---
_id: '17690'
abstract:
- lang: eng
  text: The ability of primordial gas to cool in proto-galactic haloes exposed to
    Lyman-Werner (LW) radiation is critically dependent on the self-shielding of H_2.
    We perform radiative transfer calculations of LW line photons, post-processing
    outputs from three-dimensional adaptive mesh refinement (AMR) simulations of haloes
    with T_vir > 10^4 K at redshifts around z=10. We calculate the optically thick
    photodissociation rate numerically, including the effects of density, temperature,
    and velocity gradients in the gas, as well as line overlap and shielding of H_2
    by HI, over a large number of sight-lines. In low-density regions (n<10^4 cm^-3)
    the dissociation rates exceed those obtained using most previous approximations
    by more than an order of magnitude; the correction is smaller at higher densities.
    We trace the origin of the deviations primarily to inaccuracies of (i) the most
    common fitting formula (Draine & Bertoldi 1996) for the suppression of the dissociation
    rate and (ii) estimates for the effective shielding column density from local
    properties of the gas. The combined effects of gas temperature and velocity gradients
    are comparatively less important, typically altering the spherically averaged
    rate only by a factor of less than two. We present a simple modification to the
    DB96 fitting formula for the optically thick rate which improves agreement with
    our numerical results to within approx. 15 per cent, and can be adopted in future
    simulations. We find that estimates for the effective shielding column can be
    improved by using the local Sobolev length. Our correction to the H_2 self-shielding
    reduces the critical LW flux to suppress H_2-cooling in T_vir>10^4 K haloes by
    an order of magnitude; this increases the number of such haloes in which supermassive
    (approx. M=10^5 M_sun) black holes may have formed.
alternative_title:
- H 2 self-shielding in 3D simulations
article_processing_charge: No
article_type: original
author:
- first_name: J.
  full_name: Wolcott-Green, J.
  last_name: Wolcott-Green
- first_name: Zoltán
  full_name: Haiman, Zoltán
  id: 7c006e8c-cc0d-11ee-8322-cb904ef76f36
  last_name: Haiman
- first_name: G. L.
  full_name: Bryan, G. L.
  last_name: Bryan
citation:
  ama: 'Wolcott-Green J, Haiman Z, Bryan GL. Photodissociation of H2 in protogalaxies:
    Modelling self-shielding in three-dimensional simulations. <i>Monthly Notices
    of the Royal Astronomical Society</i>. 2011;418(2):838-852. doi:<a href="https://doi.org/10.1111/j.1365-2966.2011.19538.x">10.1111/j.1365-2966.2011.19538.x</a>'
  apa: 'Wolcott-Green, J., Haiman, Z., &#38; Bryan, G. L. (2011). Photodissociation
    of H2 in protogalaxies: Modelling self-shielding in three-dimensional simulations.
    <i>Monthly Notices of the Royal Astronomical Society</i>. Oxford University Press.
    <a href="https://doi.org/10.1111/j.1365-2966.2011.19538.x">https://doi.org/10.1111/j.1365-2966.2011.19538.x</a>'
  chicago: 'Wolcott-Green, J., Zoltán Haiman, and G. L. Bryan. “Photodissociation
    of H2 in Protogalaxies: Modelling Self-Shielding in Three-Dimensional Simulations.”
    <i>Monthly Notices of the Royal Astronomical Society</i>. Oxford University Press,
    2011. <a href="https://doi.org/10.1111/j.1365-2966.2011.19538.x">https://doi.org/10.1111/j.1365-2966.2011.19538.x</a>.'
  ieee: 'J. Wolcott-Green, Z. Haiman, and G. L. Bryan, “Photodissociation of H2 in
    protogalaxies: Modelling self-shielding in three-dimensional simulations,” <i>Monthly
    Notices of the Royal Astronomical Society</i>, vol. 418, no. 2. Oxford University
    Press, pp. 838–852, 2011.'
  ista: 'Wolcott-Green J, Haiman Z, Bryan GL. 2011. Photodissociation of H2 in protogalaxies:
    Modelling self-shielding in three-dimensional simulations. Monthly Notices of
    the Royal Astronomical Society. 418(2), 838–852.'
  mla: 'Wolcott-Green, J., et al. “Photodissociation of H2 in Protogalaxies: Modelling
    Self-Shielding in Three-Dimensional Simulations.” <i>Monthly Notices of the Royal
    Astronomical Society</i>, vol. 418, no. 2, Oxford University Press, 2011, pp.
    838–52, doi:<a href="https://doi.org/10.1111/j.1365-2966.2011.19538.x">10.1111/j.1365-2966.2011.19538.x</a>.'
  short: J. Wolcott-Green, Z. Haiman, G.L. Bryan, Monthly Notices of the Royal Astronomical
    Society 418 (2011) 838–852.
date_created: 2024-09-06T08:37:08Z
date_published: 2011-11-16T00:00:00Z
date_updated: 2024-09-25T09:53:37Z
day: '16'
doi: 10.1111/j.1365-2966.2011.19538.x
extern: '1'
fulldoi: https://doi.org/10.1111/j.1365-2966.2011.19538.x
intvolume: '       418'
issue: '2'
language:
- iso: eng
main_file_link:
- open_access: '1'
  url: https://doi.org/10.1111/j.1365-2966.2011.19538.x
month: '11'
oa: 1
oa_version: Published Version
page: 838-852
publication: Monthly Notices of the Royal Astronomical Society
publication_identifier:
  issn:
  - 0035-8711
publication_status: published
publisher: Oxford University Press
quality_controlled: '1'
scopus_import: '1'
status: public
title: 'Photodissociation of H2 in protogalaxies: Modelling self-shielding in three-dimensional
  simulations'
type: journal_article
user_id: 317138e5-6ab7-11ef-aa6d-ffef3953e345
volume: 418
year: '2011'
...
---
_id: '17701'
abstract:
- lang: eng
  text: Independent lines of evidence suggest that the first stars, which ended the
    cosmic dark ages, came in pairs, rather than singly. This could change the prevailing
    view that the early Universe had a Swiss-cheese-like appearance.
article_processing_charge: No
article_type: original
arxiv: 1
author:
- first_name: Zoltán
  full_name: Haiman, Zoltán
  id: 7c006e8c-cc0d-11ee-8322-cb904ef76f36
  last_name: Haiman
citation:
  ama: Haiman Z. A smoother end to the dark ages. <i>Nature</i>. 2011;472(7341):47-48.
    doi:<a href="https://doi.org/10.1038/472047a">10.1038/472047a</a>
  apa: Haiman, Z. (2011). A smoother end to the dark ages. <i>Nature</i>. Springer
    Science and Business Media LLC. <a href="https://doi.org/10.1038/472047a">https://doi.org/10.1038/472047a</a>
  chicago: Haiman, Zoltán. “A Smoother End to the Dark Ages.” <i>Nature</i>. Springer
    Science and Business Media LLC, 2011. <a href="https://doi.org/10.1038/472047a">https://doi.org/10.1038/472047a</a>.
  ieee: Z. Haiman, “A smoother end to the dark ages,” <i>Nature</i>, vol. 472, no.
    7341. Springer Science and Business Media LLC, pp. 47–48, 2011.
  ista: Haiman Z. 2011. A smoother end to the dark ages. Nature. 472(7341), 47–48.
  mla: Haiman, Zoltán. “A Smoother End to the Dark Ages.” <i>Nature</i>, vol. 472,
    no. 7341, Springer Science and Business Media LLC, 2011, pp. 47–48, doi:<a href="https://doi.org/10.1038/472047a">10.1038/472047a</a>.
  short: Z. Haiman, Nature 472 (2011) 47–48.
date_created: 2024-09-06T08:47:22Z
date_published: 2011-04-06T00:00:00Z
date_updated: 2024-09-25T11:25:52Z
day: '06'
doi: 10.1038/472047a
extern: '1'
external_id:
  arxiv:
  - '1104.1189'
fulldoi: https://doi.org/10.1038/472047a
intvolume: '       472'
issue: '7341'
language:
- iso: eng
main_file_link:
- open_access: '1'
  url: ' https://doi.org/10.48550/arXiv.1104.1189'
month: '04'
oa: 1
oa_version: Preprint
page: 47-48
publication: Nature
publication_identifier:
  issn:
  - 0028-0836
  - 1476-4687
publication_status: published
publisher: Springer Science and Business Media LLC
quality_controlled: '1'
scopus_import: '1'
status: public
title: A smoother end to the dark ages
type: journal_article
user_id: 317138e5-6ab7-11ef-aa6d-ffef3953e345
volume: 472
year: '2011'
...
---
_id: '1775'
abstract:
- lang: eng
  text: At optical frequencies the radiation produced by a source, such as a laser,
    a black body or a single-photon emitter, is frequently characterized by analysing
    the temporal correlations of emitted photons using single-photon counters. At
    microwave frequencies, however, there are no efficient single-photon counters
    yet. Instead, well-developed linear amplifiers allow for efficient measurement
    of the amplitude of an electromagnetic field. Here, we demonstrate first- and
    second-order correlation function measurements of a pulsed microwave-frequency
    single-photon source integrated on the same chip with a 50/50 beam splitter followed
    by linear amplifiers and quadrature amplitude detectors. We clearly observe single-photon
    coherence in first-order and photon antibunching in second-order correlation function
    measurements of the propagating fields.
acknowledgement: This work was supported by the European Research Council (ERC) through
  a Starting Grant and by ETHZ. M.P.d.S. was supported by a NSERC postdoctoral fellowship.
  A.B. was supported by NSERC, CIFAR and the Alfred P. Sloan Foundation
author:
- first_name: Deniz
  full_name: Bozyigit, Deniz
  last_name: Bozyigit
- first_name: C
  full_name: Lang, C
  last_name: Lang
- first_name: L.
  full_name: Steffen, L. Kraig
  last_name: Steffen
- first_name: Johannes M
  full_name: Johannes Fink
  id: 4B591CBA-F248-11E8-B48F-1D18A9856A87
  last_name: Fink
  orcid: 0000-0001-8112-028X
- first_name: Christopher
  full_name: Eichler, Christopher
  last_name: Eichler
- first_name: Matthias
  full_name: Baur, Matthias P
  last_name: Baur
- first_name: R
  full_name: Bianchetti, R
  last_name: Bianchetti
- first_name: Peter
  full_name: Leek, Peter J
  last_name: Leek
- first_name: Stefan
  full_name: Filipp, Stefan
  last_name: Filipp
- first_name: Marcus
  full_name: Da Silva, Marcus P
  last_name: Da Silva
- first_name: Alexandre
  full_name: Blais, Alexandre
  last_name: Blais
- first_name: Andreas
  full_name: Wallraff, Andreas
  last_name: Wallraff
citation:
  ama: Bozyigit D, Lang C, Steffen L, et al. Antibunching of microwave-frequency photons
    observed in correlation measurements using linear detectors. <i>Nature Physics</i>.
    2011;7(2):154-158. doi:<a href="https://doi.org/10.1038/nphys1845">10.1038/nphys1845</a>
  apa: Bozyigit, D., Lang, C., Steffen, L., Fink, J. M., Eichler, C., Baur, M., …
    Wallraff, A. (2011). Antibunching of microwave-frequency photons observed in correlation
    measurements using linear detectors. <i>Nature Physics</i>. Nature Publishing
    Group. <a href="https://doi.org/10.1038/nphys1845">https://doi.org/10.1038/nphys1845</a>
  chicago: Bozyigit, Deniz, C Lang, L. Steffen, Johannes M Fink, Christopher Eichler,
    Matthias Baur, R Bianchetti, et al. “Antibunching of Microwave-Frequency Photons
    Observed in Correlation Measurements Using Linear Detectors.” <i>Nature Physics</i>.
    Nature Publishing Group, 2011. <a href="https://doi.org/10.1038/nphys1845">https://doi.org/10.1038/nphys1845</a>.
  ieee: D. Bozyigit <i>et al.</i>, “Antibunching of microwave-frequency photons observed
    in correlation measurements using linear detectors,” <i>Nature Physics</i>, vol.
