by confinement to volumes comparable to the dimensions of the molecules. Although such confined spaces can be found in various nanostructured materials, such as zeolites, nanoporous organic frameworks and colloidal nanocrystal assemblies, the slow diffusion of molecules in and out of these materials has greatly hampered studying the effect of confinement on their physicochemical properties. Here, we show that this diffusion limitation can be overcome by reversibly creating and destroying confined environments by means of ultraviolet and visible light irradiation. We use colloidal nanocrystals functionalized with light-responsive ligands that readily self-assemble and trap various molecules from the surrounding bulk solution. Once trapped, these molecules can undergo chemical reactions with increased rates and with stereoselectivities significantly different from those in bulk solution. Illumination with visible light disassembles these nanoflasks, releasing the product in solution and thereby establishes a catalytic cycle. These dynamic nanoflasks can be useful for studying chemical reactivities in confined environments and for synthesizing molecules that are otherwise hard to achieve in bulk solution.","lang":"eng"}],"author":[{"last_name":"Zhao","first_name":"Hui","full_name":"Zhao, Hui"},{"first_name":"Soumyo","full_name":"Sen, Soumyo","last_name":"Sen"},{"last_name":"Udayabhaskararao","first_name":"T.","full_name":"Udayabhaskararao, T."},{"last_name":"Sawczyk","full_name":"Sawczyk, Michał","first_name":"Michał"},{"last_name":"Kučanda","full_name":"Kučanda, Kristina","first_name":"Kristina"},{"last_name":"Manna","full_name":"Manna, Debasish","first_name":"Debasish"},{"first_name":"Pintu K.","full_name":"Kundu, Pintu K.","last_name":"Kundu"},{"last_name":"Lee","first_name":"Ji-Woong","full_name":"Lee, Ji-Woong"},{"full_name":"Král, Petr","first_name":"Petr","last_name":"Král"},{"full_name":"Klajn, Rafal","first_name":"Rafal","id":"8e84690e-1e48-11ed-a02b-a1e6fb8bb53b","last_name":"Klajn"}],"year":"2015","article_processing_charge":"No","article_type":"original","page":"82-88","quality_controlled":"1","month":"11","user_id":"2DF688A6-F248-11E8-B48F-1D18A9856A87","_id":"13392","title":"Reversible trapping and reaction acceleration within dynamically self-assembling nanoflasks","volume":11,"status":"public"},{"day":"01","publication_status":"published","publication":"Angewandte Chemie International Edition","language":[{"iso":"eng"}],"doi":"10.1002/anie.201502419","date_published":"2015-10-01T00:00:00Z","date_created":"2023-08-01T09:44:19Z","citation":{"short":"D. Manna, T. Udayabhaskararao, H. Zhao, R. Klajn, Angewandte Chemie International Edition 54 (2015) 12394–12397.","ama":"Manna D, Udayabhaskararao T, Zhao H, Klajn R. Orthogonal light-induced self-assembly of nanoparticles using differently substituted azobenzenes. <i>Angewandte Chemie International Edition</i>. 2015;54(42):12394-12397. doi:<a href=\"https://doi.org/10.1002/anie.201502419\">10.1002/anie.201502419</a>","apa":"Manna, D., Udayabhaskararao, T., Zhao, H., &#38; Klajn, R. (2015). Orthogonal light-induced self-assembly of nanoparticles using differently substituted azobenzenes. <i>Angewandte Chemie International Edition</i>. Wiley. <a href=\"https://doi.org/10.1002/anie.201502419\">https://doi.org/10.1002/anie.201502419</a>","ista":"Manna D, Udayabhaskararao T, Zhao H, Klajn R. 2015. Orthogonal light-induced self-assembly of nanoparticles using differently substituted azobenzenes. Angewandte Chemie International Edition. 54(42), 12394–12397.","mla":"Manna, Debasish, et al. “Orthogonal Light-Induced Self-Assembly of Nanoparticles Using Differently Substituted Azobenzenes.” <i>Angewandte Chemie International Edition</i>, vol. 54, no. 42, Wiley, 2015, pp. 12394–97, doi:<a href=\"https://doi.org/10.1002/anie.201502419\">10.1002/anie.201502419</a>.","ieee":"D. Manna, T. Udayabhaskararao, H. Zhao, and R. Klajn, “Orthogonal light-induced self-assembly of nanoparticles using differently substituted azobenzenes,” <i>Angewandte Chemie International Edition</i>, vol. 54, no. 42. Wiley, pp. 12394–12397, 2015.","chicago":"Manna, Debasish, Thumu Udayabhaskararao, Hui Zhao, and Rafal Klajn. “Orthogonal Light-Induced Self-Assembly of Nanoparticles Using Differently Substituted Azobenzenes.” <i>Angewandte Chemie International Edition</i>. Wiley, 2015. <a href=\"https://doi.org/10.1002/anie.201502419\">https://doi.org/10.1002/anie.201502419</a>."},"publisher":"Wiley","intvolume":"        54","type":"journal_article","quality_controlled":"1","month":"10","title":"Orthogonal light-induced self-assembly of nanoparticles using differently substituted azobenzenes","volume":54,"status":"public","user_id":"2DF688A6-F248-11E8-B48F-1D18A9856A87","_id":"13393","extern":"1","external_id":{"pmid":["25959725"]},"issue":"42","scopus_import":"1","publication_identifier":{"issn":["1433-7851"],"eissn":["1521-3773"]},"keyword":["General Chemistry","Catalysis"],"article_type":"original","page":"12394-12397","pmid":1,"oa_version":"None","date_updated":"2024-10-14T12:17:36Z","abstract":[{"text":"Precise control of the self-assembly of selected components within complex mixtures is a challenging goal whose realization is important for fabricating novel nanomaterials. Herein we show that by decorating the surfaces of metallic nanoparticles with differently substituted azobenzenes, it is possible to modulate the wavelength of light at which the self-assembly of these nanoparticles is induced. Exposing a mixture of two types of nanoparticles, each functionalized with a different azobenzene, to UV or blue light induces the selective self-assembly of only one type of nanoparticles. Irradiation with the other wavelength triggers the disassembly of the aggregates, and the simultaneous self-assembly of nanoparticles of the other type. By placing both types of azobenzenes on the same nanoparticles, we created unique materials (“frustrated” nanoparticles) whose self-assembly is induced irrespective of the wavelength of the incident light.","lang":"eng"}],"year":"2015","author":[{"last_name":"Manna","first_name":"Debasish","full_name":"Manna, Debasish"},{"first_name":"Thumu","full_name":"Udayabhaskararao, Thumu","last_name":"Udayabhaskararao"},{"full_name":"Zhao, Hui","first_name":"Hui","last_name":"Zhao"},{"id":"8e84690e-1e48-11ed-a02b-a1e6fb8bb53b","full_name":"Klajn, Rafal","first_name":"Rafal","last_name":"Klajn"}],"article_processing_charge":"No"},{"doi":"10.1038/nchem.2303","date_published":"2015-07-20T00:00:00Z","publication":"Nature Chemistry","language":[{"iso":"eng"}],"publication_status":"published","day":"20","publisher":"Springer Nature","intvolume":"         7","type":"journal_article","citation":{"apa":"Kundu, P. K., Samanta, D., Leizrowice, R., Margulis, B., Zhao, H., Börner, M., … Klajn, R. (2015). Light-controlled self-assembly of non-photoresponsive nanoparticles. <i>Nature Chemistry</i>. Springer Nature. <a href=\"https://doi.org/10.1038/nchem.2303\">https://doi.org/10.1038/nchem.2303</a>","short":"P.K. Kundu, D. Samanta, R. Leizrowice, B. Margulis, H. Zhao, M. Börner, T. Udayabhaskararao, D. Manna, R. Klajn, Nature Chemistry 7 (2015) 646–652.","ama":"Kundu PK, Samanta D, Leizrowice R, et al. Light-controlled self-assembly of non-photoresponsive nanoparticles. <i>Nature Chemistry</i>. 2015;7:646-652. doi:<a href=\"https://doi.org/10.1038/nchem.2303\">10.1038/nchem.2303</a>","ista":"Kundu PK, Samanta D, Leizrowice R, Margulis B, Zhao H, Börner M, Udayabhaskararao T, Manna D, Klajn R. 2015. Light-controlled self-assembly of non-photoresponsive nanoparticles. Nature Chemistry. 7, 646–652.","mla":"Kundu, Pintu K., et al. “Light-Controlled Self-Assembly of Non-Photoresponsive Nanoparticles.” <i>Nature Chemistry</i>, vol. 7, Springer Nature, 2015, pp. 646–52, doi:<a href=\"https://doi.org/10.1038/nchem.2303\">10.1038/nchem.2303</a>.","ieee":"P. K. Kundu <i>et al.</i>, “Light-controlled self-assembly of non-photoresponsive nanoparticles,” <i>Nature Chemistry</i>, vol. 7. Springer Nature, pp. 646–652, 2015.","chicago":"Kundu, Pintu K., Dipak Samanta, Ron Leizrowice, Baruch Margulis, Hui Zhao, Martin Börner, T. Udayabhaskararao, Debasish Manna, and Rafal Klajn. “Light-Controlled Self-Assembly of Non-Photoresponsive Nanoparticles.” <i>Nature Chemistry</i>. Springer Nature, 2015. <a href=\"https://doi.org/10.1038/nchem.2303\">https://doi.org/10.1038/nchem.2303</a>."},"date_created":"2023-08-01T09:44:33Z","user_id":"2DF688A6-F248-11E8-B48F-1D18A9856A87","_id":"13394","title":"Light-controlled self-assembly of non-photoresponsive nanoparticles","volume":7,"status":"public","quality_controlled":"1","month":"07","pmid":1,"oa_version":"None","abstract":[{"lang":"eng","text":"The ability to guide the assembly of nanosized objects reversibly with external stimuli, in particular light, is of fundamental importance, and it contributes to the development of applications as diverse as nanofabrication and controlled drug delivery. However, all the systems described to date are based on nanoparticles (NPs) that are inherently photoresponsive, which makes their preparation cumbersome and can markedly hamper their performance. Here we describe a conceptually new methodology to assemble NPs reversibly using light that does not require the particles to be functionalized with light-responsive ligands. Our strategy is based on the use of a photoswitchable medium that responds to light in such a way that it modulates the interparticle interactions. NP assembly proceeds quantitatively and without apparent fatigue, both in solution and in gels. Exposing the gels to light in a spatially controlled manner allowed us to draw images that spontaneously disappeared after a specific period of time."}],"date_updated":"2024-10-14T12:17:47Z","year":"2015","author":[{"first_name":"Pintu K.","full_name":"Kundu, Pintu K.","last_name":"Kundu"},{"first_name":"Dipak","full_name":"Samanta, Dipak","last_name":"Samanta"},{"first_name":"Ron","full_name":"Leizrowice, Ron","last_name":"Leizrowice"},{"first_name":"Baruch","full_name":"Margulis, Baruch","last_name":"Margulis"},{"last_name":"Zhao","full_name":"Zhao, Hui","first_name":"Hui"},{"last_name":"Börner","full_name":"Börner, Martin","first_name":"Martin"},{"last_name":"Udayabhaskararao","full_name":"Udayabhaskararao, T.","first_name":"T."},{"last_name":"Manna","first_name":"Debasish","full_name":"Manna, Debasish"},{"last_name":"Klajn","full_name":"Klajn, Rafal","first_name":"Rafal","id":"8e84690e-1e48-11ed-a02b-a1e6fb8bb53b"}],"article_processing_charge":"No","article_type":"original","page":"646-652","scopus_import":"1","keyword":["General Chemical Engineering","General Chemistry"],"publication_identifier":{"issn":["1755-4330"],"eissn":["1755-4349"]},"external_id":{"pmid":["26201741"]},"extern":"1"},{"date_created":"2023-08-01T09:44:48Z","type":"journal_article","intvolume":"        51","publisher":"Royal Society of Chemistry","citation":{"apa":"Lee, J.