---
_id: '14013'
abstract:
- lang: eng
text: The ultrafast motion of electrons and holes after light-matter interaction
is fundamental to a broad range of chemical and biophysical processes. We advanced
high-harmonic spectroscopy to resolve spatially and temporally the migration of
an electron hole immediately after ionization of iodoacetylene while simultaneously
demonstrating extensive control over the process. A multidimensional approach,
based on the measurement and accurate theoretical description of both even and
odd harmonic orders, enabled us to reconstruct both quantum amplitudes and phases
of the electronic states with a resolution of ~100 attoseconds. We separately
reconstructed quasi-field-free and laser-controlled charge migration as a function
of the spatial orientation of the molecule and determined the shape of the hole
created by ionization. Our technique opens the prospect of laser control over
electronic primary processes.
article_processing_charge: No
article_type: original
author:
- first_name: P. M.
full_name: Kraus, P. M.
last_name: Kraus
- first_name: B.
full_name: Mignolet, B.
last_name: Mignolet
- first_name: Denitsa Rangelova
full_name: Baykusheva, Denitsa Rangelova
id: 71b4d059-2a03-11ee-914d-dfa3beed6530
last_name: Baykusheva
- first_name: A.
full_name: Rupenyan, A.
last_name: Rupenyan
- first_name: L.
full_name: Horný, L.
last_name: Horný
- first_name: E. F.
full_name: Penka, E. F.
last_name: Penka
- first_name: G.
full_name: Grassi, G.
last_name: Grassi
- first_name: O. I.
full_name: Tolstikhin, O. I.
last_name: Tolstikhin
- first_name: J.
full_name: Schneider, J.
last_name: Schneider
- first_name: F.
full_name: Jensen, F.
last_name: Jensen
- first_name: L. B.
full_name: Madsen, L. B.
last_name: Madsen
- first_name: A. D.
full_name: Bandrauk, A. D.
last_name: Bandrauk
- first_name: F.
full_name: Remacle, F.
last_name: Remacle
- first_name: H. J.
full_name: Wörner, H. J.
last_name: Wörner
citation:
ama: Kraus PM, Mignolet B, Baykusheva DR, et al. Measurement and laser control of
attosecond charge migration in ionized iodoacetylene. Science. 2015;350(6262):790-795.
doi:10.1126/science.aab2160
apa: Kraus, P. M., Mignolet, B., Baykusheva, D. R., Rupenyan, A., Horný, L., Penka,
E. F., … Wörner, H. J. (2015). Measurement and laser control of attosecond charge
migration in ionized iodoacetylene. Science. American Association for the
Advancement of Science. https://doi.org/10.1126/science.aab2160
chicago: Kraus, P. M., B. Mignolet, Denitsa Rangelova Baykusheva, A. Rupenyan, L.
Horný, E. F. Penka, G. Grassi, et al. “Measurement and Laser Control of Attosecond
Charge Migration in Ionized Iodoacetylene.” Science. American Association
for the Advancement of Science, 2015. https://doi.org/10.1126/science.aab2160.
ieee: P. M. Kraus et al., “Measurement and laser control of attosecond charge
migration in ionized iodoacetylene,” Science, vol. 350, no. 6262. American
Association for the Advancement of Science, pp. 790–795, 2015.
ista: Kraus PM, Mignolet B, Baykusheva DR, Rupenyan A, Horný L, Penka EF, Grassi
G, Tolstikhin OI, Schneider J, Jensen F, Madsen LB, Bandrauk AD, Remacle F, Wörner
HJ. 2015. Measurement and laser control of attosecond charge migration in ionized
iodoacetylene. Science. 350(6262), 790–795.
mla: Kraus, P. M., et al. “Measurement and Laser Control of Attosecond Charge Migration
in Ionized Iodoacetylene.” Science, vol. 350, no. 6262, American Association
for the Advancement of Science, 2015, pp. 790–95, doi:10.1126/science.aab2160.
short: P.M. Kraus, B. Mignolet, D.R. Baykusheva, A. Rupenyan, L. Horný, E.F. Penka,
G. Grassi, O.I. Tolstikhin, J. Schneider, F. Jensen, L.B. Madsen, A.D. Bandrauk,
F. Remacle, H.J. Wörner, Science 350 (2015) 790–795.
date_created: 2023-08-10T06:37:35Z
date_published: 2015-10-22T00:00:00Z
date_updated: 2023-08-22T08:47:39Z
day: '22'
doi: 10.1126/science.aab2160
extern: '1'
external_id:
pmid:
- '26494175'
intvolume: ' 350'
issue: '6262'
keyword:
- Multidisciplinary
language:
- iso: eng
month: '10'
oa_version: None
page: 790-795
pmid: 1
publication: Science
publication_identifier:
eissn:
- 1095-9203
issn:
- 0036-8075
publication_status: published
publisher: American Association for the Advancement of Science
quality_controlled: '1'
scopus_import: '1'
status: public
title: Measurement and laser control of attosecond charge migration in ionized iodoacetylene
type: journal_article
user_id: 2DF688A6-F248-11E8-B48F-1D18A9856A87
volume: 350
year: '2015'
...
---
_id: '14014'
abstract:
- lang: eng
text: We have studied a coupled electronic-nuclear wave packet in nitric oxide using
time-resolved strong-field photoelectron holography and rescattering. We show
that the electronic dynamics mainly appears in the holographic structures whereas
nuclear motion strongly modulates the angular distribution of the rescattered
photoelectrons.
article_number: '112135'
article_processing_charge: No
article_type: original
author:
- first_name: Samuel G
full_name: Walt, Samuel G
last_name: Walt
- first_name: N Bhargava
full_name: Ram, N Bhargava
last_name: Ram
- first_name: Aaron
full_name: von Conta, Aaron
last_name: von Conta
- first_name: Denitsa Rangelova
full_name: Baykusheva, Denitsa Rangelova
id: 71b4d059-2a03-11ee-914d-dfa3beed6530
last_name: Baykusheva
- first_name: Marcos
full_name: Atala, Marcos
last_name: Atala
- first_name: Hans Jakob
full_name: Wörner, Hans Jakob
last_name: Wörner
citation:
ama: 'Walt SG, Ram NB, von Conta A, Baykusheva DR, Atala M, Wörner HJ. Resolving
the dynamics of valence-shell electrons and nuclei through laser-induced diffraction
and holography. Journal of Physics: Conference Series. 2015;635(11). doi:10.1088/1742-6596/635/11/112135'
apa: 'Walt, S. G., Ram, N. B., von Conta, A., Baykusheva, D. R., Atala, M., &
Wörner, H. J. (2015). Resolving the dynamics of valence-shell electrons and nuclei
through laser-induced diffraction and holography. Journal of Physics: Conference
Series. IOP Publishing. https://doi.org/10.1088/1742-6596/635/11/112135'
chicago: 'Walt, Samuel G, N Bhargava Ram, Aaron von Conta, Denitsa Rangelova Baykusheva,
Marcos Atala, and Hans Jakob Wörner. “Resolving the Dynamics of Valence-Shell
Electrons and Nuclei through Laser-Induced Diffraction and Holography.” Journal
of Physics: Conference Series. IOP Publishing, 2015. https://doi.org/10.1088/1742-6596/635/11/112135.'
ieee: 'S. G. Walt, N. B. Ram, A. von Conta, D. R. Baykusheva, M. Atala, and H. J.
Wörner, “Resolving the dynamics of valence-shell electrons and nuclei through
laser-induced diffraction and holography,” Journal of Physics: Conference Series,
vol. 635, no. 11. IOP Publishing, 2015.'
ista: 'Walt SG, Ram NB, von Conta A, Baykusheva DR, Atala M, Wörner HJ. 2015. Resolving
the dynamics of valence-shell electrons and nuclei through laser-induced diffraction
and holography. Journal of Physics: Conference Series. 635(11), 112135.'
mla: 'Walt, Samuel G., et al. “Resolving the Dynamics of Valence-Shell Electrons
and Nuclei through Laser-Induced Diffraction and Holography.” Journal of Physics:
Conference Series, vol. 635, no. 11, 112135, IOP Publishing, 2015, doi:10.1088/1742-6596/635/11/112135.'
short: 'S.G. Walt, N.B. Ram, A. von Conta, D.R. Baykusheva, M. Atala, H.J. Wörner,
Journal of Physics: Conference Series 635 (2015).'
date_created: 2023-08-10T06:37:44Z
date_published: 2015-11-01T00:00:00Z
date_updated: 2023-08-22T08:51:33Z
day: '01'
doi: 10.1088/1742-6596/635/11/112135
extern: '1'
intvolume: ' 635'
issue: '11'
keyword:
- General Physics and Astronomy
language:
- iso: eng
main_file_link:
- open_access: '1'
url: https://doi.org/10.1088/1742-6596/635/11/112135
month: '11'
oa: 1
oa_version: Published Version
publication: 'Journal of Physics: Conference Series'
publication_identifier:
eissn:
- 1742-6596
issn:
- 1742-6588
publication_status: published
publisher: IOP Publishing
quality_controlled: '1'
scopus_import: '1'
status: public
title: Resolving the dynamics of valence-shell electrons and nuclei through laser-induced
diffraction and holography
type: journal_article
user_id: 2DF688A6-F248-11E8-B48F-1D18A9856A87
volume: 635
year: '2015'
...
---
_id: '14015'
abstract:
- lang: eng
text: We advance high-harmonic spectroscopy to resolve molecular charge migration
in time and space and simultaneously demonstrate extensive control over the process.
A multidimensional approach enables us to reconstruct both quantum amplitudes
and phases with a resolution of better than 100 attoseconds and to separately
reconstruct field-free and laser- driven charge migration. Our techniques make
charge migration in molecules measurable on the attosecond time scale and open
new avenues for laser control of electronic primary processes.
article_number: '112136'
article_processing_charge: No
article_type: original
author:
- first_name: P M
full_name: Kraus, P M
last_name: Kraus
- first_name: B
full_name: Mignolet, B
last_name: Mignolet
- first_name: Denitsa Rangelova
full_name: Baykusheva, Denitsa Rangelova
id: 71b4d059-2a03-11ee-914d-dfa3beed6530
last_name: Baykusheva
- first_name: A
full_name: Rupenyan, A
last_name: Rupenyan
- first_name: L
full_name: Horný, L
last_name: Horný
- first_name: E F
full_name: Penka, E F
last_name: Penka
- first_name: O I
full_name: Tolstikhin, O I
last_name: Tolstikhin
- first_name: J
full_name: Schneider, J
last_name: Schneider
- first_name: F
full_name: Jensen, F
last_name: Jensen
- first_name: L B
full_name: Madsen, L B
last_name: Madsen
- first_name: A D
full_name: Bandrauk, A D
last_name: Bandrauk
- first_name: F
full_name: Remacle, F
last_name: Remacle
- first_name: H J
full_name: Wörner, H J
last_name: Wörner
citation:
ama: 'Kraus PM, Mignolet B, Baykusheva DR, et al. Attosecond charge migration and
its laser control. Journal of Physics: Conference Series. 2015;635(11).
doi:10.1088/1742-6596/635/11/112136'
apa: 'Kraus, P. M., Mignolet, B., Baykusheva, D. R., Rupenyan, A., Horný, L., Penka,
E. F., … Wörner, H. J. (2015). Attosecond charge migration and its laser control.
Journal of Physics: Conference Series. IOP Publishing. https://doi.org/10.1088/1742-6596/635/11/112136'
chicago: 'Kraus, P M, B Mignolet, Denitsa Rangelova Baykusheva, A Rupenyan, L Horný,
E F Penka, O I Tolstikhin, et al. “Attosecond Charge Migration and Its Laser Control.”
