---
OA_place: repository
OA_type: green
_id: '1376'
abstract:
- lang: eng
text: 'We consider the distributed synthesis problem for temporal logic specifications.
Traditionally, the problem has been studied for LTL, and the previous results
show that the problem is decidable iff there is no information fork in the architecture.
We consider the problem for fragments of LTL and our main results are as follows:
(1) We show that the problem is undecidable for architectures with information
forks even for the fragment of LTL with temporal operators restricted to next
and eventually. (2) For specifications restricted to globally along with non-nested
next operators, we establish decidability (in EXPSPACE) for star architectures
where the processes receive disjoint inputs, whereas we establish undecidability
for architectures containing an information fork-meet structure. (3) Finally,
we consider LTL without the next operator, and establish decidability (NEXPTIME-complete)
for all architectures for a fragment that consists of a set of safety assumptions,
and a set of guarantees where each guarantee is a safety, reachability, or liveness
condition.'
article_processing_charge: No
author:
- first_name: Krishnendu
full_name: Chatterjee, Krishnendu
id: 2E5DCA20-F248-11E8-B48F-1D18A9856A87
last_name: Chatterjee
orcid: 0000-0002-4561-241X
- first_name: Thomas A
full_name: Henzinger, Thomas A
id: 40876CD8-F248-11E8-B48F-1D18A9856A87
last_name: Henzinger
orcid: 0000−0002−2985−7724
- first_name: Jan
full_name: Otop, Jan
id: 2FC5DA74-F248-11E8-B48F-1D18A9856A87
last_name: Otop
- first_name: Andreas
full_name: Pavlogiannis, Andreas
id: 49704004-F248-11E8-B48F-1D18A9856A87
last_name: Pavlogiannis
orcid: 0000-0002-8943-0722
citation:
ama: 'Chatterjee K, Henzinger TA, Otop J, Pavlogiannis A. Distributed synthesis
for LTL fragments. In: 13th International Conference on Formal Methods in Computer-Aided
Design. IEEE; 2013:18-25. doi:10.1109/FMCAD.2013.6679386'
apa: 'Chatterjee, K., Henzinger, T. A., Otop, J., & Pavlogiannis, A. (2013).
Distributed synthesis for LTL fragments. In 13th International Conference on
Formal Methods in Computer-Aided Design (pp. 18–25). Portland, OR, United
States: IEEE. https://doi.org/10.1109/FMCAD.2013.6679386'
chicago: Chatterjee, Krishnendu, Thomas A Henzinger, Jan Otop, and Andreas Pavlogiannis.
“Distributed Synthesis for LTL Fragments.” In 13th International Conference
on Formal Methods in Computer-Aided Design, 18–25. IEEE, 2013. https://doi.org/10.1109/FMCAD.2013.6679386.
ieee: K. Chatterjee, T. A. Henzinger, J. Otop, and A. Pavlogiannis, “Distributed
synthesis for LTL fragments,” in 13th International Conference on Formal Methods
in Computer-Aided Design, Portland, OR, United States, 2013, pp. 18–25.
ista: 'Chatterjee K, Henzinger TA, Otop J, Pavlogiannis A. 2013. Distributed synthesis
for LTL fragments. 13th International Conference on Formal Methods in Computer-Aided
Design. FMCAD: Formal Methods in Computer-Aided Design, 18–25.'
mla: Chatterjee, Krishnendu, et al. “Distributed Synthesis for LTL Fragments.” 13th
International Conference on Formal Methods in Computer-Aided Design, IEEE,
2013, pp. 18–25, doi:10.1109/FMCAD.2013.6679386.
short: K. Chatterjee, T.A. Henzinger, J. Otop, A. Pavlogiannis, in:, 13th International
Conference on Formal Methods in Computer-Aided Design, IEEE, 2013, pp. 18–25.
conference:
end_date: 2013-10-23
location: Portland, OR, United States
name: 'FMCAD: Formal Methods in Computer-Aided Design'
start_date: 2013-10-20
corr_author: '1'
date_created: 2018-12-11T11:51:40Z
date_published: 2013-12-11T00:00:00Z
date_updated: 2025-06-26T08:33:43Z
day: '11'
department:
- _id: KrCh
- _id: ToHe
doi: 10.1109/FMCAD.2013.6679386
ec_funded: 1
language:
- iso: eng
main_file_link:
- open_access: '1'
url: https://doi.org/10.15479/AT:IST-2013-130-v1-1
month: '12'
oa: 1
oa_version: Preprint
page: 18 - 25
project:
- _id: 2584A770-B435-11E9-9278-68D0E5697425
call_identifier: FWF
grant_number: P 23499-N23
name: Modern Graph Algorithmic Techniques in Formal Verification
- _id: 25832EC2-B435-11E9-9278-68D0E5697425
call_identifier: FWF
grant_number: S 11407_N23
name: Rigorous Systems Engineering
- _id: 2581B60A-B435-11E9-9278-68D0E5697425
call_identifier: FP7
grant_number: '279307'
name: 'Quantitative Graph Games: Theory and Applications'
- _id: 25EE3708-B435-11E9-9278-68D0E5697425
call_identifier: FP7
grant_number: '267989'
name: Quantitative Reactive Modeling
- _id: 2587B514-B435-11E9-9278-68D0E5697425
name: Microsoft Research Faculty Fellowship
publication: 13th International Conference on Formal Methods in Computer-Aided Design
publication_status: published
publisher: IEEE
publist_id: '5835'
quality_controlled: '1'
related_material:
record:
- id: '5406'
relation: earlier_version
status: public
scopus_import: '1'
status: public
title: Distributed synthesis for LTL fragments
type: conference
user_id: 2DF688A6-F248-11E8-B48F-1D18A9856A87
year: '2013'
...
---
_id: '1385'
abstract:
- lang: eng
text: It is often difficult to correctly implement a Boolean controller for a complex
system, especially when concurrency is involved. Yet, it may be easy to formally
specify a controller. For instance, for a pipelined processor it suffices to state
that the visible behavior of the pipelined system should be identical to a non-pipelined
reference system (Burch-Dill paradigm). We present a novel procedure to efficiently
synthesize multiple Boolean control signals from a specification given as a quantified
first-order formula (with a specific quantifier structure). Our approach uses
uninterpreted functions to abstract details of the design. We construct an unsatisfiable
SMT formula from the given specification. Then, from just one proof of unsatisfiability,
we use a variant of Craig interpolation to compute multiple coordinated interpolants
that implement the Boolean control signals. Our method avoids iterative learning
and back-substitution of the control functions. We applied our approach to synthesize
a controller for a simple two-stage pipelined processor, and present first experimental
results.
acknowledgement: "This research was supported by the European Commission through project\r\nDIAMOND
\ (FP7-2009-IST-4-248613), and QUAINT (I774-N23), "
arxiv: 1
author:
- first_name: Georg
full_name: Hofferek, Georg
last_name: Hofferek
- first_name: Ashutosh
full_name: Gupta, Ashutosh
id: 335E5684-F248-11E8-B48F-1D18A9856A87
last_name: Gupta
- first_name: Bettina
full_name: Könighofer, Bettina
last_name: Könighofer
- first_name: Jie
full_name: Jiang, Jie
last_name: Jiang
- first_name: Roderick
full_name: Bloem, Roderick
last_name: Bloem
citation:
ama: 'Hofferek G, Gupta A, Könighofer B, Jiang J, Bloem R. Synthesizing multiple
boolean functions using interpolation on a single proof. In: 2013 Formal Methods
in Computer-Aided Design. IEEE; 2013:77-84. doi:10.1109/FMCAD.2013.6679394'
apa: 'Hofferek, G., Gupta, A., Könighofer, B., Jiang, J., & Bloem, R. (2013).
Synthesizing multiple boolean functions using interpolation on a single proof.
In 2013 Formal Methods in Computer-Aided Design (pp. 77–84). Portland,
OR, United States: IEEE. https://doi.org/10.1109/FMCAD.2013.6679394'
chicago: Hofferek, Georg, Ashutosh Gupta, Bettina Könighofer, Jie Jiang, and Roderick
Bloem. “Synthesizing Multiple Boolean Functions Using Interpolation on a Single
Proof.” In 2013 Formal Methods in Computer-Aided Design, 77–84. IEEE, 2013.
https://doi.org/10.1109/FMCAD.2013.6679394.
ieee: G. Hofferek, A. Gupta, B. Könighofer, J. Jiang, and R. Bloem, “Synthesizing
multiple boolean functions using interpolation on a single proof,” in 2013
Formal Methods in Computer-Aided Design, Portland, OR, United States, 2013,
pp. 77–84.
ista: 'Hofferek G, Gupta A, Könighofer B, Jiang J, Bloem R. 2013. Synthesizing multiple
boolean functions using interpolation on a single proof. 2013 Formal Methods in
Computer-Aided Design. FMCAD: Formal Methods in Computer-Aided Design, 77–84.'
mla: Hofferek, Georg, et al. “Synthesizing Multiple Boolean Functions Using Interpolation
on a Single Proof.” 2013 Formal Methods in Computer-Aided Design, IEEE,
2013, pp. 77–84, doi:10.1109/FMCAD.2013.6679394.
short: G. Hofferek, A. Gupta, B. Könighofer, J. Jiang, R. Bloem, in:, 2013 Formal
Methods in Computer-Aided Design, IEEE, 2013, pp. 77–84.
conference:
end_date: 2013-10-23
location: Portland, OR, United States
name: 'FMCAD: Formal Methods in Computer-Aided Design'
start_date: 2013-10-20
date_created: 2018-12-11T11:51:43Z
date_published: 2013-12-11T00:00:00Z
date_updated: 2024-10-21T06:02:56Z
day: '11'
department:
- _id: ToHe
doi: 10.1109/FMCAD.2013.6679394
ec_funded: 1
external_id:
arxiv:
- '1308.4767'
language:
- iso: eng
main_file_link:
- open_access: '1'
url: http://arxiv.org/abs/1308.4767
month: '12'
oa: 1
oa_version: Preprint
page: 77 - 84
project:
- _id: 25832EC2-B435-11E9-9278-68D0E5697425
call_identifier: FWF
grant_number: S 11407_N23
name: Rigorous Systems Engineering
- _id: 25EE3708-B435-11E9-9278-68D0E5697425
call_identifier: FP7
grant_number: '267989'
name: Quantitative Reactive Modeling
publication: 2013 Formal Methods in Computer-Aided Design
publication_status: published
publisher: IEEE
publist_id: '5825'
quality_controlled: '1'
scopus_import: '1'
status: public
title: Synthesizing multiple boolean functions using interpolation on a single proof
type: conference
user_id: 2DF688A6-F248-11E8-B48F-1D18A9856A87
year: '2013'
...