-W., &#38; Klajn, R. (2015). Dual-responsive nanoparticles that aggregate under the simultaneous action of light and CO2. <i>Chemical Communications</i>. Royal Society of Chemistry. <a href=\"https://doi.org/10.1039/c4cc08541h\">https://doi.org/10.1039/c4cc08541h</a>","ama":"Lee J-W, Klajn R. Dual-responsive nanoparticles that aggregate under the simultaneous action of light and CO2. <i>Chemical Communications</i>. 2015;51(11):2036-2039. doi:<a href=\"https://doi.org/10.1039/c4cc08541h\">10.1039/c4cc08541h</a>","short":"J.-W. Lee, R. Klajn, Chemical Communications 51 (2015) 2036–2039.","ieee":"J.-W. Lee and R. Klajn, “Dual-responsive nanoparticles that aggregate under the simultaneous action of light and CO2,” <i>Chemical Communications</i>, vol. 51, no. 11. Royal Society of Chemistry, pp. 2036–2039, 2015.","chicago":"Lee, Ji-Woong, and Rafal Klajn. “Dual-Responsive Nanoparticles That Aggregate under the Simultaneous Action of Light and CO2.” <i>Chemical Communications</i>. Royal Society of Chemistry, 2015. <a href=\"https://doi.org/10.1039/c4cc08541h\">https://doi.org/10.1039/c4cc08541h</a>.","ista":"Lee J-W, Klajn R. 2015. Dual-responsive nanoparticles that aggregate under the simultaneous action of light and CO2. Chemical Communications. 51(11), 2036–2039.","mla":"Lee, Ji-Woong, and Rafal Klajn. “Dual-Responsive Nanoparticles That Aggregate under the Simultaneous Action of Light and CO2.” <i>Chemical Communications</i>, vol. 51, no. 11, Royal Society of Chemistry, 2015, pp. 2036–39, doi:<a href=\"https://doi.org/10.1039/c4cc08541h\">10.1039/c4cc08541h</a>."},"publication_status":"published","day":"18","date_published":"2015-11-18T00:00:00Z","oa":1,"doi":"10.1039/c4cc08541h","language":[{"iso":"eng"}],"publication":"Chemical Communications","keyword":["Materials Chemistry","Metals and Alloys","Surfaces","Coatings and Films","General Chemistry","Ceramics and Composites","Electronic","Optical and Magnetic Materials","Catalysis"],"publication_identifier":{"issn":["1359-7345"],"eissn":["1364-548X"]},"issue":"11","scopus_import":"1","extern":"1","external_id":{"pmid":["25417754"]},"article_processing_charge":"No","author":[{"last_name":"Lee","full_name":"Lee, Ji-Woong","first_name":"Ji-Woong"},{"last_name":"Klajn","id":"8e84690e-1e48-11ed-a02b-a1e6fb8bb53b","full_name":"Klajn, Rafal","first_name":"Rafal"}],"year":"2015","abstract":[{"lang":"eng","text":"Metallic nanoparticles co-functionalised with monolayers of UV- and CO2-sensitive ligands were prepared and shown to respond to these two types of stimuli reversibly and in an orthogonal fashion. The composition of the coating could be tailored to yield nanoparticles capable of aggregating exclusively when both UV and CO2 were applied at the same time, analogously to the behaviour of an AND logic gate."}],"date_updated":"2024-10-14T12:17:58Z","oa_version":"Published Version","pmid":1,"page":"2036-2039","main_file_link":[{"url":"https://doi.org/10.1039/C4CC08541H","open_access":"1"}],"article_type":"original","month":"11","quality_controlled":"1","_id":"13395","user_id":"2DF688A6-F248-11E8-B48F-1D18A9856A87","status":"public","volume":51,"title":"Dual-responsive nanoparticles that aggregate under the simultaneous action of light and CO2"},{"date_created":"2023-08-01T09:45:02Z","intvolume":"        31","publisher":"American Chemical Society","type":"journal_article","citation":{"ista":"Moldt T, Brete D, Przyrembel D, Das S, Goldman JR, Kundu PK, Gahl C, Klajn R, Weinelt M. 2015. Tailoring the properties of surface-immobilized azobenzenes by monolayer dilution and surface curvature. Langmuir. 31(3), 1048–1057.","mla":"Moldt, Thomas, et al. “Tailoring the Properties of Surface-Immobilized Azobenzenes by Monolayer Dilution and Surface Curvature.” <i>Langmuir</i>, vol. 31, no. 3, American Chemical Society, 2015, pp. 1048–57, doi:<a href=\"https://doi.org/10.1021/la504291n\">10.1021/la504291n</a>.","ieee":"T. Moldt <i>et al.</i>, “Tailoring the properties of surface-immobilized azobenzenes by monolayer dilution and surface curvature,” <i>Langmuir</i>, vol. 31, no. 3. American Chemical Society, pp. 1048–1057, 2015.","chicago":"Moldt, Thomas, Daniel Brete, Daniel Przyrembel, Sanjib Das, Joel R. Goldman, Pintu K. Kundu, Cornelius Gahl, Rafal Klajn, and Martin Weinelt. “Tailoring the Properties of Surface-Immobilized Azobenzenes by Monolayer Dilution and Surface Curvature.” <i>Langmuir</i>. American Chemical Society, 2015. <a href=\"https://doi.org/10.1021/la504291n\">https://doi.org/10.1021/la504291n</a>.","apa":"Moldt, T., Brete, D., Przyrembel, D., Das, S., Goldman, J. R., Kundu, P. K., … Weinelt, M. (2015). Tailoring the properties of surface-immobilized azobenzenes by monolayer dilution and surface curvature. <i>Langmuir</i>. American Chemical Society. <a href=\"https://doi.org/10.1021/la504291n\">https://doi.org/10.1021/la504291n</a>","short":"T. Moldt, D. Brete, D. Przyrembel, S. Das, J.R. Goldman, P.K. Kundu, C. Gahl, R. Klajn, M. Weinelt, Langmuir 31 (2015) 1048–1057.","ama":"Moldt T, Brete D, Przyrembel D, et al. Tailoring the properties of surface-immobilized azobenzenes by monolayer dilution and surface curvature. <i>Langmuir</i>. 2015;31(3):1048-1057. doi:<a href=\"https://doi.org/10.1021/la504291n\">10.1021/la504291n</a>"},"publication_status":"published","day":"27","date_published":"2015-01-27T00:00:00Z","doi":"10.1021/la504291n","publication":"Langmuir","language":[{"iso":"eng"}],"issue":"3","scopus_import":"1","publication_identifier":{"issn":["0743-7463"],"eissn":["1520-5827"]},"keyword":["Electrochemistry","Spectroscopy","Surfaces and Interfaces","Condensed Matter Physics","General Materials Science"],"extern":"1","external_id":{"pmid":["25544061"]},"oa_version":"None","pmid":1,"article_processing_charge":"No","year":"2015","author":[{"first_name":"Thomas","full_name":"Moldt, Thomas","last_name":"Moldt"},{"full_name":"Brete, Daniel","first_name":"Daniel","last_name":"Brete"},{"last_name":"Przyrembel","first_name":"Daniel","full_name":"Przyrembel, Daniel"},{"last_name":"Das","full_name":"Das, Sanjib","first_name":"Sanjib"},{"last_name":"Goldman","first_name":"Joel R.","full_name":"Goldman, Joel R."},{"full_name":"Kundu, Pintu K.","first_name":"Pintu K.","last_name":"Kundu"},{"last_name":"Gahl","full_name":"Gahl, Cornelius","first_name":"Cornelius"},{"id":"8e84690e-1e48-11ed-a02b-a1e6fb8bb53b","first_name":"Rafal","full_name":"Klajn, Rafal","last_name":"Klajn"},{"full_name":"Weinelt, Martin","first_name":"Martin","last_name":"Weinelt"}],"date_updated":"2024-10-14T12:18:08Z","abstract":[{"text":"Photoswitching in densely packed azobenzene self-assembled monolayers (SAMs) is strongly affected by steric constraints and excitonic coupling between neighboring chromophores. Therefore, control of the chromophore density is essential for enhancing and manipulating the photoisomerization yield. We systematically compare two methods to achieve this goal: First, we assemble monocomponent azobenzene–alkanethiolate SAMs on gold nanoparticles of varying size. Second, we form mixed SAMs of azobenzene–alkanethiolates and “dummy” alkanethiolates on planar substrates. Both methods lead to a gradual decrease of the chromophore density and enable efficient photoswitching with low-power light sources. X-ray spectroscopy reveals that coadsorption from solution yields mixtures with tunable composition. The orientation of the chromophores with respect to the surface normal changes from a tilted to an upright position with increasing azobenzene density. For both systems, optical spectroscopy reveals a pronounced excitonic shift that increases with the chromophore density. In spite of exciting the optical transition of the monomer, the main spectral change in mixed SAMs occurs in the excitonic band. In addition, the photoisomerization yield decreases only slightly by increasing the azobenzene–alkanethiolate density, and we observed photoswitching even with minor dilutions. Unlike in solution, azobenzene in the planar SAM can be switched back almost completely by optical excitation from the cis to the original trans state within a short time scale. These observations indicate cooperativity in the photoswitching process of mixed SAMs.","lang":"eng"}],"article_type":"original","page":"1048-1057","month":"01","quality_controlled":"1","user_id":"2DF688A6-F248-11E8-B48F-1D18A9856A87","_id":"13396","volume":31,"title":"Tailoring the properties of surface-immobilized azobenzenes by monolayer dilution and surface curvature","status":"public"},{"month":"01","quality_controlled":"1","_id":"13397","user_id":"2DF688A6-F248-11E8-B48F-1D18A9856A87","status":"public","volume":181,"title":"Magnetic field-induced self-assembly of iron oxide nanocubes","publication_identifier":{"issn":["1359-6640"],"eissn":["1364-5498"]},"keyword":["Physical and Theoretical Chemistry"],"scopus_import":"1","external_id":{"pmid":["25920522"]},"extern":"1","article_processing_charge":"No","year":"2015","author":[{"last_name":"Singh","full_name":"Singh, Gurvinder","first_name":"Gurvinder"},{"last_name":"Chan","full_name":"Chan, Henry","first_name":"Henry"},{"last_name":"Udayabhaskararao","full_name":"Udayabhaskararao, T.","first_name":"T."},{"last_name":"Gelman","first_name":"Elijah","full_name":"Gelman, Elijah"},{"last_name":"Peddis","first_name":"Davide","full_name":"Peddis, Davide"},{"last_name":"Baskin","full_name":"Baskin, Artem","first_name":"Artem"},{"first_name":"Gregory","full_name":"Leitus, Gregory","last_name":"Leitus"},{"first_name":"Petr","full_name":"Král, Petr","last_name":"Král"},{"last_name":"Klajn","first_name":"Rafal","full_name":"Klajn, Rafal","id":"8e84690e-1e48-11ed-a02b-a1e6fb8bb53b"}],"date_updated":"2024-10-14T12:18:19Z","abstract":[{"text":"Self-assembly of inorganic nanoparticles has been studied extensively for particles having different sizes and compositions. However, relatively little attention has been devoted to how the shape and surface chemistry of magnetic nanoparticles affects their self-assembly properties. Here, we undertook a combined experiment–theory study aimed at better understanding of the self-assembly of cubic magnetite (Fe3O4) particles. We demonstrated that, depending on the experimental parameters, such as the direction of the magnetic field and nanoparticle density, a variety of superstructures can be obtained, including one-dimensional filaments and helices, as well as C-shaped assemblies described here for the first time. Furthermore, we functionalized the surfaces of the magnetic nanocubes with light-sensitive ligands. Using these modified nanoparticles, we were able to achieve orthogonal control of self-assembly using a magnetic field and light.","lang":"eng"}],"oa_version":"Published Version","pmid":1,"page":"403-421","main_file_link":[{"url":"https://doi.org/10.1039/C4FD00265B","open_access":"1"}],"article_type":"original","publication_status":"published","day":"02","oa":1,"date_published":"2015-01-02T00:00:00Z","doi":"10.1039/c4fd00265b","language":[{"iso":"eng"}],"publication":"Faraday Discussions","date_created":"2023-08-01T09:45:17Z","type":"journal_article","intvolume":"       181","publisher":"Royal Society of Chemistry","citation":{"ista":"Singh G, Chan H, Udayabhaskararao T, Gelman E, Peddis D, Baskin A, Leitus G, Král P, Klajn R. 2015. Magnetic field-induced self-assembly of iron oxide nanocubes. Faraday Discussions. 