---
_id: '14013'
abstract:
- lang: eng
  text: The ultrafast motion of electrons and holes after light-matter interaction
    is fundamental to a broad range of chemical and biophysical processes. We advanced
    high-harmonic spectroscopy to resolve spatially and temporally the migration of
    an electron hole immediately after ionization of iodoacetylene while simultaneously
    demonstrating extensive control over the process. A multidimensional approach,
    based on the measurement and accurate theoretical description of both even and
    odd harmonic orders, enabled us to reconstruct both quantum amplitudes and phases
    of the electronic states with a resolution of ~100 attoseconds. We separately
    reconstructed quasi-field-free and laser-controlled charge migration as a function
    of the spatial orientation of the molecule and determined the shape of the hole
    created by ionization. Our technique opens the prospect of laser control over
    electronic primary processes.
article_processing_charge: No
article_type: original
author:
- first_name: P. M.
  full_name: Kraus, P. M.
  last_name: Kraus
- first_name: B.
  full_name: Mignolet, B.
  last_name: Mignolet
- first_name: Denitsa Rangelova
  full_name: Baykusheva, Denitsa Rangelova
  id: 71b4d059-2a03-11ee-914d-dfa3beed6530
  last_name: Baykusheva
- first_name: A.
  full_name: Rupenyan, A.
  last_name: Rupenyan
- first_name: L.
  full_name: Horný, L.
  last_name: Horný
- first_name: E. F.
  full_name: Penka, E. F.
  last_name: Penka
- first_name: G.
  full_name: Grassi, G.
  last_name: Grassi
- first_name: O. I.
  full_name: Tolstikhin, O. I.
  last_name: Tolstikhin
- first_name: J.
  full_name: Schneider, J.
  last_name: Schneider
- first_name: F.
  full_name: Jensen, F.
  last_name: Jensen
- first_name: L. B.
  full_name: Madsen, L. B.
  last_name: Madsen
- first_name: A. D.
  full_name: Bandrauk, A. D.
  last_name: Bandrauk
- first_name: F.
  full_name: Remacle, F.
  last_name: Remacle
- first_name: H. J.
  full_name: Wörner, H. J.
  last_name: Wörner
citation:
  ama: Kraus PM, Mignolet B, Baykusheva DR, et al. Measurement and laser control of
    attosecond charge migration in ionized iodoacetylene. <i>Science</i>. 2015;350(6262):790-795.
    doi:<a href="https://doi.org/10.1126/science.aab2160">10.1126/science.aab2160</a>
  apa: Kraus, P. M., Mignolet, B., Baykusheva, D. R., Rupenyan, A., Horný, L., Penka,
    E. F., … Wörner, H. J. (2015). Measurement and laser control of attosecond charge
    migration in ionized iodoacetylene. <i>Science</i>. American Association for the
    Advancement of Science. <a href="https://doi.org/10.1126/science.aab2160">https://doi.org/10.1126/science.aab2160</a>
  chicago: Kraus, P. M., B. Mignolet, Denitsa Rangelova Baykusheva, A. Rupenyan, L.
    Horný, E. F. Penka, G. Grassi, et al. “Measurement and Laser Control of Attosecond
    Charge Migration in Ionized Iodoacetylene.” <i>Science</i>. American Association
    for the Advancement of Science, 2015. <a href="https://doi.org/10.1126/science.aab2160">https://doi.org/10.1126/science.aab2160</a>.
  ieee: P. M. Kraus <i>et al.</i>, “Measurement and laser control of attosecond charge
    migration in ionized iodoacetylene,” <i>Science</i>, vol. 350, no. 6262. American
    Association for the Advancement of Science, pp. 790–795, 2015.
  ista: Kraus PM, Mignolet B, Baykusheva DR, Rupenyan A, Horný L, Penka EF, Grassi
    G, Tolstikhin OI, Schneider J, Jensen F, Madsen LB, Bandrauk AD, Remacle F, Wörner
    HJ. 2015. Measurement and laser control of attosecond charge migration in ionized
    iodoacetylene. Science. 350(6262), 790–795.
  mla: Kraus, P. M., et al. “Measurement and Laser Control of Attosecond Charge Migration
    in Ionized Iodoacetylene.” <i>Science</i>, vol. 350, no. 6262, American Association
    for the Advancement of Science, 2015, pp. 790–95, doi:<a href="https://doi.org/10.1126/science.aab2160">10.1126/science.aab2160</a>.
  short: P.M. Kraus, B. Mignolet, D.R. Baykusheva, A. Rupenyan, L. Horný, E.F. Penka,
    G. Grassi, O.I. Tolstikhin, J. Schneider, F. Jensen, L.B. Madsen, A.D. Bandrauk,
    F. Remacle, H.J. Wörner, Science 350 (2015) 790–795.
date_created: 2023-08-10T06:37:35Z
date_published: 2015-10-22T00:00:00Z
date_updated: 2023-08-22T08:47:39Z
day: '22'
doi: 10.1126/science.aab2160
extern: '1'
external_id:
  pmid:
  - '26494175'
intvolume: '       350'
issue: '6262'
keyword:
- Multidisciplinary
language:
- iso: eng
month: '10'
oa_version: None
page: 790-795
pmid: 1
publication: Science
publication_identifier:
  eissn:
  - 1095-9203
  issn:
  - 0036-8075
publication_status: published
publisher: American Association for the Advancement of Science
quality_controlled: '1'
scopus_import: '1'
status: public
title: Measurement and laser control of attosecond charge migration in ionized iodoacetylene
type: journal_article
user_id: 2DF688A6-F248-11E8-B48F-1D18A9856A87
volume: 350
year: '2015'
...