---
_id: '1387'
abstract:
- lang: eng
text: Choices made by nondeterministic word automata depend on both the past (the
prefix of the word read so far) and the future (the suffix yet to be read). In
several applications, most notably synthesis, the future is diverse or unknown,
leading to algorithms that are based on deterministic automata. Hoping to retain
some of the advantages of nondeterministic automata, researchers have studied
restricted classes of nondeterministic automata. Three such classes are nondeterministic
automata that are good for trees (GFT; i.e., ones that can be expanded to tree
automata accepting the derived tree languages, thus whose choices should satisfy
diverse futures), good for games (GFG; i.e., ones whose choices depend only on
the past), and determinizable by pruning (DBP; i.e., ones that embody equivalent
deterministic automata). The theoretical properties and relative merits of the
different classes are still open, having vagueness on whether they really differ
from deterministic automata. In particular, while DBP ⊆ GFG ⊆ GFT, it is not known
whether every GFT automaton is GFG and whether every GFG automaton is DBP. Also
open is the possible succinctness of GFG and GFT automata compared to deterministic
automata. We study these problems for ω-regular automata with all common acceptance
conditions. We show that GFT=GFG⊃DBP, and describe a determinization construction
for GFG automata.
acknowledgement: and ERC Grant QUALITY.
alternative_title:
- LNCS
article_processing_charge: No
author:
- first_name: Udi
full_name: Boker, Udi
id: 31E297B6-F248-11E8-B48F-1D18A9856A87
last_name: Boker
- first_name: Denis
full_name: Kuperberg, Denis
last_name: Kuperberg
- first_name: Orna
full_name: Kupferman, Orna
last_name: Kupferman
- first_name: Michał
full_name: Skrzypczak, Michał
last_name: Skrzypczak
citation:
ama: Boker U, Kuperberg D, Kupferman O, Skrzypczak M. Nondeterminism in the presence
of a diverse or unknown future. 2013;7966(PART 2):89-100. doi:10.1007/978-3-642-39212-2_11
apa: 'Boker, U., Kuperberg, D., Kupferman, O., & Skrzypczak, M. (2013). Nondeterminism
in the presence of a diverse or unknown future. Presented at the ICALP: Automata,
Languages and Programming, Riga, Latvia: Springer. https://doi.org/10.1007/978-3-642-39212-2_11'
chicago: Boker, Udi, Denis Kuperberg, Orna Kupferman, and Michał Skrzypczak. “Nondeterminism
in the Presence of a Diverse or Unknown Future.” Lecture Notes in Computer Science.
Springer, 2013. https://doi.org/10.1007/978-3-642-39212-2_11.
ieee: U. Boker, D. Kuperberg, O. Kupferman, and M. Skrzypczak, “Nondeterminism in
the presence of a diverse or unknown future,” vol. 7966, no. PART 2. Springer,
pp. 89–100, 2013.
ista: Boker U, Kuperberg D, Kupferman O, Skrzypczak M. 2013. Nondeterminism in the
presence of a diverse or unknown future. 7966(PART 2), 89–100.
mla: Boker, Udi, et al. Nondeterminism in the Presence of a Diverse or Unknown
Future. Vol. 7966, no. PART 2, Springer, 2013, pp. 89–100, doi:10.1007/978-3-642-39212-2_11.
short: U. Boker, D. Kuperberg, O. Kupferman, M. Skrzypczak, 7966 (2013) 89–100.
conference:
end_date: 2013-07-12
location: Riga, Latvia
name: 'ICALP: Automata, Languages and Programming'
start_date: 2013-07-08
date_created: 2018-12-11T11:51:44Z
date_published: 2013-07-01T00:00:00Z
date_updated: 2020-08-11T10:09:09Z
day: '01'
ddc:
- '000'
department:
- _id: ToHe
doi: 10.1007/978-3-642-39212-2_11
ec_funded: 1
file:
- access_level: open_access
checksum: 98bc02e3793072e279ec8d364b381ff3
content_type: application/pdf
creator: dernst
date_created: 2020-05-15T11:05:50Z
date_updated: 2020-07-14T12:44:48Z
file_id: '7857'
file_name: 2013_ICALP_Boker.pdf
file_size: 276982
relation: main_file
file_date_updated: 2020-07-14T12:44:48Z
has_accepted_license: '1'
intvolume: ' 7966'
issue: PART 2
language:
- iso: eng
month: '07'
oa: 1
oa_version: Submitted Version
page: 89 - 100
project:
- _id: 25832EC2-B435-11E9-9278-68D0E5697425
call_identifier: FWF
grant_number: S 11407_N23
name: Rigorous Systems Engineering
- _id: 25EE3708-B435-11E9-9278-68D0E5697425
call_identifier: FP7
grant_number: '267989'
name: Quantitative Reactive Modeling
publication_status: published
publisher: Springer
publist_id: '5823'
quality_controlled: '1'
scopus_import: 1
series_title: Lecture Notes in Computer Science
status: public
title: Nondeterminism in the presence of a diverse or unknown future
type: conference
user_id: 2DF688A6-F248-11E8-B48F-1D18A9856A87
volume: 7966
year: '2013'
...
---
_id: '1442'
abstract:
- lang: eng
text: We give a cohomological interpretation of both the Kac polynomial and the
refined Donaldson-Thomas-invariants of quivers. This interpretation yields a proof
of a conjecture of Kac from 1982 and gives a new perspective on recent work of
Kontsevich-Soibelman. Thisis achieved by computing, via an arithmetic Fourier
transform, the dimensions of the isotypical components of the cohomology of associated
Nakajima quiver varieties under the action of a Weyl group. The generating function
of the corresponding Poincare polynomials is an extension of Hua's formula for
Kac polynomials of quivers involving Hall-Littlewood symmetric functions. The
resulting formulae contain a wide range of information on the geometry of the
quiver varieties.
acknowledgement: |-
The first author thanks the Royal Society for funding his research 2005-2012 in the form of a Royal Society University Research Fellowship as well as the Mathematical Institute and Wadham College in Oxford for a very productive environment. The second author is supported by Agence Nationale de la Recherche grant
ANR-09-JCJC-0102-01. The third author is supported by the NSF grant DMS-1101484 and a Research Scholarship from the Clay Mathematical Institute.
author:
- first_name: Tamas
full_name: Tamas Hausel
id: 4A0666D8-F248-11E8-B48F-1D18A9856A87
last_name: Hausel
- first_name: Emmanuel
full_name: Letellier, Emmanuel
last_name: Letellier
- first_name: Fernando
full_name: Rodríguez Villegas, Fernando
last_name: Rodríguez Villegas
citation:
ama: Hausel T, Letellier E, Rodríguez Villegas F. Positivity for Kac polynomials
and DT-invariants of quivers. Annals of Mathematics. 2013;177(3):1147-1168.
doi:10.4007/annals.2013.177.3.8
apa: Hausel, T., Letellier, E., & Rodríguez Villegas, F. (2013). Positivity
for Kac polynomials and DT-invariants of quivers. Annals of Mathematics.
Princeton University Press. https://doi.org/10.4007/annals.2013.177.3.8
chicago: Hausel, Tamás, Emmanuel Letellier, and Fernando Rodríguez Villegas. “Positivity
for Kac Polynomials and DT-Invariants of Quivers.” Annals of Mathematics.
Princeton University Press, 2013. https://doi.org/10.4007/annals.2013.177.3.8.
ieee: T. Hausel, E. Letellier, and F. Rodríguez Villegas, “Positivity for Kac polynomials
and DT-invariants of quivers,” Annals of Mathematics, vol. 177, no. 3.
Princeton University Press, pp. 1147–1168, 2013.
ista: Hausel T, Letellier E, Rodríguez Villegas F. 2013. Positivity for Kac polynomials
and DT-invariants of quivers. Annals of Mathematics. 177(3), 1147–1168.
mla: Hausel, Tamás, et al. “Positivity for Kac Polynomials and DT-Invariants of
Quivers.” Annals of Mathematics, vol. 177, no. 3, Princeton University
Press, 2013, pp. 1147–68, doi:10.4007/annals.2013.177.3.8.
short: T. Hausel, E. Letellier, F. Rodríguez Villegas, Annals of Mathematics 177
(2013) 1147–1168.
date_created: 2018-12-11T11:52:02Z
date_published: 2013-01-01T00:00:00Z
date_updated: 2021-01-12T06:50:47Z
day: '01'
doi: 10.4007/annals.2013.177.3.8
extern: 1
intvolume: ' 177'
issue: '3'
main_file_link:
- open_access: '1'
url: http://arxiv.org/abs/1204.2375
month: '01'
oa: 1
page: 1147 - 1168
publication: Annals of Mathematics
publication_status: published
publisher: Princeton University Press
publist_id: '5754'
quality_controlled: 0
status: public
title: Positivity for Kac polynomials and DT-invariants of quivers
type: journal_article
volume: 177
year: '2013'
...