181, 403–421.","mla":"Singh, Gurvinder, et al. “Magnetic Field-Induced Self-Assembly of Iron Oxide Nanocubes.” <i>Faraday Discussions</i>, vol. 181, Royal Society of Chemistry, 2015, pp. 403–21, doi:<a href=\"https://doi.org/10.1039/c4fd00265b\">10.1039/c4fd00265b</a>.","ieee":"G. Singh <i>et al.</i>, “Magnetic field-induced self-assembly of iron oxide nanocubes,” <i>Faraday Discussions</i>, vol. 181. Royal Society of Chemistry, pp. 403–421, 2015.","chicago":"Singh, Gurvinder, Henry Chan, T. Udayabhaskararao, Elijah Gelman, Davide Peddis, Artem Baskin, Gregory Leitus, Petr Král, and Rafal Klajn. “Magnetic Field-Induced Self-Assembly of Iron Oxide Nanocubes.” <i>Faraday Discussions</i>. Royal Society of Chemistry, 2015. <a href=\"https://doi.org/10.1039/c4fd00265b\">https://doi.org/10.1039/c4fd00265b</a>.","apa":"Singh, G., Chan, H., Udayabhaskararao, T., Gelman, E., Peddis, D., Baskin, A., … Klajn, R. (2015). Magnetic field-induced self-assembly of iron oxide nanocubes. <i>Faraday Discussions</i>. Royal Society of Chemistry. <a href=\"https://doi.org/10.1039/c4fd00265b\">https://doi.org/10.1039/c4fd00265b</a>","short":"G. Singh, H. Chan, T. Udayabhaskararao, E. Gelman, D. Peddis, A. Baskin, G. Leitus, P. Král, R. Klajn, Faraday Discussions 181 (2015) 403–421.","ama":"Singh G, Chan H, Udayabhaskararao T, et al. Magnetic field-induced self-assembly of iron oxide nanocubes. <i>Faraday Discussions</i>. 2015;181:403-421. doi:<a href=\"https://doi.org/10.1039/c4fd00265b\">10.1039/c4fd00265b</a>"}},{"citation":{"apa":"Sun, Y., Scarabelli, L., Kotov, N., Tebbe, M., Lin, X.-M., Brullot, W., … Ghosh, S. (2015). Field-assisted self-assembly process: General discussion. <i>Faraday Discussions</i>. Royal Society of Chemistry. <a href=\"https://doi.org/10.1039/c5fd90041g\">https://doi.org/10.1039/c5fd90041g</a>","short":"Y. Sun, L. Scarabelli, N. Kotov, M. Tebbe, X.-M. Lin, W. Brullot, L. Isa, P. Schurtenberger, H. Moehwald, I. Fedin, O. Velev, D. Faivre, C. Sorensen, R. Perzynski, M. Chanana, Z. Li, F. Bresme, P. Král, E. Firlar, D. Schiffrin, J.B. Souza Junior, A. Fery, E. Shevchenko, O. Tarhan, A.P. Alivisatos, S. Disch, R. Klajn, S. Ghosh, Faraday Discussions 181 (2015) 463–479.","ama":"Sun Y, Scarabelli L, Kotov N, et al. Field-assisted self-assembly process: General discussion. <i>Faraday Discussions</i>. 2015;181:463-479. doi:<a href=\"https://doi.org/10.1039/c5fd90041g\">10.1039/c5fd90041g</a>","ista":"Sun Y, Scarabelli L, Kotov N, Tebbe M, Lin X-M, Brullot W, Isa L, Schurtenberger P, Moehwald H, Fedin I, Velev O, Faivre D, Sorensen C, Perzynski R, Chanana M, Li Z, Bresme F, Král P, Firlar E, Schiffrin D, Souza Junior JB, Fery A, Shevchenko E, Tarhan O, Alivisatos AP, Disch S, Klajn R, Ghosh S. 2015. Field-assisted self-assembly process: General discussion. Faraday Discussions. 181, 463–479.","mla":"Sun, Yugang, et al. “Field-Assisted Self-Assembly Process: General Discussion.” <i>Faraday Discussions</i>, vol. 181, Royal Society of Chemistry, 2015, pp. 463–79, doi:<a href=\"https://doi.org/10.1039/c5fd90041g\">10.1039/c5fd90041g</a>.","ieee":"Y. Sun <i>et al.</i>, “Field-assisted self-assembly process: General discussion,” <i>Faraday Discussions</i>, vol. 181. Royal Society of Chemistry, pp. 463–479, 2015.","chicago":"Sun, Yugang, Leonardo Scarabelli, Nicholas Kotov, Moritz Tebbe, Xiao-Min Lin, Ward Brullot, Lucio Isa, et al. “Field-Assisted Self-Assembly Process: General Discussion.” <i>Faraday Discussions</i>. Royal Society of Chemistry, 2015. <a href=\"https://doi.org/10.1039/c5fd90041g\">https://doi.org/10.1039/c5fd90041g</a>."},"type":"journal_article","publisher":"Royal Society of Chemistry","intvolume":"       181","date_created":"2023-08-01T09:45:29Z","language":[{"iso":"eng"}],"publication":"Faraday Discussions","doi":"10.1039/c5fd90041g","date_published":"2015-07-07T00:00:00Z","day":"07","publication_status":"published","page":"463-479","article_type":"letter_note","date_updated":"2023-08-08T07:16:20Z","article_processing_charge":"No","author":[{"first_name":"Yugang","full_name":"Sun, Yugang","last_name":"Sun"},{"first_name":"Leonardo","full_name":"Scarabelli, Leonardo","last_name":"Scarabelli"},{"first_name":"Nicholas","full_name":"Kotov, Nicholas","last_name":"Kotov"},{"full_name":"Tebbe, Moritz","first_name":"Moritz","last_name":"Tebbe"},{"last_name":"Lin","first_name":"Xiao-Min","full_name":"Lin, Xiao-Min"},{"last_name":"Brullot","full_name":"Brullot, Ward","first_name":"Ward"},{"last_name":"Isa","first_name":"Lucio","full_name":"Isa, Lucio"},{"full_name":"Schurtenberger, Peter","first_name":"Peter","last_name":"Schurtenberger"},{"last_name":"Moehwald","full_name":"Moehwald, Helmuth","first_name":"Helmuth"},{"last_name":"Fedin","first_name":"Igor","full_name":"Fedin, Igor"},{"last_name":"Velev","full_name":"Velev, Orlin","first_name":"Orlin"},{"first_name":"Damien","full_name":"Faivre, Damien","last_name":"Faivre"},{"last_name":"Sorensen","first_name":"Christopher","full_name":"Sorensen, Christopher"},{"last_name":"Perzynski","full_name":"Perzynski, Régine","first_name":"Régine"},{"last_name":"Chanana","full_name":"Chanana, Munish","first_name":"Munish"},{"first_name":"Zhihai","full_name":"Li, Zhihai","last_name":"Li"},{"last_name":"Bresme","first_name":"Fernando","full_name":"Bresme, Fernando"},{"last_name":"Král","first_name":"Petr","full_name":"Král, Petr"},{"last_name":"Firlar","full_name":"Firlar, Emre","first_name":"Emre"},{"full_name":"Schiffrin, David","first_name":"David","last_name":"Schiffrin"},{"last_name":"Souza Junior","full_name":"Souza Junior, Joao Batista","first_name":"Joao Batista"},{"last_name":"Fery","first_name":"Andreas","full_name":"Fery, Andreas"},{"full_name":"Shevchenko, Elena","first_name":"Elena","last_name":"Shevchenko"},{"first_name":"Ozgur","full_name":"Tarhan, Ozgur","last_name":"Tarhan"},{"last_name":"Alivisatos","first_name":"Armand Paul","full_name":"Alivisatos, Armand Paul"},{"full_name":"Disch, Sabrina","first_name":"Sabrina","last_name":"Disch"},{"first_name":"Rafal","full_name":"Klajn, Rafal","id":"8e84690e-1e48-11ed-a02b-a1e6fb8bb53b","last_name":"Klajn"},{"full_name":"Ghosh, Suvojit","first_name":"Suvojit","last_name":"Ghosh"}],"year":"2015","pmid":1,"oa_version":"None","extern":"1","external_id":{"pmid":["26149295"]},"publication_identifier":{"eissn":["1364-5498"],"issn":["1359-6640"]},"keyword":["Physical and Theoretical Chemistry"],"scopus_import":"1","status":"public","title":"Field-assisted self-assembly process: General discussion","volume":181,"_id":"13398","user_id":"2DF688A6-F248-11E8-B48F-1D18A9856A87","quality_controlled":"1","month":"07"},{"department":[{"_id":"JiFr"}],"type":"journal_article","publisher":"Nature Publishing Group","isi":1,"intvolume":"         1","citation":{"short":"L. Yu, S. Scholl, A. Doering, Z. Yi, N. Irani, S. Di Rubbo, L. Neumetzler, P. Krishnamoorthy, I. Van Houtte, E. Mylle, V. Bischoff, S. Vernhettes, J. Winne, J. Friml, Y. Stierhof, K. Schumacher, S. Persson, E. Russinova, Nature Plants 1 (2015).","ama":"Yu L, Scholl S, Doering A, et al. V-ATPase activity in the TGN/EE is required for exocytosis and recycling in Arabidopsis. <i>Nature Plants</i>. 2015;1(7). doi:<a href=\"https://doi.org/10.1038/nplants.2015.94\">10.1038/nplants.2015.94</a>","apa":"Yu, L., Scholl, S., Doering, A., Yi, Z., Irani, N., Di Rubbo, S., … Russinova, E. (2015). V-ATPase activity in the TGN/EE is required for exocytosis and recycling in Arabidopsis. <i>Nature Plants</i>. Nature Publishing Group. <a href=\"https://doi.org/10.1038/nplants.2015.94\">https://doi.org/10.1038/nplants.2015.94</a>","ista":"Yu L, Scholl S, Doering A, Yi Z, Irani N, Di Rubbo S, Neumetzler L, Krishnamoorthy P, Van Houtte I, Mylle E, Bischoff V, Vernhettes S, Winne J, Friml J, Stierhof Y, Schumacher K, Persson S, Russinova E. 2015. V-ATPase activity in the TGN/EE is required for exocytosis and recycling in Arabidopsis. Nature Plants. 1(7), 15094.","mla":"Yu, Luo, et al. “V-ATPase Activity in the TGN/EE Is Required for Exocytosis and Recycling in Arabidopsis.” <i>Nature Plants</i>, vol. 1, no. 7, 15094, Nature Publishing Group, 2015, doi:<a href=\"https://doi.org/10.1038/nplants.2015.94\">10.1038/nplants.2015.94</a>.","chicago":"Yu, Luo, Stefan Scholl, Anett Doering, Zhang Yi, Niloufer Irani, Simone Di Rubbo, Lutz Neumetzler, et al. “V-ATPase Activity in the TGN/EE Is Required for Exocytosis and Recycling in Arabidopsis.” <i>Nature Plants</i>. Nature Publishing Group, 2015. <a href=\"https://doi.org/10.1038/nplants.2015.94\">https://doi.org/10.1038/nplants.2015.94</a>.","ieee":"L. Yu <i>et al.</i>, “V-ATPase activity in the TGN/EE is required for exocytosis and recycling in Arabidopsis,” <i>Nature Plants</i>, vol. 1, no. 7. Nature Publishing Group, 2015."},"date_created":"2018-12-11T11:51:42Z","doi":"10.1038/nplants.2015.94","date_published":"2015-07-06T00:00:00Z","oa":1,"language":[{"iso":"eng"}],"publication":"Nature Plants","publication_status":"published","article_number":"15094","day":"06","date_updated":"2025-09-29T11:04:05Z","abstract":[{"lang":"eng","text":"In plants, vacuolar H+-ATPase (V-ATPase) activity acidifies both the trans-Golgi network/early endosome (TGN/EE) and the vacuole. This dual V-ATPase function has impeded our understanding of how the pH homeostasis within the plant TGN/EE controls exo- and endocytosis. Here, we show that the weak V-ATPase mutant deetiolated3 (det3) displayed a pH increase in the TGN/EE, but not in the vacuole, strongly impairing secretion and recycling of the brassinosteroid receptor and the cellulose synthase complexes to the plasma membrane, in contrast to mutants lacking tonoplast-localized V-ATPase activity only. The brassinosteroid insensitivity and the cellulose deficiency defects in det3 were tightly correlated with reduced Golgi and TGN/EE motility. Thus, our results provide strong evidence that acidification of the TGN/EE, but not of the vacuole, is indispensable for functional secretion and recycling in plants."