    7, no. 2. Nature Publishing Group, pp. 154–158, 2011.
  ista: Bozyigit D, Lang C, Steffen L, Fink JM, Eichler C, Baur M, Bianchetti R, Leek
    P, Filipp S, Da Silva M, Blais A, Wallraff A. 2011. Antibunching of microwave-frequency
    photons observed in correlation measurements using linear detectors. Nature Physics.
    7(2), 154–158.
  mla: Bozyigit, Deniz, et al. “Antibunching of Microwave-Frequency Photons Observed
    in Correlation Measurements Using Linear Detectors.” <i>Nature Physics</i>, vol.
    7, no. 2, Nature Publishing Group, 2011, pp. 154–58, doi:<a href="https://doi.org/10.1038/nphys1845">10.1038/nphys1845</a>.
  short: D. Bozyigit, C. Lang, L. Steffen, J.M. Fink, C. Eichler, M. Baur, R. Bianchetti,
    P. Leek, S. Filipp, M. Da Silva, A. Blais, A. Wallraff, Nature Physics 7 (2011)
    154–158.
date_created: 2018-12-11T11:53:57Z
date_published: 2011-02-01T00:00:00Z
date_updated: 2021-01-12T06:53:07Z
day: '01'
doi: 10.1038/nphys1845
extern: 1
fulldoi: https://doi.org/10.1038/nphys1845
intvolume: '         7'
issue: '2'
month: '02'
page: 154 - 158
publication: Nature Physics
publication_status: published
publisher: Nature Publishing Group
publist_id: '5340'
quality_controlled: 0
status: public
title: Antibunching of microwave-frequency photons observed in correlation measurements
  using linear detectors
type: journal_article
volume: 7
year: '2011'
...
---
_id: '1776'
abstract:
- lang: eng
  text: Superconducting circuits have been successfully established as systems to
    prepare and investigate microwave light fields at the quantum level. In contrast
    to optical experiments where light is detected using photon counters, microwaves
    are usually measured with well developed linear amplifiers. This makes measurements
    of correlation functions - one of the important tools in optics - harder to achieve
    because they traditionally rely on photon counters and beam splitters. Here, we
    demonstrate a system where we can prepare on demand single microwave photons in
    a cavity and detect them at the two outputs of the cavity using linear amplifiers.
    Together with efficient data processing, this allows us to measure different observables
    of the cavity photons, including the first-order correlation function. Using these
    techniques we demonstrate cooling of a thermal background field in the cavity.
acknowledgement: Australian National University,Aust. Res. Counc. Cent. Excellence
  Quantum-Atom Opt.,Griffith University,Ian Potter Foundation,International Union
  of Pure and Applied Physics
alternative_title:
- 'Journal of Physics: Conference Series'
author:
- first_name: Deniz
  full_name: Bozyigit, Deniz
  last_name: Bozyigit
- first_name: C
  full_name: Lang, C
  last_name: Lang
- first_name: L.
  full_name: Steffen, L. Kraig
  last_name: Steffen
- first_name: Johannes M
  full_name: Johannes Fink
  id: 4B591CBA-F248-11E8-B48F-1D18A9856A87
  last_name: Fink
  orcid: 0000-0001-8112-028X
- first_name: Christopher
  full_name: Eichler, Christopher
  last_name: Eichler
- first_name: Matthias
  full_name: Baur, Matthias P
  last_name: Baur
- first_name: R
  full_name: Bianchetti, R
  last_name: Bianchetti
- first_name: Peter
  full_name: Leek, Peter J
  last_name: Leek
- first_name: Stefan
  full_name: Filipp, Stefan
  last_name: Filipp
- first_name: Andreas
  full_name: Wallraff, Andreas
  last_name: Wallraff
- first_name: Marcus
  full_name: Da Silva, Marcus P
  last_name: Da Silva
- first_name: Alexandre
  full_name: Blais, Alexandre
  last_name: Blais
citation:
  ama: 'Bozyigit D, Lang C, Steffen L, et al. Correlation measurements of individual
    microwave photons emitted from a symmetric cavity. In: Vol 264. IOP Publishing
    Ltd.; 2011. doi:<a href="https://doi.org/10.1088/1742-6596/264/1/012024">10.1088/1742-6596/264/1/012024</a>'
  apa: Bozyigit, D., Lang, C., Steffen, L., Fink, J. M., Eichler, C., Baur, M., …
    Blais, A. (2011). Correlation measurements of individual microwave photons emitted
    from a symmetric cavity (Vol. 264). Presented at the International Conference
    on Atomic Physics, IOP Publishing Ltd. <a href="https://doi.org/10.1088/1742-6596/264/1/012024">https://doi.org/10.1088/1742-6596/264/1/012024</a>
  chicago: Bozyigit, Deniz, C Lang, L. Steffen, Johannes M Fink, Christopher Eichler,
    Matthias Baur, R Bianchetti, et al. “Correlation Measurements of Individual Microwave
    Photons Emitted from a Symmetric Cavity,” Vol. 264. IOP Publishing Ltd., 2011.
    <a href="https://doi.org/10.1088/1742-6596/264/1/012024">https://doi.org/10.1088/1742-6596/264/1/012024</a>.
  ieee: D. Bozyigit <i>et al.</i>, “Correlation measurements of individual microwave
    photons emitted from a symmetric cavity,” presented at the International Conference
    on Atomic Physics, 2011, vol. 264, no. 1.
  ista: 'Bozyigit D, Lang C, Steffen L, Fink JM, Eichler C, Baur M, Bianchetti R,
    Leek P, Filipp S, Wallraff A, Da Silva M, Blais A. 2011. Correlation measurements
    of individual microwave photons emitted from a symmetric cavity. International
    Conference on Atomic Physics, Journal of Physics: Conference Series, vol. 264.'
  mla: Bozyigit, Deniz, et al. <i>Correlation Measurements of Individual Microwave
    Photons Emitted from a Symmetric Cavity</i>. Vol. 264, no. 1, IOP Publishing Ltd.,
    2011, doi:<a href="https://doi.org/10.1088/1742-6596/264/1/012024">10.1088/1742-6596/264/1/012024</a>.
  short: D. Bozyigit, C. Lang, L. Steffen, J.M. Fink, C. Eichler, M. Baur, R. Bianchetti,
    P. Leek, S. Filipp, A. Wallraff, M. Da Silva, A. Blais, in:, IOP Publishing Ltd.,
    2011.
conference:
  name: International Conference on Atomic Physics
date_created: 2018-12-11T11:53:57Z
date_published: 2011-01-01T00:00:00Z
date_updated: 2019-04-26T07:22:05Z
day: '01'
doi: 10.1088/1742-6596/264/1/012024
extern: 1
fulldoi: https://doi.org/10.1088/1742-6596/264/1/012024
intvolume: '       264'
issue: '1'
month: '01'
publication_status: published
publisher: IOP Publishing Ltd.
publist_id: '5339'
quality_controlled: 0
status: public
title: Correlation measurements of individual microwave photons emitted from a symmetric
  cavity
type: conference
volume: 264
year: '2011'
...
---
_id: '1777'
abstract:
- lang: eng
  text: A wide range of experiments studying microwave photons localized in superconducting
    cavities have made important contributions to our understanding of the quantum
    properties of radiation. Propagating microwave photons, however, have so far been
    studied much less intensely. Here we present measurements in which we reconstruct
    the quantum state of itinerant single photon Fock states and their superposition
    with the vacuum by analyzing moments of the measured amplitude distribution up
    to fourth order. Using linear amplifiers and quadrature amplitude detectors, we
    have developed efficient methods to separate the detected single photon signal
    from the noise added by the amplifier. From our measurement data we have also
    reconstructed the corresponding Wigner function.
acknowledgement: This work was supported by the European Research Council (ERC) through
  a Starting Grant and by ETHZ
article_processing_charge: No
author:
- first_name: Christopher
  full_name: Eichler, Christopher
  last_name: Eichler
- first_name: Deniz
  full_name: Bozyigit, Deniz
  last_name: Bozyigit
- first_name: C
  full_name: Lang, C
  last_name: Lang
- first_name: L.
  full_name: Steffen, L.
  last_name: Steffen
- first_name: Johannes M
  full_name: Fink, Johannes M
  id: 4B591CBA-F248-11E8-B48F-1D18A9856A87
  last_name: Fink
  orcid: 0000-0001-8112-028X
- first_name: Andreas
  full_name: Wallraff, Andreas
  last_name: Wallraff
citation:
  ama: Eichler C, Bozyigit D, Lang C, Steffen L, Fink JM, Wallraff A. Experimental
    state tomography of itinerant single microwave photons. <i>Physical Review Letters</i>.
    2011;106(22). doi:<a href="https://doi.org/10.1103/PhysRevLett.106.220503">10.1103/PhysRevLett.106.220503</a>
  apa: Eichler, C., Bozyigit, D., Lang, C., Steffen, L., Fink, J. M., &#38; Wallraff,
    A. (2011). Experimental state tomography of itinerant single microwave photons.
    <i>Physical Review Letters</i>. American Physical Society. <a href="https://doi.org/10.1103/PhysRevLett.106.220503">https://doi.org/10.1103/PhysRevLett.106.220503</a>
  chicago: Eichler, Christopher, Deniz Bozyigit, C Lang, L. Steffen, Johannes M Fink,
    and Andreas Wallraff. “Experimental State Tomography of Itinerant Single Microwave
    Photons.” <i>Physical Review Letters</i>. American Physical Society, 2011. <a
    href="https://doi.org/10.1103/PhysRevLett.106.220503">https://doi.org/10.1103/PhysRevLett.106.220503</a>.
  ieee: C. Eichler, D. Bozyigit, C. Lang, L. Steffen, J. M. Fink, and A. Wallraff,
    “Experimental state tomography of itinerant single microwave photons,” <i>Physical
    Review Letters</i>, vol. 106, no. 22. American Physical Society, 2011.
  ista: Eichler C, Bozyigit D, Lang C, Steffen L, Fink JM, Wallraff A. 2011. Experimental
    state tomography of itinerant single microwave photons. Physical Review Letters.
    106(22).
  mla: Eichler, Christopher, et al. “Experimental State Tomography of Itinerant Single
    Microwave Photons.” <i>Physical Review Letters</i>, vol. 106, no. 22, American
    Physical Society, 2011, doi:<a href="https://doi.org/10.1103/PhysRevLett.106.220503">10.1103/PhysRevLett.106.220503</a>.
  short: C. Eichler, D. Bozyigit, C. Lang, L. Steffen, J.M. Fink, A. Wallraff, Physical
    Review Letters 106 (2011).
date_created: 2018-12-11T11:53:57Z
date_published: 2011-06-01T00:00:00Z
date_updated: 2021-11-16T07:57:13Z
day: '01'
doi: 10.1103/PhysRevLett.106.220503
extern: '1'
fulldoi: https://doi.org/10.1103/PhysRevLett.106.220503
intvolume: '       106'
issue: '22'
language:
- iso: eng
main_file_link:
- open_access: '1'
  url: http://arxiv.org/abs/1011.6668
month: '06'
oa: 1
oa_version: None
publication: Physical Review Letters
publication_status: published
publisher: American Physical Society
publist_id: '5338'
related_material:
  link:
  - relation: erratum
    url: https://doi.org/10.1103/PhysRevLett.106.249901
status: public
title: Experimental state tomography of itinerant single microwave photons
type: journal_article
user_id: 8b945eb4-e2f2-11eb-945a-df72226e66a9
volume: 106
year: '2011'
...