Journal of Physics: Conference Series. IOP Publishing, 2015. https://doi.org/10.1088/1742-6596/635/11/112136.'
ieee: 'P. M. Kraus et al., “Attosecond charge migration and its laser control,”
Journal of Physics: Conference Series, vol. 635, no. 11. IOP Publishing,
2015.'
ista: 'Kraus PM, Mignolet B, Baykusheva DR, Rupenyan A, Horný L, Penka EF, Tolstikhin
OI, Schneider J, Jensen F, Madsen LB, Bandrauk AD, Remacle F, Wörner HJ. 2015.
Attosecond charge migration and its laser control. Journal of Physics: Conference
Series. 635(11), 112136.'
mla: 'Kraus, P. M., et al. “Attosecond Charge Migration and Its Laser Control.”
Journal of Physics: Conference Series, vol. 635, no. 11, 112136, IOP Publishing,
2015, doi:10.1088/1742-6596/635/11/112136.'
short: 'P.M. Kraus, B. Mignolet, D.R. Baykusheva, A. Rupenyan, L. Horný, E.F. Penka,
O.I. Tolstikhin, J. Schneider, F. Jensen, L.B. Madsen, A.D. Bandrauk, F. Remacle,
H.J. Wörner, Journal of Physics: Conference Series 635 (2015).'
date_created: 2023-08-10T06:37:53Z
date_published: 2015-07-01T00:00:00Z
date_updated: 2023-08-22T08:49:14Z
day: '01'
doi: 10.1088/1742-6596/635/11/112136
extern: '1'
intvolume: ' 635'
issue: '11'
keyword:
- General Physics and Astronomy
language:
- iso: eng
main_file_link:
- open_access: '1'
url: https://doi.org/10.1088/1742-6596/635/11/112136
month: '07'
oa: 1
oa_version: Published Version
publication: 'Journal of Physics: Conference Series'
publication_identifier:
eissn:
- 1742-6596
issn:
- 1742-6588
publication_status: published
publisher: IOP Publishing
quality_controlled: '1'
scopus_import: '1'
status: public
title: Attosecond charge migration and its laser control
type: journal_article
user_id: 2DF688A6-F248-11E8-B48F-1D18A9856A87
volume: 635
year: '2015'
...
---
_id: '14016'
abstract:
- lang: eng
text: All attosecond time-resolved measurements have so far relied on the use of
intense near-infrared laser pulses. In particular, attosecond streaking, laser-induced
electron diffraction and high-harmonic generation all make use of non-perturbative
light–matter interactions. Remarkably, the effect of the strong laser field on
the studied sample has often been neglected in previous studies. Here we use high-harmonic
spectroscopy to measure laser-induced modifications of the electronic structure
of molecules. We study high-harmonic spectra of spatially oriented CH3F and CH3Br
as generic examples of polar polyatomic molecules. We accurately measure intensity
ratios of even and odd-harmonic orders, and of the emission from aligned and unaligned
molecules. We show that these robust observables reveal a substantial modification
of the molecular electronic structure by the external laser field. Our insights
offer new challenges and opportunities for a range of emerging strong-field attosecond
spectroscopies.
article_number: '7039'
article_processing_charge: No
article_type: original
author:
- first_name: P. M.
full_name: Kraus, P. M.
last_name: Kraus
- first_name: O. I.
full_name: Tolstikhin, O. I.
last_name: Tolstikhin
- first_name: Denitsa Rangelova
full_name: Baykusheva, Denitsa Rangelova
id: 71b4d059-2a03-11ee-914d-dfa3beed6530
last_name: Baykusheva
- first_name: A.
full_name: Rupenyan, A.
last_name: Rupenyan
- first_name: J.
full_name: Schneider, J.
last_name: Schneider
- first_name: C. Z.
full_name: Bisgaard, C. Z.
last_name: Bisgaard
- first_name: T.
full_name: Morishita, T.
last_name: Morishita
- first_name: F.
full_name: Jensen, F.
last_name: Jensen
- first_name: L. B.
full_name: Madsen, L. B.
last_name: Madsen
- first_name: H. J.
full_name: Wörner, H. J.
last_name: Wörner
citation:
ama: Kraus PM, Tolstikhin OI, Baykusheva DR, et al. Observation of laser-induced
electronic structure in oriented polyatomic molecules. Nature Communications.
2015;6. doi:10.1038/ncomms8039
apa: Kraus, P. M., Tolstikhin, O. I., Baykusheva, D. R., Rupenyan, A., Schneider,
J., Bisgaard, C. Z., … Wörner, H. J. (2015). Observation of laser-induced electronic
structure in oriented polyatomic molecules. Nature Communications. Springer
Nature. https://doi.org/10.1038/ncomms8039
chicago: Kraus, P. M., O. I. Tolstikhin, Denitsa Rangelova Baykusheva, A. Rupenyan,
J. Schneider, C. Z. Bisgaard, T. Morishita, F. Jensen, L. B. Madsen, and H. J.
Wörner. “Observation of Laser-Induced Electronic Structure in Oriented Polyatomic
Molecules.” Nature Communications. Springer Nature, 2015. https://doi.org/10.1038/ncomms8039.
ieee: P. M. Kraus et al., “Observation of laser-induced electronic structure
in oriented polyatomic molecules,” Nature Communications, vol. 6. Springer
Nature, 2015.
ista: Kraus PM, Tolstikhin OI, Baykusheva DR, Rupenyan A, Schneider J, Bisgaard
CZ, Morishita T, Jensen F, Madsen LB, Wörner HJ. 2015. Observation of laser-induced
electronic structure in oriented polyatomic molecules. Nature Communications.
6, 7039.
mla: Kraus, P. M., et al. “Observation of Laser-Induced Electronic Structure in
Oriented Polyatomic Molecules.” Nature Communications, vol. 6, 7039, Springer
Nature, 2015, doi:10.1038/ncomms8039.
short: P.M. Kraus, O.I. Tolstikhin, D.R. Baykusheva, A. Rupenyan, J. Schneider,
C.Z. Bisgaard, T. Morishita, F. Jensen, L.B. Madsen, H.J. Wörner, Nature Communications
6 (2015).
date_created: 2023-08-10T06:38:01Z
date_published: 2015-05-05T00:00:00Z
date_updated: 2023-08-22T08:52:56Z
day: '05'
doi: 10.1038/ncomms8039
extern: '1'
external_id:
pmid:
- '25940229'
intvolume: ' 6'
keyword:
- General Physics and Astronomy
- General Biochemistry
- Genetics and Molecular Biology
- General Chemistry
- Multidisciplinary
language:
- iso: eng
main_file_link:
- open_access: '1'
url: https://doi.org/10.1038/ncomms8039
month: '05'
oa: 1
oa_version: Published Version
pmid: 1
publication: Nature Communications
publication_identifier:
eissn:
- 2041-1723
publication_status: published
publisher: Springer Nature
quality_controlled: '1'
scopus_import: '1'
status: public
title: Observation of laser-induced electronic structure in oriented polyatomic molecules
type: journal_article
user_id: 2DF688A6-F248-11E8-B48F-1D18A9856A87
volume: 6
year: '2015'
...
---
_id: '14017'
abstract:
- lang: eng
text: The detection of electron motion and electronic wave-packet dynamics is one
of the core goals of attosecond science. Recently, choosing the nitric oxide molecule
as an example, we have introduced and demonstrated an experimental approach to
measure coupled valence electronic and rotational wave packets using high-order-harmonic-generation
(HHG) spectroscopy [Kraus et al., Phys. Rev. Lett. 111, 243005 (2013)]. A short
outline of the theory to describe the combination of the pump and HHG probe process
was published together with an extensive discussion of experimental results [Baykusheva
et al., Faraday Discuss. 171, 113 (2014)]. The comparison of theory and experiment
showed good agreement on a quantitative level. Here, we present the theory in
detail, which is based on a generalized density-matrix approach that describes
the pump process and the subsequent probing of the wave packets by a semiclassical
quantitative rescattering approach. An in-depth analysis of the different Raman
scattering contributions to the creation of the coupled rotational and electronic
spin-orbit wave packets is made. We present results for parallel and perpendicular
linear polarizations of the pump and probe laser pulses. Furthermore, an analysis
of the combined rotational-electronic density matrix in terms of irreducible components
is presented that facilitates interpretation of the results.
article_number: '023421'
article_processing_charge: No
article_type: original
arxiv: 1
author:
- first_name: Song Bin
full_name: Zhang, Song Bin
last_name: Zhang
- first_name: Denitsa Rangelova
full_name: Baykusheva, Denitsa Rangelova
id: 71b4d059-2a03-11ee-914d-dfa3beed6530
last_name: Baykusheva
- first_name: Peter M.
full_name: Kraus, Peter M.
last_name: Kraus
- first_name: Hans Jakob
full_name: Wörner, Hans Jakob
last_name: Wörner
- first_name: Nina
full_name: Rohringer, Nina
last_name: Rohringer
citation:
ama: Zhang SB, Baykusheva DR, Kraus PM, Wörner HJ, Rohringer N. Theoretical study
of molecular electronic and rotational coherences by high-order-harmonic generation.
Physical Review A. 2015;91(2). doi:10.1103/physreva.91.023421
apa: Zhang, S. B., Baykusheva, D. R., Kraus, P. M., Wörner, H. J., & Rohringer,
N. (2015). Theoretical study of molecular electronic and rotational coherences
by high-order-harmonic generation. Physical Review A. American Physical
Society. https://doi.org/10.1103/physreva.91.023421
chicago: Zhang, Song Bin, Denitsa Rangelova Baykusheva, Peter M. Kraus, Hans Jakob
Wörner, and Nina Rohringer. “Theoretical Study of Molecular Electronic and Rotational
Coherences by High-Order-Harmonic Generation.” Physical Review A. American
Physical Society, 2015. https://doi.org/10.1103/physreva.91.023421.
ieee: S. B. Zhang, D. R. Baykusheva, P. M. Kraus, H. J. Wörner, and N. Rohringer,
“Theoretical study of molecular electronic and rotational coherences by high-order-harmonic
generation,” Physical Review A, vol. 91, no. 2. American Physical Society,
2015.
ista: Zhang SB, Baykusheva DR, Kraus PM, Wörner HJ, Rohringer N. 2015. Theoretical
study of molecular electronic and rotational coherences by high-order-harmonic
generation. Physical Review A. 91(2), 023421.
mla: Zhang, Song Bin, et al. “Theoretical Study of Molecular Electronic and Rotational
Coherences by High-Order-Harmonic Generation.” Physical Review A, vol.