}],"year":"2015","author":[{"first_name":"Luo","full_name":"Yu, Luo","last_name":"Yu"},{"last_name":"Scholl","full_name":"Scholl, Stefan","first_name":"Stefan"},{"first_name":"Anett","full_name":"Doering, Anett","last_name":"Doering"},{"first_name":"Zhang","full_name":"Yi, Zhang","last_name":"Yi"},{"full_name":"Irani, Niloufer","first_name":"Niloufer","last_name":"Irani"},{"full_name":"Di Rubbo, Simone","first_name":"Simone","last_name":"Di Rubbo"},{"last_name":"Neumetzler","first_name":"Lutz","full_name":"Neumetzler, Lutz"},{"full_name":"Krishnamoorthy, Praveen","first_name":"Praveen","last_name":"Krishnamoorthy"},{"first_name":"Isabelle","full_name":"Van Houtte, Isabelle","last_name":"Van Houtte"},{"last_name":"Mylle","first_name":"Evelien","full_name":"Mylle, Evelien"},{"first_name":"Volker","full_name":"Bischoff, Volker","last_name":"Bischoff"},{"last_name":"Vernhettes","full_name":"Vernhettes, Samantha","first_name":"Samantha"},{"last_name":"Winne","full_name":"Winne, Johan","first_name":"Johan"},{"last_name":"Friml","orcid":"0000-0002-8302-7596","first_name":"Jirí","full_name":"Friml, Jirí","id":"4159519E-F248-11E8-B48F-1D18A9856A87"},{"last_name":"Stierhof","first_name":"York","full_name":"Stierhof, York"},{"last_name":"Schumacher","full_name":"Schumacher, Karin","first_name":"Karin"},{"last_name":"Persson","full_name":"Persson, Staffan","first_name":"Staffan"},{"full_name":"Russinova, Eugenia","first_name":"Eugenia","last_name":"Russinova"}],"article_processing_charge":"No","pmid":1,"oa_version":"Submitted Version","main_file_link":[{"open_access":"1","url":"https://www.ncbi.nlm.nih.gov/pmc/articles/PMC4905525/"}],"article_type":"original","scopus_import":"1","issue":"7","external_id":{"pmid":["27250258"],"isi":["000364407200001"]},"_id":"1383","user_id":"317138e5-6ab7-11ef-aa6d-ffef3953e345","status":"public","title":"V-ATPase activity in the TGN/EE is required for exocytosis and recycling in Arabidopsis","volume":1,"publist_id":"5827","quality_controlled":"1","month":"07"},{"degree_awarded":"PhD","day":"01","publication_status":"published","publist_id":"5808","month":"06","alternative_title":["ISTA Thesis"],"language":[{"iso":"eng"}],"status":"public","title":"On the approximation of intrinsic volumes","date_published":"2015-06-01T00:00:00Z","_id":"1399","user_id":"2DF688A6-F248-11E8-B48F-1D18A9856A87","date_created":"2018-12-11T11:51:48Z","corr_author":"1","publication_identifier":{"issn":["2663-337X"]},"page":"144","related_material":{"record":[{"id":"1662","relation":"part_of_dissertation","status":"public"},{"status":"public","id":"1792","relation":"part_of_dissertation"},{"status":"public","id":"2255","relation":"part_of_dissertation"}]},"citation":{"ieee":"F. Pausinger, “On the approximation of intrinsic volumes,” Institute of Science and Technology Austria, 2015.","chicago":"Pausinger, Florian. “On the Approximation of Intrinsic Volumes.” Institute of Science and Technology Austria, 2015.","ista":"Pausinger F. 2015. On the approximation of intrinsic volumes. Institute of Science and Technology Austria.","mla":"Pausinger, Florian. <i>On the Approximation of Intrinsic Volumes</i>. Institute of Science and Technology Austria, 2015.","ama":"Pausinger F. On the approximation of intrinsic volumes. 2015.","short":"F. Pausinger, On the Approximation of Intrinsic Volumes, Institute of Science and Technology Austria, 2015.","apa":"Pausinger, F. (2015). <i>On the approximation of intrinsic volumes</i>. Institute of Science and Technology Austria."},"article_processing_charge":"No","year":"2015","author":[{"orcid":"0000-0002-8379-3768","last_name":"Pausinger","first_name":"Florian","full_name":"Pausinger, Florian","id":"2A77D7A2-F248-11E8-B48F-1D18A9856A87"}],"type":"dissertation","supervisor":[{"orcid":"0000-0002-9823-6833","last_name":"Edelsbrunner","id":"3FB178DA-F248-11E8-B48F-1D18A9856A87","first_name":"Herbert","full_name":"Edelsbrunner, Herbert"}],"date_updated":"2025-09-29T11:14:36Z","abstract":[{"text":"This thesis is concerned with the computation and approximation of intrinsic volumes. Given a smooth body M and a certain digital approximation of it, we develop algorithms to approximate various intrinsic volumes of M using only measurements taken from its digital approximations. The crucial idea behind our novel algorithms is to link the recent theory of persistent homology to the theory of intrinsic volumes via the Crofton formula from integral geometry and, in particular, via Euler characteristic computations. Our main contributions are a multigrid convergent digital algorithm to compute the first intrinsic volume of a solid body in R^n as well as an appropriate integration pipeline to approximate integral-geometric integrals defined over the Grassmannian manifold.","lang":"eng"}],"department":[{"_id":"HeEd"}],"oa_version":"None","publisher":"Institute of Science and Technology Austria"},{"alternative_title":["ISTA Thesis"],"month":"04","publication_status":"published","publist_id":"5807","day":"01","degree_awarded":"PhD","user_id":"2DF688A6-F248-11E8-B48F-1D18A9856A87","date_published":"2015-04-01T00:00:00Z","_id":"1400","title":"The subclonal evolution of cancer","language":[{"iso":"eng"}],"status":"public","corr_author":"1","publication_identifier":{"issn":["2663-337X"]},"date_created":"2018-12-11T11:51:48Z","publisher":"Institute of Science and Technology Austria","oa_version":"None","department":[{"_id":"KrCh"}],"abstract":[{"text":"Cancer results from an uncontrolled growth of abnormal cells. Sequentially accumulated genetic and epigenetic alterations decrease cell death and increase cell replication. We used mathematical models to quantify the effect of driver gene mutations. The recently developed targeted therapies can lead to dramatic regressions. However, in solid cancers, clinical responses are often short-lived because resistant cancer cells evolve. We estimated that approximately 50 different mutations can confer resistance to a typical targeted therapeutic agent. We find that resistant cells are likely to be present in expanded subclones before the start of the treatment. The dominant strategy to prevent the evolution of resistance is combination therapy. Our analytical results suggest that in most patients, dual therapy, but not monotherapy, can result in long-term disease control. However, long-term control can only occur if there are no possible mutations in the genome that can cause cross-resistance to both drugs. Furthermore, we showed that simultaneous therapy with two drugs is much more likely to result in long-term disease control than sequential therapy with the same drugs. To improve our understanding of the underlying subclonal evolution we reconstruct the evolutionary history of a patient's cancer from next-generation sequencing data of spatially-distinct DNA samples. Using a quantitative measure of genetic relatedness, we found that pancreatic cancers and their metastases demonstrated a higher level of relatedness than that expected for any two cells randomly taken from a normal tissue. This minimal amount of genetic divergence among advanced lesions indicates that genetic heterogeneity, when quantitatively defined, is not a fundamental feature of the natural history of untreated pancreatic cancers. Our newly developed, phylogenomic tool Treeomics finds evidence for seeding patterns of metastases and can directly be used to discover rules governing the evolution of solid malignancies to transform cancer into a more predictable disease.","lang":"eng"}],"date_updated":"2025-09-30T07:54:55Z","supervisor":[{"id":"2E5DCA20-F248-11E8-B48F-1D18A9856A87","full_name":"Chatterjee, Krishnendu","first_name":"Krishnendu","orcid":"0000-0002-4561-241X","last_name":"Chatterjee"}],"type":"dissertation","article_processing_charge":"No","author":[{"orcid":"0000-0002-0170-7353","last_name":"Reiter","id":"4A918E98-F248-11E8-B48F-1D18A9856A87","full_name":"Reiter, Johannes","first_name":"Johannes"}],"year":"2015","citation":{"ama":"Reiter J. The subclonal evolution of cancer. 2015.","short":"J. Reiter, The Subclonal Evolution of Cancer, Institute of Science and Technology Austria, 2015.","apa":"Reiter, J. (2015). <i>The subclonal evolution of cancer</i>. Institute of Science and Technology Austria.","chicago":"Reiter, Johannes. “The Subclonal Evolution of Cancer.” Institute of Science and Technology Austria, 2015.","ieee":"J. Reiter, “The subclonal evolution of cancer,” Institute of Science and Technology Austria, 2015.","mla":"Reiter, Johannes. <i>The Subclonal Evolution of Cancer</i>. Institute of Science and Technology Austria, 2015.","ista":"Reiter J. 2015. The subclonal evolution of cancer. Institute of Science and Technology Austria."},"related_material":{"record":[{"status":"public","relation":"part_of_dissertation","id":"2000"},{"status":"public","id":"1709","relation":"part_of_dissertation"},{"id":"2858","relation":"part_of_dissertation","status":"public"},{"status":"public","relation":"part_of_dissertation","id":"2816"},{"relation":"part_of_dissertation","id":"2247","status":"public"},{"id":"3260","relation":"part_of_dissertation","status":"public"},{"id":"3157","relation":"part_of_dissertation","status":"public"}]},"page":"183"},{"citation":{"ama":"Sharmanska V. Learning with attributes for object recognition: Parametric and non-parametrics views. 2015. doi:<a href=\"https://doi.org/10.15479/at:ista:1401\">10.15479/at:ista:1401</a>","short":"V. Sharmanska, Learning with Attributes for Object Recognition: Parametric and Non-Parametrics Views, Institute of Science and Technology Austria, 2015.","apa":"Sharmanska, V. (2015). <i>Learning with attributes for object recognition: Parametric and non-parametrics views</i>. Institute of Science and Technology Austria. <a href=\"https://doi.org/10.15479/at:ista:1401\">https://doi.org/10.15479/at:ista:1401</a>","chicago":"Sharmanska, Viktoriia. “Learning with Attributes for Object Recognition: Parametric and Non-Parametrics Views.” Institute of Science and Technology Austria, 2015. <a href=\"https://doi.org/10.15479/at:ista:1401\">https://doi.org/10.15479/at:ista:1401</a>.","ieee":"V. Sharmanska, “Learning with attributes for object recognition: Parametric and non-parametrics views,” Institute of Science and Technology Austria, 2015.","mla":"Sharmanska, Viktoriia. <i>Learning with Attributes for Object Recognition: Parametric and Non-Parametrics Views</i>. Institute of Science and Technology Austria, 2015, doi:<a href=\"https://doi.org/10.15479/at:ista:1401\">10.15479/at:ista:1401</a>.","ista":"Sharmanska V. 2015. Learning with attributes for object recognition: Parametric and non-parametrics views. Institute of Science and Technology Austria."