---
_id: '1778'
abstract:
- lang: eng
  text: Creating a train of single photons and monitoring its propagation and interaction
    is challenging in most physical systems, as photons generally interact very weakly
    with other systems. However, when confining microwave frequency photons in a transmission
    line resonator, effective photon-photon interactions can be mediated by qubits
    embedded in the resonator. Here, we observe the phenomenon of photon blockade
    through second-order correlation function measurements. The experiments clearly
    demonstrate antibunching in a continuously pumped source of single microwave photons
    measured by using microwave beam splitters, linear amplifiers, and quadrature
    amplitude detectors. We also investigate resonance fluorescence and Rayleigh scattering
    in Mollow-triplet-like spectra.
acknowledgement: This work was supported by the European Research Council (ERC) through
  a Starting Grant and by ETHZ. M. P. d. S. was supported by NSERC. A. B. was supported
  by NSERC, CIFAR, and the Alfred P. Sloan Foundation
author:
- first_name: C
  full_name: Lang, C
  last_name: Lang
- first_name: Deniz
  full_name: Bozyigit, Deniz
  last_name: Bozyigit
- first_name: Christopher
  full_name: Eichler, Christopher
  last_name: Eichler
- first_name: L.
  full_name: Steffen, L. Kraig
  last_name: Steffen
- first_name: Johannes M
  full_name: Johannes Fink
  id: 4B591CBA-F248-11E8-B48F-1D18A9856A87
  last_name: Fink
  orcid: 0000-0001-8112-028X
- first_name: Abdufarrukh
  full_name: Abdumalikov, Abdufarrukh A
  last_name: Abdumalikov
- first_name: Matthias
  full_name: Baur, Matthias P
  last_name: Baur
- first_name: Stefan
  full_name: Filipp, Stefan
  last_name: Filipp
- first_name: Marcus
  full_name: Da Silva, Marcus P
  last_name: Da Silva
- first_name: Alexandre
  full_name: Blais, Alexandre
  last_name: Blais
- first_name: Andreas
  full_name: Wallraff, Andreas
  last_name: Wallraff
citation:
  ama: Lang C, Bozyigit D, Eichler C, et al. Observation of resonant photon blockade
    at microwave frequencies using correlation function measurements. <i>Physical
    Review Letters</i>. 2011;106(24). doi:<a href="https://doi.org/10.1103/PhysRevLett.106.243601">10.1103/PhysRevLett.106.243601</a>
  apa: Lang, C., Bozyigit, D., Eichler, C., Steffen, L., Fink, J. M., Abdumalikov,
    A., … Wallraff, A. (2011). Observation of resonant photon blockade at microwave
    frequencies using correlation function measurements. <i>Physical Review Letters</i>.
    American Physical Society. <a href="https://doi.org/10.1103/PhysRevLett.106.243601">https://doi.org/10.1103/PhysRevLett.106.243601</a>
  chicago: Lang, C, Deniz Bozyigit, Christopher Eichler, L. Steffen, Johannes M Fink,
    Abdufarrukh Abdumalikov, Matthias Baur, et al. “Observation of Resonant Photon
    Blockade at Microwave Frequencies Using Correlation Function Measurements.” <i>Physical
    Review Letters</i>. American Physical Society, 2011. <a href="https://doi.org/10.1103/PhysRevLett.106.243601">https://doi.org/10.1103/PhysRevLett.106.243601</a>.
  ieee: C. Lang <i>et al.</i>, “Observation of resonant photon blockade at microwave
    frequencies using correlation function measurements,” <i>Physical Review Letters</i>,
    vol. 106, no. 24. American Physical Society, 2011.
  ista: Lang C, Bozyigit D, Eichler C, Steffen L, Fink JM, Abdumalikov A, Baur M,
    Filipp S, Da Silva M, Blais A, Wallraff A. 2011. Observation of resonant photon
    blockade at microwave frequencies using correlation function measurements. Physical
    Review Letters. 106(24).
  mla: Lang, C., et al. “Observation of Resonant Photon Blockade at Microwave Frequencies
    Using Correlation Function Measurements.” <i>Physical Review Letters</i>, vol.
    106, no. 24, American Physical Society, 2011, doi:<a href="https://doi.org/10.1103/PhysRevLett.106.243601">10.1103/PhysRevLett.106.243601</a>.
  short: C. Lang, D. Bozyigit, C. Eichler, L. Steffen, J.M. Fink, A. Abdumalikov,
    M. Baur, S. Filipp, M. Da Silva, A. Blais, A. Wallraff, Physical Review Letters
    106 (2011).
date_created: 2018-12-11T11:53:57Z
date_published: 2011-06-15T00:00:00Z
date_updated: 2021-01-12T06:53:08Z
day: '15'
doi: 10.1103/PhysRevLett.106.243601
extern: 1
fulldoi: https://doi.org/10.1103/PhysRevLett.106.243601
intvolume: '       106'
issue: '24'
main_file_link:
- open_access: '1'
  url: http://arxiv.org/abs/1102.0461
month: '06'
oa: 1
publication: Physical Review Letters
publication_status: published
publisher: American Physical Society
publist_id: '5336'
quality_controlled: 0
status: public
title: Observation of resonant photon blockade at microwave frequencies using correlation
  function measurements
type: journal_article
volume: 106
year: '2011'
...
---
_id: '1780'
abstract:
- lang: eng
  text: Continuous variable entanglement between two modes of a radiation field is
    usually studied at optical frequencies. Here we demonstrate experiments that show
    the entanglement between microwave photons of different energy in a broadband
    squeezed beam. We use a Josephson parametric amplifier to generate the two-mode
    correlated state and detect all four quadrature components simultaneously in a
    two-channel heterodyne setup using amplitude detectors. Analyzing two-dimensional
    phase space histograms for all possible pairs of quadratures allows us to determine
    the full covariance matrix, which is in good agreement with the one expected for
    a two-mode squeezed state.
acknowledgement: This work was supported by the European Research Council (ERC) through
  a Starting grant and by ETHZ. S. F. acknowledges the Austrian Science Foundation
  (FWF) for support
author:
- first_name: Christopher
  full_name: Eichler, Christopher
  last_name: Eichler
- first_name: Deniz
  full_name: Bozyigit, Deniz
  last_name: Bozyigit
- first_name: C
  full_name: Lang, C
  last_name: Lang
- first_name: Matthias
  full_name: Baur, Matthias P
  last_name: Baur
- first_name: L.
  full_name: Steffen, L. Kraig
  last_name: Steffen
- first_name: Johannes M
  full_name: Johannes Fink
  id: 4B591CBA-F248-11E8-B48F-1D18A9856A87
  last_name: Fink
  orcid: 0000-0001-8112-028X
- first_name: Stefan
  full_name: Filipp, Stefan
  last_name: Filipp
- first_name: Andreas
  full_name: Wallraff, Andreas
  last_name: Wallraff
citation:
  ama: Eichler C, Bozyigit D, Lang C, et al. Observation of two-mode squeezing in
    the microwave frequency domain. <i>Physical Review Letters</i>. 2011;107(11).
    doi:<a href="https://doi.org/10.1103/PhysRevLett.107.113601">10.1103/PhysRevLett.107.113601</a>
  apa: Eichler, C., Bozyigit, D., Lang, C., Baur, M., Steffen, L., Fink, J. M., …
    Wallraff, A. (2011). Observation of two-mode squeezing in the microwave frequency
    domain. <i>Physical Review Letters</i>. American Physical Society. <a href="https://doi.org/10.1103/PhysRevLett.107.113601">https://doi.org/10.1103/PhysRevLett.107.113601</a>
  chicago: Eichler, Christopher, Deniz Bozyigit, C Lang, Matthias Baur, L. Steffen,
    Johannes M Fink, Stefan Filipp, and Andreas Wallraff. “Observation of Two-Mode
    Squeezing in the Microwave Frequency Domain.” <i>Physical Review Letters</i>.
    American Physical Society, 2011. <a href="https://doi.org/10.1103/PhysRevLett.107.113601">https://doi.org/10.1103/PhysRevLett.107.113601</a>.
  ieee: C. Eichler <i>et al.</i>, “Observation of two-mode squeezing in the microwave
    frequency domain,” <i>Physical Review Letters</i>, vol. 107, no. 11. American
    Physical Society, 2011.
  ista: Eichler C, Bozyigit D, Lang C, Baur M, Steffen L, Fink JM, Filipp S, Wallraff
    A. 2011. Observation of two-mode squeezing in the microwave frequency domain.
    Physical Review Letters. 107(11).
  mla: Eichler, Christopher, et al. “Observation of Two-Mode Squeezing in the Microwave
    Frequency Domain.” <i>Physical Review Letters</i>, vol. 107, no. 11, American
    Physical Society, 2011, doi:<a href="https://doi.org/10.1103/PhysRevLett.107.113601">10.1103/PhysRevLett.107.113601</a>.
  short: C. Eichler, D. Bozyigit, C. Lang, M. Baur, L. Steffen, J.M. Fink, S. Filipp,
    A. Wallraff, Physical Review Letters 107 (2011).
date_created: 2018-12-11T11:53:58Z
date_published: 2011-09-06T00:00:00Z
date_updated: 2021-01-12T06:53:09Z
day: '06'
doi: 10.1103/PhysRevLett.107.113601
extern: 1
fulldoi: https://doi.org/10.1103/PhysRevLett.107.113601
intvolume: '       107'
issue: '11'
month: '09'
publication: Physical Review Letters
publication_status: published
publisher: American Physical Society
publist_id: '5334'
quality_controlled: 0
status: public
title: Observation of two-mode squeezing in the microwave frequency domain
type: journal_article
volume: 107
year: '2011'
...
---
_id: '1781'
abstract:
- lang: eng
  text: Microwave cavities with high quality factors enable coherent coupling of distant
    quantum systems. Virtual photons lead to a transverse interaction between qubits
    when they are nonresonant with the cavity but resonant with each other. We experimentally
    investigate the inverse scaling of the interqubit coupling with the detuning from
    a cavity mode and its proportionality to the qubit-cavity interaction strength.
    We demonstrate that the enhanced coupling at higher frequencies is mediated by
    multiple higher-harmonic cavity modes. Moreover, we observe dark states of the
    coupled qubit-qubit system and analyze their relation to the symmetry of the applied
    driving field at different frequencies.
acknowledgement: This work was supported by the Swiss National Science Foundation
  (SNF), the Austrian Science Foundation (FWF), and ETH Zurich
author:
- first_name: Stefan
  full_name: Filipp, Stefan
  last_name: Filipp
- first_name: M
  full_name: Göppl, M
  last_name: Göppl
- first_name: Johannes M
  full_name: Johannes Fink
  id: 4B591CBA-F248-11E8-B48F-1D18A9856A87
  last_name: Fink
  orcid: 0000-0001-8112-028X
- first_name: Matthias
  full_name: Baur, Matthias P
  last_name: Baur
- first_name: R
  full_name: Bianchetti, R
  last_name: Bianchetti
- first_name: L.
  full_name: Steffen, L. Kraig
  last_name: Steffen
- first_name: Andreas
  full_name: Wallraff, Andreas
  last_name: Wallraff
citation:
  ama: Filipp S, Göppl M, Fink JM, et al. Multimode mediated qubit-qubit coupling
    and dark-state symmetries in circuit quantum electrodynamics. <i>Physical Review
    A - Atomic, Molecular, and Optical Physics</i>. 2011;83(6). doi:<a href="https://doi.org/10.1103/PhysRevA.83.063827">10.1103/PhysRevA.83.063827</a>
  apa: Filipp, S., Göppl, M., Fink, J. M., Baur, M., Bianchetti, R., Steffen, L.,
    &#38; Wallraff, A. (2011). Multimode mediated qubit-qubit coupling and dark-state
    symmetries in circuit quantum electrodynamics. <i>Physical Review A - Atomic,
    Molecular, and Optical Physics</i>. American Physical Society. <a href="https://doi.org/10.1103/PhysRevA.83.063827">https://doi.org/10.1103/PhysRevA.83.063827</a>
  chicago: Filipp, Stefan, M Göppl, Johannes M Fink, Matthias Baur, R Bianchetti,
    L. Steffen, and Andreas Wallraff. “Multimode Mediated Qubit-Qubit Coupling and
    Dark-State Symmetries in Circuit Quantum Electrodynamics.” <i>Physical Review
    A - Atomic, Molecular, and Optical Physics</i>. American Physical Society, 2011.