91, no. 2, 023421, American Physical Society, 2015, doi:10.1103/physreva.91.023421.
short: S.B. Zhang, D.R. Baykusheva, P.M. Kraus, H.J. Wörner, N. Rohringer, Physical
Review A 91 (2015).
date_created: 2023-08-10T06:38:10Z
date_published: 2015-02-19T00:00:00Z
date_updated: 2023-08-22T08:56:34Z
day: '19'
doi: 10.1103/physreva.91.023421
extern: '1'
external_id:
arxiv:
- '1504.03933'
intvolume: ' 91'
issue: '2'
keyword:
- Atomic and Molecular Physics
- and Optics
language:
- iso: eng
main_file_link:
- open_access: '1'
url: https://arxiv.org/abs/1504.03933
month: '02'
oa: 1
oa_version: Preprint
publication: Physical Review A
publication_identifier:
eissn:
- 1094-1622
issn:
- 1050-2947
publication_status: published
publisher: American Physical Society
quality_controlled: '1'
scopus_import: '1'
status: public
title: Theoretical study of molecular electronic and rotational coherences by high-order-harmonic
generation
type: journal_article
user_id: 2DF688A6-F248-11E8-B48F-1D18A9856A87
volume: 91
year: '2015'
...
---
_id: '1424'
abstract:
- lang: eng
text: We consider the problem of statistical computations with persistence diagrams,
a summary representation of topological features in data. These diagrams encode
persistent homology, a widely used invariant in topological data analysis. While
several avenues towards a statistical treatment of the diagrams have been explored
recently, we follow an alternative route that is motivated by the success of methods
based on the embedding of probability measures into reproducing kernel Hilbert
spaces. In fact, a positive definite kernel on persistence diagrams has recently
been proposed, connecting persistent homology to popular kernel-based learning
techniques such as support vector machines. However, important properties of that
kernel enabling a principled use in the context of probability measure embeddings
remain to be explored. Our contribution is to close this gap by proving universality
of a variant of the original kernel, and to demonstrate its effective use in twosample
hypothesis testing on synthetic as well as real-world data.
acknowledgement: This work was partially supported by the Austrian Science FUnd, project
no. KLI 00012.
alternative_title:
- Advances in Neural Information Processing Systems
article_processing_charge: No
author:
- first_name: Roland
full_name: Kwitt, Roland
last_name: Kwitt
- first_name: Stefan
full_name: Huber, Stefan
id: 4700A070-F248-11E8-B48F-1D18A9856A87
last_name: Huber
orcid: 0000-0002-8871-5814
- first_name: Marc
full_name: Niethammer, Marc
last_name: Niethammer
- first_name: Weili
full_name: Lin, Weili
last_name: Lin
- first_name: Ulrich
full_name: Bauer, Ulrich
id: 2ADD483A-F248-11E8-B48F-1D18A9856A87
last_name: Bauer
orcid: 0000-0002-9683-0724
citation:
ama: 'Kwitt R, Huber S, Niethammer M, Lin W, Bauer U. Statistical topological data
analysis-A kernel perspective. In: Vol 28. Neural Information Processing Systems
Foundation; 2015:3070-3078.'
apa: 'Kwitt, R., Huber, S., Niethammer, M., Lin, W., & Bauer, U. (2015). Statistical
topological data analysis-A kernel perspective (Vol. 28, pp. 3070–3078). Presented
at the NIPS: Neural Information Processing Systems, Montreal, Canada: Neural Information
Processing Systems Foundation.'
chicago: Kwitt, Roland, Stefan Huber, Marc Niethammer, Weili Lin, and Ulrich Bauer.
“Statistical Topological Data Analysis-A Kernel Perspective,” 28:3070–78. Neural
Information Processing Systems Foundation, 2015.
ieee: 'R. Kwitt, S. Huber, M. Niethammer, W. Lin, and U. Bauer, “Statistical topological
data analysis-A kernel perspective,” presented at the NIPS: Neural Information
Processing Systems, Montreal, Canada, 2015, vol. 28, pp. 3070–3078.'
ista: 'Kwitt R, Huber S, Niethammer M, Lin W, Bauer U. 2015. Statistical topological
data analysis-A kernel perspective. NIPS: Neural Information Processing Systems,
Advances in Neural Information Processing Systems, vol. 28, 3070–3078.'
mla: Kwitt, Roland, et al. Statistical Topological Data Analysis-A Kernel Perspective.
Vol. 28, Neural Information Processing Systems Foundation, 2015, pp. 3070–78.
short: R. Kwitt, S. Huber, M. Niethammer, W. Lin, U. Bauer, in:, Neural Information
Processing Systems Foundation, 2015, pp. 3070–3078.
conference:
end_date: 2015-12-12
location: Montreal, Canada
name: 'NIPS: Neural Information Processing Systems'
start_date: 2015-12-07
date_created: 2018-12-11T11:51:56Z
date_published: 2015-12-01T00:00:00Z
date_updated: 2025-06-03T11:41:36Z
day: '01'
department:
- _id: HeEd
intvolume: ' 28'
language:
- iso: eng
main_file_link:
- open_access: '1'
url: https://papers.nips.cc/paper/5887-statistical-topological-data-analysis-a-kernel-perspective
month: '12'
oa: 1
oa_version: Submitted Version
page: 3070 - 3078
publication_status: published
publisher: Neural Information Processing Systems Foundation
publist_id: '5782'
quality_controlled: '1'
status: public
title: Statistical topological data analysis-A kernel perspective
type: conference
user_id: 2DF688A6-F248-11E8-B48F-1D18A9856A87
volume: 28
year: '2015'
...
---
_id: '1425'
abstract:
- lang: eng
text: 'In this work we aim at extending the theoretical foundations of lifelong
learning. Previous work analyzing this scenario is based on the assumption that
learning tasks are sampled i.i.d. from a task environment or limited to strongly
constrained data distributions. Instead, we study two scenarios when lifelong
learning is possible, even though the observed tasks do not form an i.i.d. sample:
first, when they are sampled from the same environment, but possibly with dependencies,
and second, when the task environment is allowed to change over time in a consistent
way. In the first case we prove a PAC-Bayesian theorem that can be seen as a direct
generalization of the analogous previous result for the i.i.d. case. For the second
scenario we propose to learn an inductive bias in form of a transfer procedure.
We present a generalization bound and show on a toy example how it can be used
to identify a beneficial transfer algorithm.'
alternative_title:
- Advances in Neural Information Processing Systems
article_processing_charge: No
author:
- first_name: Anastasia
full_name: Pentina, Anastasia
id: 42E87FC6-F248-11E8-B48F-1D18A9856A87
last_name: Pentina
- first_name: Christoph
full_name: Lampert, Christoph
id: 40C20FD2-F248-11E8-B48F-1D18A9856A87
last_name: Lampert
orcid: 0000-0001-8622-7887
citation:
ama: 'Pentina A, Lampert C. Lifelong learning with non-i.i.d. tasks. In: Vol 2015.
Neural Information Processing Systems Foundation; 2015:1540-1548.'
apa: 'Pentina, A., & Lampert, C. (2015). Lifelong learning with non-i.i.d. tasks
(Vol. 2015, pp. 1540–1548). Presented at the NIPS: Neural Information Processing
Systems, Montreal, Canada: Neural Information Processing Systems Foundation.'
chicago: Pentina, Anastasia, and Christoph Lampert. “Lifelong Learning with Non-i.i.d.
Tasks,” 2015:1540–48. Neural Information Processing Systems Foundation, 2015.
ieee: 'A. Pentina and C. Lampert, “Lifelong learning with non-i.i.d. tasks,” presented
at the NIPS: Neural Information Processing Systems, Montreal, Canada, 2015, vol.
2015, pp. 1540–1548.'
ista: 'Pentina A, Lampert C. 2015. Lifelong learning with non-i.i.d. tasks. NIPS:
Neural Information Processing Systems, Advances in Neural Information Processing
Systems, vol. 2015, 1540–1548.'
mla: Pentina, Anastasia, and Christoph Lampert. Lifelong Learning with Non-i.i.d.
Tasks. Vol. 2015, Neural Information Processing Systems Foundation, 2015,
pp. 1540–48.
short: A. Pentina, C. Lampert, in:, Neural Information Processing Systems Foundation,
2015, pp. 1540–1548.
conference:
end_date: 2015-12-12
location: Montreal, Canada
name: 'NIPS: Neural Information Processing Systems'
start_date: 2015-12-07
date_created: 2018-12-11T11:51:57Z
date_published: 2015-01-01T00:00:00Z
date_updated: 2025-06-03T11:41:45Z
day: '01'
department:
- _id: ChLa
ec_funded: 1
intvolume: ' 2015'
language:
- iso: eng
main_file_link:
- open_access: '1'
url: http://papers.nips.cc/paper/6007-lifelong-learning-with-non-iid-tasks
month: '01'
oa: 1
oa_version: None
page: 1540 - 1548
project:
- _id: 2532554C-B435-11E9-9278-68D0E5697425
call_identifier: FP7
grant_number: '308036'
name: Lifelong Learning of Visual Scene Understanding
publication_status: published
publisher: Neural Information Processing Systems Foundation
publist_id: '5781'
quality_controlled: '1'
scopus_import: '1'
status: public
title: Lifelong learning with non-i.i.d. tasks
type: conference
user_id: 2DF688A6-F248-11E8-B48F-1D18A9856A87
volume: 2015
year: '2015'
...
---
_id: '1430'
abstract:
- lang: eng
text: Evolutionary algorithms (EAs) form a popular optimisation paradigm inspired
by natural evolution. In recent years the field of evolutionary computation has
developed a rigorous analytical theory to analyse their runtime on many illustrative
problems. Here we apply this theory to a simple model of natural evolution. In
the Strong Selection Weak Mutation (SSWM) evolutionary regime the time between
occurrence of new mutations is much longer than the time it takes for a new beneficial
mutation to take over the population. In this situation, the population only contains
copies of one genotype and evolution can be modelled as a (1+1)-type process where
the probability of accepting a new genotype (improvements or worsenings) depends
on the change in fitness. We present an initial runtime analysis of SSWM, quantifying
its performance for various parameters and investigating differences to the (1+1)
EA. We show that SSWM can have a moderate advantage over the (1+1) EA at crossing
fitness valleys and study an example where SSWM outperforms the (1+1) EA by taking
advantage of information on the fitness gradient.
article_processing_charge: No
arxiv: 1
author:
- first_name: Tiago
full_name: Paixao, Tiago
id: 2C5658E6-F248-11E8-B48F-1D18A9856A87
last_name: Paixao
orcid: 0000-0003-2361-3953
- first_name: Dirk
full_name: Sudholt, Dirk
last_name: Sudholt
- first_name: Jorge
full_name: Heredia, Jorge
last_name: Heredia
- first_name: Barbora
full_name: Trubenova, Barbora
id: 42302D54-F248-11E8-B48F-1D18A9856A87
last_name: Trubenova
orcid: 0000-0002-6873-2967
citation:
ama: 'Paixao T, Sudholt D, Heredia J, Trubenova B. First steps towards a runtime
comparison of natural and artificial evolution. In: Proceedings of the 2015
Annual Conference on Genetic and Evolutionary Computation. ACM; 2015:1455-1462.
doi:10.1145/2739480.2754758'
apa: 'Paixao, T., Sudholt, D., Heredia, J., & Trubenova, B. (2015). First steps
towards a runtime comparison of natural and artificial evolution. In Proceedings
of the 2015 Annual Conference on Genetic and Evolutionary Computation (pp.
1455–1462). Madrid, Spain: ACM. https://doi.org/10.1145/2739480.2754758'
chicago: Paixao, Tiago, Dirk Sudholt, Jorge Heredia, and Barbora Trubenova. “First
Steps towards a Runtime Comparison of Natural and Artificial Evolution.” In Proceedings
of the 2015 Annual Conference on Genetic and Evolutionary Computation, 1455–62.