},"type":"dissertation","department":[{"_id":"ChLa"},{"_id":"GradSch"}],"supervisor":[{"last_name":"Lampert","orcid":"0000-0001-8622-7887","full_name":"Lampert, Christoph","first_name":"Christoph","id":"40C20FD2-F248-11E8-B48F-1D18A9856A87"}],"publisher":"Institute of Science and Technology Austria","date_created":"2018-12-11T11:51:48Z","file":[{"file_id":"9177","date_updated":"2021-02-22T11:33:17Z","creator":"dernst","success":1,"access_level":"open_access","content_type":"application/pdf","date_created":"2021-02-22T11:33:17Z","file_size":7964342,"relation":"main_file","checksum":"3605b402bb6934e09ae4cf672c84baf7","file_name":"2015_Thesis_Sharmanska.pdf"},{"file_id":"10297","creator":"cchlebak","date_updated":"2021-11-17T13:47:24Z","access_level":"closed","content_type":"application/pdf","date_created":"2021-11-16T14:40:45Z","file_size":7372241,"checksum":"e37593b3ee75bf3180629df2d6ca8f4e","relation":"main_file","file_name":"2015_Thesis_Sharmanska_pdfa.pdf"}],"language":[{"iso":"eng"}],"file_date_updated":"2021-11-17T13:47:24Z","doi":"10.15479/at:ista:1401","date_published":"2015-04-01T00:00:00Z","oa":1,"day":"01","publication_status":"published","alternative_title":["ISTA Thesis"],"main_file_link":[{"url":"http://users.sussex.ac.uk/~nq28/viktoriia/Thesis_Sharmanska.pdf"}],"page":"144","abstract":[{"lang":"eng","text":"The human ability to recognize objects in complex scenes has driven research in the computer vision field over couple of decades. This thesis focuses on the object recognition task in images. That is, given the image, we want the computer system to be able to predict the class of the object that appears in the image. A recent successful attempt to bridge semantic understanding of the image perceived by humans and by computers uses attribute-based models. Attributes are semantic properties of the objects shared across different categories, which humans and computers can decide on. To explore the attribute-based models we take a statistical machine learning approach, and address two key learning challenges in view of object recognition task: learning augmented attributes as mid-level discriminative feature representation, and learning with attributes as privileged information. Our main contributions are parametric and non-parametric models and algorithms to solve these frameworks. In the parametric approach, we explore an autoencoder model combined with the large margin nearest neighbor principle for mid-level feature learning, and linear support vector machines for learning with privileged information. In the non-parametric approach, we propose a supervised Indian Buffet Process for automatic augmentation of semantic attributes, and explore the Gaussian Processes classification framework for learning with privileged information. A thorough experimental analysis shows the effectiveness of the proposed models in both parametric and non-parametric views."}],"date_updated":"2024-10-09T20:56:17Z","author":[{"full_name":"Sharmanska, Viktoriia","first_name":"Viktoriia","id":"2EA6D09E-F248-11E8-B48F-1D18A9856A87","last_name":"Sharmanska","orcid":"0000-0003-0192-9308"}],"article_processing_charge":"No","year":"2015","has_accepted_license":"1","oa_version":"Published Version","corr_author":"1","publication_identifier":{"issn":["2663-337X"]},"status":"public","title":"Learning with attributes for object recognition: Parametric and non-parametrics views","_id":"1401","acknowledgement":"I would like to thank my supervisor, Christoph Lampert, for guidance throughout my studies and for patience in transforming me into a scientist, and my thesis committee, Chris Wojtan and Horst Bischof, for their help and advice. \r\n\r\nI would like to thank Elisabeth Hacker who perfectly assisted all my administrative needs and was always nice and friendly to me, and the campus team for making the IST Austria campus my second home. \r\nI was honored to collaborate with brilliant researchers and to learn from their experience. Undoubtedly, I learned most of all from Novi Quadrianto: brainstorming our projects and getting exciting results was the most enjoyable part of my work – thank you! I am also grateful to David Knowles, Zoubin Ghahramani, Daniel Hernández-Lobato, Kristian Kersting and Anastasia Pentina for the fantastic projects we worked on together, and to Kristen Grauman and Adriana Kovashka for the exceptional experience working with user studies. I would like to thank my colleagues at IST Austria and my office mates who shared their happy moods, scientific breakthroughs and thought-provoking conversations with me: Chao, Filip, Rustem, Asya, Sameh, Alex, Vlad, Mayu, Neel, Csaba, Thomas, Vladimir, Cristina, Alex Z., Avro, Amelie and Emilie, Andreas H. and Andreas E., Chris, Lena, Michael, Ali and Ipek, Vera, Igor, Katia. Special thanks to Morten for the countless games of table soccer we played together and the tournaments we teamed up for: we will definitely win next time:) A very warm hug to Asya for always being so inspiring and supportive to me, and for helping me to increase the proportion of female computer scientists in our group. ","user_id":"c635000d-4b10-11ee-a964-aac5a93f6ac1","degree_awarded":"PhD","publist_id":"5806","ddc":["000"],"month":"04"},{"intvolume":"       350","publisher":"American Association for the Advancement of Science","type":"journal_article","citation":{"chicago":"Kraus, P. M., B. Mignolet, Denitsa Rangelova Baykusheva, A. Rupenyan, L. Horný, E. F. Penka, G. Grassi, et al. “Measurement and Laser Control of Attosecond Charge Migration in Ionized Iodoacetylene.” <i>Science</i>. American Association for the Advancement of Science, 2015. <a href=\"https://doi.org/10.1126/science.aab2160\">https://doi.org/10.1126/science.aab2160</a>.","ieee":"P. M. Kraus <i>et al.</i>, “Measurement and laser control of attosecond charge migration in ionized iodoacetylene,” <i>Science</i>, vol. 350, no. 6262. American Association for the Advancement of Science, pp. 790–795, 2015.","mla":"Kraus, P. M., et al. “Measurement and Laser Control of Attosecond Charge Migration in Ionized Iodoacetylene.” <i>Science</i>, vol. 350, no. 6262, American Association for the Advancement of Science, 2015, pp. 790–95, doi:<a href=\"https://doi.org/10.1126/science.aab2160\">10.1126/science.aab2160</a>.","ista":"Kraus PM, Mignolet B, Baykusheva DR, Rupenyan A, Horný L, Penka EF, Grassi G, Tolstikhin OI, Schneider J, Jensen F, Madsen LB, Bandrauk AD, Remacle F, Wörner HJ. 2015. Measurement and laser control of attosecond charge migration in ionized iodoacetylene. Science. 350(6262), 790–795.","apa":"Kraus, P. M., Mignolet, B., Baykusheva, D. R., Rupenyan, A., Horný, L., Penka, E. F., … Wörner, H. J. (2015). Measurement and laser control of attosecond charge migration in ionized iodoacetylene. <i>Science</i>. American Association for the Advancement of Science. <a href=\"https://doi.org/10.1126/science.aab2160\">https://doi.org/10.1126/science.aab2160</a>","ama":"Kraus PM, Mignolet B, Baykusheva DR, et al. Measurement and laser control of attosecond charge migration in ionized iodoacetylene. <i>Science</i>. 2015;350(6262):790-795. doi:<a href=\"https://doi.org/10.1126/science.aab2160\">10.1126/science.aab2160</a>","short":"P.M. Kraus, B. Mignolet, D.R. Baykusheva, A. Rupenyan, L. Horný, E.F. Penka, G. Grassi, O.I. Tolstikhin, J. Schneider, F. Jensen, L.B. Madsen, A.D. Bandrauk, F. Remacle, H.J. Wörner, Science 350 (2015) 790–795."},"date_created":"2023-08-10T06:37:35Z","date_published":"2015-10-22T00:00:00Z","doi":"10.1126/science.aab2160","publication":"Science","language":[{"iso":"eng"}],"publication_status":"published","day":"22","oa_version":"None","pmid":1,"author":[{"last_name":"Kraus","full_name":"Kraus, P. M.","first_name":"P. M."},{"last_name":"Mignolet","full_name":"Mignolet, B.","first_name":"B."},{"id":"71b4d059-2a03-11ee-914d-dfa3beed6530","full_name":"Baykusheva, Denitsa Rangelova","first_name":"Denitsa Rangelova","last_name":"Baykusheva"},{"first_name":"A.","full_name":"Rupenyan, A.","last_name":"Rupenyan"},{"last_name":"Horný","first_name":"L.","full_name":"Horný, L."},{"last_name":"Penka","full_name":"Penka, E. F.","first_name":"E. F."},{"last_name":"Grassi","full_name":"Grassi, G.","first_name":"G."},{"full_name":"Tolstikhin, O. I.","first_name":"O. I.","last_name":"Tolstikhin"},{"last_name":"Schneider","full_name":"Schneider, J.","first_name":"J."},{"last_name":"Jensen","first_name":"F.","full_name":"Jensen, F."},{"last_name":"Madsen","full_name":"Madsen, L. B.","first_name":"L. B."},{"full_name":"Bandrauk, A. D.","first_name":"A. D.","last_name":"Bandrauk"},{"last_name":"Remacle","first_name":"F.","full_name":"Remacle, F."},{"last_name":"Wörner","full_name":"Wörner, H. J.","first_name":"H. J."}],"article_processing_charge":"No","year":"2015","abstract":[{"text":"The ultrafast motion of electrons and holes after light-matter interaction is fundamental to a broad range of chemical and biophysical processes. We advanced high-harmonic spectroscopy to resolve spatially and temporally the migration of an electron hole immediately after ionization of iodoacetylene while simultaneously demonstrating extensive control over the process. A multidimensional approach, based on the measurement and accurate theoretical description of both even and odd harmonic orders, enabled us to reconstruct both quantum amplitudes and phases of the electronic states with a resolution of ~100 attoseconds. We separately reconstructed quasi-field-free and laser-controlled charge migration as a function of the spatial orientation of the molecule and determined the shape of the hole created by ionization. Our technique opens the prospect of laser control over electronic primary processes.","lang":"eng"}],"date_updated":"2023-08-22T08:47:39Z","article_type":"original","page":"790-795","scopus_import":"1","issue":"6262","keyword":["Multidisciplinary"],"publication_identifier":{"issn":["0036-8075"],"eissn":["1095-9203"]},"external_id":{"pmid":["26494175"]},"extern":"1","user_id":"2DF688A6-F248-11E8-B48F-1D18A9856A87","_id":"14013","volume":350,"title":"Measurement and laser control of attosecond charge migration in ionized iodoacetylene","status":"public","month":"10","quality_controlled":"1"},{"quality_controlled":"1","month":"11","title":"Resolving the dynamics of valence-shell electrons and nuclei through laser-induced diffraction and holography","volume":635,"status":"public","user_id":"2DF688A6-F248-11E8-B48F-1D18A9856A87","_id":"14014","extern":"1","scopus_import":"1","issue":"11","keyword":["General Physics and Astronomy"],"publication_identifier":{"issn":["1742-6588"],"eissn":["1742-6596"]},"article_type":"original","main_file_link":[{"url":"https://doi.org/10.1088/1742-6596/635/11/112135","open_access":"1"}],"oa_version":"Published Version","abstract":[{"lang":"eng","text":"We have studied a coupled electronic-nuclear wave packet in nitric oxide using time-resolved strong-field photoelectron holography and rescattering. We show that the electronic dynamics mainly appears in the holographic structures whereas nuclear motion strongly modulates the angular distribution of the rescattered photoelectrons."