    <a href="https://doi.org/10.1103/PhysRevA.83.063827">https://doi.org/10.1103/PhysRevA.83.063827</a>.
  ieee: S. Filipp <i>et al.</i>, “Multimode mediated qubit-qubit coupling and dark-state
    symmetries in circuit quantum electrodynamics,” <i>Physical Review A - Atomic,
    Molecular, and Optical Physics</i>, vol. 83, no. 6. American Physical Society,
    2011.
  ista: Filipp S, Göppl M, Fink JM, Baur M, Bianchetti R, Steffen L, Wallraff A. 2011.
    Multimode mediated qubit-qubit coupling and dark-state symmetries in circuit quantum
    electrodynamics. Physical Review A - Atomic, Molecular, and Optical Physics. 83(6).
  mla: Filipp, Stefan, et al. “Multimode Mediated Qubit-Qubit Coupling and Dark-State
    Symmetries in Circuit Quantum Electrodynamics.” <i>Physical Review A - Atomic,
    Molecular, and Optical Physics</i>, vol. 83, no. 6, American Physical Society,
    2011, doi:<a href="https://doi.org/10.1103/PhysRevA.83.063827">10.1103/PhysRevA.83.063827</a>.
  short: S. Filipp, M. Göppl, J.M. Fink, M. Baur, R. Bianchetti, L. Steffen, A. Wallraff,
    Physical Review A - Atomic, Molecular, and Optical Physics 83 (2011).
date_created: 2018-12-11T11:53:58Z
date_published: 2011-06-22T00:00:00Z
date_updated: 2021-01-12T06:53:09Z
day: '22'
doi: 10.1103/PhysRevA.83.063827
extern: 1
fulldoi: https://doi.org/10.1103/PhysRevA.83.063827
intvolume: '        83'
issue: '6'
month: '06'
publication: Physical Review A - Atomic, Molecular, and Optical Physics
publication_status: published
publisher: American Physical Society
publist_id: '5335'
quality_controlled: 0
status: public
title: Multimode mediated qubit-qubit coupling and dark-state symmetries in circuit
  quantum electrodynamics
type: journal_article
volume: 83
year: '2011'
...
---
OA_type: closed access
_id: '18012'
abstract:
- lang: eng
  text: We report the first concurrent determination of conductance (G) and thermopower
    (S) of single-molecule junctions via direct measurement of electrical and thermoelectric
    currents using a scanning tunneling microscope-based break-junction technique.
    We explore several amine-Au and pyridine-Au linked molecules that are predicted
    to conduct through either the highest occupied molecular orbital (HOMO) or the
    lowest unoccupied molecular orbital (LUMO), respectively. We find that the Seebeck
    coefficient is negative for pyridine-Au linked LUMO-conducting junctions and positive
    for amine-Au linked HOMO-conducting junctions. Within the accessible temperature
    gradients (<30 K), we do not observe a strong dependence of the junction Seebeck
    coefficient on temperature. From histograms of thousands of junctions, we use
    the most probable Seebeck coefficient to determine a power factor, GS2, for each
    junction studied, and find that GS2 increases with G. Finally, we find that conductance
    and Seebeck coefficient values are in good quantitative agreement with our self-energy
    corrected density functional theory calculations.
article_processing_charge: No
article_type: letter_note
author:
- first_name: Jonathan R.
  full_name: Widawsky, Jonathan R.
  last_name: Widawsky
- first_name: Pierre
  full_name: Darancet, Pierre
  last_name: Darancet
- first_name: Jeffrey B.
  full_name: Neaton, Jeffrey B.
  last_name: Neaton
- first_name: Latha
  full_name: Venkataraman, Latha
  id: 9ebb78a5-cc0d-11ee-8322-fae086a32caf
  last_name: Venkataraman
  orcid: 0000-0002-6957-6089
citation:
  ama: Widawsky JR, Darancet P, Neaton JB, Venkataraman L. Simultaneous determination
    of conductance and thermopower of single molecule junctions. <i>Nano Letters</i>.
    2011;12(1):354-358. doi:<a href="https://doi.org/10.1021/nl203634m">10.1021/nl203634m</a>
  apa: Widawsky, J. R., Darancet, P., Neaton, J. B., &#38; Venkataraman, L. (2011).
    Simultaneous determination of conductance and thermopower of single molecule junctions.
    <i>Nano Letters</i>. American Chemical Society. <a href="https://doi.org/10.1021/nl203634m">https://doi.org/10.1021/nl203634m</a>
  chicago: Widawsky, Jonathan R., Pierre Darancet, Jeffrey B. Neaton, and Latha Venkataraman.
    “Simultaneous Determination of Conductance and Thermopower of Single Molecule
    Junctions.” <i>Nano Letters</i>. American Chemical Society, 2011. <a href="https://doi.org/10.1021/nl203634m">https://doi.org/10.1021/nl203634m</a>.
  ieee: J. R. Widawsky, P. Darancet, J. B. Neaton, and L. Venkataraman, “Simultaneous
    determination of conductance and thermopower of single molecule junctions,” <i>Nano
    Letters</i>, vol. 12, no. 1. American Chemical Society, pp. 354–358, 2011.
  ista: Widawsky JR, Darancet P, Neaton JB, Venkataraman L. 2011. Simultaneous determination
    of conductance and thermopower of single molecule junctions. Nano Letters. 12(1),
    354–358.
  mla: Widawsky, Jonathan R., et al. “Simultaneous Determination of Conductance and
    Thermopower of Single Molecule Junctions.” <i>Nano Letters</i>, vol. 12, no. 1,
    American Chemical Society, 2011, pp. 354–58, doi:<a href="https://doi.org/10.1021/nl203634m">10.1021/nl203634m</a>.
  short: J.R. Widawsky, P. Darancet, J.B. Neaton, L. Venkataraman, Nano Letters 12
    (2011) 354–358.
date_created: 2024-09-09T12:32:14Z
date_published: 2011-11-30T00:00:00Z
date_updated: 2025-01-03T09:26:26Z
day: '30'
doi: 10.1021/nl203634m
extern: '1'
external_id:
  pmid:
  - '22128800'
fulldoi: https://doi.org/10.1021/nl203634m
intvolume: '        12'
issue: '1'
language:
- iso: eng
month: '11'
oa_version: None
page: 354-358
pmid: 1
publication: Nano Letters
publication_identifier:
  eissn:
  - 1530-6992
  issn:
  - 1530-6984
publication_status: published
publisher: American Chemical Society
quality_controlled: '1'
scopus_import: '1'
status: public
title: Simultaneous determination of conductance and thermopower of single molecule
  junctions
type: journal_article
user_id: 2DF688A6-F248-11E8-B48F-1D18A9856A87
volume: 12
year: '2011'
...
---
OA_place: repository
OA_type: green
_id: '18014'
abstract:
- lang: eng
  text: We measure electronic conductance through single conjugated molecules bonded
    to Au metal electrodes with direct Au–C covalent bonds using the scanning tunneling
    microscope based break-junction technique. We start with molecules terminated
    with trimethyltin end groups that cleave off in situ, resulting in formation of
    a direct covalent σ bond between the carbon backbone and the gold metal electrodes.
    The molecular carbon backbone used in this study consist of a conjugated π system
    that has one terminal methylene group on each end, which bonds to the electrodes,
    achieving large electronic coupling of the electrodes to the π system. The junctions
    formed with the prototypical example of 1,4-dimethylenebenzene show a conductance
    approaching one conductance quantum (G0 = 2e2/h). Junctions formed with methylene-terminated
    oligophenyls with two to four phenyl units show a 100-fold increase in conductance
    compared with junctions formed with amine-linked oligophenyls. The conduction
    mechanism for these longer oligophenyls is tunneling, as they exhibit an exponential
    dependence of conductance on oligomer length. In addition, density functional
    theory based calculations for the Au–xylylene–Au junction show near-resonant transmission,
    with a crossover to tunneling for the longer oligomers.
article_processing_charge: No
article_type: letter_note
arxiv: 1
author:
- first_name: Wenbo
  full_name: Chen, Wenbo
  last_name: Chen
- first_name: Jonathan R.
  full_name: Widawsky, Jonathan R.
  last_name: Widawsky
- first_name: Héctor
  full_name: Vázquez, Héctor
  last_name: Vázquez
- first_name: Severin T.
  full_name: Schneebeli, Severin T.
  last_name: Schneebeli
- first_name: Mark S.
  full_name: Hybertsen, Mark S.
  last_name: Hybertsen
- first_name: Ronald
  full_name: Breslow, Ronald
  last_name: Breslow
- first_name: Latha
  full_name: Venkataraman, Latha
  id: 9ebb78a5-cc0d-11ee-8322-fae086a32caf
  last_name: Venkataraman
  orcid: 0000-0002-6957-6089
citation:
  ama: Chen W, Widawsky JR, Vázquez H, et al. Highly conducting π-conjugated molecular
    junctions covalently bonded to gold electrodes. <i>Journal of the American Chemical
    Society</i>. 2011;133(43):17160-17163. doi:<a href="https://doi.org/10.1021/ja208020j">10.1021/ja208020j</a>
  apa: Chen, W., Widawsky, J. R., Vázquez, H., Schneebeli, S. T., Hybertsen, M. S.,
    Breslow, R., &#38; Venkataraman, L. (2011). Highly conducting π-conjugated molecular
    junctions covalently bonded to gold electrodes. <i>Journal of the American Chemical
    Society</i>. American Chemical Society. <a href="https://doi.org/10.1021/ja208020j">https://doi.org/10.1021/ja208020j</a>
  chicago: Chen, Wenbo, Jonathan R. Widawsky, Héctor Vázquez, Severin T. Schneebeli,
    Mark S. Hybertsen, Ronald Breslow, and Latha Venkataraman. “Highly Conducting
    π-Conjugated Molecular Junctions Covalently Bonded to Gold Electrodes.” <i>Journal
    of the American Chemical Society</i>. American Chemical Society, 2011. <a href="https://doi.org/10.1021/ja208020j">https://doi.org/10.1021/ja208020j</a>.
  ieee: W. Chen <i>et al.</i>, “Highly conducting π-conjugated molecular junctions
    covalently bonded to gold electrodes,” <i>Journal of the American Chemical Society</i>,
    vol. 133, no. 43. American Chemical Society, pp. 17160–17163, 2011.
  ista: Chen W, Widawsky JR, Vázquez H, Schneebeli ST, Hybertsen MS, Breslow R, Venkataraman
    L. 2011. Highly conducting π-conjugated molecular junctions covalently bonded
    to gold electrodes. Journal of the American Chemical Society. 133(43), 17160–17163.
  mla: Chen, Wenbo, et al. “Highly Conducting π-Conjugated Molecular Junctions Covalently
    Bonded to Gold Electrodes.” <i>Journal of the American Chemical Society</i>, vol.
    133, no. 43, American Chemical Society, 2011, pp. 17160–63, doi:<a href="https://doi.org/10.1021/ja208020j">10.1021/ja208020j</a>.
  short: W. Chen, J.R. Widawsky, H. Vázquez, S.T. Schneebeli, M.S. Hybertsen, R. Breslow,
    L. Venkataraman, Journal of the American Chemical Society 133 (2011) 17160–17163.
date_created: 2024-09-09T12:33:46Z
date_published: 2011-09-22T00:00:00Z
date_updated: 2025-01-03T09:34:24Z
day: '22'
doi: 10.1021/ja208020j
extern: '1'
external_id:
  arxiv:
  - '1110.0344'
  pmid:
  - '21939263'
fulldoi: https://doi.org/10.1021/ja208020j
intvolume: '       133'
issue: '43'
language:
- iso: eng
main_file_link:
- open_access: '1'
  url: https://arxiv.org/abs/1110.0344
month: '09'
oa: 1
oa_version: Preprint
page: 17160-17163
pmid: 1
publication: Journal of the American Chemical Society
publication_identifier:
  eissn:
  - 1520-5126
  issn:
  - 0002-7863
publication_status: published
publisher: American Chemical Society
quality_controlled: '1'
scopus_import: '1'
status: public
title: Highly conducting π-conjugated molecular junctions covalently bonded to gold
  electrodes
type: journal_article
user_id: 2DF688A6-F248-11E8-B48F-1D18A9856A87
volume: 133
year: '2011'
...