ACM, 2015. https://doi.org/10.1145/2739480.2754758.
ieee: T. Paixao, D. Sudholt, J. Heredia, and B. Trubenova, “First steps towards
a runtime comparison of natural and artificial evolution,” in Proceedings of
the 2015 Annual Conference on Genetic and Evolutionary Computation, Madrid,
Spain, 2015, pp. 1455–1462.
ista: 'Paixao T, Sudholt D, Heredia J, Trubenova B. 2015. First steps towards a
runtime comparison of natural and artificial evolution. Proceedings of the 2015
Annual Conference on Genetic and Evolutionary Computation. GECCO: Genetic and
evolutionary computation conference, 1455–1462.'
mla: Paixao, Tiago, et al. “First Steps towards a Runtime Comparison of Natural
and Artificial Evolution.” Proceedings of the 2015 Annual Conference on Genetic
and Evolutionary Computation, ACM, 2015, pp. 1455–62, doi:10.1145/2739480.2754758.
short: T. Paixao, D. Sudholt, J. Heredia, B. Trubenova, in:, Proceedings of the
2015 Annual Conference on Genetic and Evolutionary Computation, ACM, 2015, pp.
1455–1462.
conference:
end_date: 2015-07-15
location: Madrid, Spain
name: 'GECCO: Genetic and evolutionary computation conference'
start_date: 2015-07-11
date_created: 2018-12-11T11:51:58Z
date_published: 2015-07-11T00:00:00Z
date_updated: 2025-09-23T08:50:33Z
day: '11'
department:
- _id: NiBa
- _id: CaGu
doi: 10.1145/2739480.2754758
ec_funded: 1
external_id:
arxiv:
- '1504.06260'
isi:
- '000358795700182'
isi: 1
language:
- iso: eng
main_file_link:
- open_access: '1'
url: http://arxiv.org/abs/1504.06260
month: '07'
oa: 1
oa_version: Preprint
page: 1455 - 1462
project:
- _id: 25B1EC9E-B435-11E9-9278-68D0E5697425
call_identifier: FP7
grant_number: '618091'
name: Speed of Adaptation in Population Genetics and Evolutionary Computation
publication: Proceedings of the 2015 Annual Conference on Genetic and Evolutionary
Computation
publication_status: published
publisher: ACM
publist_id: '5768'
quality_controlled: '1'
scopus_import: '1'
status: public
title: First steps towards a runtime comparison of natural and artificial evolution
type: conference
user_id: 317138e5-6ab7-11ef-aa6d-ffef3953e345
year: '2015'
...
---
_id: '14303'
abstract:
- lang: eng
text: Scaffolded DNA origami enables the fabrication of a variety of complex nanostructures
that promise utility in diverse fields of application, ranging from biosensing
over advanced therapeutics to metamaterials. The broad applicability of DNA origami
as a material beyond the level of proof-of-concept studies critically depends,
among other factors, on the availability of large amounts of pure single-stranded
scaffold DNA. Here, we present a method for the efficient production of M13 bacteriophage-derived
genomic DNA using high-cell-density fermentation of Escherichia coli in stirred-tank
bioreactors. We achieve phage titers of up to 1.6 × 1014 plaque-forming units
per mL. Downstream processing yields up to 410 mg of high-quality single-stranded
DNA per one liter reaction volume, thus upgrading DNA origami-based nanotechnology
from the milligram to the gram scale.
article_processing_charge: No
article_type: letter_note
author:
- first_name: B
full_name: Kick, B
last_name: Kick
- first_name: Florian M
full_name: Praetorius, Florian M
id: dfec9381-4341-11ee-8fd8-faa02bba7d62
last_name: Praetorius
- first_name: H
full_name: Dietz, H
last_name: Dietz
- first_name: D
full_name: Weuster-Botz, D
last_name: Weuster-Botz
citation:
ama: Kick B, Praetorius FM, Dietz H, Weuster-Botz D. Efficient production of single-stranded
phage DNA as scaffolds for DNA origami. Nano Letters. 2015;15(7):4672-4676.
doi:10.1021/acs.nanolett.5b01461
apa: Kick, B., Praetorius, F. M., Dietz, H., & Weuster-Botz, D. (2015). Efficient
production of single-stranded phage DNA as scaffolds for DNA origami. Nano
Letters. ACS Publications. https://doi.org/10.1021/acs.nanolett.5b01461
chicago: Kick, B, Florian M Praetorius, H Dietz, and D Weuster-Botz. “Efficient
Production of Single-Stranded Phage DNA as Scaffolds for DNA Origami.” Nano
Letters. ACS Publications, 2015. https://doi.org/10.1021/acs.nanolett.5b01461.
ieee: B. Kick, F. M. Praetorius, H. Dietz, and D. Weuster-Botz, “Efficient production
of single-stranded phage DNA as scaffolds for DNA origami,” Nano Letters,
vol. 15, no. 7. ACS Publications, pp. 4672–4676, 2015.
ista: Kick B, Praetorius FM, Dietz H, Weuster-Botz D. 2015. Efficient production
of single-stranded phage DNA as scaffolds for DNA origami. Nano Letters. 15(7),
4672–4676.
mla: Kick, B., et al. “Efficient Production of Single-Stranded Phage DNA as Scaffolds
for DNA Origami.” Nano Letters, vol. 15, no. 7, ACS Publications, 2015,
pp. 4672–76, doi:10.1021/acs.nanolett.5b01461.
short: B. Kick, F.M. Praetorius, H. Dietz, D. Weuster-Botz, Nano Letters 15 (2015)
4672–4676.
date_created: 2023-09-06T12:52:47Z
date_published: 2015-06-01T00:00:00Z
date_updated: 2023-11-07T11:56:32Z
day: '01'
doi: 10.1021/acs.nanolett.5b01461
extern: '1'
external_id:
pmid:
- '26028443'
intvolume: ' 15'
issue: '7'
language:
- iso: eng
main_file_link:
- open_access: '1'
url: https://doi.org/10.1021/acs.nanolett.5b01461
month: '06'
oa: 1
oa_version: Published Version
page: 4672-4676
pmid: 1
publication: Nano Letters
publication_identifier:
eissn:
- 1530-6992
issn:
- 1530-6984
publication_status: published
publisher: ACS Publications
quality_controlled: '1'
status: public
title: Efficient production of single-stranded phage DNA as scaffolds for DNA origami
type: journal_article
user_id: 2DF688A6-F248-11E8-B48F-1D18A9856A87
volume: 15
year: '2015'
...
---
_id: '1473'
abstract:
- lang: eng
text: In this paper we survey geometric and arithmetic techniques to study the cohomology
of semiprojective hyperkähler manifolds including toric hyperkähler varieties,
Nakajima quiver varieties and moduli spaces of Higgs bundles on Riemann surfaces.
The resulting formulae for their Poincaré polynomials are combinatorial and representation
theoretical in nature. In particular we will look at their Betti numbers and will
establish some results and state some expectations on their asymptotic shape.
author:
- first_name: Tamas
full_name: Tamas Hausel
id: 4A0666D8-F248-11E8-B48F-1D18A9856A87
last_name: Hausel
- first_name: Fernando
full_name: Rodríguez Villegas, Fernando
last_name: Rodríguez Villegas
citation:
ama: Hausel T, Rodríguez Villegas F. Cohomology of large semiprojective hyperkähler
varieties. Asterisque. 2015;2015(370):113-156.
apa: Hausel, T., & Rodríguez Villegas, F. (2015). Cohomology of large semiprojective
hyperkähler varieties. Asterisque. Societe Mathematique de France.
chicago: Hausel, Tamás, and Fernando Rodríguez Villegas. “Cohomology of Large Semiprojective
Hyperkähler Varieties.” Asterisque. Societe Mathematique de France, 2015.
ieee: T. Hausel and F. Rodríguez Villegas, “Cohomology of large semiprojective hyperkähler
varieties,” Asterisque, vol. 2015, no. 370. Societe Mathematique de France,
pp. 113–156, 2015.
ista: Hausel T, Rodríguez Villegas F. 2015. Cohomology of large semiprojective hyperkähler
varieties. Asterisque. 2015(370), 113–156.
mla: Hausel, Tamás, and Fernando Rodríguez Villegas. “Cohomology of Large Semiprojective
Hyperkähler Varieties.” Asterisque, vol. 2015, no. 370, Societe Mathematique
de France, 2015, pp. 113–56.
short: T. Hausel, F. Rodríguez Villegas, Asterisque 2015 (2015) 113–156.
date_created: 2018-12-11T11:52:13Z
date_published: 2015-01-01T00:00:00Z
date_updated: 2021-01-12T06:50:59Z
day: '01'
extern: 1
intvolume: ' 2015'
issue: '370'
main_file_link:
- open_access: '1'
url: http://arxiv.org/abs/1309.4914
month: '01'
oa: 1
page: 113 - 156
publication: Asterisque
publication_status: published
publisher: Societe Mathematique de France
publist_id: '5723'
quality_controlled: 0
status: public
title: Cohomology of large semiprojective hyperkähler varieties
type: review
volume: 2015
year: '2015'
...
---
_id: '1474'
abstract:
- lang: eng
text: Cryptographic access control offers selective access to encrypted data via
a combination of key management and functionality-rich cryptographic schemes,
such as attribute-based encryption. Using this approach, publicly available meta-data
may inadvertently leak information on the access policy that is enforced by cryptography,
which renders cryptographic access control unusable in settings where this information
is highly sensitive. We begin to address this problem by presenting rigorous definitions
for policy privacy in cryptographic access control. For concreteness we set our
results in the model of Role-Based Access Control (RBAC), where we identify and
formalize several different flavors of privacy, however, our framework should
serve as inspiration for other models of access control. Based on our insights
we propose a new system which significantly improves on the privacy properties
of state-of-the-art constructions. Our design is based on a novel type of privacy-preserving
attribute-based encryption, which we introduce and show how to instantiate. We
present our results in the context of a cryptographic RBAC system by Ferrara et
al. (CSF'13), which uses cryptography to control read access to files, while write
access is still delegated to trusted monitors. We give an extension of the construction
that permits cryptographic control over write access. Our construction assumes
that key management uses out-of-band channels between the policy enforcer and
the users but eliminates completely the need for monitoring read/write access
to the data.
article_processing_charge: No
author:
- first_name: Anna
full_name: Ferrara, Anna
last_name: Ferrara
- first_name: Georg
full_name: Fuchsbauer, Georg
id: 46B4C3EE-F248-11E8-B48F-1D18A9856A87
last_name: Fuchsbauer
- first_name: Bin
full_name: Liu, Bin
last_name: Liu
- first_name: Bogdan
full_name: Warinschi, Bogdan
last_name: Warinschi
citation:
ama: 'Ferrara A, Fuchsbauer G, Liu B, Warinschi B. Policy privacy in cryptographic
access control. In: IEEE; 2015:46-60. doi:10.1109/CSF.2015.11'
apa: 'Ferrara, A., Fuchsbauer, G., Liu, B., & Warinschi, B. (2015). Policy privacy
in cryptographic access control (pp. 46–60). Presented at the CSF: Computer Security
Foundations, Verona, Italy: IEEE. https://doi.org/10.1109/CSF.2015.11'
chicago: Ferrara, Anna, Georg Fuchsbauer, Bin Liu, and Bogdan Warinschi. “Policy
Privacy in Cryptographic Access Control,” 46–60. IEEE, 2015. https://doi.org/10.1109/CSF.2015.11.
ieee: 'A. Ferrara, G. Fuchsbauer, B. Liu, and B. Warinschi, “Policy privacy in cryptographic
access control,” presented at the CSF: Computer Security Foundations, Verona,
Italy, 2015, pp. 46–60.'
ista: 'Ferrara A, Fuchsbauer G, Liu B, Warinschi B. 2015. Policy privacy in cryptographic
access control. CSF: Computer Security Foundations, 46–60.'
mla: Ferrara, Anna, et al. Policy Privacy in Cryptographic Access Control.