---
_id: '1443'
abstract:
- lang: eng
text: 'Here we survey several results and conjectures on the cohomology of the total
space of the Hitchin system: the moduli space of semi-stable rank n and degree
d Higgs bundles on a complex algebraic curve C. The picture emerging is a dynamic
mixture of ideas originating in theoretical physics such as gauge theory and mirror
symmetry, Weil conjectures in arithmetic algebraic geometry, representation theory
of finite groups of Lie type and Langlands duality in number theory.'
alternative_title:
- Advanced Lectures in Mathematics
author:
- first_name: Tamas
full_name: Tamas Hausel
id: 4A0666D8-F248-11E8-B48F-1D18A9856A87
last_name: Hausel
citation:
ama: 'Hausel T. Global topology of the Hitchin system. In: Handbook of Moduli:
Volume II. Vol 25. International Press; 2013:29-70.'
apa: 'Hausel, T. (2013). Global topology of the Hitchin system. In Handbook of
Moduli: Volume II (Vol. 25, pp. 29–70). International Press.'
chicago: 'Hausel, Tamás. “Global Topology of the Hitchin System.” In Handbook
of Moduli: Volume II, 25:29–70. International Press, 2013.'
ieee: 'T. Hausel, “Global topology of the Hitchin system,” in Handbook of Moduli:
Volume II, vol. 25, International Press, 2013, pp. 29–70.'
ista: 'Hausel T. 2013.Global topology of the Hitchin system. In: Handbook of Moduli:
Volume II. Advanced Lectures in Mathematics, vol. 25, 29–70.'
mla: 'Hausel, Tamás. “Global Topology of the Hitchin System.” Handbook of Moduli:
Volume II, vol. 25, International Press, 2013, pp. 29–70.'
short: 'T. Hausel, in:, Handbook of Moduli: Volume II, International Press, 2013,
pp. 29–70.'
date_created: 2018-12-11T11:52:03Z
date_published: 2013-03-15T00:00:00Z
date_updated: 2021-01-12T06:50:47Z
day: '15'
extern: 1
intvolume: ' 25'
main_file_link:
- open_access: '1'
url: http://arxiv.org/abs/1102.1717
month: '03'
oa: 1
page: 29 - 70
publication: 'Handbook of Moduli: Volume II'
publication_status: published
publisher: International Press
publist_id: '5753'
quality_controlled: 0
status: public
title: Global topology of the Hitchin system
type: book_chapter
volume: 25
year: '2013'
...
---
_id: '1469'
abstract:
- lang: eng
text: We study connections between the topology of generic character varieties of
fundamental groups of punctured Riemann surfaces, Macdonald polynomials, quiver
representations, Hilbert schemes on Cx × Cx, modular forms and multiplicities
in tensor products of irreducible characters of finite general linear groups.
acknowledgement: During the preparation of this paper TH was supported by a Royal
Society University Research Fellowship at the University of Oxford. EL was supported
by ANR-09-JCJC-0102-01. FRV was supported by NSF grant DMS-0200605, an FRA from
the University of Texas at Austin, EPSRC grant EP/G027110/1, Visiting Fellowships
at All Souls and Wadham Colleges in Oxford and a Research Scholarship from the Clay
Mathematical Institute.
author:
- first_name: Tamas
full_name: Tamas Hausel
id: 4A0666D8-F248-11E8-B48F-1D18A9856A87
last_name: Hausel
- first_name: Emmanuel
full_name: Letellier, Emmanuel
last_name: Letellier
- first_name: Fernando
full_name: Rodríguez Villegas, Fernando
last_name: Rodríguez Villegas
citation:
ama: Hausel T, Letellier E, Rodríguez Villegas F. Arithmetic harmonic analysis on
character and quiver varieties II. Advances in Mathematics. 2013;234:85-128.
doi:10.1016/j.aim.2012.10.009
apa: Hausel, T., Letellier, E., & Rodríguez Villegas, F. (2013). Arithmetic
harmonic analysis on character and quiver varieties II. Advances in Mathematics.
Academic Press. https://doi.org/10.1016/j.aim.2012.10.009
chicago: Hausel, Tamás, Emmanuel Letellier, and Fernando Rodríguez Villegas. “Arithmetic
Harmonic Analysis on Character and Quiver Varieties II.” Advances in Mathematics.
Academic Press, 2013. https://doi.org/10.1016/j.aim.2012.10.009.
ieee: T. Hausel, E. Letellier, and F. Rodríguez Villegas, “Arithmetic harmonic analysis
on character and quiver varieties II,” Advances in Mathematics, vol. 234.
Academic Press, pp. 85–128, 2013.
ista: Hausel T, Letellier E, Rodríguez Villegas F. 2013. Arithmetic harmonic analysis
on character and quiver varieties II. Advances in Mathematics. 234, 85–128.
mla: Hausel, Tamás, et al. “Arithmetic Harmonic Analysis on Character and Quiver
Varieties II.” Advances in Mathematics, vol. 234, Academic Press, 2013,
pp. 85–128, doi:10.1016/j.aim.2012.10.009.
short: T. Hausel, E. Letellier, F. Rodríguez Villegas, Advances in Mathematics 234
(2013) 85–128.
date_created: 2018-12-11T11:52:12Z
date_published: 2013-02-15T00:00:00Z
date_updated: 2021-01-12T06:50:57Z
day: '15'
doi: 10.1016/j.aim.2012.10.009
extern: 1
intvolume: ' 234'
month: '02'
page: 85 - 128
publication: Advances in Mathematics
publication_status: published
publisher: Academic Press
publist_id: '5724'
quality_controlled: 0
status: public
title: Arithmetic harmonic analysis on character and quiver varieties II
type: journal_article
volume: 234
year: '2013'
...
---
_id: '1470'
abstract:
- lang: eng
text: We show that a natural isomorphism between the rational cohomology groups
of the two zero-dimensional Hilbert schemes of n-points of two surfaces, the affine
plane minus the axes and the cotangent bundle of an elliptic curve, exchanges
the weight filtration on the first set of cohomology groups with the perverse
Leray filtration associated with a natural fibration on the second set of cohomology
groups. We discuss some associated hard Lefschetz phenomena.
acknowledgement: Mark Andrea A. de Cataldo was partially supported by N.S.A. and N.S.F.
Tamás Hausel was supported by a Royal Society University Research Fellowship. Luca
Migliorini was partially supported by PRIN 2007 project "Spazi di moduli e teoria
di Lie"
author:
- first_name: Mark
full_name: De Cataldo, Mark A
last_name: De Cataldo
- first_name: Tamas
full_name: Tamas Hausel
id: 4A0666D8-F248-11E8-B48F-1D18A9856A87
last_name: Hausel
- first_name: Luca
full_name: Migliorini, Luca
last_name: Migliorini
citation:
ama: De Cataldo M, Hausel T, Migliorini L. Exchange between perverse and weight
filtration for the Hilbert schemes of points of two surfaces. Journal of Singularities.
2013;7:23-38. doi:10.5427/jsing.2013.7c
apa: De Cataldo, M., Hausel, T., & Migliorini, L. (2013). Exchange between perverse
and weight filtration for the Hilbert schemes of points of two surfaces. Journal
of Singularities. Worldwide Center of Mathematics. https://doi.org/10.5427/jsing.2013.7c
chicago: De Cataldo, Mark, Tamás Hausel, and Luca Migliorini. “Exchange between
Perverse and Weight Filtration for the Hilbert Schemes of Points of Two Surfaces.”
Journal of Singularities. Worldwide Center of Mathematics, 2013. https://doi.org/10.5427/jsing.2013.7c.
ieee: M. De Cataldo, T. Hausel, and L. Migliorini, “Exchange between perverse and
weight filtration for the Hilbert schemes of points of two surfaces,” Journal
of Singularities, vol. 7. Worldwide Center of Mathematics, pp. 23–38, 2013.
ista: De Cataldo M, Hausel T, Migliorini L. 2013. Exchange between perverse and
weight filtration for the Hilbert schemes of points of two surfaces. Journal of
Singularities. 7, 23–38.
mla: De Cataldo, Mark, et al. “Exchange between Perverse and Weight Filtration for
the Hilbert Schemes of Points of Two Surfaces.” Journal of Singularities,
vol. 7, Worldwide Center of Mathematics, 2013, pp. 23–38, doi:10.5427/jsing.2013.7c.
short: M. De Cataldo, T. Hausel, L. Migliorini, Journal of Singularities 7 (2013)
23–38.
date_created: 2018-12-11T11:52:12Z
date_published: 2013-01-01T00:00:00Z
date_updated: 2021-01-12T06:50:58Z
day: '01'
doi: 10.5427/jsing.2013.7c
extern: 1
intvolume: ' 7'
main_file_link:
- open_access: '1'
url: http://arxiv.org/abs/1012.2583
month: '01'
oa: 1
page: 23 - 38
publication: Journal of Singularities
publication_status: published
publisher: Worldwide Center of Mathematics
publist_id: '5725'
quality_controlled: 0
status: public
title: Exchange between perverse and weight filtration for the Hilbert schemes of
points of two surfaces
type: journal_article
volume: 7
year: '2013'
...
---
_id: '1785'
abstract:
- lang: eng
text: The geometric aspects of quantum mechanics are emphasized most prominently
by the concept of geometric phases, which are acquired whenever a quantum system
evolves along a path in Hilbert space, that is, the space of quantum states of
the system. The geometric phase is determined only by the shape of this path and
is, in its simplest form, a real number. However, if the system has degenerate
energy levels, then matrix-valued geometric state transformations, known as non-Abelian
holonomies-the effect of which depends on the order of two consecutive paths-can
be obtained. They are important, for example, for the creation of synthetic gauge
fields in cold atomic gases or the description of non-Abelian anyon statistics.