---
OA_type: closed access
_id: '18015'
abstract:
- lang: eng
  text: We investigate the binding and energy level alignment of 2,3,5,6-tetramethyl-1,4-benzenediamine
    (TMBDA) on Au(111) through a combination of helium atom scattering (HAS), X-ray
    photoemission (XPS), and scanning tunneling microscopy (STM). We show that TMBDA
    binds to step edges and to flat Au (111) terraces in a nearly flat-lying configuration.
    Through combination of HAS and STM data, we determine that the molecules are bound
    on step edges with an adsorption energy of about 1.2 eV, which is about 0.2 eV
    stronger than the adsorption energy we measure on flat surface. Preferential bonding
    to the under-coordinated Au atoms on step edges suggests that the molecules bind
    to Au through the nitrogen lone pair. Finally, STM measurements on TMBDA in these
    two different adsorption configurations show that the highest-occupied molecular
    orbital is deeper relative to Fermi for the more strongly bound molecules on step
    edges, confirming that the nitrogen bonds through charge donation to the Au.
article_processing_charge: No
article_type: original
author:
- first_name: M.
  full_name: Kamenetska, M.
  last_name: Kamenetska
- first_name: M.
  full_name: Dell’Angela, M.
  last_name: Dell’Angela
- first_name: J.R.
  full_name: Widawsky, J.R.
  last_name: Widawsky
- first_name: G.
  full_name: Kladnik, G.
  last_name: Kladnik
- first_name: A.
  full_name: Verdini, A.
  last_name: Verdini
- first_name: A.
  full_name: Cossaro, A.
  last_name: Cossaro
- first_name: D.
  full_name: Cvetko, D.
  last_name: Cvetko
- first_name: A.
  full_name: Morgante, A.
  last_name: Morgante
- first_name: Latha
  full_name: Venkataraman, Latha
  id: 9ebb78a5-cc0d-11ee-8322-fae086a32caf
  last_name: Venkataraman
  orcid: 0000-0002-6957-6089
citation:
  ama: Kamenetska M, Dell’Angela M, Widawsky JR, et al. Structure and energy level
    alignment of tetramethyl benzenediamine on Au(111). <i>The Journal of Physical
    Chemistry C</i>. 2011;115(25):12625-12630. doi:<a href="https://doi.org/10.1021/jp202555d">10.1021/jp202555d</a>
  apa: Kamenetska, M., Dell’Angela, M., Widawsky, J. R., Kladnik, G., Verdini, A.,
    Cossaro, A., … Venkataraman, L. (2011). Structure and energy level alignment of
    tetramethyl benzenediamine on Au(111). <i>The Journal of Physical Chemistry C</i>.
    American Chemical Society. <a href="https://doi.org/10.1021/jp202555d">https://doi.org/10.1021/jp202555d</a>
  chicago: Kamenetska, M., M. Dell’Angela, J.R. Widawsky, G. Kladnik, A. Verdini,
    A. Cossaro, D. Cvetko, A. Morgante, and Latha Venkataraman. “Structure and Energy
    Level Alignment of Tetramethyl Benzenediamine on Au(111).” <i>The Journal of Physical
    Chemistry C</i>. American Chemical Society, 2011. <a href="https://doi.org/10.1021/jp202555d">https://doi.org/10.1021/jp202555d</a>.
  ieee: M. Kamenetska <i>et al.</i>, “Structure and energy level alignment of tetramethyl
    benzenediamine on Au(111),” <i>The Journal of Physical Chemistry C</i>, vol. 115,
    no. 25. American Chemical Society, pp. 12625–12630, 2011.
  ista: Kamenetska M, Dell’Angela M, Widawsky JR, Kladnik G, Verdini A, Cossaro A,
    Cvetko D, Morgante A, Venkataraman L. 2011. Structure and energy level alignment
    of tetramethyl benzenediamine on Au(111). The Journal of Physical Chemistry C.
    115(25), 12625–12630.
  mla: Kamenetska, M., et al. “Structure and Energy Level Alignment of Tetramethyl
    Benzenediamine on Au(111).” <i>The Journal of Physical Chemistry C</i>, vol. 115,
    no. 25, American Chemical Society, 2011, pp. 12625–30, doi:<a href="https://doi.org/10.1021/jp202555d">10.1021/jp202555d</a>.
  short: M. Kamenetska, M. Dell’Angela, J.R. Widawsky, G. Kladnik, A. Verdini, A.
    Cossaro, D. Cvetko, A. Morgante, L. Venkataraman, The Journal of Physical Chemistry
    C 115 (2011) 12625–12630.
date_created: 2024-09-09T12:34:26Z
date_published: 2011-05-17T00:00:00Z
date_updated: 2025-01-03T09:36:40Z
day: '17'
doi: 10.1021/jp202555d
extern: '1'
fulldoi: https://doi.org/10.1021/jp202555d
intvolume: '       115'
issue: '25'
language:
- iso: eng
month: '05'
oa_version: None
page: 12625-12630
publication: The Journal of Physical Chemistry C
publication_identifier:
  eissn:
  - 1932-7455
  issn:
  - 1932-7447
publication_status: published
publisher: American Chemical Society
quality_controlled: '1'
scopus_import: '1'
status: public
title: Structure and energy level alignment of tetramethyl benzenediamine on Au(111)
type: journal_article
user_id: 2DF688A6-F248-11E8-B48F-1D18A9856A87
volume: 115
year: '2011'
...
---
OA_type: closed access
_id: '18016'
abstract:
- lang: eng
  text: Understanding the electrical properties of semiconducting quantum dot devices
    have been limited due to the variability of their size/composition and the chemistry
    of ligand/electrode binding. Furthermore, to probe their electrical conduction
    properties and its dependence on ligand/electrode binding, measurements must be
    carried out at the single dot/cluster level. Herein we report scanning tunneling
    microscope based break junction measurements of cobalt chalcogenide clusters with
    Te, Se and S to probe the conductance properties. Our measured conductance trends
    show that the Co–Te based clusters have the highest conductance while the Co-S
    clusters the lowest. These trends are in very good agreement with cyclic voltammetry
    measurements of the first oxidation potentials and with density functional theory
    calculations of their HOMO–LUMO gaps.
article_processing_charge: No
article_type: letter_note
author:
- first_name: Brycelyn M.
  full_name: Boardman, Brycelyn M.
  last_name: Boardman
- first_name: Jonathan R.
  full_name: Widawsky, Jonathan R.
  last_name: Widawsky
- first_name: Young S.
  full_name: Park, Young S.
  last_name: Park
- first_name: Christine L.
  full_name: Schenck, Christine L.
  last_name: Schenck
- first_name: Latha
  full_name: Venkataraman, Latha
  id: 9ebb78a5-cc0d-11ee-8322-fae086a32caf
  last_name: Venkataraman
  orcid: 0000-0002-6957-6089
- first_name: Michael L.
  full_name: Steigerwald, Michael L.
  last_name: Steigerwald
- first_name: Colin
  full_name: Nuckolls, Colin
  last_name: Nuckolls
citation:
  ama: Boardman BM, Widawsky JR, Park YS, et al. Conductance of single cobalt chalcogenide
    cluster junctions. <i>Journal of the American Chemical Society</i>. 2011;133(22):8455-8457.
    doi:<a href="https://doi.org/10.1021/ja201334s">10.1021/ja201334s</a>
  apa: Boardman, B. M., Widawsky, J. R., Park, Y. S., Schenck, C. L., Venkataraman,
    L., Steigerwald, M. L., &#38; Nuckolls, C. (2011). Conductance of single cobalt
    chalcogenide cluster junctions. <i>Journal of the American Chemical Society</i>.
    American Chemical Society. <a href="https://doi.org/10.1021/ja201334s">https://doi.org/10.1021/ja201334s</a>
  chicago: Boardman, Brycelyn M., Jonathan R. Widawsky, Young S. Park, Christine L.
    Schenck, Latha Venkataraman, Michael L. Steigerwald, and Colin Nuckolls. “Conductance
    of Single Cobalt Chalcogenide Cluster Junctions.” <i>Journal of the American Chemical
    Society</i>. American Chemical Society, 2011. <a href="https://doi.org/10.1021/ja201334s">https://doi.org/10.1021/ja201334s</a>.
  ieee: B. M. Boardman <i>et al.</i>, “Conductance of single cobalt chalcogenide cluster
    junctions,” <i>Journal of the American Chemical Society</i>, vol. 133, no. 22.
    American Chemical Society, pp. 8455–8457, 2011.
  ista: Boardman BM, Widawsky JR, Park YS, Schenck CL, Venkataraman L, Steigerwald
    ML, Nuckolls C. 2011. Conductance of single cobalt chalcogenide cluster junctions.
    Journal of the American Chemical Society. 133(22), 8455–8457.
  mla: Boardman, Brycelyn M., et al. “Conductance of Single Cobalt Chalcogenide Cluster
    Junctions.” <i>Journal of the American Chemical Society</i>, vol. 133, no. 22,
    American Chemical Society, 2011, pp. 8455–57, doi:<a href="https://doi.org/10.1021/ja201334s">10.1021/ja201334s</a>.
  short: B.M. Boardman, J.R. Widawsky, Y.S. Park, C.L. Schenck, L. Venkataraman, M.L.
    Steigerwald, C. Nuckolls, Journal of the American Chemical Society 133 (2011)
    8455–8457.
date_created: 2024-09-09T12:35:04Z
date_published: 2011-05-03T00:00:00Z
date_updated: 2025-01-03T09:38:32Z
day: '03'
doi: 10.1021/ja201334s
extern: '1'
external_id:
  pmid:
  - '21539375'
fulldoi: https://doi.org/10.1021/ja201334s
intvolume: '       133'
issue: '22'
language:
- iso: eng
month: '05'
oa_version: None
page: 8455-8457
pmid: 1
publication: Journal of the American Chemical Society
publication_identifier:
  eissn:
  - 1520-5126
  issn:
  - 0002-7863
publication_status: published
publisher: American Chemical Society
quality_controlled: '1'
scopus_import: '1'
status: public
title: Conductance of single cobalt chalcogenide cluster junctions
type: journal_article
user_id: 2DF688A6-F248-11E8-B48F-1D18A9856A87
volume: 133
year: '2011'
...
---
OA_type: closed access
_id: '18017'
abstract:
- lang: eng
  text: The conductance of individual 1,4-benzenediamine (BDA)–Au molecular junctions
    is measured in different solvent environments using a scanning tunneling microscope
    based point-contact technique. Solvents are found to increase the conductance
    of these molecular junctions by as much as 50%. Using first principles calculations,
    we explain this increase by showing that a shift in the Au contact work function
    is induced by solvents binding to undercoordinated Au sites around the junction.