IEEE, 2015, pp. 46–60, doi:10.1109/CSF.2015.11.
short: A. Ferrara, G. Fuchsbauer, B. Liu, B. Warinschi, in:, IEEE, 2015, pp. 46–60.
conference:
end_date: 2015-07-17
location: Verona, Italy
name: 'CSF: Computer Security Foundations'
start_date: 2015-07-13
date_created: 2018-12-11T11:52:14Z
date_published: 2015-09-04T00:00:00Z
date_updated: 2025-09-23T09:50:52Z
day: '04'
department:
- _id: KrPi
doi: 10.1109/CSF.2015.11
ec_funded: 1
external_id:
isi:
- '000380428500004'
isi: 1
language:
- iso: eng
main_file_link:
- open_access: '1'
url: http://epubs.surrey.ac.uk/808055/
month: '09'
oa: 1
oa_version: Submitted Version
page: 46-60
project:
- _id: 258C570E-B435-11E9-9278-68D0E5697425
call_identifier: FP7
grant_number: '259668'
name: Provable Security for Physical Cryptography
publication_status: published
publisher: IEEE
publist_id: '5722'
quality_controlled: '1'
scopus_import: '1'
status: public
title: Policy privacy in cryptographic access control
type: conference
user_id: 317138e5-6ab7-11ef-aa6d-ffef3953e345
year: '2015'
...
---
_id: '1788'
abstract:
- lang: eng
text: We fabricate and characterize a microscale silicon opto-electromechanical
system whose mechanical motion is coupled capacitively to an electrical circuit
and optically via radiation pressure to a photonic crystal cavity. To achieve
large electromechanical interaction strength, we implement an inverse shadow mask
fabrication scheme which obtains capacitor gaps as small as 30 nm while maintaining
a silicon surface quality necessary for minimizing optical loss. Using the sensitive
optical read-out of the photonic crystal cavity, we characterize the linear and
nonlinear capacitive coupling to the fundamental ωm=2π = 63 MHz in-plane flexural
motion of the structure, showing that the large electromechanical coupling in
such devices may be suitable for realizing efficient microwave-to-optical signal
conversion.
acknowledgement: This work was supported by the DARPA MESO program, the AFOSR Hybrid
Nanophotonics MURI, the Institute for Quantum Information and Matter, an NSF Physics
Frontiers Center with support of the Gordon and Betty Moore Foundation, and the
Kavli Nanoscience Institute at Caltech. AP gratefully acknowledge funding from EU
through Marie Curie Actions, project NEMO (GA 298861). AT acknowledges partial financial
support from the ERC through the advanced grant SoulMan
author:
- first_name: Alessandro
full_name: Pitanti, Alessandro
last_name: Pitanti
- first_name: Johannes M
full_name: Johannes Fink
id: 4B591CBA-F248-11E8-B48F-1D18A9856A87
last_name: Fink
orcid: 0000-0001-8112-028X
- first_name: Amir
full_name: Safavi-Naeini, Amir H
last_name: Safavi Naeini
- first_name: Jeff
full_name: Hill, Jeff T
last_name: Hill
- first_name: Chan
full_name: Lei, Chan U
last_name: Lei
- first_name: Alessandro
full_name: Tredicucci, Alessandro
last_name: Tredicucci
- first_name: Oskar
full_name: Painter, Oskar J
last_name: Painter
citation:
ama: Pitanti A, Fink JM, Safavi Naeini A, et al. Strong opto-electro-mechanical
coupling in a silicon photonic crystal cavity. Optics Express. 2015;23(3):3196-3208.
doi:10.1364/OE.23.003196
apa: Pitanti, A., Fink, J. M., Safavi Naeini, A., Hill, J., Lei, C., Tredicucci,
A., & Painter, O. (2015). Strong opto-electro-mechanical coupling in a silicon
photonic crystal cavity. Optics Express. Optical Society of America. https://doi.org/10.1364/OE.23.003196
chicago: Pitanti, Alessandro, Johannes M Fink, Amir Safavi Naeini, Jeff Hill, Chan
Lei, Alessandro Tredicucci, and Oskar Painter. “Strong Opto-Electro-Mechanical
Coupling in a Silicon Photonic Crystal Cavity.” Optics Express. Optical
Society of America, 2015. https://doi.org/10.1364/OE.23.003196.
ieee: A. Pitanti et al., “Strong opto-electro-mechanical coupling in a silicon
photonic crystal cavity,” Optics Express, vol. 23, no. 3. Optical Society
of America, pp. 3196–3208, 2015.
ista: Pitanti A, Fink JM, Safavi Naeini A, Hill J, Lei C, Tredicucci A, Painter
O. 2015. Strong opto-electro-mechanical coupling in a silicon photonic crystal
cavity. Optics Express. 23(3), 3196–3208.
mla: Pitanti, Alessandro, et al. “Strong Opto-Electro-Mechanical Coupling in a Silicon
Photonic Crystal Cavity.” Optics Express, vol. 23, no. 3, Optical Society
of America, 2015, pp. 3196–208, doi:10.1364/OE.23.003196.
short: A. Pitanti, J.M. Fink, A. Safavi Naeini, J. Hill, C. Lei, A. Tredicucci,
O. Painter, Optics Express 23 (2015) 3196–3208.
date_created: 2018-12-11T11:54:01Z
date_published: 2015-02-09T00:00:00Z
date_updated: 2021-01-12T06:53:12Z
day: '09'
doi: 10.1364/OE.23.003196
extern: 1
intvolume: ' 23'
issue: '3'
month: '02'
page: 3196 - 3208
publication: Optics Express
publication_status: published
publisher: Optical Society of America
publist_id: '5325'
quality_controlled: 0
status: public
title: Strong opto-electro-mechanical coupling in a silicon photonic crystal cavity
type: journal_article
volume: 23
year: '2015'
...
---
_id: '1789'
abstract:
- lang: eng
text: Intellectual disability (ID) has an estimated prevalence of 2-3%. Due to its
extreme heterogeneity, the genetic basis of ID remains elusive in many cases.
Recently, whole exome sequencing (WES) studies revealed that a large proportion
of sporadic cases are caused by de novo gene variants. To identify further genes
involved in ID, we performed WES in 250 patients with unexplained ID and their
unaffected parents and included exomes of 51 previously sequenced child-parents
trios in the analysis. Exome analysis revealed de novo intragenic variants in
SET domain-containing 5 (SETD5) in two patients. One patient carried a nonsense
variant, and the other an 81 bp deletion located across a splice-donor site. Chromosomal
microarray diagnostics further identified four de novo non-recurrent microdeletions
encompassing SETD5. CRISPR/Cas9 mutation modelling of the two intragenic variants
demonstrated nonsense-mediated decay of the resulting transcripts, pointing to
a loss-of-function (LoF) and haploinsufficiency as the common disease-causing
mechanism of intragenic SETD5 sequence variants and SETD5-containing microdeletions.
In silico domain prediction of SETD5, a predicted SET domain-containing histone
methyltransferase (HMT), substantiated the presence of a SET domain and identified
a novel putative PHD domain, strengthening a functional link to well-known histone-modifying
ID genes. All six patients presented with ID and certain facial dysmorphisms,
suggesting that SETD5 sequence variants contribute substantially to the microdeletion
3p25.3 phenotype. The present report of two SETD5 LoF variants in 301 patients
demonstrates a prevalence of 0.7% and thus SETD5 variants as a relatively frequent
cause of ID.
article_processing_charge: No
author:
- first_name: Alma
full_name: Kuechler, Alma
last_name: Kuechler
- first_name: Alexander
full_name: Zink, Alexander
last_name: Zink
- first_name: Thomas
full_name: Wieland, Thomas
last_name: Wieland
- first_name: Hermann
full_name: Lüdecke, Hermann
last_name: Lüdecke
- first_name: Kirsten
full_name: Cremer, Kirsten
last_name: Cremer
- first_name: Leonardo
full_name: Salviati, Leonardo
last_name: Salviati
- first_name: Pamela
full_name: Magini, Pamela
last_name: Magini
- first_name: Kimia
full_name: Najafi, Kimia
last_name: Najafi
- first_name: Christiane
full_name: Zweier, Christiane
last_name: Zweier
- first_name: Johanna
full_name: Czeschik, Johanna
last_name: Czeschik
- first_name: Stefan
full_name: Aretz, Stefan
last_name: Aretz
- first_name: Sabine
full_name: Endele, Sabine
last_name: Endele
- first_name: Federica
full_name: Tamburrino, Federica
last_name: Tamburrino
- first_name: Claudia
full_name: Pinato, Claudia
last_name: Pinato
- first_name: Maurizio
full_name: Clementi, Maurizio
last_name: Clementi
- first_name: Jasmin
full_name: Gundlach, Jasmin
last_name: Gundlach
- first_name: Carina
full_name: Maylahn, Carina
last_name: Maylahn
- first_name: Laura
full_name: Mazzanti, Laura
last_name: Mazzanti
- first_name: Eva
full_name: Wohlleber, Eva
last_name: Wohlleber
- first_name: Thomas
full_name: Schwarzmayr, Thomas
last_name: Schwarzmayr
- first_name: Roxana
full_name: Kariminejad, Roxana
last_name: Kariminejad
- first_name: Avner
full_name: Schlessinger, Avner
last_name: Schlessinger
- first_name: Dagmar
full_name: Wieczorek, Dagmar
last_name: Wieczorek
- first_name: Tim
full_name: Strom, Tim
last_name: Strom
- first_name: Gaia
full_name: Novarino, Gaia
id: 3E57A680-F248-11E8-B48F-1D18A9856A87
last_name: Novarino
orcid: 0000-0002-7673-7178
- first_name: Hartmut
full_name: Engels, Hartmut
last_name: Engels
citation:
ama: Kuechler A, Zink A, Wieland T, et al. Loss-of-function variants of SETD5 cause
intellectual disability and the core phenotype of microdeletion 3p25.3 syndrome.
