{"article_type":"original","corr_author":"1","year":"2026","publication_status":"published","oa_version":"Published Version","date_published":"2026-02-05T00:00:00Z","OA_place":"publisher","month":"02","issue":"5","citation":{"mla":"Hrast, Mateja, et al. “Bottom-up Analysis of Rovibrational Helical Dichroism.” Physical Review Letters, vol. 136, no. 5, 053204, American Physical Society, 2026, doi:10.1103/fkf1-1jml.","apa":"Hrast, M., Koutentakis, G., Maslov, M., & Lemeshko, M. (2026). Bottom-up analysis of rovibrational helical dichroism. Physical Review Letters. American Physical Society. https://doi.org/10.1103/fkf1-1jml","ieee":"M. Hrast, G. Koutentakis, M. Maslov, and M. Lemeshko, “Bottom-up analysis of rovibrational helical dichroism,” Physical Review Letters, vol. 136, no. 5. American Physical Society, 2026.","ama":"Hrast M, Koutentakis G, Maslov M, Lemeshko M. Bottom-up analysis of rovibrational helical dichroism. Physical Review Letters. 2026;136(5). doi:10.1103/fkf1-1jml","ista":"Hrast M, Koutentakis G, Maslov M, Lemeshko M. 2026. Bottom-up analysis of rovibrational helical dichroism. Physical Review Letters. 136(5), 053204.","short":"M. Hrast, G. Koutentakis, M. Maslov, M. Lemeshko, Physical Review Letters 136 (2026).","chicago":"Hrast, Mateja, Georgios Koutentakis, Mikhail Maslov, and Mikhail Lemeshko. “Bottom-up Analysis of Rovibrational Helical Dichroism.” Physical Review Letters. American Physical Society, 2026. https://doi.org/10.1103/fkf1-1jml."},"author":[{"id":"48dbb294-2a9c-11ef-905d-f56be71f0e5d","last_name":"Hrast","first_name":"Mateja","full_name":"Hrast, Mateja"},{"full_name":"Koutentakis, Georgios","last_name":"Koutentakis","first_name":"Georgios","id":"d7b23d3a-9e21-11ec-b482-f76739596b95"},{"last_name":"Maslov","first_name":"Mikhail","full_name":"Maslov, Mikhail","id":"2E65BB0E-F248-11E8-B48F-1D18A9856A87","orcid":"0000-0003-4074-2570"},{"id":"37CB05FA-F248-11E8-B48F-1D18A9856A87","orcid":"0000-0002-6990-7802","full_name":"Lemeshko, Mikhail","last_name":"Lemeshko","first_name":"Mikhail"}],"PlanS_conform":"1","department":[{"_id":"MiLe"}],"has_accepted_license":"1","ddc":["530"],"oa":1,"publication_identifier":{"eissn":["1079-7114"],"issn":["0031-9007"]},"file":[{"access_level":"open_access","date_updated":"2026-02-10T11:25:46Z","creator":"dernst","file_id":"21210","success":1,"date_created":"2026-02-10T11:25:46Z","file_size":511312,"file_name":"2026_PhysicalReviewLetters_Hrast.pdf","checksum":"805c929fff9fd4d0e733293eaace67b8","content_type":"application/pdf","relation":"main_file"}],"title":"Bottom-up analysis of rovibrational helical dichroism","_id":"21149","quality_controlled":"1","intvolume":" 136","scopus_import":"1","language":[{"iso":"eng"}],"OA_type":"hybrid","article_number":"053204","user_id":"2DF688A6-F248-11E8-B48F-1D18A9856A87","article_processing_charge":"Yes (via OA deal)","abstract":[{"text":"We present a general theoretical framework for helical dichroism (HD), establishing an explicit link between chiral resolution and orbital angular momentum (OAM) exchange in light–matter interaction. Tracing microscopic mechanisms of the OAM transfer, we derive rotational selection rules, which establish that HD emerges only from the spin–orbit coupling of light, even for beams without the far-field OAM. Our findings refine the conditions for observing HD, provide a tool to re-examine the outcome of prior experiments, and guide future designs for chiral sensing with structured light.","lang":"eng"}],"doi":"10.1103/fkf1-1jml","external_id":{"arxiv":["2505.16393"]},"project":[{"_id":"7c040762-9f16-11ee-852c-dd79eeee4ab3","name":"Coherent Optical Metrology Beyond Electric-Dipole-Allowed Transitions","grant_number":"F100403"}],"volume":136,"acknowledgement":"This research was funded in whole or in part by the Austrian Science Fund (FWF) [10.55776/F1004].","file_date_updated":"2026-02-10T11:25:46Z","tmp":{"short":"CC BY (4.0)","image":"/images/cc_by.png","name":"Creative Commons Attribution 4.0 International Public License (CC-BY 4.0)","legal_code_url":"https://creativecommons.org/licenses/by/4.0/legalcode"},"publisher":"American Physical Society","publication":"Physical Review Letters","type":"journal_article","day":"05","arxiv":1,"date_updated":"2026-02-10T11:30:37Z","date_created":"2026-02-06T10:53:17Z","status":"public"}