    Increasing the Au contact work function reduces the separation between the Au
    Fermi energy and the highest occupied molecular orbital of BDA in the junction,
    increasing the measured conductance. We demonstrate that the solvent-induced shift
    in conductance depends on the affinity of the solvent to Au binding sites and
    also on the induced dipole (relative to BDA) upon adsorption. Via this mechanism,
    molecular junction level alignment and transport properties can be statistically
    altered by solvent molecule binding to the contact surface.
article_processing_charge: No
article_type: letter_note
author:
- first_name: V.
  full_name: Fatemi, V.
  last_name: Fatemi
- first_name: M.
  full_name: Kamenetska, M.
  last_name: Kamenetska
- first_name: J. B.
  full_name: Neaton, J. B.
  last_name: Neaton
- first_name: Latha
  full_name: Venkataraman, Latha
  id: 9ebb78a5-cc0d-11ee-8322-fae086a32caf
  last_name: Venkataraman
  orcid: 0000-0002-6957-6089
citation:
  ama: Fatemi V, Kamenetska M, Neaton JB, Venkataraman L. Environmental control of
    single-molecule junction transport. <i>Nano Letters</i>. 2011;11(5):1988-1992.
    doi:<a href="https://doi.org/10.1021/nl200324e">10.1021/nl200324e</a>
  apa: Fatemi, V., Kamenetska, M., Neaton, J. B., &#38; Venkataraman, L. (2011). Environmental
    control of single-molecule junction transport. <i>Nano Letters</i>. American Chemical
    Society. <a href="https://doi.org/10.1021/nl200324e">https://doi.org/10.1021/nl200324e</a>
  chicago: Fatemi, V., M. Kamenetska, J. B. Neaton, and Latha Venkataraman. “Environmental
    Control of Single-Molecule Junction Transport.” <i>Nano Letters</i>. American
    Chemical Society, 2011. <a href="https://doi.org/10.1021/nl200324e">https://doi.org/10.1021/nl200324e</a>.
  ieee: V. Fatemi, M. Kamenetska, J. B. Neaton, and L. Venkataraman, “Environmental
    control of single-molecule junction transport,” <i>Nano Letters</i>, vol. 11,
    no. 5. American Chemical Society, pp. 1988–1992, 2011.
  ista: Fatemi V, Kamenetska M, Neaton JB, Venkataraman L. 2011. Environmental control
    of single-molecule junction transport. Nano Letters. 11(5), 1988–1992.
  mla: Fatemi, V., et al. “Environmental Control of Single-Molecule Junction Transport.”
    <i>Nano Letters</i>, vol. 11, no. 5, American Chemical Society, 2011, pp. 1988–92,
    doi:<a href="https://doi.org/10.1021/nl200324e">10.1021/nl200324e</a>.
  short: V. Fatemi, M. Kamenetska, J.B. Neaton, L. Venkataraman, Nano Letters 11 (2011)
    1988–1992.
date_created: 2024-09-09T12:35:47Z
date_published: 2011-04-18T00:00:00Z
date_updated: 2025-01-03T09:43:09Z
day: '18'
doi: 10.1021/nl200324e
extern: '1'
external_id:
  pmid:
  - '21500833'
fulldoi: https://doi.org/10.1021/nl200324e
intvolume: '        11'
issue: '5'
language:
- iso: eng
month: '04'
oa_version: None
page: 1988-1992
pmid: 1
publication: Nano Letters
publication_identifier:
  eissn:
  - 1530-6992
  issn:
  - 1530-6984
publication_status: published
publisher: American Chemical Society
quality_controlled: '1'
scopus_import: '1'
status: public
title: Environmental control of single-molecule junction transport
type: journal_article
user_id: 2DF688A6-F248-11E8-B48F-1D18A9856A87
volume: 11
year: '2011'
...
---
OA_type: closed access
_id: '18018'
abstract:
- lang: eng
  text: Controlling electron transport through a single-molecule device is key to
    the realization of nanoscale electronic components. A design requirement for single
    molecule electrical devices is that the molecule must be both structurally and
    electrically connected to the metallic electrodes. Typically, the mechanical and
    electrical contacts are achieved by the same chemical moiety. In this study, we
    demonstrate that the structural role may be played by one group (for example,
    a sulfide) while the electrical role may be played by another (a conjugated chain
    of C═C π-bonds). We can specify the electrical conductance through the molecule
    by modulating to which particular site on the oligoene chain the electrode binds.
    The result is a device that functions as a potentiometer at the single-molecule
    level.
article_processing_charge: No
article_type: letter_note
author:
- first_name: Jeffrey S.
  full_name: Meisner, Jeffrey S.
  last_name: Meisner
- first_name: Masha
  full_name: Kamenetska, Masha
  last_name: Kamenetska
- first_name: Markrete
  full_name: Krikorian, Markrete
  last_name: Krikorian
- first_name: Michael L.
  full_name: Steigerwald, Michael L.
  last_name: Steigerwald
- first_name: Latha
  full_name: Venkataraman, Latha
  id: 9ebb78a5-cc0d-11ee-8322-fae086a32caf
  last_name: Venkataraman
  orcid: 0000-0002-6957-6089
- first_name: Colin
  full_name: Nuckolls, Colin
  last_name: Nuckolls
citation:
  ama: Meisner JS, Kamenetska M, Krikorian M, Steigerwald ML, Venkataraman L, Nuckolls
    C. A single-molecule potentiometer. <i>Nano Letters</i>. 2011;11(4):1575-1579.
    doi:<a href="https://doi.org/10.1021/nl104411f">10.1021/nl104411f</a>
  apa: Meisner, J. S., Kamenetska, M., Krikorian, M., Steigerwald, M. L., Venkataraman,
    L., &#38; Nuckolls, C. (2011). A single-molecule potentiometer. <i>Nano Letters</i>.
    American Chemical Society. <a href="https://doi.org/10.1021/nl104411f">https://doi.org/10.1021/nl104411f</a>
  chicago: Meisner, Jeffrey S., Masha Kamenetska, Markrete Krikorian, Michael L. Steigerwald,
    Latha Venkataraman, and Colin Nuckolls. “A Single-Molecule Potentiometer.” <i>Nano
    Letters</i>. American Chemical Society, 2011. <a href="https://doi.org/10.1021/nl104411f">https://doi.org/10.1021/nl104411f</a>.
  ieee: J. S. Meisner, M. Kamenetska, M. Krikorian, M. L. Steigerwald, L. Venkataraman,
    and C. Nuckolls, “A single-molecule potentiometer,” <i>Nano Letters</i>, vol.
    11, no. 4. American Chemical Society, pp. 1575–1579, 2011.
  ista: Meisner JS, Kamenetska M, Krikorian M, Steigerwald ML, Venkataraman L, Nuckolls
    C. 2011. A single-molecule potentiometer. Nano Letters. 11(4), 1575–1579.
  mla: Meisner, Jeffrey S., et al. “A Single-Molecule Potentiometer.” <i>Nano Letters</i>,
    vol. 11, no. 4, American Chemical Society, 2011, pp. 1575–79, doi:<a href="https://doi.org/10.1021/nl104411f">10.1021/nl104411f</a>.
  short: J.S. Meisner, M. Kamenetska, M. Krikorian, M.L. Steigerwald, L. Venkataraman,
    C. Nuckolls, Nano Letters 11 (2011) 1575–1579.
date_created: 2024-09-09T12:36:26Z
date_published: 2011-03-17T00:00:00Z
date_updated: 2025-01-03T09:45:24Z
day: '17'
doi: 10.1021/nl104411f
extern: '1'
external_id:
  pmid:
  - '21413779'
fulldoi: https://doi.org/10.1021/nl104411f
intvolume: '        11'
issue: '4'
language:
- iso: eng
month: '03'
oa_version: None
page: 1575-1579
pmid: 1
publication: Nano Letters
publication_identifier:
  eissn:
  - 1530-6992
  issn:
  - 1530-6984
publication_status: published
publisher: American Chemical Society
quality_controlled: '1'
scopus_import: '1'
status: public
title: A single-molecule potentiometer
type: journal_article
user_id: 2DF688A6-F248-11E8-B48F-1D18A9856A87
volume: 11
year: '2011'
...
---
OA_type: closed access
_id: '18019'
abstract:
- lang: eng
  text: We simultaneously measure conductance and force across nanoscale junctions.
    A new, two-dimensional histogram technique is introduced to statistically extract
    bond rupture forces from a large data set of individual junction elongation traces.
    For the case of Au point contacts, we find a rupture force of 1.4 ± 0.2 nN, which
    is in good agreement with previous measurements. We then study systematic trends
    for single gold metal−molecule−metal junctions for a series of molecules terminated
    with amine and pyridine linkers. For all molecules studied, single molecule junctions
    rupture at the Au−N bond. Selective binding of the linker group allows us to correlate
    the N−Au bond-rupture force to the molecular backbone. We find that the rupture
    force ranges from 0.8 nN for 4,4′ bipyridine to 0.5 nN in 1,4 diaminobenzene.
    These experimental results are in excellent quantitative agreement with density
    functional theory based adiabatic molecular junction elongation and rupture calculations.
article_processing_charge: No
article_type: letter_note
author:
- first_name: Michael
  full_name: Frei, Michael
  last_name: Frei
- first_name: Sriharsha V.
  full_name: Aradhya, Sriharsha V.
  last_name: Aradhya
- first_name: Max
  full_name: Koentopp, Max
  last_name: Koentopp
- first_name: Mark S.
  full_name: Hybertsen, Mark S.
  last_name: Hybertsen
- first_name: Latha
  full_name: Venkataraman, Latha
  id: 9ebb78a5-cc0d-11ee-8322-fae086a32caf
  last_name: Venkataraman
  orcid: 0000-0002-6957-6089
citation:
  ama: 'Frei M, Aradhya SV, Koentopp M, Hybertsen MS, Venkataraman L. Mechanics and
    chemistry: Single molecule bond rupture forces correlate with molecular backbone
    structure. <i>Nano Letters</i>. 2011;11(4):1518-1523. doi:<a href="https://doi.org/10.1021/nl1042903">10.1021/nl1042903</a>'
  apa: 'Frei, M., Aradhya, S. V., Koentopp, M., Hybertsen, M. S., &#38; Venkataraman,
    L. (2011). Mechanics and chemistry: Single molecule bond rupture forces correlate
    with molecular backbone structure. <i>Nano Letters</i>. American Chemical Society.
    <a href="https://doi.org/10.1021/nl1042903">https://doi.org/10.1021/nl1042903</a>'
  chicago: 'Frei, Michael, Sriharsha V. Aradhya, Max Koentopp, Mark S. Hybertsen,
    and Latha Venkataraman. “Mechanics and Chemistry: Single Molecule Bond Rupture
    Forces Correlate with Molecular Backbone Structure.” <i>Nano Letters</i>. American
    Chemical Society, 2011. <a href="https://doi.org/10.1021/nl1042903">https://doi.org/10.1021/nl1042903</a>.'
  ieee: 'M. Frei, S. V. Aradhya, M. Koentopp, M. S. Hybertsen, and L. Venkataraman,
    “Mechanics and chemistry: Single molecule bond rupture forces correlate with molecular
    backbone structure,” <i>Nano Letters</i>, vol. 11, no. 4. American Chemical Society,
    pp. 1518–1523, 2011.'
  ista: 'Frei M, Aradhya SV, Koentopp M, Hybertsen MS, Venkataraman L. 2011. Mechanics
    and chemistry: Single molecule bond rupture forces correlate with molecular backbone
    structure. Nano Letters. 11(4), 1518–1523.'
  mla: 'Frei, Michael, et al. “Mechanics and Chemistry: Single Molecule Bond Rupture
    Forces Correlate with Molecular Backbone Structure.” <i>Nano Letters</i>, vol.
    11, no. 4, American Chemical Society, 2011, pp. 1518–23, doi:<a href="https://doi.org/10.1021/nl1042903">10.1021/nl1042903</a>.'
  short: M. Frei, S.V. Aradhya, M. Koentopp, M.S. Hybertsen, L. Venkataraman, Nano
    Letters 11 (2011) 1518–1523.
date_created: 2024-09-09T12:37:10Z
date_published: 2011-03-02T00:00:00Z
date_updated: 2025-01-03T09:47:07Z
day: '02'
doi: 10.1021/nl1042903
extern: '1'
external_id:
  pmid:
  - '21366230'
fulldoi: https://doi.org/10.1021/nl1042903
intvolume: '        11'
issue: '4'
language:
- iso: eng
month: '03'
oa_version: None
page: 1518-1523
pmid: 1
publication: Nano Letters
publication_identifier:
  eissn:
  - 1530-6992
  issn:
  - 1530-6984
publication_status: published
publisher: American Chemical Society
quality_controlled: '1'
scopus_import: '1'
status: public
title: 'Mechanics and chemistry: Single molecule bond rupture forces correlate with
  molecular backbone structure'
type: journal_article
user_id: 2DF688A6-F248-11E8-B48F-1D18A9856A87
volume: 11
year: '2011'
...