European Journal of Human Genetics. 2015;23(6):753-760. doi:10.1038/ejhg.2014.165
apa: Kuechler, A., Zink, A., Wieland, T., Lüdecke, H., Cremer, K., Salviati, L.,
… Engels, H. (2015). Loss-of-function variants of SETD5 cause intellectual disability
and the core phenotype of microdeletion 3p25.3 syndrome. European Journal of
Human Genetics. Nature Publishing Group. https://doi.org/10.1038/ejhg.2014.165
chicago: Kuechler, Alma, Alexander Zink, Thomas Wieland, Hermann Lüdecke, Kirsten
Cremer, Leonardo Salviati, Pamela Magini, et al. “Loss-of-Function Variants of
SETD5 Cause Intellectual Disability and the Core Phenotype of Microdeletion 3p25.3
Syndrome.” European Journal of Human Genetics. Nature Publishing Group,
2015. https://doi.org/10.1038/ejhg.2014.165.
ieee: A. Kuechler et al., “Loss-of-function variants of SETD5 cause intellectual
disability and the core phenotype of microdeletion 3p25.3 syndrome,” European
Journal of Human Genetics, vol. 23, no. 6. Nature Publishing Group, pp. 753–760,
2015.
ista: Kuechler A, Zink A, Wieland T, Lüdecke H, Cremer K, Salviati L, Magini P,
Najafi K, Zweier C, Czeschik J, Aretz S, Endele S, Tamburrino F, Pinato C, Clementi
M, Gundlach J, Maylahn C, Mazzanti L, Wohlleber E, Schwarzmayr T, Kariminejad
R, Schlessinger A, Wieczorek D, Strom T, Novarino G, Engels H. 2015. Loss-of-function
variants of SETD5 cause intellectual disability and the core phenotype of microdeletion
3p25.3 syndrome. European Journal of Human Genetics. 23(6), 753–760.
mla: Kuechler, Alma, et al. “Loss-of-Function Variants of SETD5 Cause Intellectual
Disability and the Core Phenotype of Microdeletion 3p25.3 Syndrome.” European
Journal of Human Genetics, vol. 23, no. 6, Nature Publishing Group, 2015,
pp. 753–60, doi:10.1038/ejhg.2014.165.
short: A. Kuechler, A. Zink, T. Wieland, H. Lüdecke, K. Cremer, L. Salviati, P.
Magini, K. Najafi, C. Zweier, J. Czeschik, S. Aretz, S. Endele, F. Tamburrino,
C. Pinato, M. Clementi, J. Gundlach, C. Maylahn, L. Mazzanti, E. Wohlleber, T.
Schwarzmayr, R. Kariminejad, A. Schlessinger, D. Wieczorek, T. Strom, G. Novarino,
H. Engels, European Journal of Human Genetics 23 (2015) 753–760.
date_created: 2018-12-11T11:54:01Z
date_published: 2015-06-15T00:00:00Z
date_updated: 2025-09-23T09:30:27Z
day: '15'
department:
- _id: GaNo
doi: 10.1038/ejhg.2014.165
external_id:
isi:
- '000354474600013'
pmid:
- '25138099'
intvolume: ' 23'
isi: 1
issue: '6'
language:
- iso: eng
main_file_link:
- open_access: '1'
url: http://www.ncbi.nlm.nih.gov/pmc/articles/PMC4795044/
month: '06'
oa: 1
oa_version: Submitted Version
page: 753 - 760
pmid: 1
publication: European Journal of Human Genetics
publication_status: published
publisher: Nature Publishing Group
publist_id: '5324'
quality_controlled: '1'
status: public
title: Loss-of-function variants of SETD5 cause intellectual disability and the core
phenotype of microdeletion 3p25.3 syndrome
type: journal_article
user_id: 317138e5-6ab7-11ef-aa6d-ffef3953e345
volume: 23
year: '2015'
...
---
_id: '1792'
abstract:
- lang: eng
text: Motivated by recent ideas of Harman (Unif. Distrib. Theory, 2010) we develop
a new concept of variation of multivariate functions on a compact Hausdorff space
with respect to a collection D of subsets. We prove a general version of the Koksma-Hlawka
theorem that holds for this notion of variation and discrepancy with respect to
D. As special cases, we obtain Koksma-Hlawka inequalities for classical notions,
such as extreme or isotropic discrepancy. For extreme discrepancy, our result
coincides with the usual Koksma-Hlawka theorem. We show that the space of functions
of bounded D-variation contains important discontinuous functions and is closed
under natural algebraic operations. Finally, we illustrate the results on concrete
integration problems from integral geometry and stereology.
acknowledgement: F.P. is supported by the Graduate School of IST Austria, A.M.S is
supported by the Centre for Stochastic Geometry and Advanced Bioimaging funded by
a grant from the Villum Foundation.
article_processing_charge: No
author:
- first_name: Florian
full_name: Pausinger, Florian
id: 2A77D7A2-F248-11E8-B48F-1D18A9856A87
last_name: Pausinger
orcid: 0000-0002-8379-3768
- first_name: Anne
full_name: Svane, Anne
last_name: Svane
citation:
ama: Pausinger F, Svane A. A Koksma-Hlawka inequality for general discrepancy systems.
Journal of Complexity. 2015;31(6):773-797. doi:10.1016/j.jco.2015.06.002
apa: Pausinger, F., & Svane, A. (2015). A Koksma-Hlawka inequality for general
discrepancy systems. Journal of Complexity. Academic Press. https://doi.org/10.1016/j.jco.2015.06.002
chicago: Pausinger, Florian, and Anne Svane. “A Koksma-Hlawka Inequality for General
Discrepancy Systems.” Journal of Complexity. Academic Press, 2015. https://doi.org/10.1016/j.jco.2015.06.002.
ieee: F. Pausinger and A. Svane, “A Koksma-Hlawka inequality for general discrepancy
systems,” Journal of Complexity, vol. 31, no. 6. Academic Press, pp. 773–797,
2015.
ista: Pausinger F, Svane A. 2015. A Koksma-Hlawka inequality for general discrepancy
systems. Journal of Complexity. 31(6), 773–797.
mla: Pausinger, Florian, and Anne Svane. “A Koksma-Hlawka Inequality for General
Discrepancy Systems.” Journal of Complexity, vol. 31, no. 6, Academic Press,
2015, pp. 773–97, doi:10.1016/j.jco.2015.06.002.
short: F. Pausinger, A. Svane, Journal of Complexity 31 (2015) 773–797.
corr_author: '1'
date_created: 2018-12-11T11:54:02Z
date_published: 2015-12-01T00:00:00Z
date_updated: 2025-09-22T14:32:05Z
day: '01'
department:
- _id: HeEd
doi: 10.1016/j.jco.2015.06.002
external_id:
isi:
- '000362926900001'
intvolume: ' 31'
isi: 1
issue: '6'
language:
- iso: eng
month: '12'
oa_version: None
page: 773 - 797
publication: Journal of Complexity
publication_status: published
publisher: Academic Press
publist_id: '5320'
quality_controlled: '1'
related_material:
record:
- id: '1399'
relation: dissertation_contains
status: public
scopus_import: '1'
status: public
title: A Koksma-Hlawka inequality for general discrepancy systems
type: journal_article
user_id: 317138e5-6ab7-11ef-aa6d-ffef3953e345
volume: 31
year: '2015'
...
---
_id: '1793'
abstract:
- lang: eng
text: We present a software platform for reconstructing and analyzing the growth
of a plant root system from a time-series of 3D voxelized shapes. It aligns the
shapes with each other, constructs a geometric graph representation together with
the function that records the time of growth, and organizes the branches into
a hierarchy that reflects the order of creation. The software includes the automatic
computation of structural and dynamic traits for each root in the system enabling
the quantification of growth on fine-scale. These are important advances in plant
phenotyping with applications to the study of genetic and environmental influences
on growth.
article_number: e0127657
article_processing_charge: No
author:
- first_name: Olga
full_name: Symonova, Olga
id: 3C0C7BC6-F248-11E8-B48F-1D18A9856A87
last_name: Symonova
orcid: 0000-0003-2012-9947
- first_name: Christopher
full_name: Topp, Christopher
last_name: Topp
- first_name: Herbert
full_name: Edelsbrunner, Herbert
id: 3FB178DA-F248-11E8-B48F-1D18A9856A87
last_name: Edelsbrunner
orcid: 0000-0002-9823-6833
citation:
ama: 'Symonova O, Topp C, Edelsbrunner H. DynamicRoots: A software platform for
the reconstruction and analysis of growing plant roots. PLoS One. 2015;10(6).
doi:10.1371/journal.pone.0127657'
apa: 'Symonova, O., Topp, C., & Edelsbrunner, H. (2015). DynamicRoots: A software
platform for the reconstruction and analysis of growing plant roots. PLoS One.
Public Library of Science. https://doi.org/10.1371/journal.pone.0127657'
chicago: 'Symonova, Olga, Christopher Topp, and Herbert Edelsbrunner. “DynamicRoots:
A Software Platform for the Reconstruction and Analysis of Growing Plant Roots.”
PLoS One. Public Library of Science, 2015. https://doi.org/10.1371/journal.pone.0127657.'
ieee: 'O. Symonova, C. Topp, and H. Edelsbrunner, “DynamicRoots: A software platform
for the reconstruction and analysis of growing plant roots,” PLoS One,
vol. 10, no. 6. Public Library of Science, 2015.'
ista: 'Symonova O, Topp C, Edelsbrunner H. 2015. DynamicRoots: A software platform
for the reconstruction and analysis of growing plant roots. PLoS One. 10(6), e0127657.'
mla: 'Symonova, Olga, et al. “DynamicRoots: A Software Platform for the Reconstruction
and Analysis of Growing Plant Roots.” PLoS One, vol. 10, no. 6, e0127657,
Public Library of Science, 2015, doi:10.1371/journal.pone.0127657.'
short: O. Symonova, C. Topp, H. Edelsbrunner, PLoS One 10 (2015).
corr_author: '1'
date_created: 2018-12-11T11:54:02Z
date_published: 2015-06-01T00:00:00Z
date_updated: 2025-09-23T08:30:43Z
day: '01'
ddc:
- '000'
department:
- _id: MaJö
- _id: HeEd
doi: 10.1371/journal.pone.0127657
external_id:
isi:
- '000356630900069'
file:
- access_level: open_access
checksum: d20f26461ca575276ad3ed9ce4bfc787
content_type: application/pdf
creator: system
date_created: 2018-12-12T10:15:30Z
date_updated: 2020-07-14T12:45:16Z
file_id: '5150'
file_name: IST-2016-454-v1+1_journal.pone.0127657.pdf
file_size: 1850825
relation: main_file
file_date_updated: 2020-07-14T12:45:16Z
has_accepted_license: '1'
intvolume: ' 10'
isi: 1
issue: '6'
language:
- iso: eng
license: https://creativecommons.org/licenses/by/4.0/
month: '06'
oa: 1
oa_version: Published Version
publication: PLoS One
publication_status: published
publisher: Public Library of Science
publist_id: '5318'
pubrep_id: '454'
quality_controlled: '1'
related_material:
record:
- id: '9737'
relation: research_data
status: public
scopus_import: '1'
status: public
title: 'DynamicRoots: A software platform for the reconstruction and analysis of growing
plant roots'
tmp:
image: /images/cc_by.png
legal_code_url: https://creativecommons.org/licenses/by/4.0/legalcode
name: Creative Commons Attribution 4.0 International Public License (CC-BY 4.0)
short: CC BY (4.0)
type: journal_article
user_id: 317138e5-6ab7-11ef-aa6d-ffef3953e345
volume: 10
year: '2015'
...
