Deep eutectic solvent as a solution for polyester/cotton textile recycling Depope, Nika Depope, Al Archodoulaki, Vasiliki Maria Ipsmiller, Wolfgang Bartl, Andreas ddc:572 Global fibre production has expanded rapidly, with polyester and cotton dominating, significantly contributing to textile waste and increasing demand for sustainable solutions. This study presents innovative method to recycle polyester/cotton (PET/CO) blends using hydrophobic deep eutectic solvents (DESs), eliminating the need for toxic chemicals while achieving high dissolution yields. PET was completely dissolved within 5 min, substantially outperforming state-of-the-art methods and facilitating the efficient and selective recovery of both components, PET (97%) and CO (100%). SEM imaging confirmed no morphological changes in cotton fibres after treatment. The thermal stability of the recovered materials was validated using DSC and TGA analyses, while ATR-FTIR spectroscopy indicated no chemical changes. Mechanical testing confirmed recovered cotton’s tenacity and elongation are within expected ranges despite showing a decrease of 28% in tenacity and 34% in elongation. Hence, the proposed process provides an efficient and sustainable recycling solution for PET/CO blends, retaining both polymers in a condition similar to virgin materials used in textile manufacturing with minimal processing time. Elsevier 2025 info:eu-repo/semantics/article doc-type:article text http://purl.org/coar/resource_type/c_2df8fbb1 https://research-explorer.ista.ac.at/record/20491 https://research-explorer.ista.ac.at/download/20491/20501 Depope N, Depope A, Archodoulaki VM, Ipsmiller W, Bartl A. Deep eutectic solvent as a solution for polyester/cotton textile recycling. <i>Waste Management</i>. 2025;208. doi:<a href="https://doi.org/10.1016/j.wasman.2025.115177">10.1016/j.wasman.2025.115177</a> eng info:eu-repo/semantics/altIdentifier/doi/10.1016/j.wasman.2025.115177 info:eu-repo/semantics/altIdentifier/issn/0956-053X info:eu-repo/semantics/altIdentifier/e-issn/1879-2456 info:eu-repo/semantics/altIdentifier/wos/001594629200003 info:eu-repo/semantics/altIdentifier/pmid/41066876 https://creativecommons.org/licenses/by/4.0/ info:eu-repo/semantics/openAccess