---
OA_type: closed access
_id: '18020'
abstract:
- lang: eng
  text: Understanding electron transport across π−π-stacked systems will help to answer
    fundamental questions about biochemical redox processes and benefit the design
    of new materials and molecular devices. Herein we employed the STM break-junction
    technique to measure the single-molecule conductance of multiple π−π-stacked aromatic
    rings. We studied electron transport through up to four stacked benzene rings
    held together in an eclipsed fashion via a paracyclophane scaffold. We found that
    the strained hydrocarbons studied herein couple directly to gold electrodes during
    the measurements; hence, we did not require any heteroatom binding groups as electrical
    contacts. Density functional theory-based calculations suggest that the gold atoms
    of the electrodes bind to two neighboring carbon atoms of the outermost cyclophane
    benzene rings in η2 fashion. Our measurements show an exponential decay of the
    conductance with an increasing number of stacked benzene rings, indicating a nonresonant
    tunneling mechanism. Furthermore, STM tip−substrate displacement data provide
    additional evidence that the electrodes bind to the outermost benzene rings of
    the π−π-stacked molecular wires.
article_processing_charge: No
article_type: letter_note
author:
- first_name: Severin T.
  full_name: Schneebeli, Severin T.
  last_name: Schneebeli
- first_name: Maria
  full_name: Kamenetska, Maria
  last_name: Kamenetska
- first_name: Zhanling
  full_name: Cheng, Zhanling
  last_name: Cheng
- first_name: Rachid
  full_name: Skouta, Rachid
  last_name: Skouta
- first_name: Richard A.
  full_name: Friesner, Richard A.
  last_name: Friesner
- first_name: Latha
  full_name: Venkataraman, Latha
  id: 9ebb78a5-cc0d-11ee-8322-fae086a32caf
  last_name: Venkataraman
  orcid: 0000-0002-6957-6089
- first_name: Ronald
  full_name: Breslow, Ronald
  last_name: Breslow
citation:
  ama: Schneebeli ST, Kamenetska M, Cheng Z, et al. Single-molecule conductance through
    multiple π−π-stacked benzene rings determined with direct electrode-to-benzene
    ring connections. <i>Journal of the American Chemical Society</i>. 2011;133(7):2136-2139.
    doi:<a href="https://doi.org/10.1021/ja111320n">10.1021/ja111320n</a>
  apa: Schneebeli, S. T., Kamenetska, M., Cheng, Z., Skouta, R., Friesner, R. A.,
    Venkataraman, L., &#38; Breslow, R. (2011). Single-molecule conductance through
    multiple π−π-stacked benzene rings determined with direct electrode-to-benzene
    ring connections. <i>Journal of the American Chemical Society</i>. American Chemical
    Society. <a href="https://doi.org/10.1021/ja111320n">https://doi.org/10.1021/ja111320n</a>
  chicago: Schneebeli, Severin T., Maria Kamenetska, Zhanling Cheng, Rachid Skouta,
    Richard A. Friesner, Latha Venkataraman, and Ronald Breslow. “Single-Molecule
    Conductance through Multiple Π−π-Stacked Benzene Rings Determined with Direct
    Electrode-to-Benzene Ring Connections.” <i>Journal of the American Chemical Society</i>.
    American Chemical Society, 2011. <a href="https://doi.org/10.1021/ja111320n">https://doi.org/10.1021/ja111320n</a>.
  ieee: S. T. Schneebeli <i>et al.</i>, “Single-molecule conductance through multiple
    π−π-stacked benzene rings determined with direct electrode-to-benzene ring connections,”
    <i>Journal of the American Chemical Society</i>, vol. 133, no. 7. American Chemical
    Society, pp. 2136–2139, 2011.
  ista: Schneebeli ST, Kamenetska M, Cheng Z, Skouta R, Friesner RA, Venkataraman
    L, Breslow R. 2011. Single-molecule conductance through multiple π−π-stacked benzene
    rings determined with direct electrode-to-benzene ring connections. Journal of
    the American Chemical Society. 133(7), 2136–2139.
  mla: Schneebeli, Severin T., et al. “Single-Molecule Conductance through Multiple
    Π−π-Stacked Benzene Rings Determined with Direct Electrode-to-Benzene Ring Connections.”
    <i>Journal of the American Chemical Society</i>, vol. 133, no. 7, American Chemical
    Society, 2011, pp. 2136–39, doi:<a href="https://doi.org/10.1021/ja111320n">10.1021/ja111320n</a>.
  short: S.T. Schneebeli, M. Kamenetska, Z. Cheng, R. Skouta, R.A. Friesner, L. Venkataraman,
    R. Breslow, Journal of the American Chemical Society 133 (2011) 2136–2139.
date_created: 2024-09-09T12:57:08Z
date_published: 2011-01-25T00:00:00Z
date_updated: 2025-01-03T09:49:00Z
day: '25'
doi: 10.1021/ja111320n
extern: '1'
external_id:
  pmid:
  - '21265533'
fulldoi: https://doi.org/10.1021/ja111320n
intvolume: '       133'
issue: '7'
language:
- iso: eng
month: '01'
oa_version: None
page: 2136-2139
pmid: 1
publication: Journal of the American Chemical Society
publication_identifier:
  eissn:
  - 1520-5126
  issn:
  - 0002-7863
publication_status: published
publisher: American Chemical Society
quality_controlled: '1'
scopus_import: '1'
status: public
title: Single-molecule conductance through multiple π−π-stacked benzene rings determined
  with direct electrode-to-benzene ring connections
type: journal_article
user_id: 2DF688A6-F248-11E8-B48F-1D18A9856A87
volume: 133
year: '2011'
...
---
OA_type: closed access
_id: '18021'
abstract:
- lang: eng
  text: Charge transport across metal–molecule interfaces has an important role in
    organic electronics1. Typically, chemical link groups such as thiols2 or amines3
    are used to bind organic molecules to metal electrodes in single-molecule circuits,
    with these groups controlling both the physical structure and the electronic coupling
    at the interface. Direct metal–carbon coupling has been shown through C60, benzene
    and π-stacked benzene4,5,6,7, but ideally the carbon backbone of the molecule
    should be covalently bonded to the electrode without intervening link groups.
    Here, we demonstrate a method to create junctions with such contacts. Trimethyl
    tin (SnMe3)-terminated polymethylene chains are used to form single-molecule junctions
    with a break-junction technique2,3. Gold atoms at the electrode displace the SnMe3
    linkers, leading to the formation of direct Au–C bonded single-molecule junctions
    with a conductance that is ∼100 times larger than analogous alkanes with most
    other terminations. The conductance of these Au–C bonded alkanes decreases exponentially
    with molecular length, with a decay constant of 0.97 per methylene, consistent
    with a non-resonant transport mechanism. Control experiments and ab initio calculations
    show that high conductances are achieved because a covalent Au–C sigma (σ) bond
    is formed. This offers a new method for making reproducible and highly conducting
    metal–organic contacts.
article_processing_charge: No
article_type: letter_note
author:
- first_name: Z.-L.
  full_name: Cheng, Z.-L.
  last_name: Cheng
- first_name: R.
  full_name: Skouta, R.
  last_name: Skouta
- first_name: H.
  full_name: Vazquez, H.
  last_name: Vazquez
- first_name: J. R.
  full_name: Widawsky, J. R.
  last_name: Widawsky
- first_name: S.
  full_name: Schneebeli, S.
  last_name: Schneebeli
- first_name: W.
  full_name: Chen, W.
  last_name: Chen
- first_name: M. S.
  full_name: Hybertsen, M. S.
  last_name: Hybertsen
- first_name: R.
  full_name: Breslow, R.
  last_name: Breslow
- first_name: Latha
  full_name: Venkataraman, Latha
  id: 9ebb78a5-cc0d-11ee-8322-fae086a32caf
  last_name: Venkataraman
  orcid: 0000-0002-6957-6089
citation:
  ama: Cheng Z-L, Skouta R, Vazquez H, et al. In situ formation of highly conducting
    covalent Au–C contacts for single-molecule junctions. <i>Nature Nanotechnology</i>.
    2011;6(6):353-357. doi:<a href="https://doi.org/10.1038/nnano.2011.66">10.1038/nnano.2011.66</a>
  apa: Cheng, Z.-L., Skouta, R., Vazquez, H., Widawsky, J. R., Schneebeli, S., Chen,
    W., … Venkataraman, L. (2011). In situ formation of highly conducting covalent
    Au–C contacts for single-molecule junctions. <i>Nature Nanotechnology</i>. Springer
    Nature. <a href="https://doi.org/10.1038/nnano.2011.66">https://doi.org/10.1038/nnano.2011.66</a>
  chicago: Cheng, Z.-L., R. Skouta, H. Vazquez, J. R. Widawsky, S. Schneebeli, W.
    Chen, M. S. Hybertsen, R. Breslow, and Latha Venkataraman. “In Situ Formation
    of Highly Conducting Covalent Au–C Contacts for Single-Molecule Junctions.” <i>Nature
    Nanotechnology</i>. Springer Nature, 2011. <a href="https://doi.org/10.1038/nnano.2011.66">https://doi.org/10.1038/nnano.2011.66</a>.
  ieee: Z.-L. Cheng <i>et al.</i>, “In situ formation of highly conducting covalent
    Au–C contacts for single-molecule junctions,” <i>Nature Nanotechnology</i>, vol.
    6, no. 6. Springer Nature, pp. 353–357, 2011.
  ista: Cheng Z-L, Skouta R, Vazquez H, Widawsky JR, Schneebeli S, Chen W, Hybertsen
    MS, Breslow R, Venkataraman L. 2011. In situ formation of highly conducting covalent
    Au–C contacts for single-molecule junctions. Nature Nanotechnology. 6(6), 353–357.
  mla: Cheng, Z. L., et al. “In Situ Formation of Highly Conducting Covalent Au–C
    Contacts for Single-Molecule Junctions.” <i>Nature Nanotechnology</i>, vol. 6,
    no. 6, Springer Nature, 2011, pp. 353–57, doi:<a href="https://doi.org/10.1038/nnano.2011.66">10.1038/nnano.2011.66</a>.
  short: Z.-L. Cheng, R. Skouta, H. Vazquez, J.R. Widawsky, S. Schneebeli, W. Chen,
    M.S. Hybertsen, R. Breslow, L. Venkataraman, Nature Nanotechnology 6 (2011) 353–357.
date_created: 2024-09-09T12:57:48Z
date_published: 2011-06-01T00:00:00Z
date_updated: 2025-01-03T09:51:33Z
day: '01'
doi: 10.1038/nnano.2011.66
extern: '1'
external_id:
  pmid:
  - '21552252'
fulldoi: https://doi.org/10.1038/nnano.2011.66
intvolume: '         6'
issue: '6'
language:
- iso: eng
month: '06'
oa_version: None
page: 353-357
pmid: 1
publication: Nature Nanotechnology
publication_identifier:
  eissn:
  - 1748-3395
  issn:
  - 1748-3387
publication_status: published
publisher: Springer Nature
quality_controlled: '1'
scopus_import: '1'
status: public
title: In situ formation of highly conducting covalent Au–C contacts for single-molecule
  junctions
type: journal_article
user_id: 2DF688A6-F248-11E8-B48F-1D18A9856A87
volume: 6
year: '2011'
...
---
_id: '1815'
abstract:
- lang: eng
  text: Many membrane channels and receptors exhibit adaptive, or desensitized, response
    to a strong sustained input stimulus, often supported by protein activity-dependent
    inactivation. Adaptive response is thought to be related to various cellular functions
    such as homeostasis and enlargement of dynamic range by background compensation.