}],"date_updated":"2023-08-22T08:51:33Z","year":"2015","article_processing_charge":"No","author":[{"full_name":"Walt, Samuel G","first_name":"Samuel G","last_name":"Walt"},{"full_name":"Ram, N Bhargava","first_name":"N Bhargava","last_name":"Ram"},{"last_name":"von Conta","full_name":"von Conta, Aaron","first_name":"Aaron"},{"last_name":"Baykusheva","full_name":"Baykusheva, Denitsa Rangelova","first_name":"Denitsa Rangelova","id":"71b4d059-2a03-11ee-914d-dfa3beed6530"},{"full_name":"Atala, Marcos","first_name":"Marcos","last_name":"Atala"},{"first_name":"Hans Jakob","full_name":"Wörner, Hans Jakob","last_name":"Wörner"}],"day":"01","article_number":"112135","publication_status":"published","publication":"Journal of Physics: Conference Series","language":[{"iso":"eng"}],"doi":"10.1088/1742-6596/635/11/112135","date_published":"2015-11-01T00:00:00Z","oa":1,"date_created":"2023-08-10T06:37:44Z","citation":{"chicago":"Walt, Samuel G, N Bhargava Ram, Aaron von Conta, Denitsa Rangelova Baykusheva, Marcos Atala, and Hans Jakob Wörner. “Resolving the Dynamics of Valence-Shell Electrons and Nuclei through Laser-Induced Diffraction and Holography.” <i>Journal of Physics: Conference Series</i>. IOP Publishing, 2015. <a href=\"https://doi.org/10.1088/1742-6596/635/11/112135\">https://doi.org/10.1088/1742-6596/635/11/112135</a>.","ieee":"S. G. Walt, N. B. Ram, A. von Conta, D. R. Baykusheva, M. Atala, and H. J. Wörner, “Resolving the dynamics of valence-shell electrons and nuclei through laser-induced diffraction and holography,” <i>Journal of Physics: Conference Series</i>, vol. 635, no. 11. IOP Publishing, 2015.","mla":"Walt, Samuel G., et al. “Resolving the Dynamics of Valence-Shell Electrons and Nuclei through Laser-Induced Diffraction and Holography.” <i>Journal of Physics: Conference Series</i>, vol. 635, no. 11, 112135, IOP Publishing, 2015, doi:<a href=\"https://doi.org/10.1088/1742-6596/635/11/112135\">10.1088/1742-6596/635/11/112135</a>.","ista":"Walt SG, Ram NB, von Conta A, Baykusheva DR, Atala M, Wörner HJ. 2015. Resolving the dynamics of valence-shell electrons and nuclei through laser-induced diffraction and holography. Journal of Physics: Conference Series. 635(11), 112135.","apa":"Walt, S. G., Ram, N. B., von Conta, A., Baykusheva, D. R., Atala, M., &#38; Wörner, H. J. (2015). Resolving the dynamics of valence-shell electrons and nuclei through laser-induced diffraction and holography. <i>Journal of Physics: Conference Series</i>. IOP Publishing. <a href=\"https://doi.org/10.1088/1742-6596/635/11/112135\">https://doi.org/10.1088/1742-6596/635/11/112135</a>","ama":"Walt SG, Ram NB, von Conta A, Baykusheva DR, Atala M, Wörner HJ. Resolving the dynamics of valence-shell electrons and nuclei through laser-induced diffraction and holography. <i>Journal of Physics: Conference Series</i>. 2015;635(11). doi:<a href=\"https://doi.org/10.1088/1742-6596/635/11/112135\">10.1088/1742-6596/635/11/112135</a>","short":"S.G. Walt, N.B. Ram, A. von Conta, D.R. Baykusheva, M. Atala, H.J. Wörner, Journal of Physics: Conference Series 635 (2015)."},"publisher":"IOP Publishing","intvolume":"       635","type":"journal_article"},{"date_created":"2023-08-10T06:37:53Z","type":"journal_article","publisher":"IOP Publishing","intvolume":"       635","citation":{"ieee":"P. M. Kraus <i>et al.</i>, “Attosecond charge migration and its laser control,” <i>Journal of Physics: Conference Series</i>, vol. 635, no. 11. IOP Publishing, 2015.","chicago":"Kraus, P M, B Mignolet, Denitsa Rangelova Baykusheva, A Rupenyan, L Horný, E F Penka, O I Tolstikhin, et al. “Attosecond Charge Migration and Its Laser Control.” <i>Journal of Physics: Conference Series</i>. IOP Publishing, 2015. <a href=\"https://doi.org/10.1088/1742-6596/635/11/112136\">https://doi.org/10.1088/1742-6596/635/11/112136</a>.","mla":"Kraus, P. M., et al. “Attosecond Charge Migration and Its Laser Control.” <i>Journal of Physics: Conference Series</i>, vol. 635, no. 11, 112136, IOP Publishing, 2015, doi:<a href=\"https://doi.org/10.1088/1742-6596/635/11/112136\">10.1088/1742-6596/635/11/112136</a>.","ista":"Kraus PM, Mignolet B, Baykusheva DR, Rupenyan A, Horný L, Penka EF, Tolstikhin OI, Schneider J, Jensen F, Madsen LB, Bandrauk AD, Remacle F, Wörner HJ. 2015. Attosecond charge migration and its laser control. Journal of Physics: Conference Series. 635(11), 112136.","apa":"Kraus, P. M., Mignolet, B., Baykusheva, D. R., Rupenyan, A., Horný, L., Penka, E. F., … Wörner, H. J. (2015). Attosecond charge migration and its laser control. <i>Journal of Physics: Conference Series</i>. IOP Publishing. <a href=\"https://doi.org/10.1088/1742-6596/635/11/112136\">https://doi.org/10.1088/1742-6596/635/11/112136</a>","ama":"Kraus PM, Mignolet B, Baykusheva DR, et al. Attosecond charge migration and its laser control. <i>Journal of Physics: Conference Series</i>. 2015;635(11). doi:<a href=\"https://doi.org/10.1088/1742-6596/635/11/112136\">10.1088/1742-6596/635/11/112136</a>","short":"P.M. Kraus, B. Mignolet, D.R. Baykusheva, A. Rupenyan, L. Horný, E.F. Penka, O.I. Tolstikhin, J. Schneider, F. Jensen, L.B. Madsen, A.D. Bandrauk, F. Remacle, H.J. Wörner, Journal of Physics: Conference Series 635 (2015)."},"publication_status":"published","article_number":"112136","day":"01","doi":"10.1088/1742-6596/635/11/112136","date_published":"2015-07-01T00:00:00Z","oa":1,"language":[{"iso":"eng"}],"publication":"Journal of Physics: Conference Series","keyword":["General Physics and Astronomy"],"publication_identifier":{"eissn":["1742-6596"],"issn":["1742-6588"]},"scopus_import":"1","issue":"11","extern":"1","date_updated":"2023-08-22T08:49:14Z","abstract":[{"text":"We advance high-harmonic spectroscopy to resolve molecular charge migration in time and space and simultaneously demonstrate extensive control over the process. A multidimensional approach enables us to reconstruct both quantum amplitudes and phases with a resolution of better than 100 attoseconds and to separately reconstruct field-free and laser- driven charge migration. Our techniques make charge migration in molecules measurable on the attosecond time scale and open new avenues for laser control of electronic primary processes.","lang":"eng"}],"year":"2015","article_processing_charge":"No","author":[{"last_name":"Kraus","full_name":"Kraus, P M","first_name":"P M"},{"last_name":"Mignolet","first_name":"B","full_name":"Mignolet, B"},{"last_name":"Baykusheva","full_name":"Baykusheva, Denitsa Rangelova","first_name":"Denitsa Rangelova","id":"71b4d059-2a03-11ee-914d-dfa3beed6530"},{"last_name":"Rupenyan","first_name":"A","full_name":"Rupenyan, A"},{"last_name":"Horný","first_name":"L","full_name":"Horný, L"},{"last_name":"Penka","first_name":"E F","full_name":"Penka, E F"},{"last_name":"Tolstikhin","first_name":"O I","full_name":"Tolstikhin, O I"},{"first_name":"J","full_name":"Schneider, J","last_name":"Schneider"},{"full_name":"Jensen, F","first_name":"F","last_name":"Jensen"},{"first_name":"L B","full_name":"Madsen, L B","last_name":"Madsen"},{"first_name":"A D","full_name":"Bandrauk, A D","last_name":"Bandrauk"},{"last_name":"Remacle","full_name":"Remacle, F","first_name":"F"},{"last_name":"Wörner","first_name":"H J","full_name":"Wörner, H J"}],"oa_version":"Published Version","main_file_link":[{"open_access":"1","url":"https://doi.org/10.1088/1742-6596/635/11/112136"}],"article_type":"original","quality_controlled":"1","month":"07","_id":"14015","user_id":"2DF688A6-F248-11E8-B48F-1D18A9856A87","status":"public","title":"Attosecond charge migration and its laser control","volume":635},{"publication":"Nature Communications","language":[{"iso":"eng"}],"doi":"10.1038/ncomms8039","date_published":"2015-05-05T00:00:00Z","oa":1,"day":"05","article_number":"7039","publication_status":"published","citation":{"apa":"Kraus, P. M., Tolstikhin, O. I., Baykusheva, D. R., Rupenyan, A., Schneider, J., Bisgaard, C. Z., … Wörner, H. J. (2015). Observation of laser-induced electronic structure in oriented polyatomic molecules. <i>Nature Communications</i>. Springer Nature. <a href=\"https://doi.org/10.1038/ncomms8039\">https://doi.org/10.1038/ncomms8039</a>","short":"P.M. Kraus, O.I. Tolstikhin, D.R. Baykusheva, A. Rupenyan, J. Schneider, C.Z. Bisgaard, T. Morishita, F. Jensen, L.B. Madsen, H.J. Wörner, Nature Communications 6 (2015).","ama":"Kraus PM, Tolstikhin OI, Baykusheva DR, et al. Observation of laser-induced electronic structure in oriented polyatomic molecules. <i>Nature Communications</i>. 2015;6. doi:<a href=\"https://doi.org/10.1038/ncomms8039\">10.1038/ncomms8039</a>","mla":"Kraus, P. M., et al. “Observation of Laser-Induced Electronic Structure in Oriented Polyatomic Molecules.” <i>Nature Communications</i>, vol. 6, 7039, Springer Nature, 2015, doi:<a href=\"https://doi.org/10.1038/ncomms8039\">10.1038/ncomms8039</a>.","ista":"Kraus PM, Tolstikhin OI, Baykusheva DR, Rupenyan A, Schneider J, Bisgaard CZ, Morishita T, Jensen F, Madsen LB, Wörner HJ. 2015. Observation of laser-induced electronic structure in oriented polyatomic molecules. Nature Communications. 6, 7039.","chicago":"Kraus, P. M., O. I. Tolstikhin, Denitsa Rangelova Baykusheva, A. Rupenyan, J. Schneider, C. Z. Bisgaard, T. Morishita, F. Jensen, L. B. Madsen, and H. J. Wörner. “Observation of Laser-Induced Electronic Structure in Oriented Polyatomic Molecules.” <i>Nature Communications</i>. Springer Nature, 2015. <a href=\"https://doi.org/10.1038/ncomms8039\">https://doi.org/10.1038/ncomms8039</a>.","ieee":"P. M. Kraus <i>et al.</i>, “Observation of laser-induced electronic structure in oriented polyatomic molecules,” <i>Nature Communications</i>, vol. 6. Springer Nature, 2015."},"publisher":"Springer Nature","intvolume":"         6","type":"journal_article","date_created":"2023-08-10T06:38:01Z","title":"Observation of laser-induced electronic structure in oriented polyatomic molecules","volume":6,"status":"public","user_id":"2DF688A6-F248-11E8-B48F-1D18A9856A87","_id":"14016","quality_controlled":"1","month":"05","article_type":"original","main_file_link":[{"open_access":"1","url":"https://doi.org/10.1038/ncomms8039"}],"pmid":1,"oa_version":"Published Version","abstract":[{"text":"All attosecond time-resolved measurements have so far relied on the use of intense near-infrared laser pulses. In particular, attosecond streaking, laser-induced electron diffraction and high-harmonic generation all make use of non-perturbative light–matter interactions. Remarkably, the effect of the strong laser field on the studied sample has often been neglected in previous studies. Here we use high-harmonic spectroscopy to measure laser-induced modifications of the electronic structure of molecules. We study high-harmonic spectra of spatially oriented CH3F and CH3Br as generic examples of polar polyatomic molecules. We accurately measure intensity ratios of even and odd-harmonic orders, and of the emission from aligned and unaligned molecules. We show that these robust observables reveal a substantial modification of the molecular electronic structure by the external laser field. Our insights offer new challenges and opportunities for a range of emerging strong-field attosecond spectroscopies.","lang":"eng"}],"date_updated":"2023-08-22T08:52:56Z","author":[{"first_name":"P. M.","full_name":"Kraus, P. M.","last_name":"Kraus"},{"full_name":"Tolstikhin, O. I.","first_name":"O. I.","last_name":"Tolstikhin"},{"last_name":"Baykusheva","first_name":"Denitsa Rangelova","full_name":"Baykusheva, Denitsa Rangelova","id":"71b4d059-2a03-11ee-914d-dfa3beed6530"},{"last_name":"Rupenyan","first_name":"A.","full_name":"Rupenyan, A."},{"first_name":"J.","full_name":"Schneider, J.","last_name":"Schneider"},{"last_name":"Bisgaard","first_name":"C. Z.","full_name":"Bisgaard, C. Z."},{"full_name":"Morishita, T.","first_name":"T.","last_name":"Morishita"},{"last_name":"Jensen","full_name":"Jensen, F.","first_name":"F."