Fully independent response in disordered solids

Zu M, Desai AA, Goodrich CP. 2025. Fully independent response in disordered solids. Physical Review Letters. 134(23), 238201.

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Journal Article | Published | English

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Corresponding author has ISTA affiliation

Abstract
Unlike in crystals, it is difficult to trace emergent material properties of amorphous solids to their underlying structure. Nevertheless, one can tune features of a disordered spring network, ranging from bulk elastic constants to specific allosteric responses, through highly precise alterations of the structure. This has been understood through the notion of independent bond-level response—the observation that, in many cases, different springs have different effects on different properties. While this idea has motivated inverse design in numerous contexts, it has not been formalized and quantified in a general context that not just informs but enables and predicts inverse design. Here, we show how to quantify independent response by linearizing the simultaneous change in multiple emergent features, and introduce the much stronger notion of fully independent response. Remarkably, we find that the mechanical properties of disordered solids are always fully independent across a wide array of scenarios, regardless of the target features, tunable parameters, system size, dimensionality, and class of interactions. Furthermore, our formulation quantifies the susceptibility of features to parameter changes, which is correlated with the maximum linear tunability. We also demonstrate the implications for multifeature inverse design beyond the linear regime. These results formalize our understanding of a key fundamental difference between ordered and disordered solids while also creating a practical tool to both understand and perform inverse design.
Publishing Year
Date Published
2025-06-13
Journal Title
Physical Review Letters
Publisher
American Physical Society
Acknowledgement
We gratefully acknowledge Edouard Hannezo for helpful comments on the manuscript. The work was funded by the Institute of Science and Technology Austria.
Volume
134
Issue
23
Article Number
238201
ISSN
eISSN
IST-REx-ID

Cite this

Zu M, Desai AA, Goodrich CP. Fully independent response in disordered solids. Physical Review Letters. 2025;134(23). doi:10.1103/PhysRevLett.134.238201
Zu, M., Desai, A. A., & Goodrich, C. P. (2025). Fully independent response in disordered solids. Physical Review Letters. American Physical Society. https://doi.org/10.1103/PhysRevLett.134.238201
Zu, Mengjie, Aayush A Desai, and Carl Peter Goodrich. “Fully Independent Response in Disordered Solids.” Physical Review Letters. American Physical Society, 2025. https://doi.org/10.1103/PhysRevLett.134.238201.
M. Zu, A. A. Desai, and C. P. Goodrich, “Fully independent response in disordered solids,” Physical Review Letters, vol. 134, no. 23. American Physical Society, 2025.
Zu M, Desai AA, Goodrich CP. 2025. Fully independent response in disordered solids. Physical Review Letters. 134(23), 238201.
Zu, Mengjie, et al. “Fully Independent Response in Disordered Solids.” Physical Review Letters, vol. 134, no. 23, 238201, American Physical Society, 2025, doi:10.1103/PhysRevLett.134.238201.
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2025-06-23
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