    Here we study the quantitative relation between adaptive response and background
    compensation within a modeling framework. We show that any particular type of
    adaptive response is neither sufficient nor necessary for adaptive enlargement
    of dynamic range. In particular a precise adaptive response, where system activity
    is maintained at a constant level at steady state, does not ensure a large dynamic
    range neither in input signal nor in system output. A general mechanism for input
    dynamic range enlargement can come about from the activity-dependent modulation
    of protein responsiveness by multiple biochemical modification, regardless of
    the type of adaptive response it induces. Therefore hierarchical biochemical processes
    such as methylation and phosphorylation are natural candidates to induce this
    property in signaling systems.
author:
- first_name: Tamar
  full_name: Tamar Friedlander
  id: 36A5845C-F248-11E8-B48F-1D18A9856A87
  last_name: Friedlander
- first_name: Naama
  full_name: Brenner, Naama
  last_name: Brenner
citation:
  ama: Friedlander T, Brenner N. Adaptive response and enlargement of dynamic range.
    <i>Mathematical Biosciences and Engineering</i>. 2011;8(2):515-526. doi:<a href="https://doi.org/10.3934/mbe.2011.8.515">10.3934/mbe.2011.8.515</a>
  apa: Friedlander, T., &#38; Brenner, N. (2011). Adaptive response and enlargement
    of dynamic range. <i>Mathematical Biosciences and Engineering</i>. Arizona State
    University. <a href="https://doi.org/10.3934/mbe.2011.8.515">https://doi.org/10.3934/mbe.2011.8.515</a>
  chicago: Friedlander, Tamar, and Naama Brenner. “Adaptive Response and Enlargement
    of Dynamic Range.” <i>Mathematical Biosciences and Engineering</i>. Arizona State
    University, 2011. <a href="https://doi.org/10.3934/mbe.2011.8.515">https://doi.org/10.3934/mbe.2011.8.515</a>.
  ieee: T. Friedlander and N. Brenner, “Adaptive response and enlargement of dynamic
    range,” <i>Mathematical Biosciences and Engineering</i>, vol. 8, no. 2. Arizona
    State University, pp. 515–526, 2011.
  ista: Friedlander T, Brenner N. 2011. Adaptive response and enlargement of dynamic
    range. Mathematical Biosciences and Engineering. 8(2), 515–526.
  mla: Friedlander, Tamar, and Naama Brenner. “Adaptive Response and Enlargement of
    Dynamic Range.” <i>Mathematical Biosciences and Engineering</i>, vol. 8, no. 2,
    Arizona State University, 2011, pp. 515–26, doi:<a href="https://doi.org/10.3934/mbe.2011.8.515">10.3934/mbe.2011.8.515</a>.
  short: T. Friedlander, N. Brenner, Mathematical Biosciences and Engineering 8 (2011)
    515–526.
date_created: 2018-12-11T11:54:10Z
date_published: 2011-04-02T00:00:00Z
date_updated: 2021-01-12T06:53:23Z
day: '02'
doi: 10.3934/mbe.2011.8.515
extern: 1
fulldoi: https://doi.org/10.3934/mbe.2011.8.515
intvolume: '         8'
issue: '2'
main_file_link:
- open_access: '1'
  url: http://arxiv.org/abs/1003.2791
month: '04'
oa: 1
page: 515 - 526
publication: Mathematical Biosciences and Engineering
publication_status: published
publisher: Arizona State University
publist_id: '5291'
quality_controlled: 0
status: public
title: Adaptive response and enlargement of dynamic range
type: journal_article
volume: 8
year: '2011'
...
---
OA_place: repository
OA_type: green
_id: '18362'
abstract:
- lang: eng
  text: Maximally stable component detection is a very popular method for feature
    analysis in images, mainly due to its low computation cost and high repeatability.
    With the recent advance of feature-based methods in geometric shape analysis,
    there is significant interest in finding analogous approaches in the 3D world.
    In this paper, we formulate a diffusion-geometric framework for stable component
    detection in non-rigid 3D shapes, which can be used for geometric feature detection
    and description. A quantitative evaluation of our method on the SHREC’10 feature
    detection benchmark shows its potential as a source of high-quality features.
article_processing_charge: No
article_type: original
arxiv: 1
author:
- first_name: Roee
  full_name: Litman, Roee
  last_name: Litman
- first_name: Alexander
  full_name: Bronstein, Alexander
  id: 58f3726e-7cba-11ef-ad8b-e6e8cb3904e6
  last_name: Bronstein
  orcid: 0000-0001-9699-8730
- first_name: Michael M.
  full_name: Bronstein, Michael M.
  last_name: Bronstein
citation:
  ama: Litman R, Bronstein AM, Bronstein MM. Diffusion-geometric maximally stable
    component detection in deformable shapes. <i>Computers &#38; Graphics</i>. 2011;35(3):549-560.
    doi:<a href="https://doi.org/10.1016/j.cag.2011.03.011">10.1016/j.cag.2011.03.011</a>
  apa: Litman, R., Bronstein, A. M., &#38; Bronstein, M. M. (2011). Diffusion-geometric
    maximally stable component detection in deformable shapes. <i>Computers &#38;
    Graphics</i>. Elsevier. <a href="https://doi.org/10.1016/j.cag.2011.03.011">https://doi.org/10.1016/j.cag.2011.03.011</a>
  chicago: Litman, Roee, Alex M. Bronstein, and Michael M. Bronstein. “Diffusion-Geometric
    Maximally Stable Component Detection in Deformable Shapes.” <i>Computers &#38;
    Graphics</i>. Elsevier, 2011. <a href="https://doi.org/10.1016/j.cag.2011.03.011">https://doi.org/10.1016/j.cag.2011.03.011</a>.
  ieee: R. Litman, A. M. Bronstein, and M. M. Bronstein, “Diffusion-geometric maximally
    stable component detection in deformable shapes,” <i>Computers &#38; Graphics</i>,
    vol. 35, no. 3. Elsevier, pp. 549–560, 2011.
  ista: Litman R, Bronstein AM, Bronstein MM. 2011. Diffusion-geometric maximally
    stable component detection in deformable shapes. Computers &#38; Graphics. 35(3),
    549–560.
  mla: Litman, Roee, et al. “Diffusion-Geometric Maximally Stable Component Detection
    in Deformable Shapes.” <i>Computers &#38; Graphics</i>, vol. 35, no. 3, Elsevier,
    2011, pp. 549–60, doi:<a href="https://doi.org/10.1016/j.cag.2011.03.011">10.1016/j.cag.2011.03.011</a>.
  short: R. Litman, A.M. Bronstein, M.M. Bronstein, Computers &#38; Graphics 35 (2011)
    549–560.
date_created: 2024-10-15T11:20:54Z
date_published: 2011-06-01T00:00:00Z
date_updated: 2024-11-12T08:40:40Z
day: '01'
doi: 10.1016/j.cag.2011.03.011
extern: '1'
external_id:
  arxiv:
  - '1012.3951'
fulldoi: https://doi.org/10.1016/j.cag.2011.03.011
intvolume: '        35'
issue: '3'
language:
- iso: eng
main_file_link:
- open_access: '1'
  url: https://doi.org/10.48550/arXiv.1012.3951
month: '06'
oa: 1
oa_version: Preprint
page: 549-560
publication: Computers & Graphics
publication_identifier:
  issn:
  - 0097-8493
publication_status: published
publisher: Elsevier
quality_controlled: '1'
scopus_import: '1'
status: public
title: Diffusion-geometric maximally stable component detection in deformable shapes
type: journal_article
user_id: 2DF688A6-F248-11E8-B48F-1D18A9856A87
volume: 35
year: '2011'
...
---
OA_place: repository
OA_type: green
_id: '18363'
abstract:
- lang: eng
  text: "Natural objects can be subject to various transformations yet still preserve
    properties that we refer to as invariants. Here, we use definitions of affine-invariant
    arclength for surfaces in \r\n in order to extend the set of existing non-rigid
    shape analysis tools. We show that by re-defining the surface metric as its equi-affine
    version, the surface with its modified metric tensor can be treated as a canonical
    Euclidean object on which most classical Euclidean processing and analysis tools
    can be applied. The new definition of a metric is used to extend the fast marching
    method technique for computing geodesic distances on surfaces, where now, the
    distances are defined with respect to an affine-invariant arclength. Applications
    of the proposed framework demonstrate its invariance, efficiency, and accuracy
    in shape analysis."
article_processing_charge: No
article_type: letter_note
arxiv: 1
author:
- first_name: Dan
  full_name: Raviv, Dan
  last_name: Raviv
- first_name: Alexander
  full_name: Bronstein, Alexander
  id: 58f3726e-7cba-11ef-ad8b-e6e8cb3904e6
  last_name: Bronstein
  orcid: 0000-0001-9699-8730
- first_name: Michael M.
  full_name: Bronstein, Michael M.
  last_name: Bronstein
- first_name: Ron
  full_name: Kimmel, Ron
  last_name: Kimmel
- first_name: Nir
  full_name: Sochen, Nir
  last_name: Sochen
citation:
  ama: Raviv D, Bronstein AM, Bronstein MM, Kimmel R, Sochen N. Affine-invariant geodesic
    geometry of deformable 3D shapes. <i>Computers &#38; Graphics</i>. 2011;35(3):692-697.
    doi:<a href="https://doi.org/10.1016/j.cag.2011.03.030">10.1016/j.cag.2011.03.030</a>
  apa: Raviv, D., Bronstein, A. M., Bronstein, M. M., Kimmel, R., &#38; Sochen, N.
    (2011). Affine-invariant geodesic geometry of deformable 3D shapes. <i>Computers
    &#38; Graphics</i>. Elsevier. <a href="https://doi.org/10.1016/j.cag.2011.03.030">https://doi.org/10.1016/j.cag.2011.03.030</a>
  chicago: Raviv, Dan, Alex M. Bronstein, Michael M. Bronstein, Ron Kimmel, and Nir
    Sochen. “Affine-Invariant Geodesic Geometry of Deformable 3D Shapes.” <i>Computers
    &#38; Graphics</i>. Elsevier, 2011. <a href="https://doi.org/10.1016/j.cag.2011.03.030">https://doi.org/10.1016/j.cag.2011.03.030</a>.
  ieee: D. Raviv, A. M. Bronstein, M. M. Bronstein, R. Kimmel, and N. Sochen, “Affine-invariant
    geodesic geometry of deformable 3D shapes,” <i>Computers &#38; Graphics</i>, vol.
    35, no. 3. Elsevier, pp. 692–697, 2011.
  ista: Raviv D, Bronstein AM, Bronstein MM, Kimmel R, Sochen N. 2011. Affine-invariant
    geodesic geometry of deformable 3D shapes. Computers &#38; Graphics. 35(3), 692–697.
  mla: Raviv, Dan, et al. “Affine-Invariant Geodesic Geometry of Deformable 3D Shapes.”
    <i>Computers &#38; Graphics</i>, vol. 35, no. 3, Elsevier, 2011, pp. 692–97, doi:<a
    href="https://doi.org/10.1016/j.cag.2011.03.030">10.1016/j.cag.2011.03.030</a>.
  short: D. Raviv, A.M. Bronstein, M.M. Bronstein, R. Kimmel, N. Sochen, Computers
    &#38; Graphics 35 (2011) 692–697.
date_created: 2024-10-15T11:20:54Z
date_published: 2011-06-01T00:00:00Z
date_updated: 2024-11-12T08:37:24Z
day: '01'
doi: 10.1016/j.cag.2011.03.030
extern: '1'
external_id:
  arxiv:
  - '1012.5936'
fulldoi: https://doi.org/10.1016/j.cag.2011.03.030
intvolume: '        35'
issue: '3'
language:
- iso: eng
main_file_link:
- open_access: '1'
  url: https://doi.org/10.48550/arXiv.1012.5936
month: '06'
oa: 1
oa_version: Preprint
page: 692-697
publication: Computers & Graphics
publication_identifier:
  issn:
  - 0097-8493
publication_status: published
publisher: Elsevier
quality_controlled: '1'
scopus_import: '1'
status: public
title: Affine-invariant geodesic geometry of deformable 3D shapes
type: journal_article
user_id: 2DF688A6-F248-11E8-B48F-1D18A9856A87
volume: 35
year: '2011'
...
