{"date_updated":"2023-08-22T07:30:25Z","type":"journal_article","user_id":"2DF688A6-F248-11E8-B48F-1D18A9856A87","doi":"10.1126/sciadv.abj8121","oa_version":"Published Version","article_type":"original","status":"public","keyword":["Multidisciplinary"],"_id":"13995","extern":"1","publication_status":"published","month":"12","date_created":"2023-08-09T13:09:02Z","external_id":{"pmid":["34860540"]},"publisher":"American Association for the Advancement of Science","publication":"Science Advances","issue":"49","publication_identifier":{"eissn":["2375-2548"]},"intvolume":"         7","citation":{"ieee":"S. Heck <i>et al.</i>, “Attosecond interferometry of shape resonances in the recoil frame of CF4,” <i>Science Advances</i>, vol. 7, no. 49. American Association for the Advancement of Science, 2021.","short":"S. Heck, D.R. Baykusheva, M. Han, J.-B. Ji, C. Perry, X. Gong, H.J. Wörner, Science Advances 7 (2021).","ama":"Heck S, Baykusheva DR, Han M, et al. Attosecond interferometry of shape resonances in the recoil frame of CF4. <i>Science Advances</i>. 2021;7(49). doi:<a href=\"https://doi.org/10.1126/sciadv.abj8121\">10.1126/sciadv.abj8121</a>","chicago":"Heck, Saijoscha, Denitsa Rangelova Baykusheva, Meng Han, Jia-Bao Ji, Conaill Perry, Xiaochun Gong, and Hans Jakob Wörner. “Attosecond Interferometry of Shape Resonances in the Recoil Frame of CF4.” <i>Science Advances</i>. American Association for the Advancement of Science, 2021. <a href=\"https://doi.org/10.1126/sciadv.abj8121\">https://doi.org/10.1126/sciadv.abj8121</a>.","apa":"Heck, S., Baykusheva, D. R., Han, M., Ji, J.-B., Perry, C., Gong, X., &#38; Wörner, H. J. (2021). Attosecond interferometry of shape resonances in the recoil frame of CF4. <i>Science Advances</i>. American Association for the Advancement of Science. <a href=\"https://doi.org/10.1126/sciadv.abj8121\">https://doi.org/10.1126/sciadv.abj8121</a>","mla":"Heck, Saijoscha, et al. “Attosecond Interferometry of Shape Resonances in the Recoil Frame of CF4.” <i>Science Advances</i>, vol. 7, no. 49, abj8121, American Association for the Advancement of Science, 2021, doi:<a href=\"https://doi.org/10.1126/sciadv.abj8121\">10.1126/sciadv.abj8121</a>.","ista":"Heck S, Baykusheva DR, Han M, Ji J-B, Perry C, Gong X, Wörner HJ. 2021. Attosecond interferometry of shape resonances in the recoil frame of CF4. Science Advances. 7(49), abj8121."},"title":"Attosecond interferometry of shape resonances in the recoil frame of CF4","article_processing_charge":"No","article_number":"abj8121","pmid":1,"date_published":"2021-12-03T00:00:00Z","volume":7,"quality_controlled":"1","scopus_import":"1","year":"2021","oa":1,"abstract":[{"text":"Shape resonances play a central role in many areas of science, but the real-time measurement of the associated many-body dynamics remains challenging. Here, we present measurements of recoil frame angle-resolved photoionization delays in the vicinity of shape resonances of CF4. This technique provides insights into the spatiotemporal photoionization dynamics of molecular shape resonances. We find delays of up to ∼600 as in the ionization out of the highest occupied molecular orbital (HOMO) with a strong dependence on the emission direction and a pronounced asymmetry along the dissociation axis. Comparison with quantum-scattering calculations traces the asymmetries to the interference of a small subset of partial waves at low kinetic energies and, additionally, to the interference of two overlapping shape resonances in the HOMO-1 channel. Our experimental and theoretical results establish a broadly applicable approach to space- and time-resolved photoionization dynamics in the molecular frame.","lang":"eng"}],"author":[{"first_name":"Saijoscha","last_name":"Heck","full_name":"Heck, Saijoscha"},{"full_name":"Baykusheva, Denitsa Rangelova","id":"71b4d059-2a03-11ee-914d-dfa3beed6530","first_name":"Denitsa Rangelova","last_name":"Baykusheva"},{"full_name":"Han, Meng","last_name":"Han","first_name":"Meng"},{"full_name":"Ji, Jia-Bao","last_name":"Ji","first_name":"Jia-Bao"},{"first_name":"Conaill","last_name":"Perry","full_name":"Perry, Conaill"},{"first_name":"Xiaochun","last_name":"Gong","full_name":"Gong, Xiaochun"},{"full_name":"Wörner, Hans Jakob","first_name":"Hans Jakob","last_name":"Wörner"}],"language":[{"iso":"eng"}],"day":"03","main_file_link":[{"open_access":"1","url":"https://doi.org/10.1126/sciadv.abj8121"}]}