Moreover, there are proposals to exploit non-Abelian holonomic gates for the purposes
of noise-resilient quantum computation. In contrast to Abelian geometric operations,
non-Abelian ones have been observed only in nuclear quadrupole resonance experiments
with a large number of spins, and without full characterization of the geometric
process and its non-commutative nature. Here we realize non-Abelian non-adiabatic
holonomic quantum operations on a single, superconducting, artificial three-level
atom by applying a well-controlled, two-tone microwave drive. Using quantum process
tomography, we determine fidelities of the resulting non-commuting gates that
exceed 95 per cent. We show that two different quantum gates, originating from
two distinct paths in Hilbert space, yield non-equivalent transformations when
applied in different orders. This provides evidence for the non-Abelian character
of the implemented holonomic quantum operations. In combination with a non-trivial
two-quantum-bit gate, our method suggests a way to universal holonomic quantum
computing.
acknowledgement: This work is supported financially by GEOMDISS, the Swiss National
Science Foundation and ETH Zurich
author:
- first_name: Abdufarrukh
full_name: Abdumalikov, Abdufarrukh A
last_name: Abdumalikov
- first_name: Johannes M
full_name: Johannes Fink
id: 4B591CBA-F248-11E8-B48F-1D18A9856A87
last_name: Fink
orcid: 0000-0001-8112-028X
- first_name: K
full_name: Juliusson, K
last_name: Juliusson
- first_name: M
full_name: Pechal, M
last_name: Pechal
- first_name: Stefan
full_name: Berger, Stefan T
last_name: Berger
- first_name: Andreas
full_name: Wallraff, Andreas
last_name: Wallraff
- first_name: Stefan
full_name: Filipp, Stefan
last_name: Filipp
citation:
ama: Abdumalikov A, Fink JM, Juliusson K, et al. Experimental realization of non-Abelian
non-adiabatic geometric gates. Nature. 2013;496(7446):482-485. doi:10.1038/nature12010
apa: Abdumalikov, A., Fink, J. M., Juliusson, K., Pechal, M., Berger, S., Wallraff,
A., & Filipp, S. (2013). Experimental realization of non-Abelian non-adiabatic
geometric gates. Nature. Nature Publishing Group. https://doi.org/10.1038/nature12010
chicago: Abdumalikov, Abdufarrukh, Johannes M Fink, K Juliusson, M Pechal, Stefan
Berger, Andreas Wallraff, and Stefan Filipp. “Experimental Realization of Non-Abelian
Non-Adiabatic Geometric Gates.” Nature. Nature Publishing Group, 2013.
https://doi.org/10.1038/nature12010.
ieee: A. Abdumalikov et al., “Experimental realization of non-Abelian non-adiabatic
geometric gates,” Nature, vol. 496, no. 7446. Nature Publishing Group,
pp. 482–485, 2013.
ista: Abdumalikov A, Fink JM, Juliusson K, Pechal M, Berger S, Wallraff A, Filipp
S. 2013. Experimental realization of non-Abelian non-adiabatic geometric gates.
Nature. 496(7446), 482–485.
mla: Abdumalikov, Abdufarrukh, et al. “Experimental Realization of Non-Abelian Non-Adiabatic
Geometric Gates.” Nature, vol. 496, no. 7446, Nature Publishing Group,
2013, pp. 482–85, doi:10.1038/nature12010.
short: A. Abdumalikov, J.M. Fink, K. Juliusson, M. Pechal, S. Berger, A. Wallraff,
S. Filipp, Nature 496 (2013) 482–485.
date_created: 2018-12-11T11:54:00Z
date_published: 2013-04-25T00:00:00Z
date_updated: 2021-01-12T06:53:11Z
day: '25'
doi: 10.1038/nature12010
extern: 1
intvolume: ' 496'
issue: '7446'
month: '04'
page: 482 - 485
publication: Nature
publication_status: published
publisher: Nature Publishing Group
publist_id: '5329'
quality_controlled: 0
status: public
title: Experimental realization of non-Abelian non-adiabatic geometric gates
type: journal_article
volume: 496
year: '2013'
...
---
_id: '1786'
abstract:
- lang: eng
text: We report the experimental observation and a theoretical explanation of collective
suppression of linewidths for multiple superconducting qubits coupled to a good
cavity. This demonstrates how strong qubit-cavity coupling can significantly modify
the dephasing and dissipation processes that might be expected for individual
qubits, and can potentially improve coherence times in many-body circuit QED.
acknowledgement: J. K. acknowledges financial support from EPSRC program “TOPNES”
(EP/I031014/1) and EPSRC (EP/G004714/2)
author:
- first_name: Felix
full_name: Nissen, Felix
last_name: Nissen
- first_name: Johannes M
full_name: Johannes Fink
id: 4B591CBA-F248-11E8-B48F-1D18A9856A87
last_name: Fink
orcid: 0000-0001-8112-028X
- first_name: Jonas
full_name: Mlynek, Jonas A
last_name: Mlynek
- first_name: Andreas
full_name: Wallraff, Andreas
last_name: Wallraff
- first_name: Jonathan
full_name: Keeling, Jonathan M
last_name: Keeling
citation:
ama: Nissen F, Fink JM, Mlynek J, Wallraff A, Keeling J. Collective suppression
of linewidths in circuit QED. Physical Review Letters. 2013;110(20). doi:10.1103/PhysRevLett.110.203602
apa: Nissen, F., Fink, J. M., Mlynek, J., Wallraff, A., & Keeling, J. (2013).
Collective suppression of linewidths in circuit QED. Physical Review Letters.
American Physical Society. https://doi.org/10.1103/PhysRevLett.110.203602
chicago: Nissen, Felix, Johannes M Fink, Jonas Mlynek, Andreas Wallraff, and Jonathan
Keeling. “Collective Suppression of Linewidths in Circuit QED.” Physical Review
Letters. American Physical Society, 2013. https://doi.org/10.1103/PhysRevLett.110.203602.
ieee: F. Nissen, J. M. Fink, J. Mlynek, A. Wallraff, and J. Keeling, “Collective
suppression of linewidths in circuit QED,” Physical Review Letters, vol.
110, no. 20. American Physical Society, 2013.
ista: Nissen F, Fink JM, Mlynek J, Wallraff A, Keeling J. 2013. Collective suppression
of linewidths in circuit QED. Physical Review Letters. 110(20).
mla: Nissen, Felix, et al. “Collective Suppression of Linewidths in Circuit QED.”
Physical Review Letters, vol. 110, no. 20, American Physical Society, 2013,
doi:10.1103/PhysRevLett.110.203602.
short: F. Nissen, J.M. Fink, J. Mlynek, A. Wallraff, J. Keeling, Physical Review
Letters 110 (2013).
date_created: 2018-12-11T11:54:00Z
date_published: 2013-05-15T00:00:00Z
date_updated: 2021-01-12T06:53:11Z
day: '15'
doi: 10.1103/PhysRevLett.110.203602
extern: 1
intvolume: ' 110'
issue: '20'
main_file_link:
- open_access: '1'
url: http://arxiv.org/abs/1302.0665
month: '05'
oa: 1
publication: Physical Review Letters
publication_status: published
publisher: American Physical Society
publist_id: '5328'
quality_controlled: 0
status: public
title: Collective suppression of linewidths in circuit QED
type: journal_article
volume: 110
year: '2013'
...
---
_id: '1787'
abstract:
- lang: eng
text: When two indistinguishable single photons impinge at the two inputs of a beam
splitter they coalesce into a pair of photons appearing in either one of its two
outputs. This effect is due to the bosonic nature of photons and was first experimentally
observed by Hong, Ou and Mandel. Here, we present the observation of the Hong-Ou-Mandel
effect with two independent single-photon sources in the microwave frequency domain.
We probe the indistinguishability of single photons, created with a controllable
delay, in time-resolved second-order cross- and auto-correlation function measurements.
Using quadrature amplitude detection we are able to resolve different photon numbers
and detect coherence in and between the output arms. This scheme allows us to
fully characterize the two-mode entanglement of the spatially separated beam-splitter
output modes. Our experiments constitute a first step towards using two-photon
interference at microwave frequencies for quantum communication and information
processing.
acknowledgement: This work was supported by the European Research Council (ERC) through
a Starting Grant and by ETHZ. L.S. was supported by EU IP SOLID. A.B. and M.J.W.
were supported by NSERC, CIFAR and the Alfred P. Sloan Foundation
author:
- first_name: C
full_name: Lang, C
last_name: Lang
- first_name: Christopher
full_name: Eichler, Christopher
last_name: Eichler
- first_name: L.
full_name: Steffen, L. Kraig
last_name: Steffen
- first_name: Johannes M
full_name: Johannes Fink
id: 4B591CBA-F248-11E8-B48F-1D18A9856A87
last_name: Fink
orcid: 0000-0001-8112-028X
- first_name: Matthew
full_name: Woolley, Matthew J
last_name: Woolley
- first_name: Alexandre
full_name: Blais, Alexandre
last_name: Blais
- first_name: Andreas
full_name: Wallraff, Andreas
last_name: Wallraff
citation:
ama: Lang C, Eichler C, Steffen L, et al. Correlations, indistinguishability and
entanglement in Hong-Ou-Mandel experiments at microwave frequencies. Nature
Physics. 2013;9(6):345-348. doi:10.1038/nphys2612
apa: Lang, C., Eichler, C., Steffen, L., Fink, J. M., Woolley, M., Blais, A., &
Wallraff, A. (2013). Correlations, indistinguishability and entanglement in Hong-Ou-Mandel
experiments at microwave frequencies. Nature Physics. Nature Publishing
Group. https://doi.org/10.1038/nphys2612
chicago: Lang, C, Christopher Eichler, L. Steffen, Johannes M Fink, Matthew Woolley,
Alexandre Blais, and Andreas Wallraff. “Correlations, Indistinguishability and
Entanglement in Hong-Ou-Mandel Experiments at Microwave Frequencies.” Nature
Physics. Nature Publishing Group, 2013. https://doi.org/10.1038/nphys2612.
ieee: C. Lang et al., “Correlations, indistinguishability and entanglement
in Hong-Ou-Mandel experiments at microwave frequencies,” Nature Physics,
vol. 9, no. 6. Nature Publishing Group, pp. 345–348, 2013.
ista: Lang C, Eichler C, Steffen L, Fink JM, Woolley M, Blais A, Wallraff A. 2013.
Correlations, indistinguishability and entanglement in Hong-Ou-Mandel experiments
at microwave frequencies. Nature Physics. 9(6), 345–348.
mla: Lang, C., et al. “Correlations, Indistinguishability and Entanglement in Hong-Ou-Mandel
Experiments at Microwave Frequencies.” Nature Physics, vol. 9, no. 6, Nature
Publishing Group, 2013, pp. 345–48, doi:10.1038/nphys2612.
short: C. Lang, C. Eichler, L. Steffen, J.M. Fink, M. Woolley, A. Blais, A. Wallraff,
Nature Physics 9 (2013) 345–348.
date_created: 2018-12-11T11:54:00Z
date_published: 2013-06-01T00:00:00Z
date_updated: 2021-01-12T06:53:11Z
day: '01'
doi: 10.1038/nphys2612
extern: 1
intvolume: ' 9'
issue: '6'
month: '06'
page: 345 - 348
publication: Nature Physics
publication_status: published
publisher: Nature Publishing Group
publist_id: '5327'
quality_controlled: 0
status: public
title: Correlations, indistinguishability and entanglement in Hong-Ou-Mandel experiments
at microwave frequencies
type: journal_article
volume: 9
year: '2013'
...