---
_id: '17965'
abstract:
- lang: eng
text: 'We investigate bidirectional femtosecond charge transfer dynamics using the
core–hole clock implementation of resonant photoemission spectroscopy from 4,4′-bipyridine
molecular layers on three different surfaces: Au(111), epitaxial graphene on Ni(111),
and graphene nanoribbons. We show that the lowest unoccupied molecular orbital
(LUMO) of the molecule drops partially below the Fermi level upon core–hole creation
in all systems, opening an additional decay channel for the core–hole, involving
electron donation from substrate to the molecule. Furthermore, using the core–hole
clock method, we find that the bidirectional charge transfer time between the
substrate and the molecule is fastest on Au(111), with a 2 fs time, then around
4 fs for epitaxial graphene and slowest with graphene nanoribbon surface, taking
around 10 fs. Finally, we provide evidence for fast phase decoherence of the core-excited
LUMO* electron through an interaction with the substrate providing the first observation
of such a fast bidirectional charge transfer across an organic/graphene interface.'
article_processing_charge: No
article_type: letter_note
author:
- first_name: Olgun
full_name: Adak, Olgun
last_name: Adak
- first_name: Gregor
full_name: Kladnik, Gregor
last_name: Kladnik
- first_name: Gregor
full_name: Bavdek, Gregor
last_name: Bavdek
- first_name: Albano
full_name: Cossaro, Albano
last_name: Cossaro
- first_name: Alberto
full_name: Morgante, Alberto
last_name: Morgante
- first_name: Dean
full_name: Cvetko, Dean
last_name: Cvetko
- first_name: Latha
full_name: Venkataraman, Latha
id: 9ebb78a5-cc0d-11ee-8322-fae086a32caf
last_name: Venkataraman
orcid: 0000-0002-6957-6089
citation:
ama: 'Adak O, Kladnik G, Bavdek G, et al. Ultrafast bidirectional charge transport
and electron decoherence at molecule/surface interfaces: A comparison of gold,
graphene, and graphene nanoribbon surfaces. Nano Letters. 2015;15(12):8316-8321.
doi:10.1021/acs.nanolett.5b03962'
apa: 'Adak, O., Kladnik, G., Bavdek, G., Cossaro, A., Morgante, A., Cvetko, D.,
& Venkataraman, L. (2015). Ultrafast bidirectional charge transport and electron
decoherence at molecule/surface interfaces: A comparison of gold, graphene, and
graphene nanoribbon surfaces. Nano Letters. American Chemical Society.
https://doi.org/10.1021/acs.nanolett.5b03962'
chicago: 'Adak, Olgun, Gregor Kladnik, Gregor Bavdek, Albano Cossaro, Alberto Morgante,
Dean Cvetko, and Latha Venkataraman. “Ultrafast Bidirectional Charge Transport
and Electron Decoherence at Molecule/Surface Interfaces: A Comparison of Gold,
Graphene, and Graphene Nanoribbon Surfaces.” Nano Letters. American Chemical
Society, 2015. https://doi.org/10.1021/acs.nanolett.5b03962.'
ieee: 'O. Adak et al., “Ultrafast bidirectional charge transport and electron
decoherence at molecule/surface interfaces: A comparison of gold, graphene, and
graphene nanoribbon surfaces,” Nano Letters, vol. 15, no. 12. American
Chemical Society, pp. 8316–8321, 2015.'
ista: 'Adak O, Kladnik G, Bavdek G, Cossaro A, Morgante A, Cvetko D, Venkataraman
L. 2015. Ultrafast bidirectional charge transport and electron decoherence at
molecule/surface interfaces: A comparison of gold, graphene, and graphene nanoribbon
surfaces. Nano Letters. 15(12), 8316–8321.'
mla: 'Adak, Olgun, et al. “Ultrafast Bidirectional Charge Transport and Electron
Decoherence at Molecule/Surface Interfaces: A Comparison of Gold, Graphene, and
Graphene Nanoribbon Surfaces.” Nano Letters, vol. 15, no. 12, American
Chemical Society, 2015, pp. 8316–21, doi:10.1021/acs.nanolett.5b03962.'
short: O. Adak, G. Kladnik, G. Bavdek, A. Cossaro, A. Morgante, D. Cvetko, L. Venkataraman,
Nano Letters 15 (2015) 8316–8321.
date_created: 2024-09-09T09:40:21Z
date_published: 2015-11-17T00:00:00Z
date_updated: 2024-12-18T10:22:39Z
day: '17'
doi: 10.1021/acs.nanolett.5b03962
extern: '1'
external_id:
pmid:
- '26574713'
intvolume: ' 15'
issue: '12'
language:
- iso: eng
month: '11'
oa_version: None
page: 8316-8321
pmid: 1
publication: Nano Letters
publication_identifier:
eissn:
- 1530-6992
issn:
- 1530-6984
publication_status: published
publisher: American Chemical Society
quality_controlled: '1'
scopus_import: '1'
status: public
title: 'Ultrafast bidirectional charge transport and electron decoherence at molecule/surface
interfaces: A comparison of gold, graphene, and graphene nanoribbon surfaces'
type: journal_article
user_id: 2DF688A6-F248-11E8-B48F-1D18A9856A87
volume: 15
year: '2015'
...
---
OA_type: closed access
_id: '17966'
article_processing_charge: No
article_type: letter_note
author:
- first_name: Mikkel
full_name: Strange, Mikkel
last_name: Strange
- first_name: Gemma C.
full_name: Solomon, Gemma C.
last_name: Solomon
- first_name: Latha
full_name: Venkataraman, Latha
id: 9ebb78a5-cc0d-11ee-8322-fae086a32caf
last_name: Venkataraman
orcid: 0000-0002-6957-6089
- first_name: Luis M.
full_name: Campos, Luis M.
last_name: Campos
citation:
ama: Strange M, Solomon GC, Venkataraman L, Campos LM. Reply to “Comment on ‘Breakdown
of Interference Rules in Azulene, a Nonalternant Hydrocarbon.’” Nano Letters.
2015;15(11):7177-7178. doi:10.1021/acs.nanolett.5b04154
apa: Strange, M., Solomon, G. C., Venkataraman, L., & Campos, L. M. (2015).
Reply to “Comment on ‘Breakdown of Interference Rules in Azulene, a Nonalternant
Hydrocarbon.’” Nano Letters. American Chemical Society. https://doi.org/10.1021/acs.nanolett.5b04154
chicago: Strange, Mikkel, Gemma C. Solomon, Latha Venkataraman, and Luis M. Campos.
“Reply to ‘Comment on “Breakdown of Interference Rules in Azulene, a Nonalternant
Hydrocarbon.”’” Nano Letters. American Chemical Society, 2015. https://doi.org/10.1021/acs.nanolett.5b04154.
ieee: M. Strange, G. C. Solomon, L. Venkataraman, and L. M. Campos, “Reply to ‘Comment
on “Breakdown of Interference Rules in Azulene, a Nonalternant Hydrocarbon,”’”
Nano Letters, vol. 15, no. 11. American Chemical Society, pp. 7177–7178,
2015.
ista: Strange M, Solomon GC, Venkataraman L, Campos LM. 2015. Reply to “Comment
on ‘Breakdown of Interference Rules in Azulene, a Nonalternant Hydrocarbon’”.
Nano Letters. 15(11), 7177–7178.
mla: Strange, Mikkel, et al. “Reply to ‘Comment on “Breakdown of Interference Rules
in Azulene, a Nonalternant Hydrocarbon.”’” Nano Letters, vol. 15, no. 11,
American Chemical Society, 2015, pp. 7177–78, doi:10.1021/acs.nanolett.5b04154.
short: M. Strange, G.C. Solomon, L. Venkataraman, L.M. Campos, Nano Letters 15 (2015)
7177–7178.
date_created: 2024-09-09T09:41:17Z
date_published: 2015-10-20T00:00:00Z
date_updated: 2024-12-18T10:28:04Z
day: '20'
doi: 10.1021/acs.nanolett.5b04154
extern: '1'
external_id:
pmid:
- '24745894'
intvolume: ' 15'
issue: '11'
language:
- iso: eng
month: '10'
oa_version: None
page: 7177-7178
pmid: 1
publication: Nano Letters
publication_identifier:
eissn:
- 1530-6992
issn:
- 1530-6984
publication_status: published
publisher: American Chemical Society
quality_controlled: '1'
scopus_import: '1'
status: public
title: Reply to “Comment on ‘Breakdown of Interference Rules in Azulene, a Nonalternant
Hydrocarbon’”
type: journal_article
user_id: 2DF688A6-F248-11E8-B48F-1D18A9856A87
volume: 15
year: '2015'
...
---
OA_type: closed access
_id: '17967'
abstract:
- lang: eng
text: We report a systematic computational search of molecular frameworks for intrinsic
rectification of electron transport. The screening of molecular rectifiers includes
52 molecules and conformers spanning over 9 series of structural motifs. N-Phenylbenzamide
is found to be a promising framework with both suitable conductance and rectification
properties. A targeted screening performed on 30 additional derivatives and conformers
of N-phenylbenzamide yielded enhanced rectification based on asymmetric functionalization.
We demonstrate that electron-donating substituent groups that maintain an asymmetric
distribution of charge in the dominant transport channel (e.g., HOMO) enhance
rectification by raising the channel closer to the Fermi level. These findings
are particularly valuable for the design of molecular assemblies that could ensure
directionality of electron transport in a wide range of applications, from molecular
electronics to catalytic reactions.
article_processing_charge: No
article_type: original
author:
- first_name: Wendu
full_name: Ding, Wendu
last_name: Ding
- first_name: Matthieu
full_name: Koepf, Matthieu
last_name: Koepf
- first_name: Christopher
full_name: Koenigsmann, Christopher
last_name: Koenigsmann
- first_name: Arunabh
full_name: Batra, Arunabh
last_name: Batra
- first_name: Latha
full_name: Venkataraman, Latha
id: 9ebb78a5-cc0d-11ee-8322-fae086a32caf
last_name: Venkataraman
orcid: 0000-0002-6957-6089
- first_name: Christian F. A.
full_name: Negre, Christian F. A.
last_name: Negre
- first_name: Gary W.
full_name: Brudvig, Gary W.
last_name: Brudvig
- first_name: Robert H.
full_name: Crabtree, Robert H.
last_name: Crabtree
- first_name: Charles A.
full_name: Schmuttenmaer, Charles A.
last_name: Schmuttenmaer
- first_name: Victor S.
full_name: Batista, Victor S.
last_name: Batista
citation:
ama: Ding W, Koepf M, Koenigsmann C, et al. Computational design of intrinsic molecular
rectifiers based on asymmetric functionalization of N-Phenylbenzamide. Journal
of Chemical Theory and Computation. 2015;11(12):5888-5896. doi:10.1021/acs.jctc.5b00823
apa: Ding, W., Koepf, M., Koenigsmann, C., Batra, A., Venkataraman, L., Negre, C.
F. A., … Batista, V. S. (2015). Computational design of intrinsic molecular rectifiers
based on asymmetric functionalization of N-Phenylbenzamide. Journal of Chemical
Theory and Computation. American Chemical Society. https://doi.org/10.1021/acs.jctc.5b00823
chicago: Ding, Wendu, Matthieu Koepf, Christopher Koenigsmann, Arunabh Batra, Latha
Venkataraman, Christian F. A. Negre, Gary W. Brudvig, Robert H. Crabtree, Charles
A. Schmuttenmaer, and Victor S. Batista. “Computational Design of Intrinsic Molecular
Rectifiers Based on Asymmetric Functionalization of N-Phenylbenzamide.” Journal
of Chemical Theory and Computation. American Chemical Society, 2015. https://doi.org/10.1021/acs.jctc.5b00823.
ieee: W. Ding et al., “Computational design of intrinsic molecular rectifiers
based on asymmetric functionalization of N-Phenylbenzamide,” Journal of Chemical
Theory and Computation, vol. 11, no. 12. American Chemical Society, pp. 5888–5896,
2015.
ista: Ding W, Koepf M, Koenigsmann C, Batra A, Venkataraman L, Negre CFA, Brudvig
GW, Crabtree RH, Schmuttenmaer CA, Batista VS. 2015. Computational design of intrinsic
molecular rectifiers based on asymmetric functionalization of N-Phenylbenzamide.