},{"first_name":"L. B.","full_name":"Madsen, L. B.","last_name":"Madsen"},{"first_name":"H. J.","full_name":"Wörner, H. J.","last_name":"Wörner"}],"year":"2015","article_processing_charge":"No","external_id":{"pmid":["25940229"]},"extern":"1","scopus_import":"1","publication_identifier":{"eissn":["2041-1723"]},"keyword":["General Physics and Astronomy","General Biochemistry","Genetics and Molecular Biology","General Chemistry","Multidisciplinary"]},{"scopus_import":"1","issue":"2","publication_identifier":{"eissn":["1094-1622"],"issn":["1050-2947"]},"keyword":["Atomic and Molecular Physics","and Optics"],"extern":"1","external_id":{"arxiv":["1504.03933"]},"oa_version":"Preprint","arxiv":1,"author":[{"last_name":"Zhang","full_name":"Zhang, Song Bin","first_name":"Song Bin"},{"full_name":"Baykusheva, Denitsa Rangelova","first_name":"Denitsa Rangelova","id":"71b4d059-2a03-11ee-914d-dfa3beed6530","last_name":"Baykusheva"},{"first_name":"Peter M.","full_name":"Kraus, Peter M.","last_name":"Kraus"},{"first_name":"Hans Jakob","full_name":"Wörner, Hans Jakob","last_name":"Wörner"},{"last_name":"Rohringer","full_name":"Rohringer, Nina","first_name":"Nina"}],"article_processing_charge":"No","year":"2015","abstract":[{"text":"The detection of electron motion and electronic wave-packet dynamics is one of the core goals of attosecond science. Recently, choosing the nitric oxide molecule as an example, we have introduced and demonstrated an experimental approach to measure coupled valence electronic and rotational wave packets using high-order-harmonic-generation (HHG) spectroscopy [Kraus et al., Phys. Rev. Lett. 111, 243005 (2013)]. A short outline of the theory to describe the combination of the pump and HHG probe process was published together with an extensive discussion of experimental results [Baykusheva et al., Faraday Discuss. 171, 113 (2014)]. The comparison of theory and experiment showed good agreement on a quantitative level. Here, we present the theory in detail, which is based on a generalized density-matrix approach that describes the pump process and the subsequent probing of the wave packets by a semiclassical quantitative rescattering approach. An in-depth analysis of the different Raman scattering contributions to the creation of the coupled rotational and electronic spin-orbit wave packets is made. We present results for parallel and perpendicular linear polarizations of the pump and probe laser pulses. Furthermore, an analysis of the combined rotational-electronic density matrix in terms of irreducible components is presented that facilitates interpretation of the results.","lang":"eng"}],"date_updated":"2023-08-22T08:56:34Z","article_type":"original","main_file_link":[{"open_access":"1","url":"https://arxiv.org/abs/1504.03933"}],"month":"02","quality_controlled":"1","user_id":"2DF688A6-F248-11E8-B48F-1D18A9856A87","_id":"14017","volume":91,"title":"Theoretical study of molecular electronic and rotational coherences by high-order-harmonic generation","status":"public","date_created":"2023-08-10T06:38:10Z","intvolume":"        91","publisher":"American Physical Society","type":"journal_article","citation":{"mla":"Zhang, Song Bin, et al. “Theoretical Study of Molecular Electronic and Rotational Coherences by High-Order-Harmonic Generation.” <i>Physical Review A</i>, vol. 91, no. 2, 023421, American Physical Society, 2015, doi:<a href=\"https://doi.org/10.1103/physreva.91.023421\">10.1103/physreva.91.023421</a>.","ista":"Zhang SB, Baykusheva DR, Kraus PM, Wörner HJ, Rohringer N. 2015. Theoretical study of molecular electronic and rotational coherences by high-order-harmonic generation. Physical Review A. 91(2), 023421.","ieee":"S. B. Zhang, D. R. Baykusheva, P. M. Kraus, H. J. Wörner, and N. Rohringer, “Theoretical study of molecular electronic and rotational coherences by high-order-harmonic generation,” <i>Physical Review A</i>, vol. 91, no. 2. American Physical Society, 2015.","chicago":"Zhang, Song Bin, Denitsa Rangelova Baykusheva, Peter M. Kraus, Hans Jakob Wörner, and Nina Rohringer. “Theoretical Study of Molecular Electronic and Rotational Coherences by High-Order-Harmonic Generation.” <i>Physical Review A</i>. American Physical Society, 2015. <a href=\"https://doi.org/10.1103/physreva.91.023421\">https://doi.org/10.1103/physreva.91.023421</a>.","apa":"Zhang, S. B., Baykusheva, D. R., Kraus, P. M., Wörner, H. J., &#38; Rohringer, N. (2015). Theoretical study of molecular electronic and rotational coherences by high-order-harmonic generation. <i>Physical Review A</i>. American Physical Society. <a href=\"https://doi.org/10.1103/physreva.91.023421\">https://doi.org/10.1103/physreva.91.023421</a>","short":"S.B. Zhang, D.R. Baykusheva, P.M. Kraus, H.J. Wörner, N. Rohringer, Physical Review A 91 (2015).","ama":"Zhang SB, Baykusheva DR, Kraus PM, Wörner HJ, Rohringer N. Theoretical study of molecular electronic and rotational coherences by high-order-harmonic generation. <i>Physical Review A</i>. 2015;91(2). doi:<a href=\"https://doi.org/10.1103/physreva.91.023421\">10.1103/physreva.91.023421</a>"},"article_number":"023421","publication_status":"published","day":"19","date_published":"2015-02-19T00:00:00Z","oa":1,"doi":"10.1103/physreva.91.023421","publication":"Physical Review A","language":[{"iso":"eng"}]},{"date_created":"2018-12-11T11:51:56Z","citation":{"mla":"Kwitt, Roland, et al. <i>Statistical Topological Data Analysis-A Kernel Perspective</i>. Vol. 28, Neural Information Processing Systems Foundation, 2015, pp. 3070–78.","ista":"Kwitt R, Huber S, Niethammer M, Lin W, Bauer U. 2015. Statistical topological data analysis-A kernel perspective. NIPS: Neural Information Processing Systems, Advances in Neural Information Processing Systems, vol. 28, 3070–3078.","chicago":"Kwitt, Roland, Stefan Huber, Marc Niethammer, Weili Lin, and Ulrich Bauer. “Statistical Topological Data Analysis-A Kernel Perspective,” 28:3070–78. Neural Information Processing Systems Foundation, 2015.","ieee":"R. Kwitt, S. Huber, M. Niethammer, W. Lin, and U. Bauer, “Statistical topological data analysis-A kernel perspective,” presented at the NIPS: Neural Information Processing Systems, Montreal, Canada, 2015, vol. 28, pp. 3070–3078.","apa":"Kwitt, R., Huber, S., Niethammer, M., Lin, W., &#38; Bauer, U. (2015). Statistical topological data analysis-A kernel perspective (Vol. 28, pp. 3070–3078). Presented at the NIPS: Neural Information Processing Systems, Montreal, Canada: Neural Information Processing Systems Foundation.","short":"R. Kwitt, S. Huber, M. Niethammer, W. Lin, U. Bauer, in:, Neural Information Processing Systems Foundation, 2015, pp. 3070–3078.","ama":"Kwitt R, Huber S, Niethammer M, Lin W, Bauer U. Statistical topological data analysis-A kernel perspective. In: Vol 28. Neural Information Processing Systems Foundation; 2015:3070-3078."},"main_file_link":[{"open_access":"1","url":"https://papers.nips.cc/paper/5887-statistical-topological-data-analysis-a-kernel-perspective"}],"page":"3070 - 3078","publisher":"Neural Information Processing Systems Foundation","intvolume":"        28","oa_version":"Submitted Version","type":"conference","date_updated":"2025-06-03T11:41:36Z","abstract":[{"lang":"eng","text":"We consider the problem of statistical computations with persistence diagrams, a summary representation of topological features in data. These diagrams encode persistent homology, a widely used invariant in topological data analysis. While several avenues towards a statistical treatment of the diagrams have been explored recently, we follow an alternative route that is motivated by the success of methods based on the embedding of probability measures into reproducing kernel Hilbert spaces. In fact, a positive definite kernel on persistence diagrams has recently been proposed, connecting persistent homology to popular kernel-based learning techniques such as support vector machines. However, important properties of that kernel enabling a principled use in the context of probability measure embeddings remain to be explored. Our contribution is to close this gap by proving universality of a variant of the original kernel, and to demonstrate its effective use in twosample hypothesis testing on synthetic as well as real-world data."}],"department":[{"_id":"HeEd"}],"article_processing_charge":"No","author":[{"full_name":"Kwitt, Roland","first_name":"Roland","last_name":"Kwitt"},{"orcid":"0000-0002-8871-5814","last_name":"Huber","id":"4700A070-F248-11E8-B48F-1D18A9856A87","first_name":"Stefan","full_name":"Huber, Stefan"},{"full_name":"Niethammer, Marc","first_name":"Marc","last_name":"Niethammer"},{"first_name":"Weili","full_name":"Lin, Weili","last_name":"Lin"},{"id":"2ADD483A-F248-11E8-B48F-1D18A9856A87","full_name":"Bauer, Ulrich","first_name":"Ulrich","orcid":"0000-0002-9683-0724","last_name":"Bauer"}],"year":"2015","day":"01","alternative_title":["Advances in Neural Information Processing Systems"],"quality_controlled":"1","month":"12","publication_status":"published","publist_id":"5782","title":"Statistical topological data analysis-A kernel perspective","volume":28,"status":"public","language":[{"iso":"eng"}],"acknowledgement":"This work was partially supported by the Austrian Science FUnd, project no. KLI 00012.","user_id":"2DF688A6-F248-11E8-B48F-1D18A9856A87","date_published":"2015-12-01T00:00:00Z","_id":"1424","oa":1,"conference":{"location":"Montreal, Canada","name":"NIPS: Neural Information Processing Systems","start_date":"2015-12-07","end_date":"2015-12-12"}},{"publication_status":"published","alternative_title":["Advances in Neural Information Processing Systems"],"day":"01","conference":{"start_date":"2015-12-07","end_date":"2015-12-12","location":"Montreal, Canada","name":"NIPS: Neural Information Processing Systems"},"oa":1,"date_published":"2015-01-01T00:00:00Z","language":[{"iso":"eng"}],"project":[{"call_identifier":"FP7","_id":"2532554C-B435-11E9-9278-68D0E5697425","grant_number":"308036","name":"Lifelong Learning of Visual Scene Understanding"}],"date_created":"2018-12-11T11:51:57Z","type":"conference","department":[{"_id":"ChLa"}],"publisher":"Neural Information Processing Systems Foundation","intvolume":"      2015","citation":{"short":"A. Pentina, C. Lampert, in:, Neural Information Processing Systems Foundation, 2015, pp. 1540–1548.","ama":"Pentina A, Lampert C. Lifelong learning with non-i.i.d. tasks. In: Vol 2015. Neural Information Processing Systems Foundation; 2015:1540-1548.","apa":"Pentina, A., &#38; Lampert, C. (2015). Lifelong learning with non-i.i.d. tasks (Vol. 2015, pp. 1540–1548). Presented at the NIPS: Neural Information Processing Systems, Montreal, Canada: Neural Information Processing Systems Foundation.","mla":"Pentina, Anastasia, and Christoph Lampert. <i>Lifelong Learning with Non-i.i.d. Tasks</i>. Vol. 2015, Neural Information Processing Systems Foundation, 2015, pp. 1540–48.","ista":"Pentina A, Lampert C. 2015. Lifelong learning with non-i.i.d. tasks. NIPS: Neural Information Processing Systems, Advances in Neural Information Processing Systems, vol. 2015, 1540–1548.","chicago":"Pentina, Anastasia, and Christoph Lampert. “Lifelong Learning with Non-i.i.d. Tasks,” 2015:1540–48. Neural Information Processing Systems Foundation, 2015.","ieee":"A. Pentina and C. Lampert, “Lifelong learning with non-i.i.d. tasks,” presented at the NIPS: Neural Information Processing Systems, Montreal, Canada, 2015, vol. 2015, pp. 1540–1548."