---
_id: '1790'
abstract:
- lang: eng
text: In the September 12, 2013 issue of Nature, the Epi4K Consortium (. Allen etal.,
2013) reported sequencing 264patient trios with epileptic encephalopathies. The
Consortium focused on genes exceptionally intolerant to sequence variations and
found substantial interconnections with autism and intellectual disability gene
networks.
author:
- first_name: Gaia
full_name: Gaia Novarino
id: 3E57A680-F248-11E8-B48F-1D18A9856A87
last_name: Novarino
orcid: 0000-0002-7673-7178
- first_name: Seungtae
full_name: Baek, SeungTae
last_name: Baek
- first_name: Joseph
full_name: Gleeson, Joseph G
last_name: Gleeson
citation:
ama: 'Novarino G, Baek S, Gleeson J. The sacred disease: The puzzling genetics of
epileptic disorders. Neuron. 2013;80(1):9-11. doi:10.1016/j.neuron.2013.09.019'
apa: 'Novarino, G., Baek, S., & Gleeson, J. (2013). The sacred disease: The
puzzling genetics of epileptic disorders. Neuron. Elsevier. https://doi.org/10.1016/j.neuron.2013.09.019'
chicago: 'Novarino, Gaia, Seungtae Baek, and Joseph Gleeson. “The Sacred Disease:
The Puzzling Genetics of Epileptic Disorders.” Neuron. Elsevier, 2013.
https://doi.org/10.1016/j.neuron.2013.09.019.'
ieee: 'G. Novarino, S. Baek, and J. Gleeson, “The sacred disease: The puzzling genetics
of epileptic disorders,” Neuron, vol. 80, no. 1. Elsevier, pp. 9–11, 2013.'
ista: 'Novarino G, Baek S, Gleeson J. 2013. The sacred disease: The puzzling genetics
of epileptic disorders. Neuron. 80(1), 9–11.'
mla: 'Novarino, Gaia, et al. “The Sacred Disease: The Puzzling Genetics of Epileptic
Disorders.” Neuron, vol. 80, no. 1, Elsevier, 2013, pp. 9–11, doi:10.1016/j.neuron.2013.09.019.'
short: G. Novarino, S. Baek, J. Gleeson, Neuron 80 (2013) 9–11.
date_created: 2018-12-11T11:54:01Z
date_published: 2013-10-02T00:00:00Z
date_updated: 2021-01-12T06:53:13Z
day: '02'
doi: 10.1016/j.neuron.2013.09.019
extern: 1
intvolume: ' 80'
issue: '1'
month: '10'
page: 9 - 11
publication: Neuron
publication_status: published
publisher: Elsevier
publist_id: '5323'
quality_controlled: 0
status: public
title: 'The sacred disease: The puzzling genetics of epileptic disorders'
type: journal_article
volume: 80
year: '2013'
...
---
OA_place: repository
OA_type: green
_id: '17991'
abstract:
- lang: eng
text: Electrical and thermal transport properties of C60 molecules are investigated
with density-functional-theory based calculations. These calculations suggest
that the optimum contact geometry for an electrode terminated with a single-Au
atom is through binding to one or two C-atoms of C60 with a tendency to promote
the sp2-hybridization into an sp3-type one. Transport in these junctions is
primarily through an unoccupied molecular orbital that is partly hybridized with
the Au, which results in splitting the degeneracy of the lowest unoccupied molecular
orbital triplet. The transmission through these junctions, however, cannot be
modeled by a single Lorentzian resonance, as our results show evidence of quantum
interference between an occupied and an unoccupied orbital. The interference results
in a suppression of conductance around the Fermi energy. Our numerical findings
are readily analyzed analytically within a simple two-level model.
article_number: '234701'
article_processing_charge: No
article_type: original
arxiv: 1
author:
- first_name: G.
full_name: Géranton, G.
last_name: Géranton
- first_name: C.
full_name: Seiler, C.
last_name: Seiler
- first_name: A.
full_name: Bagrets, A.
last_name: Bagrets
- first_name: Latha
full_name: Venkataraman, Latha
id: 9ebb78a5-cc0d-11ee-8322-fae086a32caf
last_name: Venkataraman
orcid: 0000-0002-6957-6089
- first_name: F.
full_name: Evers, F.
last_name: Evers
citation:
ama: Géranton G, Seiler C, Bagrets A, Venkataraman L, Evers F. Transport properties
of individual C60-molecules. The Journal of Chemical Physics. 2013;139(23).
doi:10.1063/1.4840535
apa: Géranton, G., Seiler, C., Bagrets, A., Venkataraman, L., & Evers, F. (2013).
Transport properties of individual C60-molecules. The Journal of Chemical Physics.
AIP Publishing. https://doi.org/10.1063/1.4840535
chicago: Géranton, G., C. Seiler, A. Bagrets, Latha Venkataraman, and F. Evers.
“Transport Properties of Individual C60-Molecules.” The Journal of Chemical
Physics. AIP Publishing, 2013. https://doi.org/10.1063/1.4840535.
ieee: G. Géranton, C. Seiler, A. Bagrets, L. Venkataraman, and F. Evers, “Transport
properties of individual C60-molecules,” The Journal of Chemical Physics,
vol. 139, no. 23. AIP Publishing, 2013.
ista: Géranton G, Seiler C, Bagrets A, Venkataraman L, Evers F. 2013. Transport
properties of individual C60-molecules. The Journal of Chemical Physics. 139(23),
234701.
mla: Géranton, G., et al. “Transport Properties of Individual C60-Molecules.” The
Journal of Chemical Physics, vol. 139, no. 23, 234701, AIP Publishing, 2013,
doi:10.1063/1.4840535.
short: G. Géranton, C. Seiler, A. Bagrets, L. Venkataraman, F. Evers, The Journal
of Chemical Physics 139 (2013).
date_created: 2024-09-09T11:27:23Z
date_published: 2013-12-16T00:00:00Z
date_updated: 2025-01-03T07:51:59Z
day: '16'
doi: 10.1063/1.4840535
extern: '1'
external_id:
arxiv:
- '1206.1226'
intvolume: ' 139'
issue: '23'
language:
- iso: eng
main_file_link:
- open_access: '1'
url: https://arxiv.org/abs/1206.1226
month: '12'
oa: 1
oa_version: Preprint
publication: The Journal of Chemical Physics
publication_identifier:
eissn:
- 1089-7690
issn:
- 0021-9606
publication_status: published
publisher: AIP Publishing
quality_controlled: '1'
scopus_import: '1'
status: public
title: Transport properties of individual C60-molecules
type: journal_article
user_id: 2DF688A6-F248-11E8-B48F-1D18A9856A87
volume: 139
year: '2013'
...
---
OA_type: closed access
_id: '17992'
abstract:
- lang: eng
text: Here we demonstrate for the first time that strained silanes couple directly
to gold electrodes in break-junction conductance measurements. We find that strained
silicon molecular wires terminated by alkyl sulfide aurophiles behave effectively
as single-molecule parallel circuits with competing sulfur-to-sulfur (low G) and
sulfur-to-silacycle (high G) pathways. We can switch off the high conducting sulfur-to-silacycle
pathway by altering the environment of the electrode surface to disable the Au–silacycle
coupling. Additionally, we can switch between conductive pathways in a single
molecular junction by modulating the tip–substrate electrode distance. This study
provides a new molecular design to control electronics in silicon-based single
molecule wires.
article_processing_charge: No
article_type: letter_note
author:
- first_name: Timothy A.
full_name: Su, Timothy A.
last_name: Su
- first_name: Jonathan R.
full_name: Widawsky, Jonathan R.
last_name: Widawsky
- first_name: Haixing
full_name: Li, Haixing
last_name: Li
- first_name: Rebekka S.
full_name: Klausen, Rebekka S.
last_name: Klausen
- first_name: James L.
full_name: Leighton, James L.
last_name: Leighton
- first_name: Michael L.
full_name: Steigerwald, Michael L.
last_name: Steigerwald
- first_name: Latha
full_name: Venkataraman, Latha
id: 9ebb78a5-cc0d-11ee-8322-fae086a32caf
last_name: Venkataraman
orcid: 0000-0002-6957-6089
- first_name: Colin
full_name: Nuckolls, Colin
last_name: Nuckolls
citation:
ama: Su TA, Widawsky JR, Li H, et al. Silicon ring strain creates high-conductance
pathways in single-molecule circuits. Journal of the American Chemical Society.
2013;135(49):18331-18334. doi:10.1021/ja410656a
apa: Su, T. A., Widawsky, J. R., Li, H., Klausen, R. S., Leighton, J. L., Steigerwald,
M. L., … Nuckolls, C. (2013). Silicon ring strain creates high-conductance pathways
in single-molecule circuits. Journal of the American Chemical Society.
American Chemical Society. https://doi.org/10.1021/ja410656a
chicago: Su, Timothy A., Jonathan R. Widawsky, Haixing Li, Rebekka S. Klausen, James
L. Leighton, Michael L. Steigerwald, Latha Venkataraman, and Colin Nuckolls. “Silicon
Ring Strain Creates High-Conductance Pathways in Single-Molecule Circuits.” Journal
of the American Chemical Society. American Chemical Society, 2013. https://doi.org/10.1021/ja410656a.
ieee: T. A. Su et al., “Silicon ring strain creates high-conductance pathways
in single-molecule circuits,” Journal of the American Chemical Society,
vol. 135, no. 49. American Chemical Society, pp. 18331–18334, 2013.
ista: Su TA, Widawsky JR, Li H, Klausen RS, Leighton JL, Steigerwald ML, Venkataraman
L, Nuckolls C. 2013. Silicon ring strain creates high-conductance pathways in
single-molecule circuits. Journal of the American Chemical Society. 135(49), 18331–18334.
mla: Su, Timothy A., et al. “Silicon Ring Strain Creates High-Conductance Pathways
in Single-Molecule Circuits.” Journal of the American Chemical Society,
vol. 135, no. 49, American Chemical Society, 2013, pp. 18331–34, doi:10.1021/ja410656a.
short: T.A. Su, J.R. Widawsky, H. Li, R.S. Klausen, J.L. Leighton, M.L. Steigerwald,
L. Venkataraman, C. Nuckolls, Journal of the American Chemical Society 135 (2013)
18331–18334.
date_created: 2024-09-09T11:29:00Z
date_published: 2013-11-21T00:00:00Z
date_updated: 2025-01-03T07:54:49Z
day: '21'
doi: 10.1021/ja410656a
extern: '1'
external_id:
pmid:
- '24261548'
intvolume: ' 135'
issue: '49'
language:
- iso: eng
month: '11'
oa_version: None
page: 18331-18334
pmid: 1
publication: Journal of the American Chemical Society
publication_identifier:
eissn:
- 1520-5126
issn:
- 0002-7863
publication_status: published
publisher: American Chemical Society
quality_controlled: '1'
scopus_import: '1'
status: public
title: Silicon ring strain creates high-conductance pathways in single-molecule circuits
type: journal_article
user_id: 2DF688A6-F248-11E8-B48F-1D18A9856A87
volume: 135
year: '2013'
...