Journal of Chemical Theory and Computation. 11(12), 5888–5896.
mla: Ding, Wendu, et al. “Computational Design of Intrinsic Molecular Rectifiers
Based on Asymmetric Functionalization of N-Phenylbenzamide.” Journal of Chemical
Theory and Computation, vol. 11, no. 12, American Chemical Society, 2015,
pp. 5888–96, doi:10.1021/acs.jctc.5b00823.
short: W. Ding, M. Koepf, C. Koenigsmann, A. Batra, L. Venkataraman, C.F.A. Negre,
G.W. Brudvig, R.H. Crabtree, C.A. Schmuttenmaer, V.S. Batista, Journal of Chemical
Theory and Computation 11 (2015) 5888–5896.
date_created: 2024-09-09T09:42:20Z
date_published: 2015-11-03T00:00:00Z
date_updated: 2024-12-18T10:33:40Z
day: '03'
doi: 10.1021/acs.jctc.5b00823
extern: '1'
external_id:
pmid:
- '26642992'
intvolume: ' 11'
issue: '12'
language:
- iso: eng
month: '11'
oa_version: None
page: 5888-5896
pmid: 1
publication: Journal of Chemical Theory and Computation
publication_identifier:
eissn:
- 1549-9626
issn:
- 1549-9618
publication_status: published
publisher: American Chemical Society
quality_controlled: '1'
scopus_import: '1'
status: public
title: Computational design of intrinsic molecular rectifiers based on asymmetric
functionalization of N-Phenylbenzamide
type: journal_article
user_id: 2DF688A6-F248-11E8-B48F-1D18A9856A87
volume: 11
year: '2015'
...
---
OA_type: closed access
_id: '17968'
abstract:
- lang: eng
text: While the electrical conductivity of bulk-scale group 14 materials such as
diamond carbon, silicon, and germanium is well understood, there is a gap in knowledge
regarding the conductivity of these materials at the nano and molecular scales.
Filling this gap is important because integrated circuits have shrunk so far that
their active regions, which rely so heavily on silicon and germanium, begin to
resemble ornate molecules rather than extended solids. Here we unveil a new approach
for synthesizing atomically discrete wires of germanium and present the first
conductance measurements of molecular germanium using a scanning tunneling microscope-based
break-junction (STM-BJ) technique. Our findings show that germanium and silicon
wires are nearly identical in conductivity at the molecular scale, and that both
are much more conductive than aliphatic carbon. We demonstrate that the strong
donor ability of C–Ge σ-bonds can be used to raise the energy of the anchor lone
pair and increase conductance. Furthermore, the oligogermane wires behave as conductance
switches that function through stereoelectronic logic. These devices can be trained
to operate with a higher switching factor by repeatedly compressing and elongating
the molecular junction.
article_processing_charge: No
article_type: original
author:
- first_name: Timothy A.
full_name: Su, Timothy A.
last_name: Su
- first_name: Haixing
full_name: Li, Haixing
last_name: Li
- first_name: Vivian
full_name: Zhang, Vivian
last_name: Zhang
- first_name: Madhav
full_name: Neupane, Madhav
last_name: Neupane
- first_name: Arunabh
full_name: Batra, Arunabh
last_name: Batra
- first_name: Rebekka S.
full_name: Klausen, Rebekka S.
last_name: Klausen
- first_name: Bharat
full_name: Kumar, Bharat
last_name: Kumar
- first_name: Michael L.
full_name: Steigerwald, Michael L.
last_name: Steigerwald
- first_name: Latha
full_name: Venkataraman, Latha
id: 9ebb78a5-cc0d-11ee-8322-fae086a32caf
last_name: Venkataraman
orcid: 0000-0002-6957-6089
- first_name: Colin
full_name: Nuckolls, Colin
last_name: Nuckolls
citation:
ama: Su TA, Li H, Zhang V, et al. Single-molecule conductance in atomically precise
Germanium wires. Journal of the American Chemical Society. 2015;137(38):12400-12405.
doi:10.1021/jacs.5b08155
apa: Su, T. A., Li, H., Zhang, V., Neupane, M., Batra, A., Klausen, R. S., … Nuckolls,
C. (2015). Single-molecule conductance in atomically precise Germanium wires.
Journal of the American Chemical Society. American Chemical Society. https://doi.org/10.1021/jacs.5b08155
chicago: Su, Timothy A., Haixing Li, Vivian Zhang, Madhav Neupane, Arunabh Batra,
Rebekka S. Klausen, Bharat Kumar, Michael L. Steigerwald, Latha Venkataraman,
and Colin Nuckolls. “Single-Molecule Conductance in Atomically Precise Germanium
Wires.” Journal of the American Chemical Society. American Chemical Society,
2015. https://doi.org/10.1021/jacs.5b08155.
ieee: T. A. Su et al., “Single-molecule conductance in atomically precise
Germanium wires,” Journal of the American Chemical Society, vol. 137, no.
38. American Chemical Society, pp. 12400–12405, 2015.
ista: Su TA, Li H, Zhang V, Neupane M, Batra A, Klausen RS, Kumar B, Steigerwald
ML, Venkataraman L, Nuckolls C. 2015. Single-molecule conductance in atomically
precise Germanium wires. Journal of the American Chemical Society. 137(38), 12400–12405.
mla: Su, Timothy A., et al. “Single-Molecule Conductance in Atomically Precise Germanium
Wires.” Journal of the American Chemical Society, vol. 137, no. 38, American
Chemical Society, 2015, pp. 12400–05, doi:10.1021/jacs.5b08155.
short: T.A. Su, H. Li, V. Zhang, M. Neupane, A. Batra, R.S. Klausen, B. Kumar, M.L.
Steigerwald, L. Venkataraman, C. Nuckolls, Journal of the American Chemical Society
137 (2015) 12400–12405.
date_created: 2024-09-09T09:43:25Z
date_published: 2015-09-16T00:00:00Z
date_updated: 2024-12-18T11:24:37Z
day: '16'
doi: 10.1021/jacs.5b08155
extern: '1'
external_id:
pmid:
- '26373928'
intvolume: ' 137'
issue: '38'
language:
- iso: eng
month: '09'
oa_version: None
page: 12400-12405
pmid: 1
publication: Journal of the American Chemical Society
publication_identifier:
eissn:
- 1520-5126
issn:
- 0002-7863
publication_status: published
publisher: American Chemical Society
quality_controlled: '1'
scopus_import: '1'
status: public
title: Single-molecule conductance in atomically precise Germanium wires
type: journal_article
user_id: 2DF688A6-F248-11E8-B48F-1D18A9856A87
volume: 137
year: '2015'
...
---
OA_place: repository
OA_type: green
_id: '17969'
abstract:
- lang: eng
text: Recent experiments have shown that transport properties of molecular-scale
devices can be reversibly altered by the surrounding solvent. Here, we use a combination
of first-principles calculations and experiment to explain this change in transport
properties through a shift in the local electrostatic potential at the junction
caused by nearby conducting and solvent molecules chemically bound to the electrodes.
This effect is found to alter the conductance of 4,4′-bipyridine-gold junctions
by more than 50%. Moreover, we develop a general electrostatic model that quantitatively
relates the conductance and dipoles associated with the bound solvent and conducting
molecules. Our work shows that solvent-induced effects can be used to control
charge and energy transport at molecular-scale interfaces.
article_processing_charge: No
article_type: letter_note
arxiv: 1
author:
- first_name: Michele
full_name: Kotiuga, Michele
last_name: Kotiuga
- first_name: Pierre
full_name: Darancet, Pierre
last_name: Darancet
- first_name: Carlos R.
full_name: Arroyo, Carlos R.
last_name: Arroyo
- first_name: Latha
full_name: Venkataraman, Latha
id: 9ebb78a5-cc0d-11ee-8322-fae086a32caf
last_name: Venkataraman
orcid: 0000-0002-6957-6089
- first_name: Jeffrey B.
full_name: Neaton, Jeffrey B.
last_name: Neaton
citation:
ama: Kotiuga M, Darancet P, Arroyo CR, Venkataraman L, Neaton JB. Adsorption-induced
solvent-based electrostatic gating of charge transport through molecular junctions.
Nano Letters. 2015;15(7):4498-4503. doi:10.1021/acs.nanolett.5b00990
apa: Kotiuga, M., Darancet, P., Arroyo, C. R., Venkataraman, L., & Neaton, J.
B. (2015). Adsorption-induced solvent-based electrostatic gating of charge transport
through molecular junctions. Nano Letters. American Chemical Society. https://doi.org/10.1021/acs.nanolett.5b00990
chicago: Kotiuga, Michele, Pierre Darancet, Carlos R. Arroyo, Latha Venkataraman,
and Jeffrey B. Neaton. “Adsorption-Induced Solvent-Based Electrostatic Gating
of Charge Transport through Molecular Junctions.” Nano Letters. American
Chemical Society, 2015. https://doi.org/10.1021/acs.nanolett.5b00990.
ieee: M. Kotiuga, P. Darancet, C. R. Arroyo, L. Venkataraman, and J. B. Neaton,
“Adsorption-induced solvent-based electrostatic gating of charge transport through
molecular junctions,” Nano Letters, vol. 15, no. 7. American Chemical Society,
pp. 4498–4503, 2015.
ista: Kotiuga M, Darancet P, Arroyo CR, Venkataraman L, Neaton JB. 2015. Adsorption-induced
solvent-based electrostatic gating of charge transport through molecular junctions.
Nano Letters. 15(7), 4498–4503.
mla: Kotiuga, Michele, et al. “Adsorption-Induced Solvent-Based Electrostatic Gating
of Charge Transport through Molecular Junctions.” Nano Letters, vol. 15,
no. 7, American Chemical Society, 2015, pp. 4498–503, doi:10.1021/acs.nanolett.5b00990.
short: M. Kotiuga, P. Darancet, C.R. Arroyo, L. Venkataraman, J.B. Neaton, Nano
Letters 15 (2015) 4498–4503.
date_created: 2024-09-09T09:44:13Z
date_published: 2015-06-12T00:00:00Z
date_updated: 2024-12-18T11:28:49Z
day: '12'
doi: 10.1021/acs.nanolett.5b00990
extern: '1'
external_id:
arxiv:
- '1410.1439'
intvolume: ' 15'
issue: '7'
language:
- iso: eng
main_file_link:
- open_access: '1'
url: https://doi.org/10.48550/arXiv.1410.1439
month: '06'
oa: 1
oa_version: Preprint
page: 4498-4503
publication: Nano Letters
publication_identifier:
eissn:
- 1530-6992
issn:
- 1530-6984
publication_status: published
publisher: American Chemical Society
quality_controlled: '1'
scopus_import: '1'
status: public
title: Adsorption-induced solvent-based electrostatic gating of charge transport through
molecular junctions
type: journal_article
user_id: 2DF688A6-F248-11E8-B48F-1D18A9856A87
volume: 15
year: '2015'
...