Strain-induced multiferroicity in Cr1/3NbS2

Multiferroic materials, in which electric polarization and magnetic order coexist and couple, offer rich opportunities for both fundamental discovery and technology. However, multiferroicity remains rare due to conflicting electronic requirements for ferroelectricity and magnetism. One route to circumvent this challenge is to exploit the noncollinear ordering of spin cycloids, whose symmetry permits the emergence of polar order. In this work, we introduce another pathway to multiferroic order in which strain generates polarization in materials that host nonpolar spin spirals. To demonstrate this phenomenon, we chose the spin spiral in the well-studied helimagnet Cr1/3NbS2. To detect the induced polarization, we introduce the technique of magnetoelectric birefringence (MEB), an optical probe that enables spatially-resolved and unambiguous detection of polar order. By combining MEB imaging with strain engineering, we confirm the onset of a polar vector at the magnetic transition, establishing strained Cr1/3NbS2 as a type-II multiferroic.