---
OA_type: closed access
_id: '17993'
abstract:
- lang: eng
text: We demonstrate a new method of achieving rectification in single molecule
devices using the high-bias properties of gold–carbon bonds. Our design for molecular
rectifiers uses a symmetric, conjugated molecular backbone with a single methylsulfide
group linking one end to a gold electrode and a covalent gold–carbon bond at the
other end. The gold–carbon bond results in a hybrid gold-molecule “gateway” state
pinned close to the Fermi level of one electrode. Through nonequilibrium transport
calculations, we show that the energy of this state shifts drastically with applied
bias, resulting in rectification at surprisingly low voltages. We use this concept
to design and synthesize a family of diodes and demonstrate through single-molecule
current–voltage measurements that the rectification ratio can be predictably and
efficiently tuned. This result constitutes the first experimental demonstration
of a rationally tunable system of single-molecule rectifiers. More generally,
the results demonstrate that the high-bias properties of “gateway” states can
be used to provide additional functionality to molecular electronic systems.
article_processing_charge: No
article_type: letter_note
author:
- first_name: Arunabh
full_name: Batra, Arunabh
last_name: Batra
- first_name: Pierre
full_name: Darancet, Pierre
last_name: Darancet
- first_name: Qishui
full_name: Chen, Qishui
last_name: Chen
- first_name: Jeffrey S.
full_name: Meisner, Jeffrey S.
last_name: Meisner
- first_name: Jonathan R.
full_name: Widawsky, Jonathan R.
last_name: Widawsky
- first_name: Jeffrey B.
full_name: Neaton, Jeffrey B.
last_name: Neaton
- first_name: Colin
full_name: Nuckolls, Colin
last_name: Nuckolls
- first_name: Latha
full_name: Venkataraman, Latha
id: 9ebb78a5-cc0d-11ee-8322-fae086a32caf
last_name: Venkataraman
orcid: 0000-0002-6957-6089
citation:
ama: Batra A, Darancet P, Chen Q, et al. Tuning rectification in single-molecular
diodes. Nano Letters. 2013;13(12):6233-6237. doi:10.1021/nl403698m
apa: Batra, A., Darancet, P., Chen, Q., Meisner, J. S., Widawsky, J. R., Neaton,
J. B., … Venkataraman, L. (2013). Tuning rectification in single-molecular diodes.
Nano Letters. American Chemical Society. https://doi.org/10.1021/nl403698m
chicago: Batra, Arunabh, Pierre Darancet, Qishui Chen, Jeffrey S. Meisner, Jonathan
R. Widawsky, Jeffrey B. Neaton, Colin Nuckolls, and Latha Venkataraman. “Tuning
Rectification in Single-Molecular Diodes.” Nano Letters. American Chemical
Society, 2013. https://doi.org/10.1021/nl403698m.
ieee: A. Batra et al., “Tuning rectification in single-molecular diodes,”
Nano Letters, vol. 13, no. 12. American Chemical Society, pp. 6233–6237,
2013.
ista: Batra A, Darancet P, Chen Q, Meisner JS, Widawsky JR, Neaton JB, Nuckolls
C, Venkataraman L. 2013. Tuning rectification in single-molecular diodes. Nano
Letters. 13(12), 6233–6237.
mla: Batra, Arunabh, et al. “Tuning Rectification in Single-Molecular Diodes.” Nano
Letters, vol. 13, no. 12, American Chemical Society, 2013, pp. 6233–37, doi:10.1021/nl403698m.
short: A. Batra, P. Darancet, Q. Chen, J.S. Meisner, J.R. Widawsky, J.B. Neaton,
C. Nuckolls, L. Venkataraman, Nano Letters 13 (2013) 6233–6237.
date_created: 2024-09-09T11:29:47Z
date_published: 2013-11-25T00:00:00Z
date_updated: 2025-01-03T07:57:04Z
day: '25'
doi: 10.1021/nl403698m
extern: '1'
external_id:
pmid:
- '24274757'
intvolume: ' 13'
issue: '12'
language:
- iso: eng
month: '11'
oa_version: None
page: 6233-6237
pmid: 1
publication: Nano Letters
publication_identifier:
eissn:
- 1530-6992
issn:
- 1530-6984
publication_status: published
publisher: American Chemical Society
quality_controlled: '1'
scopus_import: '1'
status: public
title: Tuning rectification in single-molecular diodes
type: journal_article
user_id: 2DF688A6-F248-11E8-B48F-1D18A9856A87
volume: 13
year: '2013'
...
---
OA_type: closed access
_id: '17994'
abstract:
- lang: eng
text: Charge transfer through noncovalent interactions is crucial to a variety of
chemical phenomena. These interactions are often weak and nonspecific and can
coexist, making it difficult to isolate the transfer efficiency of one type of
bond versus another. Here, we show how core-hole clock spectroscopy can be used
to measure charge transfer through noncovalent interactions. We study the model
system 1,4-benzenediamine molecules bound on an Au surface through an Au–N donor–acceptor
bond as these are known to provide a pathway for electronic conduction in molecular
devices. We study different phases of the molecule/Au system and map charge delocalization
times from carbon and nitrogen sites on the molecule. We show that charge delocalization
across Au–N donor–acceptor bond occurs in less than 500 as. Furthermore, the Au–N
bond also enhances delocalization times from neighboring carbon sites, demonstrating
that fast charge transfer across a metal–organic interface does not require a
covalently bonded system.
article_processing_charge: No
article_type: original
author:
- first_name: Gregor
full_name: Kladnik, Gregor
last_name: Kladnik
- first_name: Dean
full_name: Cvetko, Dean
last_name: Cvetko
- first_name: Arunabh
full_name: Batra, Arunabh
last_name: Batra
- first_name: Martina
full_name: Dell’Angela, Martina
last_name: Dell’Angela
- first_name: Albano
full_name: Cossaro, Albano
last_name: Cossaro
- first_name: Maria
full_name: Kamenetska, Maria
last_name: Kamenetska
- first_name: Latha
full_name: Venkataraman, Latha
id: 9ebb78a5-cc0d-11ee-8322-fae086a32caf
last_name: Venkataraman
orcid: 0000-0002-6957-6089
- first_name: Alberto
full_name: Morgante, Alberto
last_name: Morgante
citation:
ama: Kladnik G, Cvetko D, Batra A, et al. Ultrafast charge transfer through noncovalent
Au–N interactions in molecular systems. The Journal of Physical Chemistry C.
2013;117(32):16477-16482. doi:10.1021/jp405229b
apa: Kladnik, G., Cvetko, D., Batra, A., Dell’Angela, M., Cossaro, A., Kamenetska,
M., … Morgante, A. (2013). Ultrafast charge transfer through noncovalent Au–N
interactions in molecular systems. The Journal of Physical Chemistry C.
American Chemical Society. https://doi.org/10.1021/jp405229b
chicago: Kladnik, Gregor, Dean Cvetko, Arunabh Batra, Martina Dell’Angela, Albano
Cossaro, Maria Kamenetska, Latha Venkataraman, and Alberto Morgante. “Ultrafast
Charge Transfer through Noncovalent Au–N Interactions in Molecular Systems.” The
Journal of Physical Chemistry C. American Chemical Society, 2013. https://doi.org/10.1021/jp405229b.
ieee: G. Kladnik et al., “Ultrafast charge transfer through noncovalent Au–N
interactions in molecular systems,” The Journal of Physical Chemistry C,
vol. 117, no. 32. American Chemical Society, pp. 16477–16482, 2013.
ista: Kladnik G, Cvetko D, Batra A, Dell’Angela M, Cossaro A, Kamenetska M, Venkataraman
L, Morgante A. 2013. Ultrafast charge transfer through noncovalent Au–N interactions
in molecular systems. The Journal of Physical Chemistry C. 117(32), 16477–16482.
mla: Kladnik, Gregor, et al. “Ultrafast Charge Transfer through Noncovalent Au–N
Interactions in Molecular Systems.” The Journal of Physical Chemistry C,
vol. 117, no. 32, American Chemical Society, 2013, pp. 16477–82, doi:10.1021/jp405229b.
short: G. Kladnik, D. Cvetko, A. Batra, M. Dell’Angela, A. Cossaro, M. Kamenetska,
L. Venkataraman, A. Morgante, The Journal of Physical Chemistry C 117 (2013) 16477–16482.
date_created: 2024-09-09T11:30:45Z
date_published: 2013-07-17T00:00:00Z
date_updated: 2025-01-03T07:59:05Z
day: '17'
doi: 10.1021/jp405229b
extern: '1'
intvolume: ' 117'
issue: '32'
language:
- iso: eng
month: '07'
oa_version: None
page: 16477-16482
publication: The Journal of Physical Chemistry C
publication_identifier:
eissn:
- 1932-7455
issn:
- 1932-7447
publication_status: published
publisher: American Chemical Society
quality_controlled: '1'
scopus_import: '1'
status: public
title: Ultrafast charge transfer through noncovalent Au–N interactions in molecular
systems
type: journal_article
user_id: 2DF688A6-F248-11E8-B48F-1D18A9856A87
volume: 117
year: '2013'
...