},"publist_id":"5781","quality_controlled":"1","month":"01","_id":"1425","user_id":"2DF688A6-F248-11E8-B48F-1D18A9856A87","status":"public","title":"Lifelong learning with non-i.i.d. tasks","volume":2015,"scopus_import":"1","ec_funded":1,"date_updated":"2025-06-03T11:41:45Z","abstract":[{"text":"In this work we aim at extending the theoretical foundations of lifelong learning. Previous work analyzing this scenario is based on the assumption that learning tasks are sampled i.i.d. from a task environment or limited to strongly constrained data distributions. Instead, we study two scenarios when lifelong learning is possible, even though the observed tasks do not form an i.i.d. sample: first, when they are sampled from the same environment, but possibly with dependencies, and second, when the task environment is allowed to change over time in a consistent way. In the first case we prove a PAC-Bayesian theorem that can be seen as a direct generalization of the analogous previous result for the i.i.d. case. For the second scenario we propose to learn an inductive bias in form of a transfer procedure. We present a generalization bound and show on a toy example how it can be used to identify a beneficial transfer algorithm.","lang":"eng"}],"author":[{"last_name":"Pentina","first_name":"Anastasia","full_name":"Pentina, Anastasia","id":"42E87FC6-F248-11E8-B48F-1D18A9856A87"},{"full_name":"Lampert, Christoph","first_name":"Christoph","id":"40C20FD2-F248-11E8-B48F-1D18A9856A87","last_name":"Lampert","orcid":"0000-0001-8622-7887"}],"article_processing_charge":"No","year":"2015","oa_version":"None","main_file_link":[{"url":"http://papers.nips.cc/paper/6007-lifelong-learning-with-non-iid-tasks","open_access":"1"}],"page":"1540 - 1548"},{"date_created":"2018-12-11T11:51:58Z","citation":{"ama":"Paixao T, Sudholt D, Heredia J, Trubenova B. First steps towards a runtime comparison of natural and artificial evolution. In: <i>Proceedings of the 2015 Annual Conference on Genetic and Evolutionary Computation</i>. ACM; 2015:1455-1462. doi:<a href=\"https://doi.org/10.1145/2739480.2754758\">10.1145/2739480.2754758</a>","short":"T. Paixao, D. Sudholt, J. Heredia, B. Trubenova, in:, Proceedings of the 2015 Annual Conference on Genetic and Evolutionary Computation, ACM, 2015, pp. 1455–1462.","apa":"Paixao, T., Sudholt, D., Heredia, J., &#38; Trubenova, B. (2015). First steps towards a runtime comparison of natural and artificial evolution. In <i>Proceedings of the 2015 Annual Conference on Genetic and Evolutionary Computation</i> (pp. 1455–1462). Madrid, Spain: ACM. <a href=\"https://doi.org/10.1145/2739480.2754758\">https://doi.org/10.1145/2739480.2754758</a>","ieee":"T. Paixao, D. Sudholt, J. Heredia, and B. Trubenova, “First steps towards a runtime comparison of natural and artificial evolution,” in <i>Proceedings of the 2015 Annual Conference on Genetic and Evolutionary Computation</i>, Madrid, Spain, 2015, pp. 1455–1462.","chicago":"Paixao, Tiago, Dirk Sudholt, Jorge Heredia, and Barbora Trubenova. “First Steps towards a Runtime Comparison of Natural and Artificial Evolution.” In <i>Proceedings of the 2015 Annual Conference on Genetic and Evolutionary Computation</i>, 1455–62. ACM, 2015. <a href=\"https://doi.org/10.1145/2739480.2754758\">https://doi.org/10.1145/2739480.2754758</a>.","mla":"Paixao, Tiago, et al. “First Steps towards a Runtime Comparison of Natural and Artificial Evolution.” <i>Proceedings of the 2015 Annual Conference on Genetic and Evolutionary Computation</i>, ACM, 2015, pp. 1455–62, doi:<a href=\"https://doi.org/10.1145/2739480.2754758\">10.1145/2739480.2754758</a>.","ista":"Paixao T, Sudholt D, Heredia J, Trubenova B. 2015. First steps towards a runtime comparison of natural and artificial evolution. Proceedings of the 2015 Annual Conference on Genetic and Evolutionary Computation. GECCO: Genetic and evolutionary computation conference, 1455–1462."},"type":"conference","department":[{"_id":"NiBa"},{"_id":"CaGu"}],"isi":1,"publisher":"ACM","day":"11","publication_status":"published","language":[{"iso":"eng"}],"project":[{"grant_number":"618091","_id":"25B1EC9E-B435-11E9-9278-68D0E5697425","name":"Speed of Adaptation in Population Genetics and Evolutionary Computation","call_identifier":"FP7"}],"publication":"Proceedings of the 2015 Annual Conference on Genetic and Evolutionary Computation","date_published":"2015-07-11T00:00:00Z","conference":{"start_date":"2015-07-11","end_date":"2015-07-15","location":"Madrid, Spain","name":"GECCO: Genetic and evolutionary computation conference"},"oa":1,"doi":"10.1145/2739480.2754758","external_id":{"arxiv":["1504.06260"],"isi":["000358795700182"]},"scopus_import":"1","page":"1455 - 1462","main_file_link":[{"url":"http://arxiv.org/abs/1504.06260","open_access":"1"}],"year":"2015","author":[{"id":"2C5658E6-F248-11E8-B48F-1D18A9856A87","full_name":"Paixao, Tiago","first_name":"Tiago","orcid":"0000-0003-2361-3953","last_name":"Paixao"},{"first_name":"Dirk","full_name":"Sudholt, Dirk","last_name":"Sudholt"},{"first_name":"Jorge","full_name":"Heredia, Jorge","last_name":"Heredia"},{"full_name":"Trubenova, Barbora","first_name":"Barbora","id":"42302D54-F248-11E8-B48F-1D18A9856A87","orcid":"0000-0002-6873-2967","last_name":"Trubenova"}],"article_processing_charge":"No","date_updated":"2025-09-23T08:50:33Z","ec_funded":1,"abstract":[{"lang":"eng","text":"Evolutionary algorithms (EAs) form a popular optimisation paradigm inspired by natural evolution. In recent years the field of evolutionary computation has developed a rigorous analytical theory to analyse their runtime on many illustrative problems. Here we apply this theory to a simple model of natural evolution. In the Strong Selection Weak Mutation (SSWM) evolutionary regime the time between occurrence of new mutations is much longer than the time it takes for a new beneficial mutation to take over the population. In this situation, the population only contains copies of one genotype and evolution can be modelled as a (1+1)-type process where the probability of accepting a new genotype (improvements or worsenings) depends on the change in fitness. We present an initial runtime analysis of SSWM, quantifying its performance for various parameters and investigating differences to the (1+1) EA. We show that SSWM can have a moderate advantage over the (1+1) EA at crossing fitness valleys and study an example where SSWM outperforms the (1+1) EA by taking advantage of information on the fitness gradient."}],"arxiv":1,"oa_version":"Preprint","publist_id":"5768","month":"07","quality_controlled":"1","status":"public","title":"First steps towards a runtime comparison of natural and artificial evolution","_id":"1430","user_id":"317138e5-6ab7-11ef-aa6d-ffef3953e345"},{"title":"Efficient production of single-stranded phage DNA as scaffolds for DNA origami","volume":15,"status":"public","user_id":"2DF688A6-F248-11E8-B48F-1D18A9856A87","_id":"14303","quality_controlled":"1","month":"06","article_type":"letter_note","main_file_link":[{"open_access":"1","url":"https://doi.org/10.1021/acs.nanolett.5b01461"}],"page":"4672-4676","pmid":1,"oa_version":"Published Version","abstract":[{"lang":"eng","text":"Scaffolded DNA origami enables the fabrication of a variety of complex nanostructures that promise utility in diverse fields of application, ranging from biosensing over advanced therapeutics to metamaterials. The broad applicability of DNA origami as a material beyond the level of proof-of-concept studies critically depends, among other factors, on the availability of large amounts of pure single-stranded scaffold DNA. Here, we present a method for the efficient production of M13 bacteriophage-derived genomic DNA using high-cell-density fermentation of Escherichia coli in stirred-tank bioreactors. We achieve phage titers of up to 1.6 × 1014 plaque-forming units per mL. Downstream processing yields up to 410 mg of high-quality single-stranded DNA per one liter reaction volume, thus upgrading DNA origami-based nanotechnology from the milligram to the gram scale."}],"date_updated":"2023-11-07T11:56:32Z","author":[{"last_name":"Kick","first_name":"B","full_name":"Kick, B"},{"last_name":"Praetorius","id":"dfec9381-4341-11ee-8fd8-faa02bba7d62","full_name":"Praetorius, Florian M","first_name":"Florian M"},{"full_name":"Dietz, H","first_name":"H","last_name":"Dietz"},{"full_name":"Weuster-Botz, D","first_name":"D","last_name":"Weuster-Botz"}],"article_processing_charge":"No","year":"2015","extern":"1","external_id":{"pmid":["26028443"]},"issue":"7","publication_identifier":{"issn":["1530-6984"],"eissn":["1530-6992"]},"publication":"Nano Letters","language":[{"iso":"eng"}],"doi":"10.1021/acs.nanolett.5b01461","oa":1,"date_published":"2015-06-01T00:00:00Z","day":"01","publication_status":"published","citation":{"apa":"Kick, B., Praetorius, F. M., Dietz, H., &#38; Weuster-Botz, D. (2015). Efficient production of single-stranded phage DNA as scaffolds for DNA origami. <i>Nano Letters</i>. ACS Publications. <a href=\"https://doi.org/10.1021/acs.nanolett.5b01461\">https://doi.org/10.1021/acs.nanolett.5b01461</a>","short":"B. Kick, F.M. Praetorius, H. Dietz, D. Weuster-Botz, Nano Letters 15 (2015) 4672–4676.","ama":"Kick B, Praetorius FM, Dietz H, Weuster-Botz D. Efficient production of single-stranded phage DNA as scaffolds for DNA origami. <i>Nano Letters</i>. 2015;15(7):4672-4676. doi:<a href=\"https://doi.org/10.1021/acs.nanolett.5b01461\">10.1021/acs.nanolett.5b01461</a>","mla":"Kick, B., et al. “Efficient Production of Single-Stranded Phage DNA as Scaffolds for DNA Origami.” <i>Nano Letters</i>, vol. 15, no. 7, ACS Publications, 2015, pp. 4672–76, doi:<a href=\"https://doi.org/10.1021/acs.nanolett.5b01461\">10.1021/acs.nanolett.5b01461</a>.","ista":"Kick B, Praetorius FM, Dietz H, Weuster-Botz D. 2015. Efficient production of single-stranded phage DNA as scaffolds for DNA origami. Nano Letters. 15(7), 4672–4676.","ieee":"B. Kick, F. M. Praetorius, H. Dietz, and D. Weuster-Botz, “Efficient production of single-stranded phage DNA as scaffolds for DNA origami,” <i>Nano Letters</i>, vol. 15, no. 7. ACS Publications, pp. 4672–4676, 2015.","chicago":"Kick, B, Florian M Praetorius, H Dietz, and D Weuster-Botz. “Efficient Production of Single-Stranded Phage DNA as Scaffolds for DNA Origami.” <i>Nano Letters</i>. ACS Publications, 2015. <a href=\"https://doi.org/10.1021/acs.nanolett.5b01461\">https://doi.org/10.1021/acs.nanolett.5b01461</a>."},"publisher":"ACS Publications","intvolume":"        15","type":"journal_article","date_created":"2023-09-06T12:52:47Z"}]