---
OA_type: closed access
_id: '17995'
abstract:
- lang: eng
text: We have measured the single-molecule conductance of a family of bithiophene
derivatives terminated with methyl sulfide gold-binding linkers using a scanning
tunneling microscope based break-junction technique. We find a broad distribution
in the single-molecule conductance of bithiophene compared with that of a methyl
sulfide terminated biphenyl. Using a combination of experiments and calculations,
we show that this increased breadth in the conductance distribution is explained
by the difference in 5-fold symmetry of thiophene rings as compared to the 6-fold
symmetry of benzene rings. The reduced symmetry of thiophene rings results in
a restriction on the torsion angle space available to these molecules when bound
between two metal electrodes in a junction, causing each molecular junction to
sample a different set of conformers in the conductance measurements. In contrast,
the rotations of biphenyl are essentially unimpeded by junction binding, allowing
each molecular junction to sample similar conformers. This work demonstrates that
the conductance of bithiophene displays a strong dependence on the conformational
fluctuations accessible within a given junction configuration, and that the symmetry
of such small molecules can significantly influence their conductance behaviors.
article_processing_charge: No
article_type: letter_note
arxiv: 1
author:
- first_name: Emma J.
full_name: Dell, Emma J.
last_name: Dell
- first_name: Brian
full_name: Capozzi, Brian
last_name: Capozzi
- first_name: Kateri H.
full_name: DuBay, Kateri H.
last_name: DuBay
- first_name: Timothy C.
full_name: Berkelbach, Timothy C.
last_name: Berkelbach
- first_name: Jose Ricardo
full_name: Moreno, Jose Ricardo
last_name: Moreno
- first_name: David R.
full_name: Reichman, David R.
last_name: Reichman
- first_name: Latha
full_name: Venkataraman, Latha
id: 9ebb78a5-cc0d-11ee-8322-fae086a32caf
last_name: Venkataraman
orcid: 0000-0002-6957-6089
- first_name: Luis M.
full_name: Campos, Luis M.
last_name: Campos
citation:
ama: Dell EJ, Capozzi B, DuBay KH, et al. Impact of molecular symmetry on single-molecule
conductance. Journal of the American Chemical Society. 2013;135(32):11724-11727.
doi:10.1021/ja4055367
apa: Dell, E. J., Capozzi, B., DuBay, K. H., Berkelbach, T. C., Moreno, J. R., Reichman,
D. R., … Campos, L. M. (2013). Impact of molecular symmetry on single-molecule
conductance. Journal of the American Chemical Society. American Chemical
Society. https://doi.org/10.1021/ja4055367
chicago: Dell, Emma J., Brian Capozzi, Kateri H. DuBay, Timothy C. Berkelbach, Jose
Ricardo Moreno, David R. Reichman, Latha Venkataraman, and Luis M. Campos. “Impact
of Molecular Symmetry on Single-Molecule Conductance.” Journal of the American
Chemical Society. American Chemical Society, 2013. https://doi.org/10.1021/ja4055367.
ieee: E. J. Dell et al., “Impact of molecular symmetry on single-molecule
conductance,” Journal of the American Chemical Society, vol. 135, no. 32.
American Chemical Society, pp. 11724–11727, 2013.
ista: Dell EJ, Capozzi B, DuBay KH, Berkelbach TC, Moreno JR, Reichman DR, Venkataraman
L, Campos LM. 2013. Impact of molecular symmetry on single-molecule conductance.
Journal of the American Chemical Society. 135(32), 11724–11727.
mla: Dell, Emma J., et al. “Impact of Molecular Symmetry on Single-Molecule Conductance.”
Journal of the American Chemical Society, vol. 135, no. 32, American Chemical
Society, 2013, pp. 11724–27, doi:10.1021/ja4055367.
short: E.J. Dell, B. Capozzi, K.H. DuBay, T.C. Berkelbach, J.R. Moreno, D.R. Reichman,
L. Venkataraman, L.M. Campos, Journal of the American Chemical Society 135 (2013)
11724–11727.
date_created: 2024-09-09T11:32:00Z
date_published: 2013-08-01T00:00:00Z
date_updated: 2025-01-03T08:00:57Z
day: '01'
doi: 10.1021/ja4055367
extern: '1'
external_id:
arxiv:
- '23905714'
intvolume: ' 135'
issue: '32'
language:
- iso: eng
month: '08'
oa_version: None
page: 11724-11727
publication: Journal of the American Chemical Society
publication_identifier:
eissn:
- 1520-5126
issn:
- 0002-7863
publication_status: published
publisher: American Chemical Society
quality_controlled: '1'
scopus_import: '1'
status: public
title: Impact of molecular symmetry on single-molecule conductance
type: journal_article
user_id: 2DF688A6-F248-11E8-B48F-1D18A9856A87
volume: 135
year: '2013'
...
---
OA_type: closed access
_id: '17996'
abstract:
- lang: eng
text: We compare the conductance of a series of amine-terminated oligophenyl and
alkane molecular junctions formed with Ag and Au electrodes using the scanning
tunneling microscope based break-junction technique. For these molecules that
conduct through the highest occupied molecular orbital, junctions formed with
Au electrodes are more conductive than those formed with Ag electrodes, consistent
with the lower work function for Ag. The measured conductance decays exponentially
with molecular backbone length with a decay constant that is essentially the same
for Ag and Au electrodes. However, the formation and evolution of molecular junctions
upon elongation are very different for these two metals. Specifically, junctions
formed with Ag electrodes sustain significantly longer elongation when compared
with Au due to a difference in the initial gap opened up when the metal point-contact
is broken. Using this observation and density functional theory calculations of
junction structure and conductance we explain the trends observed in the single
molecule junction conductance. Our work thus opens a new path to the conductance
measurements of a single molecule junction in Ag electrodes.
article_processing_charge: No
article_type: letter_note
author:
- first_name: Taekyeong
full_name: Kim, Taekyeong
last_name: Kim
- first_name: Héctor
full_name: Vázquez, Héctor
last_name: Vázquez
- first_name: Mark S.
full_name: Hybertsen, Mark S.
last_name: Hybertsen
- first_name: Latha
full_name: Venkataraman, Latha
id: 9ebb78a5-cc0d-11ee-8322-fae086a32caf
last_name: Venkataraman
orcid: 0000-0002-6957-6089
citation:
ama: Kim T, Vázquez H, Hybertsen MS, Venkataraman L. Conductance of molecular junctions
formed with silver electrodes. Nano Letters. 2013;13(7):3358-3364. doi:10.1021/nl401654s
apa: Kim, T., Vázquez, H., Hybertsen, M. S., & Venkataraman, L. (2013). Conductance
of molecular junctions formed with silver electrodes. Nano Letters. American
Chemical Society. https://doi.org/10.1021/nl401654s
chicago: Kim, Taekyeong, Héctor Vázquez, Mark S. Hybertsen, and Latha Venkataraman.
“Conductance of Molecular Junctions Formed with Silver Electrodes.” Nano Letters.
American Chemical Society, 2013. https://doi.org/10.1021/nl401654s.
ieee: T. Kim, H. Vázquez, M. S. Hybertsen, and L. Venkataraman, “Conductance of
molecular junctions formed with silver electrodes,” Nano Letters, vol.
13, no. 7. American Chemical Society, pp. 3358–3364, 2013.
ista: Kim T, Vázquez H, Hybertsen MS, Venkataraman L. 2013. Conductance of molecular
junctions formed with silver electrodes. Nano Letters. 13(7), 3358–3364.
mla: Kim, Taekyeong, et al. “Conductance of Molecular Junctions Formed with Silver
Electrodes.” Nano Letters, vol. 13, no. 7, American Chemical Society, 2013,
pp. 3358–64, doi:10.1021/nl401654s.
short: T. Kim, H. Vázquez, M.S. Hybertsen, L. Venkataraman, Nano Letters 13 (2013)
3358–3364.
date_created: 2024-09-09T11:32:49Z
date_published: 2013-06-03T00:00:00Z
date_updated: 2025-01-03T08:02:58Z
day: '03'
doi: 10.1021/nl401654s
extern: '1'
external_id:
pmid:
- '23731268'
intvolume: ' 13'
issue: '7'
language:
- iso: eng
month: '06'
oa_version: None
page: 3358-3364
pmid: 1
publication: Nano Letters
publication_identifier:
eissn:
- 1530-6992
issn:
- 1530-6984
publication_status: published
publisher: American Chemical Society
quality_controlled: '1'
scopus_import: '1'
status: public
title: Conductance of molecular junctions formed with silver electrodes
type: journal_article
user_id: 2DF688A6-F248-11E8-B48F-1D18A9856A87
volume: 13
year: '2013'
...
---
OA_type: closed access
_id: '17997'
abstract:
- lang: eng
text: We report the simultaneous measurement of conductance and thermopower of highly
conducting single-molecule junctions using a scanning tunneling microscope-based
break-junction setup. We start with molecular backbones (alkanes and oligophenyls)
terminated with trimethyltin end groups that cleave off in situ to create junctions
where terminal carbons are covalently bonded to the Au electrodes. We apply a
thermal gradient across these junctions and measure their conductance and thermopower.
Because of the electronic properties of the highly conducting Au–C links, the
thermoelectric properties and power factor are very high. Our results show that
the molecular thermopower increases nonlinearly with the molecular length while
conductance decreases exponentially with increasing molecular length. Density
functional theory calculations show that a gateway state representing the Au–C
covalent bond plays a key role in the conductance. With this as input, we analyze
a series of simplified models and show that a tight-binding model that explicitly
includes the gateway states and the molecular backbone states accurately captures
the experimentally measured conductance and thermopower trends.
article_processing_charge: No
article_type: letter_note
author:
- first_name: J. R.
full_name: Widawsky, J. R.
last_name: Widawsky
- first_name: W.
full_name: Chen, W.
last_name: Chen
- first_name: H.
full_name: Vázquez, H.
last_name: Vázquez
- first_name: T.
full_name: Kim, T.
last_name: Kim
- first_name: R.
full_name: Breslow, R.
last_name: Breslow
- first_name: M. S.
full_name: Hybertsen, M. S.
last_name: Hybertsen
- first_name: Latha
full_name: Venkataraman, Latha
id: 9ebb78a5-cc0d-11ee-8322-fae086a32caf
last_name: Venkataraman
orcid: 0000-0002-6957-6089
citation:
ama: Widawsky JR, Chen W, Vázquez H, et al. Length-dependent thermopower of highly
conducting Au–C bonded single molecule junctions. Nano Letters. 2013;13(6):2889-2894.
doi:10.1021/nl4012276
apa: Widawsky, J. R., Chen, W., Vázquez, H., Kim, T., Breslow, R., Hybertsen, M.
S., & Venkataraman, L. (2013). Length-dependent thermopower of highly conducting
Au–C bonded single molecule junctions. Nano Letters. American Chemical
Society. https://doi.org/10.1021/nl4012276
chicago: Widawsky, J. R., W. Chen, H. Vázquez, T. Kim, R. Breslow, M. S. Hybertsen,
and Latha Venkataraman. “Length-Dependent Thermopower of Highly Conducting Au–C
Bonded Single Molecule Junctions.” Nano Letters. American Chemical Society,
2013. https://doi.org/10.1021/nl4012276.
ieee: J. R. Widawsky et al., “Length-dependent thermopower of highly conducting
Au–C bonded single molecule junctions,” Nano Letters, vol. 13, no. 6. American
Chemical Society, pp. 2889–2894, 2013.
ista: Widawsky JR, Chen W, Vázquez H, Kim T, Breslow R, Hybertsen MS, Venkataraman
L. 2013. Length-dependent thermopower of highly conducting Au–C bonded single
molecule junctions. Nano Letters. 13(6), 2889–2894.
mla: Widawsky, J. R., et al. “Length-Dependent Thermopower of Highly Conducting
Au–C Bonded Single Molecule Junctions.” Nano Letters, vol. 13, no. 6, American
Chemical Society, 2013, pp. 2889–94, doi:10.1021/nl4012276.
short: J.R. Widawsky, W. Chen, H. Vázquez, T. Kim, R. Breslow, M.S. Hybertsen, L.
Venkataraman, Nano Letters 13 (2013) 2889–2894.
date_created: 2024-09-09T11:33:33Z
date_published: 2013-05-17T00:00:00Z
date_updated: 2025-01-03T08:05:44Z
day: '17'
doi: 10.1021/nl4012276
extern: '1'
external_id:
pmid:
- '23682792'
intvolume: ' 13'
issue: '6'
language:
- iso: eng
month: '05'
oa_version: None
page: 2889-2894
pmid: 1
publication: Nano Letters
publication_identifier:
eissn:
- 1530-6992
issn:
- 1530-6984
publication_status: published
publisher: American Chemical Society
quality_controlled: '1'
scopus_import: '1'
status: public
title: Length-dependent thermopower of highly conducting Au–C bonded single molecule
junctions
type: journal_article
user_id: 2DF688A6-F248-11E8-B48F-1D18A9856A87
volume: 13
year: '2013'
...
---
OA_type: closed access
_id: '17998'
abstract:
- lang: eng
text: We measure simultaneously force and conductance of Ag metal point-contacts
under ambient conditions at room temperature. We observe the formation of contacts
with a conductance close to 1 G0, the quantum of conductance, which can be attributed
to a single-atom contact, similar to those formed by Au. We also find two additional
conductance features at ∼0.4 G0 and ∼1.3 G0, which have been previously ascribed
to contacts with oxygen contaminations. Here, using a conductance cross-correlation
technique, we distinguish three different atomic-scale structural motifs and analyze
their rupture forces and stiffness. Our results allow us to assign the ∼0.4 G0
conductance feature to an Ag–O–Ag contact and the ∼1.3 G0 feature to an Ag–Ag
single-atom contact with an oxygen atom in parallel. Utilizing complementary information
from force and conductance, we thus demonstrate the correlation of conductance
with the structural evolution at the atomic scale.
article_processing_charge: No
article_type: original
author:
- first_name: Sriharsha V.
full_name: Aradhya, Sriharsha V.
last_name: Aradhya
- first_name: Michael
full_name: Frei, Michael
last_name: Frei
- first_name: András
full_name: Halbritter, András
last_name: Halbritter
- first_name: Latha
full_name: Venkataraman, Latha
id: 9ebb78a5-cc0d-11ee-8322-fae086a32caf
last_name: Venkataraman
orcid: 0000-0002-6957-6089
citation:
ama: Aradhya SV, Frei M, Halbritter A, Venkataraman L. Correlating structure, conductance,
and mechanics of silver atomic-scale contacts. ACS Nano. 2013;7(4):3706-3712.
doi:10.1021/nn4007187
apa: Aradhya, S. V., Frei, M., Halbritter, A., & Venkataraman, L. (2013). Correlating
structure, conductance, and mechanics of silver atomic-scale contacts. ACS
Nano. American Chemical Society. https://doi.org/10.1021/nn4007187
chicago: Aradhya, Sriharsha V., Michael Frei, András Halbritter, and Latha Venkataraman.
“Correlating Structure, Conductance, and Mechanics of Silver Atomic-Scale Contacts.”
ACS Nano. American Chemical Society, 2013. https://doi.org/10.1021/nn4007187.
ieee: S. V. Aradhya, M. Frei, A. Halbritter, and L. Venkataraman, “Correlating structure,
conductance, and mechanics of silver atomic-scale contacts,” ACS Nano,
vol. 7, no. 4. American Chemical Society, pp. 3706–3712, 2013.
ista: Aradhya SV, Frei M, Halbritter A, Venkataraman L. 2013. Correlating structure,
conductance, and mechanics of silver atomic-scale contacts. ACS Nano. 7(4), 3706–3712.
mla: Aradhya, Sriharsha V., et al. “Correlating Structure, Conductance, and Mechanics
of Silver Atomic-Scale Contacts.” ACS Nano, vol. 7, no. 4, American Chemical
Society, 2013, pp. 3706–12, doi:10.1021/nn4007187.
short: S.V. Aradhya, M. Frei, A. Halbritter, L. Venkataraman, ACS Nano 7 (2013)
3706–3712.
date_created: 2024-09-09T11:34:27Z
date_published: 2013-03-23T00:00:00Z
date_updated: 2025-01-03T08:07:54Z
day: '23'
doi: 10.1021/nn4007187
extern: '1'
external_id:
pmid:
- '23521342'
intvolume: ' 7'
issue: '4'
language:
- iso: eng
month: '03'
oa_version: None
page: 3706-3712
pmid: 1
publication: ACS Nano
publication_identifier:
eissn:
- 1936-086X
issn:
- 1936-0851
publication_status: published
publisher: American Chemical Society
quality_controlled: '1'
scopus_import: '1'
status: public
title: Correlating structure, conductance, and mechanics of silver atomic-scale contacts
type: journal_article
user_id: 2DF688A6-F248-11E8-B48F-1D18A9856A87
volume: 7
year: '2013'
...
---
OA_type: closed access
_id: '17999'
abstract:
- lang: eng
text: The idea of using individual molecules as active electronic components provided
the impetus to develop a variety of experimental platforms to probe their electronic
transport properties. Among these, single-molecule junctions in a metal–molecule–metal
motif have contributed significantly to our fundamental understanding of the principles
required to realize molecular-scale electronic components from resistive wires
to reversible switches. The success of these techniques and the growing interest
of other disciplines in single-molecule-level characterization are prompting new
approaches to investigate metal–molecule–metal junctions with multiple probes.
Going beyond electronic transport characterization, these new studies are highlighting
both the fundamental and applied aspects of mechanical, optical and thermoelectric
properties at the atomic and molecular scales. Furthermore, experimental demonstrations
of quantum interference and manipulation of electronic and nuclear spins in single-molecule
circuits are heralding new device concepts with no classical analogues. In this
Review, we present the emerging methods being used to interrogate multiple properties
in single molecule-based devices, detail how these measurements have advanced
our understanding of the structure–function relationships in molecular junctions,
and discuss the potential for future research and applications.
article_processing_charge: No
article_type: original
author:
- first_name: Sriharsha V.
full_name: Aradhya, Sriharsha V.
last_name: Aradhya
- first_name: Latha
full_name: Venkataraman, Latha
id: 9ebb78a5-cc0d-11ee-8322-fae086a32caf
last_name: Venkataraman
orcid: 0000-0002-6957-6089
citation:
ama: Aradhya SV, Venkataraman L. Single-molecule junctions beyond electronic transport.
Nature Nanotechnology. 2013;8(6):399-410. doi:10.1038/nnano.2013.91
apa: Aradhya, S. V., & Venkataraman, L. (2013). Single-molecule junctions beyond
electronic transport. Nature Nanotechnology. Springer Nature. https://doi.org/10.1038/nnano.2013.91
chicago: Aradhya, Sriharsha V., and Latha Venkataraman. “Single-Molecule Junctions
beyond Electronic Transport.” Nature Nanotechnology. Springer Nature, 2013.
https://doi.org/10.1038/nnano.2013.91.
ieee: S. V. Aradhya and L. Venkataraman, “Single-molecule junctions beyond electronic
transport,” Nature Nanotechnology, vol. 8, no. 6. Springer Nature, pp.
399–410, 2013.
ista: Aradhya SV, Venkataraman L. 2013. Single-molecule junctions beyond electronic
transport. Nature Nanotechnology. 8(6), 399–410.
mla: Aradhya, Sriharsha V., and Latha Venkataraman. “Single-Molecule Junctions beyond
Electronic Transport.” Nature Nanotechnology, vol. 8, no. 6, Springer Nature,
2013, pp. 399–410, doi:10.1038/nnano.2013.91.
short: S.V. Aradhya, L. Venkataraman, Nature Nanotechnology 8 (2013) 399–410.
date_created: 2024-09-09T11:35:13Z
date_published: 2013-06-01T00:00:00Z
date_updated: 2025-01-03T08:10:06Z
day: '01'
doi: 10.1038/nnano.2013.91
extern: '1'
external_id:
pmid:
- '23736215'
intvolume: ' 8'
issue: '6'
language:
- iso: eng
month: '06'
oa_version: None
page: 399-410
pmid: 1
publication: Nature Nanotechnology
publication_identifier:
eissn:
- 1748-3395
issn:
- 1748-3387
publication_status: published
publisher: Springer Nature
quality_controlled: '1'
scopus_import: '1'
status: public
title: Single-molecule junctions beyond electronic transport
type: journal_article
user_id: 2DF688A6-F248-11E8-B48F-1D18A9856A87
volume: 8
year: '2013'
...